A new approach to HDO/H2O ratio profile retrieval in the atmosphere from TANSO-FTS/GOSAT-2 spectrum data by using TIR and SWIR spectral ranges simultaneously: method and software

Author(s):  
Zadvornykh Ilya ◽  
Gribanov Konstantin ◽  
Zakharov Vyacheslav ◽  
Denisova Nina ◽  
Imasu Ryoichi ◽  
...  

<p><span>Global monitoring of isotopic composition of water vapor in the atmosphere provides information regarding atmospheric hydgrological cycle in the Earth’s climate system. The observed HDO to H</span><sub><span>2</span></sub><span>O ratio (δD) in atmospheric water vapor gives information on origin and history of air masses in the atmosphere.</span></p><p><span>In this study we present a method, software tool and some results on δD ratio retrieval from spectra, measured simultaneously in the thermal (TIR) and short wave infrared (SWIR) spectral ranges. The TANSO-FTS high spectral resolution spectrometer on board GOSAT-2 satellite is unique to perform simultaneous measurements in TIR and SWIR spectral bands. A method of simultaneous using of these both bands can improve vertical resolution of δD retrieved profile.</span></p><p><span>We applied conventional optimal estimation method to solve inverse problem. The output data of atmospheric general circulation model ECHAM5-wiso were used as a statistical ensemble of HDO and H2O a priori profiles. The averaging kernels, a posteriori covariance matrices and degrees of freedom are calculated. The retrieval algorithm is implemented using original FIRE-ARMS software and VLIDORT radiation transfer model.</span></p><p><span>This study is supported by the Russian Science Foundation grant No. 18-11-00024.</span></p>

2015 ◽  
Vol 54 (2) ◽  
pp. 408-422 ◽  
Author(s):  
Gregory S. Elsaesser ◽  
Christian D. Kummerow

AbstractThe Goddard profiling algorithm (GPROF) uses Bayesian probability theory to retrieve rainfall over the global oceans. A critical component of GPROF and most Bayes theorem–based retrieval frameworks is the specification of uncertainty in the observations being utilized to retrieve the parameter of interest. In the case of GPROF, for any sensor, uncertainties in microwave brightness temperatures (Tbs) arise from radiative transfer model errors, satellite sensor noise and/or degradation, and nonlinear, scene-dependent Tb offsets added during sensor intercalibration procedures. All mentioned sources impact sensors in a varying fashion, in part because of sensor-dependent fields of view. It is found that small errors in assumed Tb uncertainty (ranging from 0.57 K at 10 GHz to 2.29 K at 85 GHz) lead to a 3.6% change in the retrieved global-average oceanic rainfall rate, and 10%–20% (20%–40%) shifts in the pixel-level (monthly) frequency distributions for given rainfall bins. A mathematical expression describing the sensitivity of retrieved rainfall to uncertainty is developed here. The strong global sensitivity is linked to rainfall variance scaling systematically as Tb varies. For ocean scenes, the same emission-dominated rainfall–Tb physics used in passive microwave rainfall retrieval is also responsible for the substantial underestimation (overestimation) of global rainfall if uncertainty is overestimated (underestimated). Proper uncertainties are required to quantify variability in surface rainfall, assess long-term trends, and provide robust rainfall benchmarks for general circulation model evaluations. The implications for assessing global and regional biases in active versus passive microwave rainfall products, and for achieving rainfall product agreement among a constellation of orbiting microwave radiometers [employed in the Global Precipitation Measurement (GPM) mission], are also discussed.


