scholarly journals The global methane budget 2000–2012

2016 ◽  
Vol 8 (2) ◽  
pp. 697-751 ◽  
Author(s):  
Marielle Saunois ◽  
Philippe Bousquet ◽  
Ben Poulter ◽  
Anna Peregon ◽  
Philippe Ciais ◽  
...  

Abstract. The global methane (CH4) budget is becoming an increasingly important component for managing realistic pathways to mitigate climate change. This relevance, due to a shorter atmospheric lifetime and a stronger warming potential than carbon dioxide, is challenged by the still unexplained changes of atmospheric CH4 over the past decade. Emissions and concentrations of CH4 are continuing to increase, making CH4 the second most important human-induced greenhouse gas after carbon dioxide. Two major difficulties in reducing uncertainties come from the large variety of diffusive CH4 sources that overlap geographically, and from the destruction of CH4 by the very short-lived hydroxyl radical (OH). To address these difficulties, we have established a consortium of multi-disciplinary scientists under the umbrella of the Global Carbon Project to synthesize and stimulate research on the methane cycle, and producing regular (∼ biennial) updates of the global methane budget. This consortium includes atmospheric physicists and chemists, biogeochemists of surface and marine emissions, and socio-economists who study anthropogenic emissions. Following Kirschke et al. (2013), we propose here the first version of a living review paper that integrates results of top-down studies (exploiting atmospheric observations within an atmospheric inverse-modelling framework) and bottom-up models, inventories and data-driven approaches (including process-based models for estimating land surface emissions and atmospheric chemistry, and inventories for anthropogenic emissions, data-driven extrapolations). For the 2003–2012 decade, global methane emissions are estimated by top-down inversions at 558 Tg CH4 yr−1, range 540–568. About 60 % of global emissions are anthropogenic (range 50–65 %). Since 2010, the bottom-up global emission inventories have been closer to methane emissions in the most carbon-intensive Representative Concentrations Pathway (RCP8.5) and higher than all other RCP scenarios. Bottom-up approaches suggest larger global emissions (736 Tg CH4 yr−1, range 596–884) mostly because of larger natural emissions from individual sources such as inland waters, natural wetlands and geological sources. Considering the atmospheric constraints on the top-down budget, it is likely that some of the individual emissions reported by the bottom-up approaches are overestimated, leading to too large global emissions. Latitudinal data from top-down emissions indicate a predominance of tropical emissions (∼ 64 % of the global budget, < 30° N) as compared to mid (∼ 32 %, 30–60° N) and high northern latitudes (∼ 4 %, 60–90° N). Top-down inversions consistently infer lower emissions in China (∼ 58 Tg CH4 yr−1, range 51–72, −14 %) and higher emissions in Africa (86 Tg CH4 yr−1, range 73–108, +19 %) than bottom-up values used as prior estimates. Overall, uncertainties for anthropogenic emissions appear smaller than those from natural sources, and the uncertainties on source categories appear larger for top-down inversions than for bottom-up inventories and models. The most important source of uncertainty on the methane budget is attributable to emissions from wetland and other inland waters. We show that the wetland extent could contribute 30–40 % on the estimated range for wetland emissions. Other priorities for improving the methane budget include the following: (i) the development of process-based models for inland-water emissions, (ii) the intensification of methane observations at local scale (flux measurements) to constrain bottom-up land surface models, and at regional scale (surface networks and satellites) to constrain top-down inversions, (iii) improvements in the estimation of atmospheric loss by OH, and (iv) improvements of the transport models integrated in top-down inversions. The data presented here can be downloaded from the Carbon Dioxide Information Analysis Center (http://doi.org/10.3334/CDIAC/GLOBAL_METHANE_BUDGET_2016_V1.1) and the Global Carbon Project.

2020 ◽  
Vol 12 (3) ◽  
pp. 1561-1623 ◽  
Author(s):  
Marielle Saunois ◽  
Ann R. Stavert ◽  
Ben Poulter ◽  
Philippe Bousquet ◽  
Josep G. Canadell ◽  
...  

