scholarly journals Strong coupling of a plasmonic nanoparticle to a semiconductor nanowire

Nanophotonics ◽  
2021 ◽  
Vol 0 (0) ◽  
Author(s):  
Yingying Jin ◽  
Liu Yang ◽  
Chenxinyu Pan ◽  
Zhangxing Shi ◽  
Bowen Cui ◽  
...  
Keyword(s):  
Strong Coupling ◽  
Coupled System ◽  
Resonance Wavelength ◽  
Transverse Magnetic ◽  
Spectral Shift ◽  
Au Nanoparticle ◽  
Localized Surface Plasmon ◽  
Nanowire Diameter ◽  
Plasmonic Nanoparticle ◽  
Au Nanosphere

Abstract By placing a single Au nanoparticle on the surface of a cadmium sulfide (CdS) nanowire, we demonstrate strong coupling of localized surface plasmon resonance (LSPR) modes in the nanoparticle and whispering gallery modes (WGMs) in the nanowire. For a 50-nm-diameter Au-nanosphere particle, strong coupling occurs when the nanowire diameter is between 300 and 600 nm, with a mode splitting up to 80 meV. Using a temperature-induced spectral shift of the resonance wavelength, we also observe the anticrossing behavior in the strongly coupled system. In addition, since the Au nanosphere has spherical symmetry, the supported LSPR mode can be selectively coupled with transverse electric (TE) and transverse magnetic (TM) WGMs in the nanowire. The ultracompact strong-coupling system shown here may provide a versatile platform for studying hybrid “photon–plasmon” nanolasers, nonlinear optical devices, and nanosensors.

scholarly journals Effects of gap thickness and emitter location on the photoluminescence enhancement of monolayer MoS2 in a plasmonic nanoparticle-film coupled system

Nanophotonics ◽  
2020 ◽  
Vol 9 (7) ◽  
pp. 2097-2105
Author(s):  
Xiaozhuo Qi ◽  
Tsz Wing Lo ◽  
Di Liu ◽  
Lantian Feng ◽  
Yang Chen ◽  
...  
Keyword(s):  
Near Field ◽  
Central Area ◽  
Field Enhancement ◽  
Coupled System ◽  
Film Structure ◽  
Plasmonic Nanoparticle ◽  
Emitter Location ◽  
Radiation Properties ◽  
Radiation Enhancement ◽  
Quantum Emitters

AbstractPlasmonic nanocavities comprised of metal film-coupled nanoparticles have emerged as a versatile nanophotonic platform benefiting from their ultrasmall mode volume and large Purcell factors. In the weak-coupling regime, the particle-film gap thickness affects the photoluminescence (PL) of quantum emitters sandwiched therein. Here, we investigated the Purcell effect-enhanced PL of monolayer MoS2 inserted in the gap of a gold nanoparticle (AuNP)–alumina (Al2O3)–gold film (Au Film) structure. Under confocal illumination by a 532 nm CW laser, we observed a 7-fold PL peak intensity enhancement for the cavity-sandwiched MoS2 at an optimal Al2O3 thickness of 5 nm, corresponding to a local PL enhancement of ∼350 by normalizing the actual illumination area to the cavity’s effective near-field enhancement area. Full-wave simulations reveal a counterintuitive fact that radiation enhancement comes from the non-central area of the cavity rather than the cavity center. By scanning an electric dipole across the nanocavity, we obtained an average radiation enhancement factor of about 65 for an Al2O3 spacer thickness of 4 nm, agreeing well with the experimental thickness and indicating further PL enhancement optimization. Our results indicate the importance of configuration optimization, emitter location and excitation condition when using such plasmonic nanocavities to modulate the radiation properties of quantum emitters.

Determination of pseudo-refractive index in self-assembled ligand layers from spectral shift of surface plasmon resonances in colloidal silver nanoplates

2021 ◽  
Vol 0 (0) ◽  
Author(s):  
Pavel Malakhovsky ◽  
Dmitry Murausky ◽  
Dmitry Guzatov ◽  
Sergey Gaponenko ◽  
Mikhail Artemyev
Keyword(s):  
Refractive Index ◽  
Surface Plasmon ◽  
Mie Theory ◽  
Spectral Shift ◽  
Localized Surface Plasmon ◽  
Clear Trend ◽  
Silver Nanoplates ◽  
Assembled Monolayers ◽  
Self Assembled