2019 ◽  
Author(s):  
Camille Risi ◽  
Joseph Galewsky ◽  
Gilles Reverdin ◽  
Florent Brient

Abstract. Understanding what controls the water vapor isotopic composition of the sub-cloud layer (SCL) over tropical oceans (δD0) is a first step towards understanding the water vapor isotopic composition everywhere in the troposphere. We propose an analytical model to predict δD0 as a function of sea surface conditions, humidity and temperature profiles, and the altitude from which the free tropospheric air originates (zorig). To do so, we extend previous studies by (1) prescribing the shape of δD0 vertical profiles, and (2) linking δD0 to zorig. The model relies on the hypotheses that δD0 profiles are steeper than mixing lines and no clouds are precipitating. We show that δD0 does not depend on the intensity of entrainment, dampening hope that δD0 measurements could help constrain this long-searched quantity. Based on an isotope-enabled general circulation model simulation, we show that δD0 variations are mainly controlled by mid-tropospheric depletion and rain evaporation in ascending regions, and by sea surface temperature and zorig in subsiding regions. When the air mixing into the SCL is lower in altitude, it is moister, and thus it depletes more efficiently the SCL. In turn, could δD0 measurements help estimate zorig and thus discriminate between different mixing processes? Estimates that are accurate enough to be useful would be difficult to achieve in practice, requiring measuring daily δD profiles, and measuring δD0 with an accuracy of 0.1 ‰ and 0.4 ‰ in trade-wind cumulus and strato-cumulus clouds respectively.


2020 ◽  
Vol 12 (24) ◽  
pp. 4107
Author(s):  
Charlotte Segonne ◽  
Nathalie Huret ◽  
Sébastien Payan ◽  
Mathieu Gouhier ◽  
Valéry Catoire

Fast and accurate quantification of gas fluxes emitted by volcanoes is essential for the risk mitigation of explosive eruption, and for the fundamental understanding of shallow eruptive processes. Sulphur dioxide (SO2), in particular, is a reliable indicator to predict upcoming eruptions, and its systemic characterization allows the rapid assessment of sudden changes in eruptive dynamics. In this regard, infrared (IR) hyperspectral imaging is a promising new technology for accurately measure SO2 fluxes day and night at a frame rate down to 1 image per second. The thermal infrared region is not very sensitive to particle scattering, which is an asset for the study of volcanic plume. A ground based infrared hyperspectral imager was deployed during the IMAGETNA campaign in 2015 and provided high spectral resolution images of the Mount Etna (Sicily, Italy) plume from the North East Crater (NEC), mainly. The LongWave InfraRed (LWIR) hyperspectral imager, hereafter name Hyper-Cam, ranges between 850–1300 cm−1 (7.7–11.8 µm). The LATMOS (Laboratoire Atmosphères Milieux Observations Spatiales) Atmospheric Retrieval Algorithm (LARA), which is used to retrieve the slant column densities (SCD) of SO2, is a robust and a complete radiative transfer model, well adapted to the inversion of ground-based remote measurements. However, the calculation time to process the raw data and retrieve the infrared spectra, which is about seven days for the retrieval of one image of SO2 SCD, remains too high to infer near real-time (NRT) SO2 emission fluxes. A spectral image classification methodology based on two parameters extracting spectral features in the O3 and SO2 emission bands was developed to create a library. The relevance is evaluated in detail through tests. From data acquisition to the generation of SO2 SCD images, this method requires only ~40 s per image, which opens the possibility to infer NRT estimation of SO2 emission fluxes from IR hyperspectral imager measurements.


2006 ◽  
Vol 19 (9) ◽  
pp. 1652-1672 ◽  
Author(s):  
Mike Bauer ◽  
Anthony D. Del Genio

Abstract The role of midlatitude baroclinic cyclones in maintaining the extratropical winter distribution of water vapor in an operational global climate model is investigated. A cyclone identification and tracking algorithm is used to compare the frequency of occurrence, propagation characteristics, and composite structure of 10 winters of storms in the Goddard Institute for Space Studies general circulation model (GCM) and in two reanalysis products. Cyclones are the major dynamical source of water vapor over the extratropical oceans in the reanalyses. The GCM produces fewer, generally weaker, and slower-moving cyclones than the reanalyses and is especially deficient in storms associated with secondary cyclogenesis. Composite fields show that GCM cyclones are shallower and drier aloft than those in the reanalyses and that their vertical structure is less tilted in the frontal region because of the GCM’s weaker ageostrophic circulation. This is consistent with the GCM’s underprediction of midlatitude cirrus. The GCM deficiencies do not appear to be primarily due to parameterization errors; the model is too dry despite producing less storm precipitation than is present in the reanalyses and in an experimental satellite precipitation dataset, and the weakness and shallow structure of GCM cyclones is already present at storm onset. These shortcomings may be common to most climate GCMs that do not resolve the mesoscale structure of frontal zones, and this may account for some universal problems in climate GCM midlatitude cloud properties.