Abstract. Understanding and quantifying the global methane (CH4) budget is important for assessing realistic pathways to mitigate climate change. Atmospheric emissions and concentrations of CH4 continue to increase, making CH4 the second most important human-influenced greenhouse gas in terms of climate forcing, after carbon dioxide (CO2). The relative importance of CH4 compared to CO2 depends on its shorter atmospheric lifetime, stronger warming potential, and variations in atmospheric growth rate over the past decade, the causes of which are still debated. Two major challenges in reducing uncertainties in the atmospheric growth rate arise from the variety of geographically overlapping CH4 sources and from the destruction of CH4 by short-lived hydroxyl radicals (OH). To address these challenges, we have established a consortium of multidisciplinary scientists under the umbrella of the Global Carbon Project to synthesize and stimulate new research aimed at improving and regularly updating the global methane budget. Following Saunois et al. (2016), we present here the second version of the living review paper dedicated to the decadal methane budget, integrating results of top-down studies (atmospheric observations within an atmospheric inverse-modelling framework) and bottom-up estimates (including process-based models for estimating land surface emissions and atmospheric chemistry, inventories of anthropogenic emissions, and data-driven extrapolations). For the 2008–2017 decade, global methane emissions are estimated by atmospheric inversions (a top-down approach) to be 576 Tg CH4 yr−1 (range 550–594, corresponding to the minimum and maximum estimates of the model ensemble). Of this total, 359 Tg CH4 yr−1 or ∼ 60 % is attributed to anthropogenic sources, that is emissions caused by direct human activity (i.e. anthropogenic emissions; range 336–376 Tg CH4 yr−1 or 50 %–65 %). The mean annual total emission for the new decade (2008–2017) is 29 Tg CH4 yr−1 larger than our estimate for the previous decade (2000–2009), and 24 Tg CH4 yr−1 larger than the one reported in the previous budget for 2003–2012 (Saunois et al., 2016). Since 2012, global CH4 emissions have been tracking the warmest scenarios assessed by the Intergovernmental Panel on Climate Change. Bottom-up methods suggest almost 30 % larger global emissions (737 Tg CH4 yr−1, range 594–881) than top-down inversion methods. Indeed, bottom-up estimates for natural sources such as natural wetlands, other inland water systems, and geological sources are higher than top-down estimates. The atmospheric constraints on the top-down budget suggest that at least some of these bottom-up emissions are overestimated. The latitudinal distribution of atmospheric observation-based emissions indicates a predominance of tropical emissions (∼ 65 % of the global budget, < 30∘ N) compared to mid-latitudes (∼ 30 %, 30–60∘ N) and high northern latitudes (∼ 4 %, 60–90∘ N). The most important source of uncertainty in the methane budget is attributable to natural emissions, especially those from wetlands and other inland waters. Some of our global source estimates are smaller than those in previously published budgets (Saunois et al., 2016; Kirschke et al., 2013). In particular wetland emissions are about 35 Tg CH4 yr−1 lower due to improved partition wetlands and other inland waters. Emissions from geological sources and wild animals are also found to be smaller by 7 Tg CH4 yr−1 by 8 Tg CH4 yr−1, respectively. However, the overall discrepancy between bottom-up and top-down estimates has been reduced by only 5 % compared to Saunois et al. (2016), due to a higher estimate of emissions from inland waters, highlighting the need for more detailed research on emissions factors. Priorities for improving the methane budget include (i) a global, high-resolution map of water-saturated soils and inundated areas emitting methane based on a robust classification of different types of emitting habitats; (ii) further development of process-based models for inland-water emissions; (iii) intensification of methane observations at local scales (e.g., FLUXNET-CH4 measurements) and urban-scale monitoring to constrain bottom-up land surface models, and at regional scales (surface networks and satellites) to constrain atmospheric inversions; (iv) improvements of transport models and the representation of photochemical sinks in top-down inversions; and (v) development of a 3D variational inversion system using isotopic and/or co-emitted species such as ethane to improve source partitioning. The data presented here can be downloaded from https://doi.org/10.18160/GCP-CH4-2019 (Saunois et al., 2020) and from the Global Carbon Project.


2016 ◽  
Author(s):  
Marielle Saunois ◽  
Philippe Bousquet ◽  
Ben Poulter ◽  
Anna Peregon ◽  
Philippe Ciais ◽  
...  

