scholarly journals Spatial and Temporal Characteristics of Environmental Air Quality and Its Relationship with Seasonal Climatic Conditions in Eastern China during 2015–2018

Author(s):  
Zhiyuan Wang ◽  
Xiaoyi Shi ◽  
Chunhua Pan ◽  
Sisi Wang

Exploring the relationship between environmental air quality (EAQ) and climatic conditions on a large scale can help better understand the main distribution characteristics and the mechanisms of EAQ in China, which is significant for the implementation of policies of joint prevention and control of regional air pollution. In this study, we used the concentrations of six conventional air pollutants, i.e., carbon monoxide (CO), sulfur dioxide (SO2), nitrogen dioxide (NO2), fine particulate matter (PM2.5), coarse particulate matter (PM10), and ozone (O3), derived from about 1300 monitoring sites in eastern China (EC) from January 2015 to December 2018. Exploiting the grading concentration limit (GB3095-2012) of various pollutants in China, we also calculated the monthly average air quality index (AQI) in EC. The results show that, generally, the EAQ has improved in all seasons in EC from 2015 to 2018. In particular, the concentrations of conventional air pollutants, such as CO, SO2, and NO2, have been decreasing year by year. However, the concentrations of particulate matter, such as PM2.5 and PM10, have changed little, and the O3 concentration increased from 2015 to 2018. Empirical mode decomposition (EOF) was used to analyze the major patterns of AQI in EC. The first mode (EOF1) was characterized by a uniform structure in AQI over EC. These phenomena are due to the precipitation variability associated with the East Asian summer monsoon (EASM), referred to as the “summer–winter” pattern. The second EOF mode (EOF2) showed that the AQI over EC is a north–south dipole pattern, which is bound by the Qinling Mountains and Huaihe River (about 35° N). The EOF2 is mainly caused by seasonal variations of the mixed concentration of PM2.5 and O3. Associated with EOF2, the Mongolia–Siberian High influences the AQI variation over northern EC by dominating the low-level winds (10 m and 850 hPa) in autumn and winter, and precipitation affects the AQI variation over southern EC in spring and summer.

2017 ◽  
Vol 17 (11) ◽  
pp. 7261-7276 ◽  
Author(s):  
Tobias Wolf-Grosse ◽  
Igor Esau ◽  
Joachim Reuder

Abstract. Street-level urban air pollution is a challenging concern for modern urban societies. Pollution dispersion models assume that the concentrations decrease monotonically with raising wind speed. This convenient assumption breaks down when applied to flows with local recirculations such as those found in topographically complex coastal areas. This study looks at a practically important and sufficiently common case of air pollution in a coastal valley city. Here, the observed concentrations are determined by the interaction between large-scale topographically forced and local-scale breeze-like recirculations. Analysis of a long observational dataset in Bergen, Norway, revealed that the most extreme cases of recurring wintertime air pollution episodes were accompanied by increased large-scale wind speeds above the valley. Contrary to the theoretical assumption and intuitive expectations, the maximum NO2 concentrations were not found for the lowest 10 m ERA-Interim wind speeds but in situations with wind speeds of 3 m s−1. To explain this phenomenon, we investigated empirical relationships between the large-scale forcing and the local wind and air quality parameters. We conducted 16 large-eddy simulation (LES) experiments with the Parallelised Large-Eddy Simulation Model (PALM) for atmospheric and oceanic flows. The LES accounted for the realistic relief and coastal configuration as well as for the large-scale forcing and local surface condition heterogeneity in Bergen. They revealed that emerging local breeze-like circulations strongly enhance the urban ventilation and dispersion of the air pollutants in situations with weak large-scale winds. Slightly stronger large-scale winds, however, can counteract these local recirculations, leading to enhanced surface air stagnation. Furthermore, this study looks at the concrete impact of the relative configuration of warmer water bodies in the city and the major transport corridor. We found that a relatively small local water body acted as a barrier for the horizontal transport of air pollutants from the largest street in the valley and along the valley bottom, transporting them vertically instead and hence diluting them. We found that the stable stratification accumulates the street-level pollution from the transport corridor in shallow air pockets near the surface. The polluted air pockets are transported by the local recirculations to other less polluted areas with only slow dilution. This combination of relatively long distance and complex transport paths together with weak dispersion is not sufficiently resolved in classical air pollution models. The findings have important implications for the air quality predictions over urban areas. Any prediction not resolving these, or similar local dynamic features, might not be able to correctly simulate the dispersion of pollutants in cities.


