scholarly journals Aerosol–Ice Formation Closure: A Southern Great Plains Field Campaign

Author(s):  
D. A. Knopf ◽  
K. R. Barry ◽  
T. A. Brubaker ◽  
L. G. Jahl ◽  
K. A., L. Jankowski ◽  
...  

AbstractPrediction of ice formation in clouds presents one of the grand challenges in the atmospheric sciences. Immersion freezing initiated by ice-nucleating particles (INPs) is the dominant pathway of primary ice crystal formation in mixed-phase clouds, where supercooled water droplets and ice crystals coexist, with important implications for the hydrological cycle and climate. However, derivation of INP number concentrations from an ambient aerosol population in cloud-resolving and climate models remains highly uncertain. We conducted an aerosol-ice formation closure pilot study using a field-observational approach to evaluate the predictive capability of immersion freezing INPs. The closure study relies on co-located measurements of the ambient size-resolved and single-particle composition and INP number concentrations. The acquired particle data serve as input in several immersion freezing parameterizations, that are employed in cloud-resolving and climate models, for prediction of INP number concentrations. We discuss in detail one closure case study in which a front passed through the measurement site, resulting in a change of ambient particle and INP populations. We achieved closure in some circumstances within uncertainties, but we emphasize the need for freezing parameterization of potentially missing INP types and evaluation of the choice of parameterization to be employed. Overall, this closure pilot study aims to assess the level of parameter details and measurement strategies needed to achieve aerosol-ice formation closure. The closure approach is designed to accurately guide immersion freezing schemes in models, and ultimately identify the leading causes for climate model bias in INP predictions.

2017 ◽  
Vol 30 (20) ◽  
pp. 8275-8298 ◽  
Author(s):  
Melissa S. Bukovsky ◽  
Rachel R. McCrary ◽  
Anji Seth ◽  
Linda O. Mearns

Abstract Global and regional climate model ensembles project that the annual cycle of rainfall over the southern Great Plains (SGP) will amplify by midcentury. Models indicate that warm-season precipitation will increase during the early spring wet season but shift north earlier in the season, intensifying late summer drying. Regional climate models (RCMs) project larger precipitation changes than their global climate model (GCM) counterparts. This is particularly true during the dry season. The credibility of the RCM projections is established by exploring the larger-scale dynamical and local land–atmosphere feedback processes that drive future changes in the simulations, that is, the responsible mechanisms or processes. In this case, it is found that out of 12 RCM simulations produced for the North American Regional Climate Change Assessment Program (NARCCAP), the majority are mechanistically credible and consistent in the mean changes they are producing in the SGP. Both larger-scale dynamical processes and local land–atmosphere feedbacks drive an earlier end to the spring wet period and deepening of the summer dry season in the SGP. The midlatitude upper-level jet shifts northward, the monsoon anticyclone expands, and the Great Plains low-level jet increases in strength, all supporting a poleward shift in precipitation in the future. This dynamically forced shift causes land–atmosphere coupling to strengthen earlier in the summer, which in turn leads to earlier evaporation of soil moisture in the summer, resulting in extreme drying later in the summer.


2019 ◽  
Vol 32 (13) ◽  
pp. 4089-4102 ◽  
Author(s):  
Ryan J. Kramer ◽  
Brian J. Soden ◽  
Angeline G. Pendergrass

Abstract We analyze the radiative forcing and radiative response at Earth’s surface, where perturbations in the radiation budget regulate the atmospheric hydrological cycle. By applying a radiative kernel-regression technique to CMIP5 climate model simulations where CO2 is instantaneously quadrupled, we evaluate the intermodel spread in surface instantaneous radiative forcing, radiative adjustments to this forcing, and radiative responses to surface warming. The cloud radiative adjustment to CO2 forcing and the temperature-mediated cloud radiative response exhibit significant intermodel spread. In contrast to its counterpart at the top of the atmosphere, the temperature-mediated cloud radiative response at the surface is found to be positive in some models and negative in others. Also, the compensation between the temperature-mediated lapse rate and water vapor radiative responses found in top-of-atmosphere calculations is not present for surface radiative flux changes. Instantaneous radiative forcing at the surface is rarely reported for model simulations; as a result, intermodel differences have not previously been evaluated in global climate models. We demonstrate that the instantaneous radiative forcing is the largest contributor to intermodel spread in effective radiative forcing at the surface. We also find evidence of differences in radiative parameterizations in current models and argue that this is a significant, but largely overlooked, source of bias in climate change simulations.


