scholarly journals A Stratospheric Intrusion-Influenced Ozone Pollution Episode Associated with an Intense Horizontal-Trough Event

Atmosphere ◽  
2020 ◽  
Vol 11 (2) ◽  
pp. 164 ◽  
Author(s):  
Yiping Wang ◽  
Hongyue Wang ◽  
Wuke Wang
Keyword(s):  
Climate Model ◽  
Stratospheric Ozone ◽  
Surface Ozone ◽  
Eastern China ◽  
Particle Dispersion ◽  
Dispersion Modeling ◽  
Ozone Pollution ◽  
Ozone Forecast ◽  
Stratospheric Intrusion ◽  
Pollution Episode

Ozone pollution is currently a serious issue in China. As an important source of tropospheric ozone, the stratospheric ozone has received less concern. This study uses a combination of ground-based ozone measurements, the latest ERA5 reanalysis data as well as chemistry-climate model and Lagrangian Particle Dispersion Modeling (LPDM) simulations to investigate the potential impacts of stratospheric intrusion (SI) on surface ozone pollution episodes in eastern China. Station-based observations indicate that severe ozone pollution occurred from 27 April to 28 April 2018 in eastern China, with maximal values over 140 ppbv. ERA5 meteorological and ozone data suggest that a strong horizontal-trough exists at the same time, which leads to an evident SI event and brings ozone-rich air from the stratosphere to the troposphere. Using a stratospheric ozone tracer defined by NCAR’s Community Atmosphere Model with Chemistry (CAM-Chem), we conclude that this SI event contributed about 15 ppbv (15%) to the surface ozone pollution episode during 27–28 April in eastern China. The potential impacts of SI events on surface ozone variations should be therefore considered in ozone forecast and control.

Impacts of Stratospheric Intrusion on Surface Ozone over Eastern China

2020 ◽  
Author(s):  
Wuke Wang
Keyword(s):  
Yangtze River ◽  
Surface Ozone ◽  
Eastern China ◽  
Yangtze River Delta ◽  
River Delta ◽  
Anthropogenic Sources ◽  
The Yangtze River ◽  
Ozone Pollution ◽  
Stratospheric Intrusion ◽  
The Yangtze River Delta

<p><span>Ozone pollution is currently a serious environmental issue in China. Most of studies have attributed the surface ozone pollution over China to the strong photochemical production from anthropogenic sources. As another important source of tropospheric ozone, the stratospheric intrusion (SI), however, has been less concerned. This study investigates the SI events over the Yangtze River Delta in eastern China using the newest ERA5 (the fifth generation of ECMWF atmospheric reanalysis) meteorological and ozone data, the In-service Aircraft for a Global Observing System (IAGOS) ozone profiles and the station-based ground-level ozone measurements. Results indicate that SI plays important roles in spring and summer ozone pollution episodes over the Yangtze River Delta, eastern China. Based on CAM-Chem (the Community Atmosphere Model with Chemistry) and LPDM (Lagrangian Particle Dispersion Modeling) model simulations, we found that deep SIs contribute ~15 ppbv in spring and ~10 ppbv in summer to surface ozone variations in eastern China. A deep SI event occurred in 2018 spring associated with a strong horizontal-trough, which brought ozone-rich air from the stratosphere to the troposphere and resulted in severe surface ozone pollution over the Yangtze River Delta. From 7-year statistics, we found that strong SI events during summer are associated with a cyclonic valley between the South Asian High and the Subtropical High, accompanied by downward fast transport of ozone from the stratosphere to the troposphere. Our results provide important information for surface ozone prediction and control in eastern China.</span></p>

scholarly journals Transport analysis of ozone enhancement in Southern Ontario during BAQS-Met

2011 ◽  
Vol 11 (6) ◽  
pp. 2569-2583 ◽  
Author(s):  
H. He ◽  
D. W. Tarasick ◽  
W. K. Hocking ◽  
T. K. Carey-Smith ◽  
Y. Rochon ◽  
...  
Keyword(s):  
Air Quality ◽  
Numerical Models ◽  
Stratospheric Ozone ◽  
Weather Prediction ◽  
Surface Ozone ◽  
Air Quality Model ◽  
Quality Model ◽  
Stratospheric Intrusion ◽  
Continuous Surface ◽  
Consistent Picture

