scholarly journals The applicability of C-14 measurements in the soil gas for the assessment of leakage out of underground carbon dioxide reservoirs

Nukleonika ◽  
2014 ◽  
Vol 59 (1) ◽  
pp. 3-7
Author(s):  
Stanisław Chałupnik ◽  
Małgorzata Wysocka

Abstract Poland, due to the ratification of the Kioto Protocol, is obliged to diminish the emission of greenhouse gases. One of the possible solutions of this problem is CO2 sequestration (CCS - carbon capture and storage). Such an option is a priority in the European Union. On the other hand, CO2 sequestration may be potentially risky in the case of gas leakage from underground reservoirs. The most dangerous event may be a sudden release of the gas onto the surface. Therefore, it is very important to know if there is any escape of CO2 from underground gas reservoirs, created as a result of sequestration. Such information is crucial to ensure safety of the population in areas located above geological reservoirs. It is possible to assess the origin of carbon dioxide, if the measurement of radiocarbon 14C concentration in this gas is done. If CO2 contains no 14C, it means, that the origin of the gas is either geological or the gas has been produced as a result of combustion of fossil fuels, like coal. A lot of efforts are focused on the development of monitoring methods to ensure safety of CO2 sequestration in geological formations. A radiometric method has been tested for such a purpose. The main goal of the investigations was to check the application possibility of such a method. The technique is based on the liquid scintillation counting of samples. The gas sample is at first bubbled through the carbon dioxide adsorbent, afterwards the adsorbent is mixed with a dedicated cocktail and measured in a low-background liquid scintillation spectrometer Quantulus. The described method enables measurements of 14C in mine and soil gas samples.

2007 ◽  
Vol 25 (5) ◽  
pp. 357-392 ◽  
Author(s):  
Havva Balat ◽  
Cahide Öz

This article deals with review of technical and economic aspects of Carbon Capture and Storage. Since the late 1980s a new concept is being developed which enables to make use of fossil fuels with a considerably reduced emission of carbon dioxide to the atmosphere. The concept is often called ‘Carbon Capture and Storage’ (CCS). CCS technologies are receiving increasing attention, mainly for their potential contribution to the optimal mitigation of carbon dioxide emissions that is intended to avoid future, dangerous climate change. CCS technologies attract a lot of attention because they could allow “to reduce our carbon dioxide emissions to the atmosphere whilst continuing to use fossil fuels”. CCS is not a completely new technology, e.g., the United States alone is sequestering about 8.5 MtC for enhanced oil recovery each year. Today, CCS technologies are widely recognised as an important means of progress in industrialized countries.


Author(s):  
Dan Allason ◽  
Keith Armstrong ◽  
Julian Barnett ◽  
Phil Cleaver ◽  
Ann Halford

A large Research and Development programme has been executed by National Grid to determine the feasibility of transporting carbon dioxide (CO2) by pipeline. Such pipelines would be required to form a transportation system to take the CO2 from its place of capture at an emitter’s site to a place of safe storage within a Carbon Capture and Storage (CCS) scheme. This programme received financial support from the European Union. As part of this programme, National Grid commissioned a series of experimental studies to investigate the behaviour of releases of CO2 mixtures in the gaseous and the liquid (or dense) phase. This has included simulating accidental releases in the form of punctures or ruptures of a buried pipeline and deliberate releases through different venting arrangements. This work is required, as CO2 has the potential to cause some harm to people if they are exposed to it for long enough at high concentrations. This paper gives an overview of the findings from this work and shows how the data has been used to help develop a number of the more pragmatic, predictive models for outflow and dispersion. This work complements the more theoretical studies carried out using state of the art advanced computational fluid dynamic models, employed by other UK based participants (University College London, University of Leeds, Kingston University and the University of Warwick) in the research programme.


2021 ◽  
Author(s):  
Ángel Galán-Martín ◽  
Daniel Vázquez ◽  
Selene Cobo ◽  
Niall Mac Dowell ◽  
José Caballero ◽  
...  

Abstract Carbon dioxide removal (CDR) will be essential to meet the climate targets, so enabling its deployment at the right time will be decisive. Here, we investigate the still poorly understood implications of delaying CDR actions, focusing on integrating direct air capture and bioenergy with carbon capture and storage (DACCS and BECCS) into the European Union power mix. Under an indicative target of − 50 Gt of net CO2 by 2100, delayed CDR would cost an extra of 0.12 − 0.19 trillion EUR per year of inaction. Moreover, postponing CDR beyond mid-century would substantially reduce the removal potential to almost half (− 35.60 Gt CO2) due to the underused biomass and land resources and the maximum technology diffusion speed. The effective design of BECCS and DACCS systems calls for long-term planning starting from now and aligned with the evolving power systems. Our quantitative analysis of the consequences of inaction on CDR —with climate targets at risk and fair CDR contributions at stake —should help to break the current impasse and incentivize early actions worldwide.


