scholarly journals Quantification of the radiative impact of light-absorbing particles during two contrasted snow seasons at Col du Lautaret (2058 m a.s.l., French Alps)

2020 ◽  
Vol 14 (12) ◽  
pp. 4553-4579
Author(s):  
François Tuzet ◽  
Marie Dumont ◽  
Ghislain Picard ◽  
Maxim Lamare ◽  
Didier Voisin ◽  
...  

Abstract. The presence of light-absorbing particles (LAPs) in snow leads to a decrease in short-wave albedo affecting the surface energy budget. However, the understanding of the impacts of LAPs is hampered by the lack of dedicated datasets, as well as the scarcity of models able to represent the interactions between LAPs and snow metamorphism. The present study aims to address both these limitations by introducing a survey of LAP concentrations over two snow seasons in the French Alps and an estimation of their impacts based on the Crocus snowpack model that represents the complex interplays between LAP dynamics and snow metamorphism. First, a unique dataset collected at Col du Lautaret (2058 m a.s.l., above sea level, French Alps) for the two snow seasons 2016–2017 and 2017–2018 is presented. This dataset consists of spectral albedo measurements, vertical profiles of snow specific surface area (SSA), density and concentrations of different LAP species. Spectral albedos are processed to estimate SSA and LAP absorption-equivalent concentrations near the surface of the snowpack. These estimates are then compared to chemical measurements of LAP concentrations and SSA measurements. Our dataset highlights, among others, large discrepancies between two measurement techniques of black carbon (BC) concentrations in snow (namely thermal-optical and laser-induced incandescence). Second, we present ensemble snowpack simulations of the multi-physics version of the detailed snowpack model Crocus, forced with in situ meteorological data, as well as dust and BC deposition fluxes from an atmospheric model. The temporal variations of near-surface LAP concentrations and SSA are most of the time correctly simulated. The simulated seasonal radiative forcing of LAPs is 33 % higher for the 2017–2018 snow season than for the 2016–2017 one, highlighting a strong variability between these two seasons. However, the shortening of the snow season caused by LAPs is similar with 10 ± 5 and 11 ± 1 d for the first and the second snow seasons, respectively. This counter-intuitive result is attributed to two small snowfalls at the end of the first season and highlights the importance in accounting for meteorological conditions to correctly predict the impact of LAPs. The strong variability of season shortening caused by LAPs in the multi-physics ensemble for the first season (10 ± 5 d) also points out the sensitivity of model-based estimations of LAP impact on modelling uncertainties of other processes. Finally, the indirect impact of LAPs (i.e. the enhancement of energy absorption due to the acceleration of the metamorphism by LAPs) is negligible for the 2 years considered here, which is contrary to what was found in previous studies for other sites.

2020 ◽  
Author(s):  
François Tuzet ◽  
Marie Dumont ◽  
Ghislain Picard ◽  
Maxim Lamare ◽  
Didier Voisin ◽  
...  