2016 ◽  
Vol 9 (9) ◽  
pp. 4673-4686 ◽  
Author(s):  
Andreas Reichert ◽  
Markus Rettinger ◽  
Ralf Sussmann

Abstract. Quantitative knowledge of water vapor absorption is crucial for accurate climate simulations. An open science question in this context concerns the strength of the water vapor continuum in the near infrared (NIR) at atmospheric temperatures, which is still to be quantified by measurements. This issue can be addressed with radiative closure experiments using solar absorption spectra. However, the spectra used for water vapor continuum quantification have to be radiometrically calibrated. We present for the first time a method that yields sufficient calibration accuracy for NIR water vapor continuum quantification in an atmospheric closure experiment. Our method combines the Langley method with spectral radiance measurements of a high-temperature blackbody calibration source (<  2000 K). The calibration scheme is demonstrated in the spectral range 2500 to 7800 cm−1, but minor modifications to the method enable calibration also throughout the remainder of the NIR spectral range. The resulting uncertainty (2σ) excluding the contribution due to inaccuracies in the extra-atmospheric solar spectrum (ESS) is below 1 % in window regions and up to 1.7 % within absorption bands. The overall radiometric accuracy of the calibration depends on the ESS uncertainty, on which at present no firm consensus has been reached in the NIR. However, as is shown in the companion publication Reichert and Sussmann (2016), ESS uncertainty is only of minor importance for the specific aim of this study, i.e., the quantification of the water vapor continuum in a closure experiment. The calibration uncertainty estimate is substantiated by the investigation of calibration self-consistency, which yields compatible results within the estimated errors for 91.1 % of the 2500 to 7800 cm−1 range. Additionally, a comparison of a set of calibrated spectra to radiative transfer model calculations yields consistent results within the estimated errors for 97.7 % of the spectral range.


2021 ◽  
Vol 14 (10) ◽  
pp. 6483-6507
Author(s):  
Zhao-Cheng Zeng ◽  
Vijay Natraj ◽  
Feng Xu ◽  
Sihe Chen ◽  
Fang-Ying Gong ◽  
...  

Abstract. Remote sensing of greenhouse gases (GHGs) in cities, where high GHG emissions are typically associated with heavy aerosol loading, is challenging due to retrieval uncertainties caused by the imperfect characterization of scattering by aerosols. We investigate this problem by developing GFIT3, a full physics algorithm to retrieve GHGs (CO2 and CH4) by accounting for aerosol scattering effects in polluted urban atmospheres. In particular, the algorithm includes coarse- (including sea salt and dust) and fine- (including organic carbon, black carbon, and sulfate) mode aerosols in the radiative transfer model. The performance of GFIT3 is assessed using high-spectral-resolution observations over the Los Angeles (LA) megacity made by the California Laboratory for Atmospheric Remote Sensing Fourier transform spectrometer (CLARS-FTS). CLARS-FTS is located on Mt. Wilson, California, at 1.67 km a.s.l. overlooking the LA Basin, and it makes observations of reflected sunlight in the near-infrared spectral range. The first set of evaluations are performed by conducting retrieval experiments using synthetic spectra. We find that errors in the retrievals of column-averaged dry air mole fractions of CO2 (XCO2) and CH4 (XCH4) due to uncertainties in the aerosol optical properties and atmospheric a priori profiles are less than 1 % on average. This indicates that atmospheric scattering does not induce a large bias in the retrievals when the aerosols are properly characterized. The methodology is then further evaluated by comparing GHG retrievals using GFIT3 with those obtained from the CLARS-GFIT algorithm (used for currently operational CLARS retrievals) that does not account for aerosol scattering. We find a significant correlation between retrieval bias and aerosol optical depth (AOD). A comparison of GFIT3 AOD retrievals with collocated ground-based observations from AErosol RObotic NETwork (AERONET) shows that the developed algorithm produces very accurate results, with biases in AOD estimates of about 0.02. Finally, we assess the uncertainty in the widely used tracer–tracer ratio method to obtain CH4 emissions based on CO2 emissions and find that using the CH4/CO2 ratio effectively cancels out biases due to aerosol scattering. Overall, this study of applying GFIT3 to CLARS-FTS observations improves our understanding of the impact of aerosol scattering on the remote sensing of GHGs in polluted urban atmospheric environments. GHG retrievals from CLARS-FTS are potentially complementary to existing ground-based and spaceborne observations to monitor anthropogenic GHG fluxes in megacities.