Author(s):  
Naimish Agarwal

Abstract: More than ever, the fate of anthropogenic CO2 emissions is in our hands. Since the advent of industrialization, there has been an increase in the use of fossil fuels to fulfil rising energy demands. The usage of such fuels results in the release of carbon dioxide (CO2) and other greenhouse gases, which result in increased temperature. Such warming is extremely harmful to life on Earth. The development of technology to counter the climate change and spreading it for widespread adoptions. We need to establish a framework to provide overarching guidance for the well-functioning of technology and mechanism development of Carbon Capture and Storage. Carbon capture and storage (CCS) is widely regarded as a critical approach for achieving the desired CO2 emission reduction. Various elements of CCS, such as state-of-the-art technology for CO2 collection, separation, transport, storage, politics, opportunities, and innovations, are examined and explored in this paper. Carbon capture and storage is the process of capturing and storing carbon dioxide (CO2) before it is discharged into the environment (CCS). The technology can capture high amounts of CO2 produced by fossil fuel combustion in power plants and industrial processes. CO2 is compressed and transferred by pipeline, ship, or road tanker once it has been captured. CO2 can then be piped underground, usually to depths of 1km or more, and stored in depleted oil and gas reservoirs, coalbeds, or deep saline aquifers, depending on the geology. CO2 could also be used to produce commercially marketable products. With the goal of keeping world average temperatures below 1.5°C (2.7°F) and preventing global average temperature rises of more than 2°C (3.6°F) over pre-industrial levels, CCS model should be our priority to be implemented with the proper economical map


Author(s):  
Anand Pavithran ◽  
Meeta Sharma ◽  
Anoop Kumar Shukla

The energy generation from the fossil fuels results to emit a tremendous amount of carbon dioxide into the atmosphere. The rise in the atmospheric carbon dioxide level is the primary reason for global warming and other climate change problems for which energy generation from renewable sources is an alternative solution to overcome this problem. However, the renewables sources are not as reliable for the higher amount of energy production and cannot fulfil the world’s energy demand; fossil fuels will continue to be consumed heavily for the energy generation requirements in the immediate future. The only possible solution to overcome the greenhouse gas emission from the power plant is by capturing and storing the carbon dioxide within the power plants instead of emitting it into the atmosphere. The oxy-fuel combustion power cycle with a carbon capture and storage system is an effective way to minimize emissions from the energy sectors. The oxy-fuel power cycle can reduce 90–99% of carbon dioxide emissions from the atmosphere. Moreover, the oxy-fuel power cycles have several advantages over the conventional power plants, these include high efficiency, lesser plant footprint, much easier carbon-capturing processes, etc. Because of these advantages, the oxy-fuel combustion power cycles capture more attention. In the last decades, the number of studies has risen exponentially, leading to many experimental and demonstrational projects under development today. This paper reviews the works related to oxy-fuel combustion power generation technologies with carbon capture and storage system. The cycle concepts and the advancements in this technology have been briefly discussed in this paper.


Energies ◽  
2021 ◽  
Vol 14 (9) ◽  
pp. 2406
Author(s):  
Maria João Regufe ◽  
Ana Pereira ◽  
Alexandre F. P. Ferreira ◽  
Ana Mafalda Ribeiro ◽  
Alírio E. Rodrigues

An essential line of worldwide research towards a sustainable energy future is the materials and processes for carbon dioxide capture and storage. Energy from fossil fuels combustion always generates carbon dioxide, leading to a considerable environmental concern with the values of CO2 produced in the world. The increase in emissions leads to a significant challenge in reducing the quantity of this gas in the atmosphere. Many research areas are involved solving this problem, such as process engineering, materials science, chemistry, waste management, and politics and public engagement. To decrease this problem, green and efficient solutions have been extensively studied, such as Carbon Capture Utilization and Storage (CCUS) processes. In 2015, the Paris Agreement was established, wherein the global temperature increase limit of 1.5 °C above pre-industrial levels was defined as maximum. To achieve this goal, a global balance between anthropogenic emissions and capture of greenhouse gases in the second half of the 21st century is imperative, i.e., net-zero emissions. Several projects and strategies have been implemented in the existing systems and facilities for greenhouse gas reduction, and new processes have been studied. This review starts with the current data of CO2 emissions to understand the need for drastic reduction. After that, the study reviews the recent progress of CCUS facilities and the implementation of climate-positive solutions, such as Bioenergy with Carbon Capture and Storage and Direct Air Capture. Future changes in industrial processes are also discussed.