Author(s):  
Janis Kleperis ◽  
Gunars Bajars ◽  
Ingrida Bremere ◽  
Martins Menniks ◽  
Arturs Viksna ◽  
...  

Air Quality in Riga and Its Improvement Options Air quality in the city of Riga is evaluated from direct monitoring results and from accounting registered air pollutants in the city. It is concluded that from all air polluting substances listed in the European Commission directives, only nitrogen dioxide NO2 and particulate matter PM10 exceed the limits. In assessing the projected measures to improve air quality in Riga, it can be concluded that the implementation of cleaner fuels and improvements in energy efficiency of household and industrial sectors will decrease particle pollution, but measures in the transport sector will also contribute to reducing air pollution from nitrogen oxides.


2021 ◽  
Author(s):  
Drew C. Pendergrass ◽  
Daniel J. Jacob ◽  
Shixian Zhai ◽  
Jhoon Kim ◽  
Ja-Ho Koo ◽  
...  

Abstract. We use 2011–2019 aerosol optical depth (AOD) observations from the Geostationary Ocean Color Imager (GOCI) instrument over East Asia to infer 24-h daily surface fine particulate matter (PM2.5) concentrations at continuous 6x6 km2 resolution over eastern China, South Korea, and Japan. This is done with a random forest (RF) algorithm applied to the gap-filled GOCI AODs and other data and trained with PM2.5 observations from the three national networks. The predicted 24-h PM2.5 concentrations for sites entirely withheld from training in a ten-fold crossvalidation procedure correlate highly with network observations (R2 = 0.89) with single-value precision of 26–32 % depending on country. Prediction of annual mean values has R2 = 0.96 and single-value precision of 12 %. The RF algorithm is only moderately successful for diagnosing local exceedances of the National Ambient Air Quality Standard (NAAQS) because these exceedances are typically within the single-value precisions of the RF, and also because of RF smoothing of extreme PM2.5 concentrations. The area-weighted and population-weighted trends of RF PM2.5 concentrations for eastern China, South Korea, and Japan show steady 2015–2019 declines consistent with surface networks, but the surface networks in eastern China and South Korea underestimate population exposure. Further examination of RF PM2.5 fields for South Korea identifies hotspots where surface network sites were initially lacking and shows 2015–2019 PM2.5 decreases across the country except for flat concentrations in the Seoul metropolitan area. Inspection of monthly PM2.5 time series in Beijing, Seoul, and Tokyo shows that the RF algorithm successfully captures observed seasonal variations of PM2.5 even though AOD and PM2.5 often have opposite seasonalities. Application of the RF algorithm to urban pollution episodes in Seoul and Beijing demonstrates high skill in reproducing the observed day-to-day variations in air quality as well as spatial patterns on the 6 km scale. Comparison to a CMAQ simulation for the Korean peninsula demonstrates the value of the continuous RF PM2.5 fields for testing air quality models, including over North Korea where they offer a unique resource.


Author(s):  
Edmilson D. Freitas ◽  
Sergio A. Ibarra-Espinosa ◽  
Mario E. Gavidia-Calderón ◽  
Amanda Rehbein ◽  
Sameh A. Abou Rafee ◽  
...  

Social distancing policies put in place during COVID-19 epidemic in addition to helping to limit the spread of the disease also contributed to improving urban air quality. Here we show a decrease in air pollutant concentration as a consequence of mobility reduction in São Paulo during the containment measure which began on 22nd March 2020. When comparing to foregoing weeks to equivalent periods of 2019, the concentration of most air pollutants sharply decreased in the first days of mobility restriction, to then increase again after government officials downplayed the threat of the disease. This trend is also followed by a decrease in hospital admissions by SARS-influenza. Therefore, despite the great economic and social unrest caused by the pandemic, this unique situation shows that large-scale mobility reduction policy had a significant impact on air quality, benefiting, directly and indirectly, the public health system.