Abstract. Twice-daily ozonesondes were launched from Harrow, in southwestern Ontario, Canada, during the BAQS-Met (Border Air Quality and Meteorology Study) field campaign in June and July of 2007. A co-located radar windprofiler measured tropopause height continuously. These data, in combination with continuous surface ozone measurements and geo-statistical interpolation of satellite ozone observations, present a consistent picture and indicate that a number of significant ozone enhancements in the troposphere were observed that were the result of stratospheric intrusion events. The combined observations have also been compared with results from two Environment Canada numerical models, the operational weather prediction model GEM (as input to FLEXPART), and a new version of the regional air quality model AURAMS, in order to examine the ability of these models to accurately represent sporadic cross-tropopause ozone transport events. The models appear to reproduce intrusion events with some skill, implying that GEM dynamics (which also drive AURAMS) are able to represent such events well. There are important differences in the quantitative comparison, however; in particular, the poor vertical resolution of AURAMS around the tropopause causes it to bring down too much ozone in individual intrusions. These campaign results imply that stratospheric intrusions are important to the ozone budget of the mid-latitude troposphere, and appear to be responsible for much of the variability of ozone in the free troposphere. GEM-FLEXPART calculations indicate that stratospheric ozone intrusions contributed significantly to surface ozone on several occasions during the BAQS-Met campaign, and made a moderate but significant contribution to the overall tropospheric ozone budget.

scholarly journals Local and synoptic meteorological influences on daily variability in summertime surface ozone in eastern China

2020 ◽  
Vol 20 (1) ◽  
pp. 203-222 ◽  
Author(s):  
Han Han ◽  
Jane Liu ◽  
Lei Shu ◽  
Tijian Wang ◽  
Huiling Yuan
Keyword(s):  
Surface Ozone ◽  
Eastern China ◽  
River Delta ◽  
Daily Maximum ◽  
Ozone Pollution ◽  
Study Region ◽  
Synoptic Weather ◽  
Daily Variability ◽  
Influential Variable ◽  
The Impact

Abstract. Ozone pollution in China is influenced by meteorological processes on multiple scales. Using regression analysis and weather classification, we statistically assess the impacts of local and synoptic meteorology on daily variability in surface ozone in eastern China in summer during 2013–2018. In this period, summertime surface ozone in eastern China (20–42∘ N, 110–130∘ E) is among the highest in the world, with regional means of 73.1 and 114.7 µg m−3, respectively, in daily mean and daily maximum 8 h average. Through developing a multiple linear regression (MLR) model driven by local and synoptic weather factors, we establish a quantitative linkage between the daily mean ozone concentrations and meteorology in the study region. The meteorology described by the MLR can explain ∼43 % of the daily variability in summertime surface ozone across eastern China. Among local meteorological factors, relative humidity is the most influential variable in the center and south of eastern China, including the Yangtze River Delta and the Pearl River Delta regions, while temperature is the most influential variable in the north, covering the Beijing–Tianjin–Hebei region. To further examine the synoptic influence of weather conditions explicitly, six predominant synoptic weather patterns (SWPs) over eastern China in summer are objectively identified using the self-organizing map clustering technique. The six SWPs are formed under the integral influence of the East Asian summer monsoon, the western Pacific subtropical high, the Meiyu front, and the typhoon activities. On average, regionally, two SWPs bring about positive ozone anomalies (1.1 µg m−3 or 1.7 % and 2.7 µg m−3 or 4.6 %), when eastern China is under a weak cyclone system or under the prevailing southerly wind. The impact of SWPs on the daily variability in surface ozone varies largely within eastern China. The maximum impact can reach ±8 µg m−3 or ±16 % of the daily mean in some areas. A combination of the regression and the clustering approaches suggests a strong performance of the MLR in predicting the sensitivity of surface ozone in eastern China to the variation of synoptic weather. Our assessment highlights the importance of meteorology in modulating ozone pollution over China.

