Since it has been shewn by various accurate experiments, that the diamond and common carbonaceous substances consume nearly the same quantity of oxygene in combustion, and produce a gas having the same obvious qualities, a number of conjectures have been formed to explain the remarkable differences in the sensible qualities of these bodies, by supposing some minute difference in their chemical composition; these conjectures have been often discussed, it will not be necessary therefore to dwell upon them: M. M. Biot and Arago, from the high refractive power of the diamond, have supposed that it may contain hydrogene; I ventured to suggest in my third Bakerian Lecture, from the circumstance of its non-conducting power, and from the action of potassium upon it, that a minute portion of oxygene may exist in it; and in my Account of some new experiments on the fluoric Compounds,I hazarded the idea that it might be the carbonaceous principle combined with some new light and subtile element of the class of supporters of combustion. M. Guyton de Morveau, who conceived he had proved by experiments made fourteen years ago, that common carbonaceous substances were, oxides of diamonds, from his last researches, conducted in the same manner as those of Messrs. Allen and Pepys, seems still inclined to adopt this opinion, though in admitting a much smaller quantity of oxygene than he originally supposed in charcoal; and he considers the diamond as pure carbonaceous matter, containing, possibly, some atoms of water of crystallisation. I have long had a desire of making some new experiments on the combustion of the diamond and other carbonaceous substances, and this desire was increased by the new facts ascertained with respect to iodine, which by uniting to hydrogene, affords an acid so analogous to muriatic acid, that it was for some time confounded with that substance. My object in these experiments, was to examine minutely whether any peculiar matter was separated from the diamond during its combustion, and to determine whether the gas, formed in this process, was precisely the same in its minute chemical nature, as that formed in the combustion of common charcoal. I have lately been able to accomplish my wishes; I shall now have the honour of communicating my results to the Royal Society.