Abstract We examined systematically how self-assembled monolayers (SAMs) of different mercaptoacids affect the spectral shift of the localized surface plasmon resonance in silver nanoplates and nanospheres. We observed a clear trend in the magnitude of a redshift with a molecular length or the SAM thickness within a homologous series of aliphatic mercaptoacids: the thicker shell the stronger the red shift. Using classic Mie theory for plasmonic core-dielectric shell spheres and oblate spheroids we developed the method for determination of a pseudo-refractive index in SAM of different molecules and obtained a good correlation with the reference refractive indices for bulk long-chain aliphatic acids, but only in case of silver nanoplates. Calculations for silver core–shell nanospheres gave overestimated values of refractive index perhaps due to restrictions of Mie theory on the minimum particle size.

scholarly journals Quad-Band Plasmonic Perfect Absorber for Visible Light with a Patchwork of Silicon Nanorod Resonators

Materials ◽  
2018 ◽  
Vol 11 (10) ◽  
pp. 1954 ◽  
Author(s):  
Can Cao ◽  
Yongzhi Cheng
Keyword(s):  
Visible Light ◽  
Transverse Electric ◽  
Transverse Magnetic ◽  
Localized Surface Plasmon ◽  
Perfect Absorber ◽  
Absorption Properties ◽  
Perfect Absorption ◽  
Potential Applications ◽  
Polarization Insensitive ◽  
Band Absorption

In this paper, a plasmonic perfect absorber (PPA) based on a silicon nanorod resonator (SNRR) for visible light is proposed and investigated numerically. The proposed PPA is only a two-layer nanostructure consisting of a SNRR periodic array and metal substrate. The perfect absorption mainly originates from excitation of the localized surface plasmon resonance (LSPR) mode in the SNRR structure. The absorption properties of this design can be adjusted by varying the radius (r) and height (h) of the SNRR structure. What is more, the stronger quad-band absorption can be achieved by combing four different radius of the SNRR in one period as a super unit-cell. Numerical simulation indicates that the designed quad-band PPA can achieve the absorbance of 99.99%, 99.8%, 99.8%, and 92.2% at 433.5 THz, 456 THz, 482 THz, and 504.5 THz, respectively. Further simulations show that the proposed PPA is polarization-insensitive for both transverse electric (TE) and transverse magnetic (TM) modes. The proposed PPA can be a desirable candidate for some potential applications in detecting, sensing, and visible spectroscopy.

scholarly journals Dynamics of Strong Coupling Between Free Charge Carriers in Organometal Halide Perovskites and Aluminum Plasmonic States

2022 ◽  
Vol 9 ◽  
Author(s):  
Yang Luo ◽  
Hai Wang ◽  
Le-Yi Zhao ◽  
Yong-Lai Zhang
Keyword(s):  
Strong Coupling ◽  
Transient Absorption ◽  
Perovskite Solar Cells ◽  
Coupled System ◽  
Free Carrier ◽  
Charge Carriers ◽  
Free Charge ◽  
Free Carriers ◽  
Halide Perovskites ◽  
Poor Absorption

We have investigated a strong coupled system composed of a MAPbIxCl3-x perovskite film and aluminum conical nanopits array. The hybrid states formed by surface plasmons and free carriers, rather than the traditional excitons, is observed in both steady-state reflection measurements and transient absorption spectra. In particular, under near upper band resonant excitation, the bleaching signal from the band edge of uncoupled perovskite was completely separated into two distinctive bleaching signals of the hybrid system, which is clear evidence for the formation of strong coupling states between the free carrier–plasmon state. Besides this, a Rabi splitting up to 260 meV is achieved. The appearance of the lower bands can compensate for the poor absorption of the perovskite in the NIR region. Finally, we found that the lifetime of the free carrier–SP hybrid states is slightly shorter than that of uncoupled perovskite film, which can be caused by the ultrafast damping of the SPs modes. These peculiar features on the strong coupled hybrid states based on free charge carriers can open new perspectives for novel plasmonic perovskite solar cells.

scholarly journals Enhanced Plasmonic Resonance Characteristics of AgNRs–Gold Film Hybrid System

2021 ◽  
Vol 8 ◽  
Author(s):  
Yanping Yin ◽  
Jin Zhu ◽  
Zaoji Wang ◽  
Guojun Ma ◽  
Huining Yuan ◽  
...  
Keyword(s):  
Refractive Index ◽  
Aspect Ratio ◽  
Gold Film ◽  
Spectral Response ◽  
Surrounding Medium ◽  
Resonance Wavelength ◽  
Spectral Shift ◽  
Refractive Index Sensor ◽  
Gap Size ◽  
Refractive Index Sensitivity