scholarly journals Stratospheric ozone changes under solar geoengineering: implications for UV exposure and air quality

2016 ◽  
Vol 16 (6) ◽  
pp. 4191-4203 ◽  
Author(s):  
Peer Johannes Nowack ◽  
Nathan Luke Abraham ◽  
Peter Braesicke ◽  
John Adrian Pyle
Keyword(s):  
Air Quality ◽  
Atmospheric Carbon Dioxide ◽  
Climate Model ◽  
Stratospheric Ozone ◽  
Surface Ozone ◽  
Atmospheric Composition ◽  
Specific Humidity ◽  
Uv Exposure ◽  
Solar Radiation Management ◽  
Global Mean

Abstract. Various forms of geoengineering have been proposed to counter anthropogenic climate change. Methods which aim to modify the Earth's energy balance by reducing insolation are often subsumed under the term solar radiation management (SRM). Here, we present results of a standard SRM modelling experiment in which the incoming solar irradiance is reduced to offset the global mean warming induced by a quadrupling of atmospheric carbon dioxide. For the first time in an atmosphere–ocean coupled climate model, we include atmospheric composition feedbacks for this experiment. While the SRM scheme considered here could offset greenhouse gas induced global mean surface warming, it leads to important changes in atmospheric composition. We find large stratospheric ozone increases that induce significant reductions in surface UV-B irradiance, which would have implications for vitamin D production. In addition, the higher stratospheric ozone levels lead to decreased ozone photolysis in the troposphere. In combination with lower atmospheric specific humidity under SRM, this results in overall surface ozone concentration increases in the idealized G1 experiment. Both UV-B and surface ozone changes are important for human health. We therefore highlight that both stratospheric and tropospheric ozone changes must be considered in the assessment of any SRM scheme, due to their important roles in regulating UV exposure and air quality.

Summertime surface ozone variation over East Asia in CCMI

2020 ◽  
Author(s):  
Jieun Wie ◽  
Hyo-Jin Park ◽  
Hyomee Lee ◽  
Byung-Kwon Moon
Keyword(s):  
East Asia ◽  
Climate Model ◽  
Southern Oscillation ◽  
Surface Ozone ◽  
Eastern China ◽  
Empirical Orthogonal Functions ◽  
Ozone Production ◽  
Shortwave Radiation ◽  
Horizontal Wind ◽  
Second Mode

<p>The concentration of surface ozone in East Asia is high due to strong solar radiation, but decreases in areas affected by summer monsoons. This study analyzes the summer surface ozone variations in East Asia using meteorological and atmospheric chemistry variables in 12 models participating in Chemistry-Climate Model Initiative (CCMI) for the period of 1979 to 2010. The concentration of 850 hPa ozone was identified two modes by Empirical Orthogonal Functions (EOF) analysis. The first mode is an increase in all regions over East Asia, mainly in eastern China. This mode was associated with downward wind, weak horizontal wind speed, increase in temperatures, decrease in precipitation. The second mode showed high ozone concentrations in eastern China and low in northern Japan. In eastern China, temperatures and precipitation are decreased, and shortwave radiation reaches the surface is increased. In addition, the concentration of nitrogen oxides and carbon monoxide and the net ozone production are increased. The second mode was highly correlated with El Nino-Southern Oscillation (ENSO) and western North Pacific subtropical high (WNPSH) indices and was found to be closely associated with East Asian summer monsoons.</p><p> </p><p>Acknowledgements: This work was supported by a National Research Foundation of Korea (NRF) grant funded by the Korean government (MSIT) (No. 2019R1A2C1008549). We acknowledge the modeling groups for making their simulations available for this analysis, the joint WCRP SPARC/IGAC Chemistry–Climate Model Initiative (CCMI) for organizing and coordinating the model simulations and data analysis activity, and the British Atmospheric Data Centre (BADC) for collecting and archiving the CCMI model output.</p>

scholarly journals Influence of Stratospheric Intrusion on the Surface Ozone Levels in India

