CdSe and CsPbBr3 Quantum Dots Co-doped Monolithic Glasses as Tunable Wavelength Convertors

Author(s):  
Orhan Kıbrıslı ◽  
Erdinc Erol ◽  
Ali Erçin Ersundu ◽  
Miray Çelikbilek Ersundu

Abstract CdSe and CsPbBr3 quantum dots are well studied photoluminescent materials due to their extraordinary emission properties. However, their vulnerability against environmental conditions limits their integration into further applications. At this point, glass encapsulation offers promising durability features due to its robust and dense structure. In this study, CdSe and CsPbBr3 QDs are successfully synthesized in the same glass host through melt-quenching technique followed by a single heat-treatment process. Excitation wavelength dependent photoluminescence properties are investigated and emission color tunability of monolithic glasses from yellow-green to red is demonstrated. Favorable quantum yield values are obtained as 21.78% and 16.63% under 345 and 365 nm excitation wavelengths, respectively. Prepared glasses demonstrate high potential to be used as tunable wavelength convertors for state-of-the-art photonic and opto-electronic applications.

2017 ◽  
Vol 19 (26) ◽  
pp. 17349-17355 ◽  
Author(s):  
Bing Ai ◽  
Chao Liu ◽  
Zhao Deng ◽  
Jing Wang ◽  
Jianjun Han ◽  
...  

Size dependence of exciton activation energy, electron–phonon coupling strength, and thermal expansion of the bandgap of CsPbBr3 QDs were studied.


2019 ◽  
Vol 215 ◽  
pp. 116584
Author(s):  
Hui Gao ◽  
Siyuan Liu ◽  
Zhipeng Xue ◽  
Wenjing Liu ◽  
Yanguang Nie ◽  
...  

MRS Advances ◽  
2016 ◽  
Vol 1 (19) ◽  
pp. 1371-1376 ◽  
Author(s):  
George R. S. Andrade ◽  
Silvânio S. L. Costa ◽  
Cristiane C. Nascimento ◽  
Iara F. Gimenez

ABSTRACTIn this work, 3 simple, fast, labour and energy efficient methodologies were used to prepare carbon quantum dots (C-dots) using a red beetroot (Beta vulgaris subsp. vulgaris var. vulgaris) aqueous extract as the carbon source: alkali-assisted (AA), microwave-assisted (MA) and alkali-microwave-assisted (AMA) synthesis. TEM images shows nanoparticles with a nearly spherical morphology and diameters around 7.0 nm. FTIR spectra show characteristic peaks of C-H, C-O, O-H and C=C bonds for all the samples. The emission spectra show an interesting feature of the as-prepared samples: the emission band position can be tunable by changing the excitation wavelength. Comparing the 3 different methodologies in terms of photoluminescence properties, the one based only on the microwave-assisted heating has showed the most improved emission.


Author(s):  
Haibo Zeng ◽  
Dandan Yang ◽  
Zhiheng Xu ◽  
Chunhui Gong ◽  
Xiaoming Li ◽  
...  

One of the main reasons for the stability issue of inorganic perovskite quantum dots (PQDs) is the fragile protection of surface ligands. Here, an armor-like passivation strategy is proposed to...


2021 ◽  
Author(s):  
Huiqi Wang ◽  
Duo An ◽  
Mei Wang ◽  
Liwen Sun ◽  
Ying Li ◽  
...  

Crystalline borophene quantum dots with two-photo fluorescence and their derivative boron nanospheres with hydrazine hydrate-dependent photoluminescence properties were prepared by efficient high-power sonication method combined with chemical exfoliation and one-step...


Nanoscale ◽  
2021 ◽  
Author(s):  
Dongdong Yan ◽  
Qionghua Mo ◽  
Shuangyi Zhao ◽  
Wensi Cai ◽  
Zhigang Zang

With a high photoluminescence quantum yield (PLQY) being able to exceed 90% for those prepared by hot injection method, CsPbBr3 quantum dots (QDs) have attracted intensive attentions for white light-emitting...


2020 ◽  
Vol 18 ◽  
pp. 100488 ◽  
Author(s):  
Juan Jesús Gallardo ◽  
Eduardo Blanco ◽  
Antonio Sánchez-Coronilla ◽  
José Carlos Pinero ◽  
Javier Navas

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