Abstract. The presence of light-absorbing particles (LAPs) in snow leads to a decrease in shortwave albedo, affecting the surface energy budget. Precisely quantifying the impacts of LAPs on snowpack evolution is crucial to characterise the spatio-temporal variability of snowmelt and assess snow albedo feedbacks in detail. However, the understanding of the impacts of LAPs is hampered by the lack of dedicated datasets, as well as the scarcity of models able to represent the interactions between LAPs and snow metamorphism. The present study aims to address both these limitations by introducing a survey of LAP concentrations over two snow seasons in the French Alps, as well as an estimation of their impacts based on the Crocus snowpack model that represents the complex interplays between LAP dynamics and snow metamorphism. First, we present a unique dataset collected at the Col du Lautaret (2058 m a.s.l; French Alps) for the two snow seasons 2016–2017 and 2017–2018. This dataset consists of spectral albedo measurements (manual and automated), vertical profiles of snow specific surface area (SSA), density, and concentrations of refractive Black Carbon (rBC), Elemental Carbon (EC) and mineral dust. Spectral albedo data are processed to estimate near-surface SSA and LAP absorption-equivalent concentrations near the surface of the snowpack. These estimates are then compared to chemical measurements of dust and BC concentrations, as well as to SSA measurements acquired by near-infrared reflectometry. Our dataset highlights large discrepancies between the two measurement techniques of BC concentrations, with EC concentrations being one order of magnitude higher than rBC measurements. In view of LAP absorption inferred from albedo measurements, the mass absorption efficiency (MAE) of BC used in our study (11.25 g m−2 at 550 nm) is more appropriate for EC measurements than for rBC ones. Second, we present ensemble snowpack simulations of ESCROC – the multi-physics version of the detailed snowpack model Crocus – forced with in-situ meteorological data as well as dust and BC deposition fluxes from the ALADIN-Climate atmospheric model. The results of these simulations are compared to the near-surface properties estimated from automatic albedo measurements, showing that the temporal variations of near-surface LAP concentration and SSA are correctly reproduced. The impact of dust and BC on our simulations is estimated by comparing this ensemble to a similar ensemble that does not account for LAPs. The seasonal radiative forcing of LAPs is 1.33 times higher for the 2017–2018 snow season than for the 2016–2017 one, highlighting a strong variability between these two seasons. However, the shortening of the snow season caused by LAPs are similar with 10 ± 5 and 11 ± 1 days for the first and the second snow seasons respectively. This counter-intuitive result is attributed to two small snowfalls at the end of the first season and highlights the importance to account for meteorological conditions to correctly predict the impact of LAPs. The strong variability of season shortening caused by LAPs in the multi-physics ensemble for the first season also points out the sensitivity of model-based estimations of LAP impact to modelling uncertainties of other processes. Finally, the indirect impact of LAPs (i.e. the enhancement of energy absorption due to acceleration of the metamorphism by LAPs) is negligible for the two years considered here, contrary to what was found in previous studies for other sites. This finding is mainly attributed to the meteorological conditions of the two studied snow seasons.


2020 ◽  
Author(s):  
Louis Le Toumelin ◽  
Charles Amory ◽  
Vincent Favier ◽  
Christoph Kittel ◽  
Stefan Hofer ◽  
...  

Abstract. In order to understand the evolution of the climate of Antarctica, dominant processes that control surface and low-atmosphere meteorology need to be accurately captured in climate models. We used the regional climate model MAR (v3.11) at 10 km horizontal resolution, forced by ERA5 reanalysis over a 9-year period (2010–2018), to study the impact of drifting snow (designing here the wind-driven transport of snow particles below and above 2 m) on the near-surface atmosphere and surface in Adelie Land, East Antarctica. Two model runs were performed, respectively with and without drifting snow, and compared to half-hourly in situ observations at D17, a coastal and windy location of Adelie Land. We show that sublimation of drifting-snow particles in the atmosphere drives the difference between model runs and is responsible for significant impacts on the near-surface atmosphere. By cooling the low atmosphere and increasing its relative humidity, drifting snow also reduces sensible and latent heat exchanges at the surface (−5.9 W m−2 on average). Moreover, large and dense drifting-snow layers act as near-surface cloud by interacting with incoming radiative fluxes, enhancing incoming longwave radiations and reducing incoming shortwave radiations in summer (net radiative forcing: 5.9 W m−2). Even if drifting snow modifies these processes involved in surface-atmosphere interactions, the total surface energy budget is only slightly modified by introducing drifting snow, because of compensating effects in surface energy fluxes. The drifting-snow driven effects are not prominent near the surface but peak higher in the boundary layer (fifth vertical level, 38 m) where drifting snow sublimation is the most pronounced. Accounting for drifting snow in MAR generally improves the comparison at D17, more especially for the representation of relative humidity (mean bias reduced from −11.1 % to 2.9 %) and incoming longwave radiation (mean bias reduced from −7.6 W m−2 to −1.5 W m−2). Consequently, our results suggest that a detailed representation of drifting-snow processes is required in climate models to better capture the near–surface meteorology and surface–atmosphere interactions in coastal Adelie Land.


2015 ◽  
Vol 15 (23) ◽  
pp. 13633-13646 ◽  
Author(s):  
B. L. Zhuang ◽  
T. J. Wang ◽  
J. Liu ◽  
Y. Ma ◽  
C. Q. Yin ◽  
...  