2012 ◽  
Vol 2012 ◽  
pp. 1-7 ◽  
Author(s):  
Nandita D. Ganguly
Keyword(s):  
Stratospheric Ozone ◽  
Surface Ozone ◽  
High Surface ◽  
Living System ◽  
Transport Processes ◽  
Stratospheric Intrusion ◽  
Life On Earth ◽  
Indian Cities ◽  
Enhanced Surface ◽  
Ozone Levels

The surface ozone levels in some Indian cities have increased significantly in the recent years. Ozone being toxic to the living system and an important contributor to anthropogenic global warming, enhanced surface ozone may have adverse effects on the air quality and climate. Transport of ozone from the stratosphere to the troposphere causes stratospheric ozone to decrease and tropospheric ozone to increase, which can in turn have serious consequences for life on earth. Since stratosphere-troposphere exchange (STE) is an important factor influencing the ozone concentration in the troposphere, this paper investigates probably for the first time the possible contribution of STE events to the observed enhanced surface ozone levels for cities covering from north to south of India. It is concluded that apart from transport processes and in situ photochemical production, STE also influences the observed high-surface ozone levels in Indian cities to a small extent (8%–16%). STE events producing high-surface ozone levels are found to be higher at high latitudes.

scholarly journals Dominant patterns of summer ozone pollution in eastern China and associated atmospheric circulations

2019 ◽  
Vol 19 (22) ◽  
pp. 13933-13943 ◽  
Author(s):  
Zhicong Yin ◽  
Bufan Cao ◽  
Huijun Wang
Keyword(s):  
North China ◽  
Surface Ozone ◽  
Eastern China ◽  
Western Pacific Subtropical High ◽  
Ground Level ◽  
Photochemical Reactions ◽  
Western Pacific ◽  
Subtropical High ◽  
Ozone Pollution ◽  
Atmospheric Circulations

Abstract. Surface ozone has been severe during summers in the eastern parts of China, damaging human health and flora and fauna. During 2015–2018, ground-level ozone pollution increased and intensified from south to north. In North China and the Huanghuai region, the O3 concentrations were highest. Two dominant patterns of summer ozone pollution were determined, i.e., a south–north covariant pattern and a south–north differential pattern. The anomalous atmospheric circulations composited for the first pattern manifested as a zonally enhanced East Asian deep trough and as a western Pacific subtropical high, whose western ridge point shifted northward. The local hot, dry air and intense solar radiation enhanced the photochemical reactions to elevate the O3 pollution levels in North China and the Huanghuai region; however, the removal of pollutants was decreased. For the second pattern, the broad positive geopotential height anomalies at high latitudes significantly weakened cold air advection from the north, and those extending to North China resulted in locally high temperatures near the surface. In a different manner, the western Pacific subtropical high transported sufficient water vapor to the Yangtze River Delta and resulted in a locally adverse environment for the formation of surface ozone. In addition, the most dominant pattern in 2017 and 2018 was different from that in previous years, which is investigated as a new feature.

The stratospheric ozone rich cold intrusion during El-Nino over the Indian region: implication during the Indian summer monsoon

2020 ◽  
Author(s):  
Chaitri Roy ◽  
Suvarna Fadnavis ◽  
Sabin Thazhe Purayil
Keyword(s):  
Radiative Forcing ◽  
Climate Model ◽  
Wave Train ◽  
Stratospheric Ozone ◽  
Surface Ozone ◽  
North India ◽  
Cold Wave ◽  
Upper Troposphere ◽  
Rainfall Condition ◽  
Stratospheric Intrusions