2016 ◽  
Author(s):  
Andreas Reichert ◽  
Markus Rettinger ◽  
Ralf Sussmann

Abstract. Quantitative knowledge of water vapor absorption is crucial for accurate climate simulations. An open science question in this context concerns the strength of the water vapor continuum in the near infrared (NIR) at atmospheric temperatures, which is still to be quantified by measurements. This issue can be addressed with radiative closure experiments using solar absorption spectra. However, the spectra used for water vapor continuum quantification have to be radiometrically calibrated. We present for the first time a method that yields sufficient calibration accuracy for NIR water vapor continuum quantification in an atmospheric closure experiment. Our method combines the Langley method with spectral radiance measurements of a high-temperature blackbody calibration source (< 2000 K). The calibration scheme is demonstrated in the spectral range 2500 to 7800 cm−1, but minor modifications to the method enable calibration also throughout the remainder of the NIR spectral range. The resulting uncertainty (2 σ) is below 1 % in window regions and up to 1.7 % within absorption bands. A validation of this calibration uncertainty estimate is performed by investigation of calibration self-consistency, which yields compatible results within the estimated errors for 91.1 % of the 2500 to 7800 cm−1-range. A second validation effort consists in a comparison of a set of calibrated spectra to radiative transfer model calculations, which are consistent within the estimated errors for 97.7 % of the spectral range.


2009 ◽  
Vol 5 (2) ◽  
pp. 1133-1162 ◽  
Author(s):  
A. N. LeGrande ◽  
G. A. Schmidt

Abstract. Variability in water isotopes has been captured in numerous archives and used to infer climate change. Here we examine water isotope variability over the course of the Holocene using the water-isotope enabled, coupled atmosphere-ocean general circulation model, GISS ModelE-R. Eight Holocene time slices, mostly 1000 years apart are simulated using estimated changes in orbital configuration, greenhouse gases, and ice sheet extent. We find that water isotopes in the model match well with those captured in proxy climate archives in ice cores, ocean sediment cores, and speleothems. The climate changes associated with the water isotope changes, however, are more complex than simple modern analog interpretations. In particular, water isotope variability in Asian speleothems is linked to alterations in landward water vapor transport, not local precipitation, and ice sheet changes over North America lead to masking of temperature signals in Summit, Greenland. Salinity-seawater isotope variability is complicated by inter-ocean basin exchanges of water vapor. Water isotopes do reflect variability in the hydrologic cycle, but are better interpreted in terms of regional changes rather than local climate variables.


2020 ◽  
Vol 10 (1) ◽  
Author(s):  
Xiaoxin Yang ◽  
Tandong Yao

Abstract This study integrated isotopic composition in precipitation at 50 stations on and around the Tibetan Plateau (TP) and demonstrated the distinct seasonality of isotopic composition in precipitation across the study period. The potential effect of water vapor isotopes on precipitation isotopes is studied by comparing the station precipitation data with extensive isotopic patterns in atmospheric water vapor, revealing the close linkage between the two. The analysis of contemporary water vapor transport and potential helps confirm the different mechanisms behind precipitation isotopic compositions in different areas, as the southern TP is more closely related to large-scale atmospheric circulation such as local Hadley and summer monsoon circulations during other seasons than winter, while the northern TP is subject to the westerly prevalence and advective moisture supply and precipitation processes. The new data presented in this manuscript also enrich the current dataset for the study of precipitation isotopes in this region and together provide a valuable database for verification of the isotope-integrated general circulation model and explanation of related physical processes.


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