Abstract. Absorbing aerosols can significantly modulate short-wave solar radiation in the atmosphere, affecting regional and global climate. The aerosol absorption coefficient (AAC) is an indicator that assesses the impact of absorbing aerosols on radiative forcing. In this study, the near-surface AAC and absorption Ångström exponent (AAE) in the urban area of Nanjing, China, are characterized on the basis of measurements in 2012 and 2013 using the seven-channel Aethalometer (model AE-31, Magee Scientific, USA). The AAC is estimated with direct and indirect corrections, which result in consistent temporal variations and magnitudes of AAC at 532 nm. The mean AAC at 532 nm is about 43.23 ± 28.13 M m−1 in the urban area of Nanjing, which is much lower than that in Pearl River Delta and the same as in rural areas (Lin'an) in Yangtze River Delta. The AAC in the urban area of Nanjing shows strong seasonality (diurnal variations); it is high in cold seasons (at rush hour) and low in summer (in the afternoon). It also shows synoptic and quasi-2-week cycles in response to weather systems. Its frequency distribution follows a typical log-normal pattern. The 532 nm AAC ranging from 15 to 65 M m−1 dominates, accounting for more than 72 % of the total data samples in the entire study period. Frequent high pollution episodes, such as those observed in June 2012 and in winter 2013, greatly enhanced AAC and altered its temporal variations and frequency distributions. These episodes are mostly due to local emissions and regional pollution. Air masses flowing from northern China to Nanjing can sometimes be highly polluted and lead to high AAC at the site. AAE at 660/470 nm from the Schmid correction (Schmid et al., 2006) is about 1.56, which might be more reasonable than from the Weingartner correction (Weingartner et al., 2003). Low AAEs mainly occur in summer, likely due to high relative humidity (RH) in the season. AAC increases with increasing AAE at a fixed aerosol loading. The RH–AAC relationship is more complex. Overall, AAC peaks at RH values of around 40 % (1.3 < AAE < 1.6), 65 % (AAE < 1.3 and AAE > 1.6), and 80 % (1.3 < AAE < 1.6).


2019 ◽  
Author(s):  
Gaurav Govardhan ◽  
Sreedharan Krishnakumari Satheesh ◽  
Krishnaswamy Krishna Moorthy ◽  
Ravi Nanjundiah

Abstract. With a view to improving the performance of WRF-Chem over the Indian region in simulating BC (black Carbon) mass concentrations as well as its short-term variations, especially on diurnal scale, a region-specific diurnal variation scheme has been introduced in the model emissios and the performance of the modified simulations has been evaluated against high-resolution measurements carried out over 8 ARFI (Aerosol Radiative Forcing over India) network observatories spread across India for distinct seasons; pre-monsoon (represented by May), post-monsoon (represented by October) and winter (represented by December). In addition to an overall improvement in the simulated concentrations and their temporal variations, it has also been found that the effects of prescribing diurnally varying emissions on the simulated near-surface concentrations largely depend on the boundary layer turbulence. The effects are perceived fast (within about 2–3 hours) during the evening–early morning hours when the atmospheric boundary layer is shallow and convective mixing is weak, while they are delayed, taking as much as about 5–6 hours, during periods when the boundary layer is deep and convective mixing is strong. This information would also serve as an important input for agencies concerned with urban planning and pollution mitigation. Despite these improvements in the near-surface concentrations, the simulated columnar aerosol optical depth (AOD) still remains largely underestimated vis-a-vis the satellite retrieved products. These modifications will serve as a guideline for further model-improvement initiatives at regional scale.


2019 ◽  
Vol 19 (12) ◽  
pp. 8229-8241 ◽  
Author(s):  
Gaurav Govardhan ◽  
Sreedharan Krishnakumari Satheesh ◽  
Krishnaswamy Krishna Moorthy ◽  
Ravi Nanjundiah

Abstract. With a view to improving the performance of WRF-Chem over the Indian region in simulating BC (black carbon) mass concentrations as well as its short-term variations, especially on a diurnal scale, a region-specific diurnal variation scheme has been introduced in the model emissions and the performance of the modified simulations has been evaluated against high-resolution measurements carried out over eight ARFI (Aerosol Radiative Forcing over India) network observatories spread across India for distinct seasons: pre-monsoon (represented by May), post-monsoon (represented by October) and winter (represented by December). In addition to an overall improvement in the simulated concentrations and their temporal variations, we have also found that the effects of prescribing diurnally varying emissions on the simulated near-surface concentrations largely depend on the boundary layer turbulence. The effects are perceived quickly (within about 2–3 h) during the evening–early morning hours when the atmospheric boundary layer is shallow and convective mixing is weak, while they are delayed, taking as much as about 5–6 h, during periods when the boundary layer is deep and convective mixing is strong. This information would also serve as an important input for agencies concerned with urban planning and pollution mitigation. Despite these improvements in the near-surface concentrations, the simulated columnar aerosol optical depth (AOD) still remains largely underestimated vis-à-vis the satellite-retrieved products. These modifications will serve as a guideline for further model-improvement initiatives at a regional scale.