Abstract. The global methane (CH4) budget is becoming an increasingly important component for managing realistic pathways to mitigate climate change. This relevance, due to a shorter atmospheric lifetime and a stronger warming potential than carbon dioxide, is challenged by the still unexplained changes of atmospheric CH4 over the past decade. Emissions and concentrations of CH4 are continuing to increase making CH4 the second most important human-induced greenhouse gas after carbon dioxide. Two major difficulties in reducing uncertainties come from the large variety of diffusive CH4 sources that overlap geographically, and from the destruction of CH4 by the very short-lived hydroxyl radical (OH). To address these difficulties, we have established a consortium of multi-disciplinary scientists under the umbrella of the Global Carbon Project to synthesize and stimulate research on the methane cycle, and producing regular (~biennial) updates of the global methane budget. This consortium includes atmospheric physicists and chemists, biogeochemists of surface and marine emissions, and socio-economists who study anthropogenic emissions. Following Kirschke et al. (2013), we propose here the first version of a living review paper that integrates results of top-down studies (T-D, exploiting atmospheric observations within an atmospheric inverse-modelling framework) and bottom-up models, inventories, and data-driven approaches (B-U, including process-based models for estimating land surface emissions and atmospheric chemistry, and inventories for anthropogenic emissions, data-driven extrapolations). For the 2003–2012 decade, global methane emissions are estimated by T-D inversions at 558 Tg CH4 yr−1 (range [540–568]). About 60 % of global emissions are anthropogenic (range [50–65 %]). B-U approaches suggest larger global emissions (736 Tg CH4 yr−1 [596–884]) mostly because of larger natural emissions from individual sources such as inland waters, natural wetlands and geological sources. Considering the atmospheric constraints on the T-D budget, it is likely that some of the individual emissions reported by the B-U approaches are overestimated, leading to too large global emissions. Latitudinal data from T-D emissions indicate a predominance of tropical emissions (~64 % of the global budget,


2017 ◽  
Author(s):  
Robbie M. Andrew

Abstract. Global production of cement has grown very rapidly in recent years, and after fossil fuels and land-use change, it is the third-largest source of anthropogenic emissions of carbon dioxide. The required data for estimating emissions from global cement production are poor, and it has been recognised that some global estimates are significantly inflated. Here we assemble a large variety of available datasets, prioritising official data and emission factors, including estimates submitted to the UNFCCC plus new estimates for China and India, to present a new analysis of global process emissions from cement production. We show that global emissions in 2016 were 1.45 ± 0.20 Gt CO2, equivalent to about 4 % of emissions from fossil fuels. Cumulative emissions to 2016 were 39.3 ± 2.6 Gt CO2, 66 % of which have occurred since 1990. Emissions in 2015 were 30 % lower than those recently reported by the Global Carbon Project. The data associated with this article can be found at https://doi.org/10.5281/zenodo.831455.


2021 ◽  
Vol 8 (1) ◽  
Author(s):  
Matthew W. Jones ◽  
Robbie M. Andrew ◽  
Glen P. Peters ◽  
Greet Janssens-Maenhout ◽  
Anthony J. De-Gol ◽  
...  

AbstractQuantification of CO2 fluxes at the Earth’s surface is required to evaluate the causes and drivers of observed increases in atmospheric CO2 concentrations. Atmospheric inversion models disaggregate observed variations in atmospheric CO2 concentration to variability in CO2 emissions and sinks. They require prior constraints fossil CO2 emissions. Here we describe GCP-GridFED (version 2019.1), a gridded fossil emissions dataset that is consistent with the national CO2 emissions reported by the Global Carbon Project (GCP). GCP-GridFEDv2019.1 provides monthly fossil CO2 emissions estimates for the period 1959–2018 at a spatial resolution of 0.1°. Estimates are provided separately for oil, coal and natural gas, for mixed international bunker fuels, and for the calcination of limestone during cement production. GCP-GridFED also includes gridded estimates of O2 uptake based on oxidative ratios for oil, coal and natural gas. It will be updated annually and made available for atmospheric inversions contributing to GCP global carbon budget assessments, thus aligning the prior constraints on top-down fossil CO2 emissions with the bottom-up estimates compiled by the GCP.