<p>Ozone in the upper troposphere is a dominant radiative constituent.  In this study, we investigate ozone variability due to stratospheric intrusions in the upper troposphere over India, and its associated radiative impacts during monsoon breaks co-occurring with El Niño. For this purpose, we use the ECHAM5-HAMMOZ, Global-Chemistry-climate model simulations, and ERA-Interim reanalysis data. Our analysis shows that during El Niño deep stratospheric intrusions, occurring at the North India - Tibetan Plateau (NI-TP) region and the western edge of the monsoon anticyclone, lead to an enormous increase in ozone amounts (~160 ppb) in the upper troposphere over India. These intrusions elevate the surface ozone levels by ~20 ppb and ozone radiative forcing by ~0.33 W m<sup>-2</sup> at the top of the atmosphere (TOA). </p><p>Interestingly, the stratospheric intrusions are associated with a wave train composed of cyclonic and anticyclonic circulation in the upper troposphere, emanating from El-Niño region in the east Pacific, traversing towards NI-TP locale. The wave train transports extra-tropical cold air mass, producing an anomalous cooling of ~2 - 3 K in the upper troposphere over NI-TP. The cold wave train induces Rossby wave breaking (RWB), which facilitates stratospheric intrusions, thereby enhancing subsidence over NI-TP region. Additionally, this severe cold subsidence over North India during break days may further intensify the deficit rainfall condition during break days.</p>

scholarly journals Global distribution of tropospheric ozone from satellite measurements using the empirically corrected tropospheric ozone residual technique: Identification of the regional aspects of air pollution

2003 ◽  
Vol 3 (4) ◽  
pp. 893-907 ◽  
Author(s):  
J. Fishman ◽  
A. E. Wozniak ◽  
J. K. Creilson
Keyword(s):  
Tropospheric Ozone ◽  
Total Ozone ◽  
Stratospheric Ozone ◽  
Eastern China ◽  
Daily Basis ◽  
Stratospheric Aerosol ◽  
Eastern United States ◽  
Ozone Pollution ◽  
Austral Spring ◽  
Data Set

Abstract. Using coincident observations of total ozone from the Total Ozone Mapping Spectrometer (TOMS) and stratospheric ozone profiles from the Solar Backscattered Ultraviolet (SBUV) instruments, detailed maps of tropospheric ozone have been derived on a daily basis over a time period spanning more than two decades. The resultant climatological seasonal depictions of the tropospheric ozone residual (TOR) show much more detail than an earlier analysis that had used coincident TOMS and Stratospheric Aerosol and Gas Experiment (SAGE) ozone profiles, although there are many similarities between the TOMS/SAGE TOR and the TOMS/SBUV TOR climatologies. In particular, both TOR seasonal depictions show large enhancements in the southern tropics and subtropics in austral spring and at northern temperate latitudes during the summer. The much greater detail in this new data set clearly defines the regional aspect of tropospheric ozone pollution in northeastern India, eastern United States, eastern China, and west and southern Africa. Being able to define monthly climatologies for each year of the data record provides enough temporal resolution to illustrate significant interannual variability in some of these regions.

scholarly journals Spatial distribution and temporal trend of ozone pollution in China observed with the OMI satellite instrument, 2005–2017

2018 ◽  
Author(s):  
Lu Shen ◽  
Daniel J. Jacob ◽  
Xiong Liu ◽  
Guanyu Huang ◽  
Ke Li ◽  
...  
Keyword(s):  
Surface Ozone ◽  
Eastern China ◽  
Ozone Pollution ◽  
The North ◽  
The Pacific ◽  
Extreme Value Model ◽  
The Individual ◽  
Value Model ◽  
Ozone Episodes ◽  
Ozone Episode

Abstract. We use data from the new China Ministry of Ecology and Environment (MEE) network to show that OMI satellite observations of tropospheric ozone can successfully map the distribution of surface ozone pollution in China and the frequency of high-ozone episodes. After subtracting the Pacific background, OMI ozone enhancements over China can quantify mean summer afternoon surface ozone with a precision of 10.7 ppb and a spatial correlation coefficient R=0.73. Day-to-day correlations between OMI and the MEE ozone data are statistically significant but limited by noise in the individual OMI retrievals. OMI shows significantly higher values on surface ozone episode days (>82 ppb). An extreme value model can successfully predict the probability of surface ozone episodes from the daily OMI data. The 2005–2017 OMI record shows a 0.67 ppb a−1 increase in mean summer afternoon ozone in eastern China and an increasing frequency of ozone pollution episodes particularly in the north.

Sign in / Sign up

Export Citation Format

Share Document