2021 ◽  
Vol 12 (1) ◽  
Author(s):  
Ángel Galán-Martín ◽  
Daniel Vázquez ◽  
Selene Cobo ◽  
Niall Mac Dowell ◽  
José Antonio Caballero ◽  
...  

AbstractCarbon dioxide removal (CDR) will be essential to meet the climate targets, so enabling its deployment at the right time will be decisive. Here, we investigate the still poorly understood implications of delaying CDR actions, focusing on integrating direct air capture and bioenergy with carbon capture and storage (DACCS and BECCS) into the European Union power mix. Under an indicative target of −50 Gt of net CO2 by 2100, delayed CDR would cost an extra of 0.12−0.19 trillion EUR per year of inaction. Moreover, postponing CDR beyond mid-century would substantially reduce the removal potential to almost half (−35.60 Gt CO2) due to the underused biomass and land resources and the maximum technology diffusion speed. The effective design of BECCS and DACCS systems calls for long-term planning starting from now and aligned with the evolving power systems. Our quantitative analysis of the consequences of inaction on CDR—with climate targets at risk and fair CDR contributions at stake—should help to break the current impasse and incentivize early actions worldwide.


Author(s):  
Kartika Srivastava

Abstract: Carbon dioxide capture and sequestration (CCS) is the capture and storage of carbon dioxide (CO2) that is emitted to the atmosphere as a result of combustion process. Presently majority of efforts focus on the removal of carbon dioxide directly from industrial plants and thereby storing it in geological reservoirs. The principle is to achieve a carbon neutral budget if not carbon negative, and thereby mitigate global climate change. Currently, fossil fuels are the predominant source of the global energy generation and the trend will continue for the rest of the century. Fossil fuels supply over 63% of all primary energy; the rest is contributed by nuclear, hydro-electricity and renewable energy. Although research and investments are being targeted to increase the percentage of renewable energy and foster conservation and efficiency improvements of fossil-fuel usage, development of CCS technology is the most important tool likely to play a pivotal role in addressing this crisis. [1] Keywords: Carbon Capture and Storage, Carbon dioxide, fossil fuels, Greenhouse gases


2021 ◽  
Vol 104 (2) ◽  
pp. 003685042110196
Author(s):  
Brendon Mpofu ◽  
Hembe E Mukaya ◽  
Diakanua B Nkazi

Carbon dioxide has been identified as one of the greenhouse gases responsible for global warming. Several carbon capture and storage technologies have been developed to mitigate the large quantities of carbon dioxide released into the atmosphere, but these are quite expensive and not easy to implement. Thus, this research analyses the technical and economic feasibility of using calcium leached from cow bone to capture and store carbon dioxide through the mineral carbonation process. The capturing process of carbon dioxide was successful using the proposed technique of leaching calcium from cow shinbone (the tibia) in the presence of HCl by reacting the calcium solution with gaseous carbon dioxide. AAS and XRF analysis were used to determine the concentration of calcium in leached solutions and the composition of calcium in cow bone respectively. The best leaching conditions were found to be 4 mole/L HCl and leaching time of 6 h. Under these conditions, a leaching efficiency of 91% and a calcium conversion of 83% in the carbonation reaction were obtained. Other factors such as carbonation time, agitation rate, and carbonation reaction temperature had little effect on the yield. A preliminary cost analysis showed that the cost to capture 1 ton of CO2 with the proposed technique is about US$ 268.32, which is in the acceptable range of the capturing process. However, the cost of material used and electricity should be reviewed to reduce the preliminary production cost.


2014 ◽  
Vol 68 (5) ◽  
Author(s):  
Nabilah Zaini ◽  
Khairul Sozana Nor Kamarudin

Emission of carbon dioxide (CO2) becomes a major concern in combating issues of global warming. The strategy to reduce the concentration of CO2 could be achieved by executing carbon capture and storage (CCS) technology such as adsorption. This study presents the used of kenaf as a green source for CO2 adsorption material. The modification of MEA on kenaf is a novelty work to enhance the capacity of adsorbent since MEA has been proved to have potential in separating CO2 in industrial applications. In this work, 10 wt % of MEA has been impregnated on kenaf via wet impregnation method. The adsorption of CO2 study was conducted by passing CO2/N2 mixture in a ratio of 30:70 in a Pressure Swing Adsorption (PSA) system with a pressure up to 1.5 bar at ambient temperature. Result obtained via SEM analysis shows that the morphology of kenaf was affected after modification with MEA. However, the presence of MEA on kenaf has improved the CO2 adsorption capacity by 16 %. In addition, the adsorption equilibrium data for kenaf and MEA modified kenaf are well fitted in Freundlich isotherm model at low pressure and well fitted in Langmuir model at higher pressure. This study indicates that the introduction of MEA on kenaf could enhance the CO2 adsorption process.  


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