2019 ◽  
Author(s):  
Marielle Saunois ◽  
Ann R. Stavert ◽  
Ben Poulter ◽  
Philippe Bousquet ◽  
Joseph G. Canadell ◽  
...  

Abstract. Understanding and quantifying the global methane (CH4) budget is important for assessing realistic pathways to mitigate climate change. Atmospheric emissions and concentrations of CH4 are continuing to increase, making CH4 the second most important human-influenced greenhouse gas in terms of climate forcing, after carbon dioxide (CO2). Assessing the relative importance of CH4 in comparison to CO2 is complicated by its shorter atmospheric lifetime, stronger warming potential, and atmospheric growth rate variations over the past decade, the causes of which are still debated. Two major difficulties in reducing uncertainties arise from the variety of geographically overlapping CH4 sources and from the destruction of CH4 by short-lived hydroxyl radicals (OH). To address these difficulties, we have established a consortium of multi-disciplinary scientists under the umbrella of the Global Carbon Project to synthesize and stimulate new research aimed at improving and regularly updating the global methane budget. Following Saunois et al. (2016), we present here the second version of the living review paper dedicated to the decadal methane budget, integrating results of top-down studies (atmospheric observations within an atmospheric inverse-modelling framework) and bottom-up estimates (including process-based models for estimating land surface emissions and atmospheric chemistry, inventories of anthropogenic emissions, and data-driven extrapolations). For the 2008–2017 decade, global methane emissions are estimated by atmospheric inversions (top-down approach) to be 572 Tg CH4 yr−1 (range 538–593, corresponding to the minimum and maximum estimates of the ensemble), of which 357 Tg CH4 yr−1 or ~ 60 % are attributed to anthropogenic sources (range 50–65 %). This total emission is 27 Tg CH4 yr−1 larger than the value estimated for the period 2000–2009 and 24 Tg CH4 yr−1 larger than the one reported in the previous budget for the period 2003–2012 (Saunois et al. 2016). Since 2012, global CH4 emissions have been tracking the carbon intensive scenarios developed by the Intergovernmental Panel on Climate Change (Gidden et al., 2019). Bottom-up methods suggest larger global emissions (737 Tg CH4 yr−1, range 583–880) than top-down inversion methods, mostly because of larger estimated natural emissions from sources such as natural wetlands, other inland water systems, and geological sources. However the strength of the atmospheric constraints on the top-down budget, suggest that these bottom-up emissions are overestimated. The latitudinal distribution of atmospheric-based emissions indicates a predominance of tropical emissions (~ 65 % of the global budget,


2021 ◽  
Author(s):  
Emily Dowd ◽  
Christopher Wilson ◽  
Martyn Chipperfield ◽  
Manuel Gloor