2015 ◽  
Vol 15 (13) ◽  
pp. 7173-7193 ◽  
Author(s):  
A. Veira ◽  
S. Kloster ◽  
N. A. J. Schutgens ◽  
J. W. Kaiser

Abstract. Wildfires represent a major source for aerosols impacting atmospheric radiation, atmospheric chemistry and cloud micro-physical properties. Previous case studies indicated that the height of the aerosol–radiation interaction may crucially affect atmospheric radiation, but the sensitivity to emission heights has been examined with only a few models and is still uncertain. In this study we use the general circulation model ECHAM6 extended by the aerosol module HAM2 to investigate the impact of wildfire emission heights on atmospheric long-range transport, black carbon (BC) concentrations and atmospheric radiation. We simulate the wildfire aerosol release using either various versions of a semi-empirical plume height parametrization or prescribed standard emission heights in ECHAM6-HAM2. Extreme scenarios of near-surface or free-tropospheric-only injections provide lower and upper constraints on the emission height climate impact. We find relative changes in mean global atmospheric BC burden of up to 7.9±4.4 % caused by average changes in emission heights of 1.5–3.5 km. Regionally, changes in BC burden exceed 30–40 % in the major biomass burning regions. The model evaluation of aerosol optical thickness (AOT) against Moderate Resolution Imaging Spectroradiometer (MODIS), AErosol RObotic NETwork (AERONET) and Cloud–Aerosol Lidar with Orthogonal Polarization (CALIOP) observations indicates that the implementation of a plume height parametrization slightly reduces the ECHAM6-HAM2 biases regionally, but on the global scale these improvements in model performance are small. For prescribed emission release at the surface, wildfire emissions entail a total sky top-of-atmosphere (TOA) radiative forcing (RF) of −0.16±0.06 W m−2. The application of a plume height parametrization which agrees reasonably well with observations introduces a slightly stronger negative TOA RF of −0.20±0.07 W m−2. The standard ECHAM6-HAM2 model in which 25 % of the wildfire emissions are injected into the free troposphere (FT) and 75 % into the planetary boundary layer (PBL), leads to a TOA RF of −0.24±0.06 W m−2. Overall, we conclude that simple plume height parametrizations provide sufficient representations of emission heights for global climate modeling. Significant improvements in aerosol wildfire modeling likely depend on better emission inventories and aerosol process modeling rather than on improved emission height parametrizations.


2019 ◽  
Vol 48 (3) ◽  
pp. 3-9
Author(s):  
Peter Gerginov ◽  
Dimitar Antonov

Loess and loess-like sediments cover approximately 13% of the Bulgarian territory, mainly within the Danubian plain. From the Danube River to the Fore-Balkan, the loess soils form a loess complex where its depth varies from 50–60 meters in the north to few meters in the south, respectively. Widespread loess sediments possess a specific feature: they typically form deep unsaturated zones. Quantification of the near surface water balance is extremely important for evaluating land-atmosphere interactions, and the impact of land-use change on the subsurface flow and the evapotranspiration rate is an essential term in this quantification. In the frames of a scientific project, an automatic weather station was installed in a typical plain terrain of the loess complex in Northeast Bulgaria, recording meteorological data from September 2015 to February 2017. This study provides a mathematical description of processes (i.e., Penman-Monteith and Hargreaves Methods) used to estimate daily evapotranspiration rates implemented into the numerical model HYDRUS-1D, as well as a respective rate investigation of months with and without intensive rainfalls. Overall results indicate that using the Hargreaves formula for evaluation of the potential evapotranspiration leads to overestimation between 10% and 20%, respectively for a “wet” and “dry” month.


2016 ◽  
Author(s):  
B. L. Zhuang ◽  
T. J. Wang ◽  
J. Liu ◽  
S. Li ◽  
M. Xie ◽  
...  