2021 ◽  
Author(s):  
Georgios Margazoglou ◽  
Valerio Lucarini ◽  
Tobias Grafke ◽  
Alessandro Laio

<p>We apply two independent data analysis methodologies to locate stable climate states in an intermediate complexity climate model and analyze their interplay. First, drawing from the theory of quasipotentials, and viewing the state space as an energy landscape with valleys and mountain ridges, we infer the relative likelihood of the identified multistable climate states, and investigate the most likely transition trajectories as well as the expected transition times between them. Second, harnessing techniques from data science, specifically manifold learning, we characterize  the data landscape of the simulation output to find climate states and basin boundaries within a fully agnostic and unsupervised framework. Both approaches show remarkable agreement, and reveal, apart from the well known warm and snowball earth states, a third intermediate stable state in one of the two climate models we consider. The combination of our approaches allows to identify how the negative feedback of ocean heat transport and entropy production via the hydrological cycle drastically change the topography of the dynamical landscape of Earth's climate.</p>


2005 ◽  
Vol 4 ◽  
pp. 57-62 ◽  
Author(s):  
L. F. Leon ◽  
D. Lam ◽  
W. Schertzer ◽  
D. Swayne

Abstract. Under a Canadian Foundation for Climate and Atmospheric Sciences (CFCAS) project, targeted to study the feasibility to link regional climate models with lake models, one of the tasks was to consider such a coupling in large lakes. The objective is to provide detailed information on temperature and circulation distributions of the lake to take into account the spatial variability for temperature and the heat exchange through the water's surface. The major contribution of this work is focused on realistic representation of the heat fluxes and temperature distributions to and from lakes especially during the thermally stratified ice-free periods. This paper presents the detailed 3-D ELCOM model applied in Lake Erie in order to produce, at the surface layer of the lake, the spatial distribution of temperature and heat exchanges that eventually can be coupled with a regional climate model (CRCM). Preliminary results will be presented on how this lake model may improve the regional climate models, which currently do not consider such large lake circulation effects.


2016 ◽  
Author(s):  
Cheng Zhou ◽  
Joyce E. Penner

Abstract. Observation-based studies have shown that the aerosol cloud lifetime effect or the increase of cloud liquid water (LWP) with increased aerosol loading may have been overestimated in climate models. Here, we simulate shallow warm clouds on 05/27/2011 at the Southern Great Plains (SGP) measurement site established by Department of Energy's Atmospheric Radiation Measurement (ARM) Program using a single column version of a global climate model (CAM5.3) and a cloud resolving model (CRM). The LWP simulated by CAM increases substantially with aerosol loading while that in the CRM does not. The increase of LWP in CAM is caused by a large decrease of the autoconversion rate when cloud droplet number increases. In the CRM, the autoconversion rate is also reduced, but this is offset or even outweighed by the increased evaporation of cloud droplets near cloud top, resulting in an overall decrease in LWP. Our results suggest that climate models need to include the dependence of cloud top growth and the evaporation/condensation process on cloud droplet number concentrations.


2021 ◽  
Author(s):  
Charline Ragon ◽  
Valerio Lembo ◽  
Valerio Lucarini ◽  
Christian Vérard ◽  
Jérôme Kasparian ◽  
...  