&lt;p&gt;Methane (CH&lt;sub&gt;4&lt;/sub&gt;) is the second most important atmospheric greenhouse gas after carbon dioxide. Global concentrations of CH&lt;sub&gt;4&lt;/sub&gt; have been rising in the last decade and our understanding of what is driving the increase remains incomplete. Natural sources, such as wetlands, contribute to the uncertainty of the methane budget. However, anthropogenic sources, such as fossil fuels, present an opportunity to mitigate the human contribution to climate change on a relatively short timescale, since CH&lt;sub&gt;4&lt;/sub&gt; has a much shorter lifetime than carbon dioxide. Therefore, it is important to know the relative contributions of these sources in different regions.&lt;/p&gt;&lt;p&gt;We have investigated the inter-annual variation (IAV) and rising trend of CH&lt;sub&gt;4&lt;/sub&gt; concentrations using a global 3-D chemical transport model, TOMCAT. We independently tagged several regional natural and anthropogenic CH&lt;sub&gt;4&lt;/sub&gt; tracers in TOMCAT to identify their contribution to the atmospheric CH&lt;sub&gt;4&lt;/sub&gt; concentrations over the period 2009 &amp;#8211; 2018. The tagged regions were selected based on the land surface types and the predominant flux sector within each region and include subcontinental regions, such as tropical South America, boreal regions and anthropogenic regions such as Europe. We used surface CH&lt;sub&gt;4&lt;/sub&gt; fluxes derived from a previous TOMCAT-based atmospheric inversion study (Wilson et al., 2020). These atmospheric inversions were constrained by satellite and surface flask observations of CH&lt;sub&gt;4&lt;/sub&gt;, giving optimised monthly estimates for fossil fuel and non-fossil fuel emissions on a 5.6&amp;#176; horizontal grid. During the study period, the total optimised CH&lt;sub&gt;4&lt;/sub&gt; flux grew from 552 Tg/yr to 593 Tg/yr. This increase in emissions, particularly in the tropics, contributed to the increase in atmospheric CH&lt;sub&gt;4 &lt;/sub&gt;concentrations and added to the imbalance in the CH&lt;sub&gt;4&lt;/sub&gt; budget. We will use the results of the regional tagged tracers to quantify the contribution of regional methane emissions at surface observation sites, and to quantify the contributions of the natural and anthropogenic emissions from the tagged regions to the IAV and the rising methane concentrations.&lt;/p&gt;&lt;p&gt;Wilson, C., Chipperfield, M. P., Gloor, M., Parker, R. J., Boesch, H., McNorton, J., Gatti, L. V., Miller, J. B., Basso, L. S., and Monks, S. A.: Large and increasing methane emissions from Eastern Amazonia derived from satellite data, 2010&amp;#8211;2018, Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2020-1136, in review, 2020.&lt;/p&gt;


2016 ◽  
Author(s):  
Francesco Graziosi ◽  
Jgor Arduini ◽  
Paolo Bonasoni ◽  
Francesco Furlani ◽  
Umberto Giostra ◽  
...  

Abstract. Carbon tetrachloride (CCl4) is a long-lived radiatively-active compound able to destroy stratospheric ozone. Due to its inclusion in the Montreal Protocol on Substances that Deplete the Ozone Layer, the last two decades have seen a sharp decrease in its large scale emissive use with a consequent decline of its atmospheric mole fractions. However, the Montreal Protocol restrictions do not apply to the use of carbon tetrachloride as feedstock for the production of other chemicals, implying the risk of fugitive emissions from the industry sector. The occurrence of such unintended emissions is suggested by a significant discrepancy between global emissions as derived by reported production and feedstock usage (bottom-up emissions), and those based on atmospheric observations (top-down emissions). In order to better constrain the atmospheric budget of carbon tetrachloride, several studies based on a combination of atmospheric observations and inverse modelling have been conducted in recent years in various regions of the world. This study is focused on the European scale and based on long-term high-frequency observations at three European sites, combined with a Bayesian inversion methodology. We estimated that average European emissions for 2006–2014 were 2.3 (± 0.8) Gg yr−1, with an average decreasing trend of 7.3 % per year. Our analysis identified France as the main source of emissions over the whole study period, with an average contribution to total European emissions of 25 %. The inversion was also able to allow the localisation of emission "hot-spots" in the domain, with major source areas in Southern France, Central England (UK) and Benelux (Belgium, The Netherlands, Luxembourg), where most of industrial scale production of basic organic chemicals are located. According to our results, European emissions correspond to 4.0 % of global emissions for 2006–2012. Together with other regional studies, our results allow a better constraint of the global budget of carbon tetrachloride and a better quantification of the gap between top-down and bottom-up estimates.


2003 ◽  
Vol 33 (3) ◽  
pp. 480-489 ◽  
Author(s):  
Boris Zeide

So far, process-based models use largely the bottom-up approach. They start by describing physiological processes in a single plant element and then integrate the constituent processes to predict growth and dimensions of the tree and stand. Although bottom-up process models are praised for their contribution to knowledge of growth processes, their predictions are poor. The complementary top-down approach begins where the bottom-up model ends: with measurable variables such as height or diameter. This approach intends to uncover the ecophysiological processes responsible for the observed tree dimensions rather than to provide growth information for forest management. As foresters, we would like to utilize measurable variables to uncover inner mechanisms of growth in hope of predicting future diameter, number of trees, volume, and other practical variables. This means that we need to combine the top-down and bottom-up approaches. Examples of the united U-approach (so called because of its descending and ascending branches) are described. They demonstrate that growth models can be both meaningful and accurate.