In recent years, the plasma gap resonance maintained by metal-film-coupled nanostructures has attracted extensive attention. This mainly originates from its flexible control of the spectral response and significantly enhanced field strength at the nanoparticle–film junction. In the present study, the tunability of local surface plasmon resonances (LSPRs) of nanorods coupled to a gold film is studied theoretically. To this end, the plasmonic resonances in the nanostructure of individual silver nanorod–gold film (AgNR-film) with different parameters are investigated. Obtained results show that the refractive index sensitivity (S) of nanostructures to the environment increases as the aspect ratio (Ar) of nanostructures increase. It is found that when the aspect ratio (Ar) is set to 3.5, the figure of merit (FOM) is the highest. Moreover, the variation in the gap distances of the nanorod monomer–gold film, electric field distribution of nanorods dimer, and the corresponding impact on the gold film are studied. It is concluded that the gap size of nanostructures has an exponential correlation with the resonance wavelength. Considering the remarkable influence of the gap size and the surrounding medium environment on the spectral shift of AgNR-film nanostructures, potential applications of the structure as a refractive index sensor and biomolecule measurement are proposed.

scholarly journals Ultrabroadband Absorption Enhancement via Hybridization of Localized and Propagating Surface Plasmons

Nanomaterials ◽  
2020 ◽  
Vol 10 (9) ◽  
pp. 1625
Author(s):  
Tian Sang ◽  
Honglong Qi ◽  
Xun Wang ◽  
Xin Yin ◽  
Guoqing Li ◽  
...  
Keyword(s):  
Surface Plasmon ◽  
Near Infrared ◽  
Low Cost ◽  
Polarized Light ◽  
Wavelength Region ◽  
Transverse Magnetic ◽  
Localized Surface Plasmon ◽  
Absorption Enhancement ◽  
Geometrical Parameters ◽  
Light Illumination

Broadband metamaterial absorbers (MAs) are critical for applications of photonic and optoelectronic devices. Despite long-standing efforts on broadband MAs, it has been challenging to achieve ultrabroadband absorption with high absorptivity and omnidirectional characteristics within a comparatively simple and low-cost architecture. Here we design, fabricate, and characterize a novel compact Cr-based MA to achieve ultrabroadband absorption in the visible to near-infrared wavelength region. The Cr-based MA consists of Cr nanorods and Cr substrate sandwiched by three pairs of SiO2/Cr stacks. Both simulated and experimental results show that an average absorption over 93.7% can be achieved in the range of 400–1000 nm. Specifically, the ultrabroadband features result from the co-excitations of localized surface plasmon (LSP) and propagating surface plasmon (PSP) and their synergistic absorption effects, where absorption in the shorter and longer wavelengths are mainly contributed bythe LSP and PSP modes, respectively. The Cr-based MA is very robust to variations of the geometrical parameters, and angle-and polarization-insensitive absorption can be operated well over a large range of anglesunder both transverse magnetic(TM)- and transverse electric (TE)-polarized light illumination.

scholarly journals Double-resonant enhancement of third-harmonic generation in graphene nanostructures

2017 ◽  
Vol 375 (2090) ◽  
pp. 20160313 ◽  
Author(s):  
Jian Wei You ◽  
Jie You ◽  
Martin Weismann ◽  
Nicolae C. Panoiu
Keyword(s):  
Harmonic Generation ◽  
Spectral Response ◽  
Near Field ◽  
Field Enhancement ◽  
Third Harmonic Generation ◽  
Resonance Wavelength ◽  
Localized Surface Plasmon ◽  
Third Harmonic ◽  
New Horizons ◽  
Geometry Dependence

Intriguing and unusual physical properties of graphene offer remarkable potential for advanced, photonics-related technological applications, particularly in the area of nonlinear optics at the deep-subwavelength scale. In this study, we use a recently developed numerical method to illustrate an efficient mechanism that can lead to orders of magnitude enhancement of the third-harmonic generation in graphene diffraction gratings. In particular, we demonstrate that by taking advantage of the geometry dependence of the resonance wavelength of localized surface-plasmon polaritons of graphene ribbons and discs one can engineer the spectral response of graphene gratings so that strong plasmonic resonances exist at both the fundamental frequency and third-harmonic (TH). As a result of this double-resonant mechanism for optical near-field enhancement, the intensity of the TH can be increased by more than six orders of magnitude. This article is part of the themed issue ‘New horizons for nanophotonics’.

Sign in / Sign up

Export Citation Format

Share Document