Abstract. Observational studies of aerosol optical properties are useful to reducing uncertainties in estimating aerosol radiative forcing and forecasting visibility. In this study, the observed near-surface aerosol optical properties in urban Nanjing are analyzed from Mar 2014 to Feb 2016. Results show that near-surface urban aerosols in Nanjing are mainly from local emissions and the regions around. They have lower loadings but are more scattering than in most cities in China. The annual mean aerosol extinction coefficient (EC), single scattering albedo (SSA) and asymmetry parameter (ASP) at 550 nm are 381.96 Mm−1, 0.9 and 0.57, respectively. The aerosol absorption coefficient (AAC) is about one order of magnitude smaller than its scattering coefficient (SC). However, the absorbing aerosol has larger Ångström exponent (AAE) value, 1.58 at 470/660 nm, about 0.2 larger than the scattering aerosols' (SAE). All the aerosol optical properties followed a near unimodal pattern, the ranges around their averages accounting for more than 60 % of the total samplings. Additionally, they have substantial seasonality and diurnal variations. High levels of SC and AAC all appear in winter due to higher aerosol and trace gas emissions. AAE (ASP) is the smallest (largest) in summer because of high relative humidity (RH) which also causes considerably larger SC and smaller SAE, although intensive gas-to-particle transformation could produce a large number of finer scattering aerosols in this season. Seasonality of EC is different from the columnar aerosol optical depth. Larger AACs appear at the rush hours of the day while SC and Bsp only peak in the early morning. Aerosols are fresher at daytime than at nighttime, leading to their larger AE and smaller ASP. Different temporal variations between AAC and SC cause the aerosols more absorbing (smaller SSA) in autumn and around rush hours. ASP has a good quasi-LogNormal growth trend with increasing SC when RH is below 60 %. The correlation between AAC and SC at the site is close but a little smaller than that in suburban Nanjing in spring. Atmospheric visibility decreases exponentially with increasing EC or SC, more sharply in spring and summer. It could be further deteriorated with increasing SSA and ASP.


2018 ◽  
Vol 31 (20) ◽  
pp. 8381-8399 ◽  
Author(s):  
S. Undorf ◽  
M. A. Bollasina ◽  
G. C. Hegerl

The impact of North American and European (NAEU) anthropogenic aerosol emissions on Eurasian summer climate during the twentieth century is studied using historical single- and all-forcing (including anthropogenic aerosols, greenhouse gases, and natural forcings) simulations from phase 5 of the Coupled Model Intercomparison Project (CMIP5). Intermodel agreement on significant linear trends during a period of increasing NAEU sulfate emissions (1900–74) reveals robust features of NAEU aerosol impact, supported by opposite changes during the subsequent period of decreasing emissions. Regionally, these include a large-scale cooling and associated anticyclonic circulation, as well as a narrowing of the diurnal temperature range (DTR) over Eurasian midlatitudes. Remotely, NAEU aerosols induce a drying over the western African and northern Indian monsoon regions and a strengthening and southward shift of the subtropical jet consistent with the pattern of temperature change. Over Europe, the temporal variations of observed temperature, pressure, and DTR tend to agree better with simulations that include aerosols. Throughout the twentieth century, aerosols are estimated to explain more than a third of the simulated interdecadal forced variability of European near-surface temperature and more than half between 1940 and 1970. These results highlight the substantial aerosol impact on Eurasian climate, already identifiable in the first half of the twentieth century. This may be relevant for understanding future patterns of change related to further emission reductions.


2012 ◽  
Vol 6 (2) ◽  
pp. 353-363 ◽  
Author(s):  
P. Kuipers Munneke ◽  
M. R. van den Broeke ◽  
J. C. King ◽  
T. Gray ◽  
C. H. Reijmer

Abstract. Data collected by two automatic weather stations (AWS) on the Larsen C ice shelf, Antarctica, between 22 January 2009 and 1 February 2011 are analyzed and used as input for a model that computes the surface energy budget (SEB), which includes melt energy. The two AWSs are separated by about 70 km in the north–south direction, and both the near-surface meteorology and the SEB show similarities, although small differences in all components (most notably the melt flux) can be seen. The impact of subsurface absorption of shortwave radiation on melt and snow temperature is significant, and discussed. In winter, longwave cooling of the surface is entirely compensated by a downward turbulent transport of sensible heat. In summer, the positive net radiative flux is compensated by melt, and quite frequently by upward turbulent diffusion of heat and moisture, leading to sublimation and weak convection over the ice shelf. The month of November 2010 is highlighted, when strong westerly flow over the Antarctic Peninsula led to a dry and warm föhn wind over the ice shelf, resulting in warm and sunny conditions. Under these conditions the increase in shortwave and sensible heat fluxes is larger than the decrease of net longwave and latent heat fluxes, providing energy for significant melt.


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