<p><span>The climate can be regarded as a stationary non-equilibrium statistical system (Gallavotti 2006): a continuous and spatially inhomogeneous input of solar energy enters at the top-of-atmosphere and compensates the action of non-conservative forces, mainly occurring at small scales, to give rise to a statistically steady state (or attractor) for the whole climate. </span></p><p><span>Depending on the initial conditions and the range of forcing, all other parameters being the same, some climate models have the property to settle down on different attractors. </span><span>Multi-stability reflects how energy, water mass and entropy can be re-distributed in multiple ways among the climate components, such as the atmosphere, the ocean or the ice, through a different balance between nonlinear mechanisms. </span></p><p><span>Starting from a configuration where competing climate attractors occur under the same forcing, we have explored their robustness performing two kinds of numerical experiment. </span><span>First, we have investigated the impact of frictional heating on the overall energy balance and we have shown that such contribution, generally neglected in the atmospheric component of climate models, has crucial </span><span>consequences on conservation properties: it improves the energy imbalance at top-of-atmosphere, typically non negligible in coarse simulations (Wild et al. 2020), strengthens the hydrological cycle, </span><span>mitigates the mechanical work associated to atmospheric circulation intensity </span><span>and reduces the heat transport peaks in the ocean. </span><span>Second, we have compared two bulk formulas for the cloud albedo, one where it is constant everywhere and the other where it increases with latitude, as implemented in the new version of the atmospheric module SPEEDY in order to improve comparisons with observational data (Kucharski 2013). We have che</span><span>cked that this new parameterization does not affect energy and water-mass imbalances, while reduces global temperature and water-mass transport on the attractor, giving rise to a larger conversion of heat into mechanical work in the atmosphere.</span></p><p><span>In order to perform such studies, we have run the climate model MITgcm on coupled aquaplanets at 2.8 horizontal resolution until steady states are reached (Brunetti el al. 2019) and we have applied the Thermodynamic Diagnostic Tool (<em>TheDiaTo</em>, Lembo et al. 2019). </span></p><p> </p><p><span>References: </span></p><p><span>Brunetti, Kasparian, Vérard, Climate Dynamics 53, 6293 (2019)</span></p><p><span>Gallavotti, </span>Math. Phys. 3, 530<span> (2006)</span></p><p>Kucharski<span> et al.</span>, Bulletin of the American Meteorological Society 94, 25<span> (2013)</span></p><p>Lembo, Lunkeit, Lucarini, Geoscientific Model Development 12, 3805<span> (2019)</span></p><p><span>Wild, </span>Climate Dynamics 55, 553<span> (2020)</span></p>


2021 ◽  
Author(s):  
Alberto Sanchez-Marroquin ◽  
Olafur Arnalds ◽  
Kelly J. Baustian-Dorsi ◽  
Jo Browse ◽  
Pavla Dagsson-Waldhauserova ◽  
...  

<p>Although most of the dust present in the atmosphere originates from low-latitude arid deserts, it has been increasingly recognised that there are significant sources of High-Latitude Dust (HLD) in locations such as Iceland, Greenland, North American Arctic or North Eurasia [1]. The emission, transport and deposition of HLD can interact with the atmosphere, cryosphere and the marine ecosystem in several ways. Particularly, HLD has the potential to act as significant source of atmospheric Ice-Nucleating Particles (INP), competing with other sources such as dust and other INP types from lower-latitude arid sources [2, 3]. INPs are the fraction of aerosol particles that can trigger ice-formation in supercooled water droplets, that otherwise would remain unfrozen until temperatures of about -36 <sup>o</sup>C.</p><p>Ice formation initiated by the presence of INPs dramatically affects the amount of solar radiation reflected by clouds containing both liquid water and ice, known as mixed-phase clouds. However, ice-related processes in mixed-phase clouds such as the INP concentration are commonly oversimplified in most climate models, which leads to large discrepancies in the amount of water and ice that the models simulate at mid- to high-latitudes [4]. These present-day divergences in simulated mixed-phase clouds lead to a large uncertainty in the cloud climate feedback. This feedback is associated to the fact that mid- to high-latitude mixed-phase clouds dampen a part of the of the global temperature rise associated with greenhouse gases [5] [6].</p><p>Here we will explain the importance of understanding the chemical and ice-nucleating properties of HLD, as well as how it is emitted, transported and deposited for the cloud climate feedback. We will present new results from aircraft studies of the ice nucleating ability of HLD as well as modelling work which shows that this dust can be transported to altitudes and regions where it has the potential to influence mixed-phase clouds and climate.</p>