2020 ◽  
Author(s):  
Gesa Meyer ◽  
Elyn R. Humphreys ◽  
Joe R. Melton ◽  
Alex J. Cannon ◽  
Peter M. Lafleur

Abstract. The Arctic is warming more rapidly than other regions of the world leading to ecosystem change including shifts in vegetation communities, permafrost degradation and alteration of tundra surface-atmosphere energy and carbon (C) fluxes, among others. However, year-round C and energy flux measurements at high-latitude sites remain rare. This poses a challenge for evaluating the impacts of climate change on Arctic tundra ecosystems and for developing and evaluating process-based models, which may be used to predict regional and global energy and C feedbacks to the climate system. Our study used 14 years of seasonal eddy covariance (EC) measurements of carbon dioxide (CO2), water and energy fluxes and winter soil chamber CO2 flux measurements at a dwarf-shrub tundra site underlain by continuous permafrost in Canada's Southern Arctic ecozone to evaluate the incorporation of shrub plant functional types (PFTs) in the Canadian Land Surface Scheme Including biogeochemical Cycles (CLASSIC), the land surface component of the Canadian Earth System Model. In addition to new PFTs, a modification of the efficiency with which water evaporates from the ground surface was applied. This modification addressed a high ground evaporation bias that reduced model performance when soils became very dry, limited heat flow into the ground and reduced plant productivity through water stress effects. Compared to the grass and tree PFTs previously used by CLASSIC to represent the vegetation in Arctic permafrost-affected regions, simulations with the new shrub PFTs better capture the physical and biogeochemical impact of shrubs on the magnitude and seasonality of energy and CO2 fluxes at the dwarf-shrub tundra evaluation site. The revised model, however, tends to overestimate gross primary productivity, particularly in spring, and overestimated late winter CO2 emissions. On average, annual net ecosystem CO2 exchange was positive for all simulations, suggesting this site was a net CO2 source of 18 ± 4 g C m−2 year−1 using shrub PFTs, 15 ± 6 g C m−2 year−1 using grass PFTs, and 25 ± 5 g C m−2 year−1 using tree PFTs. These results highlight the importance of using appropriate PFTs in process-based models to simulate current and future Arctic surface-atmosphere interactions.


2020 ◽  
Author(s):  
Gilles Y. Brocard ◽  
Jane K. Willenbring ◽  
Tristan Salles ◽  
Michael Cosca ◽  
Axel Guttiérez-Orrego ◽  
...  

Abstract. The presence of a mountain affects the circulation of water in the atmosphere and over the land surface. These effects are felt over some distance, beyond the extent of the mountain, controlling precipitation delivery and river incision over surrounding landmasses. The rise of a new mountain range therefore affects the erosion of pre-existing mountains located in close proximity. We document here this phenomenon in the mountains of Central Guatemala. The 40Ar-39Ar dating of lava flows shows that two parallel, closely spaced mountain ranges formed during two consecutive pulses of single-stepped uplift, one from 12 to 7 Ma, and the second one since 7 Ma. The distribution of erosion rates derived from the analysis of detrital cosmogenic 10Be in river sediments shows that the younger range erodes faster (~300 m/My) than the older one (20–150 m/My), and that erosion correlates with the amount of precipitation. Moisture tracking form the Caribbean Sea is intercepted by the younger range, which casts a rain shadow over the older one. The analysis of river long-profiles provides a record of longer-term interactions between the two ranges. The rivers that drain the older range were diverted by the younger range during the early stages of its rise. A few rivers were able to maintain their course across the young range, through profile steepening, but incision completely stalled along their upper reaches, upstream of the younger range. As a result, the older range has been passively uplifted, and entered a phase of a slow topographic decay: pediments have formed along its base, while ancient upstream-migrating waves of erosion, located farther up the mountain flanks, have almost stopped migrating. Aridification and cessation of river incision together explain the slowing down of erosion over the older range. They represent top-down and bottom-up processes whereby the younger range controls erosion over the older one. These controls are regarded as instrumental in the nucleation and enlargement of orogenic plateaus forming above continental accretionary wedges.


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