2018 ◽  
Vol 11 (10) ◽  
pp. 4021-4041 ◽  
Author(s):  
Sara Bacer ◽  
Sylvia C. Sullivan ◽  
Vlassis A. Karydis ◽  
Donifan Barahona ◽  
Martina Krämer ◽  
...  

Abstract. A comprehensive ice nucleation parameterization has been implemented in the global chemistry-climate model EMAC to improve the representation of ice crystal number concentrations (ICNCs). The parameterization of Barahona and Nenes (2009, hereafter BN09) allows for the treatment of ice nucleation taking into account the competition for water vapour between homogeneous and heterogeneous nucleation in cirrus clouds. Furthermore, the influence of chemically heterogeneous, polydisperse aerosols is considered by applying one of the multiple ice nucleating particle parameterizations which are included in BN09 to compute the heterogeneously formed ice crystals. BN09 has been modified in order to consider the pre-existing ice crystal effect and implemented to operate both in the cirrus and in the mixed-phase regimes. Compared to the standard EMAC parameterizations, BN09 produces fewer ice crystals in the upper troposphere but higher ICNCs in the middle troposphere, especially in the Northern Hemisphere where ice nucleating mineral dust particles are relatively abundant. Overall, ICNCs agree well with the observations, especially in cold cirrus clouds (at temperatures below 205 K), although they are underestimated between 200 and 220 K. As BN09 takes into account processes which were previously neglected by the standard version of the model, it is recommended for future EMAC simulations.


2021 ◽  
Author(s):  
Georgia Sotiropoulou ◽  
Anna Lewinschal ◽  
Annica Ekman ◽  
Athanasios Nenes

<p>Arctic clouds are among the largest sources of uncertainty in predictions of Arctic weather and climate. This is mainly due to errors in the representation of the cloud thermodynamic phase and the associated radiative impacts, which largely depends on the parameterization of cloud microphysical processes. Secondary ice processes (SIP) are among the microphysical processes that are poorly represented, or completely absent, in climate models. In most models, including the Norwegian Earth System Model -version 2 (NorESM2), Hallet-Mossop (H-M) is the only SIP mechanism available. In this study we further improve the description of H-M and include two additional SIP mechanisms (collisional break-up and drop-shattering) in NorESM2. Our results indicate that these additions improve the agreement between observed and modeled ice crystal number concentrations and liquid water path in mixed-phase clouds observed at Ny-Alesund in 2016-2017. We then conclude by quantifying the impact of these overlooked SIP mechanisms for cloud microphysical characteristics, properties and the radiative balance throughout the Arctic.</p><p> </p>


2011 ◽  
Vol 4 (3) ◽  
pp. 2545-2576
Author(s):  
C. E. Brennan ◽  
A. J. Weaver ◽  
M. Eby ◽  
K. J. Meissner

Abstract. Implementing oxygen isotopes (H218O, H216O) in coupled climate models provides both an important test of the individual model's hydrological cycle, and a powerful tool to mechanistically explore past climate changes while producing results directly comparable to isotope proxy records. Here we describe the addition of oxygen isotopes in the University of Victoria Earth System Climate Model (UVic ESCM). Equilibrium simulations are performed for preindustrial and Last Glacial Maximum conditions. The oxygen isotope content in the model preindustrial climate is compared against observations for precipitation and seawater. The distribution of oxygen isotopes during the LGM is compared against available paleo-reconstructions.


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