2020 ◽  
Vol 20 (10) ◽  
pp. 5899-5909 ◽  
Author(s):  
Yucong Miao ◽  
Huizheng Che ◽  
Xiaoye Zhang ◽  
Shuhua Liu

Abstract. Rapid urbanization and industrialization have led to deterioration of air quality in the Beijing–Tianjin–Hebei (BTH) region due to high loadings of PM2.5. Heavy aerosol pollution frequently occurs in winter, in close relation to the planetary boundary layer (PBL) meteorology. To unravel the physical processes that influence PBL structure and aerosol pollution in BTH, this study combined long-term observational data analyses, synoptic pattern classification, and meteorology–chemistry coupled simulations. During the winter of 2017 and 2018, Beijing and Tangshan often experienced heavy PM2.5 pollution simultaneously, accompanied by strong thermal inversion aloft. These concurrences of pollution in different cities were primarily regulated by the large-scale synoptic conditions. Using principal component analysis with geopotential height fields at the 850 hPa level during winter, two typical synoptic patterns associated with heavy pollution in BTH were identified. One pattern is characterized by a southeast-to-north pressure gradient across BTH, and the other is associated with high pressure in eastern China. Both synoptic types feature warmer air temperature at 1000 m a.g.l., which could suppress the development of the PBL. Under these unfavorable synoptic conditions, aerosols can modulate PBL structure through the radiative effect, which was examined using numerical simulations. The aerosol radiative effect can significantly lower the daytime boundary layer height through cooling the surface layer and heating the upper part of the PBL, leading to the deterioration of air quality. This PBL–aerosol feedback is sensitive to the aerosol vertical structure, which is more effective when the synoptic pattern can distribute more aerosols to the upper PBL.


2020 ◽  
Vol 24 (2) ◽  
pp. 373-379
Author(s):  
I.B. Abaje ◽  
Y. Bello ◽  
S.A. Ahmad

This study generally classifies air pollutants on the basis of: primary or secondary, natural or anthropogenic, chemical composition, physical state, and the space scales of their effects. Air pollutants that affect air quality in Nigeria were discussed based on natural and anthropogenic sources. The natural sources include: sand dust, sea spray, volcanic activities, smoke and carbon monoxide from wildfires among others, while the anthropogenic sources include: vehicular emissions, mining activities, industries such as cement companies and quarry factories, agricultural practices and solid waste dumps among others. Some of the atmospheric pollutants that posed greatest threat to human health were equally examined. They include: Sulphur dioxide (SO2) which can react with water vapor (H2O) in the atmosphere to form sulphuric acid (H2SO4) and thus acid rain; particulate matter (PM) with less than 10 μm, particularly fine particles (PM2.5 ) and particles in the fine fraction that are smaller than 0.1 μm (ultrafine particles), can carry toxic chemicals which are linked to cancer; carbon monoxide (CO), even in very small concentrations, can prevent oxygen from being delivered through the body major organs; ozone which is a highly reactive gas causes oxidation of a number of macromolecules within a biological system and produces free radicals that can damage DNA molecules and cause carcinogenesis. Based on the aforementioned, this study recommends that priority should be given to the establishment of air monitoring stations in all urban centers of the country in order to provide accurate and continuous information on air quality. Keywords: anthropogenic pollutants, atmosphere, particulate matter, pollution


2020 ◽  
Author(s):  
Jana Handschuh ◽  
Frank Baier ◽  
Thilo Erbertseder ◽  
Martijn Schaap

<p>Particulate matter and other air pollutants have become an increasing burden on the environment and human health. Especially in metropolitan and high-traffic areas, air quality is often remarkably reduced. For a better understanding of the air quality in specific areas, which is of great environment-political interest, data with high resolution in space and time is required. The combination of satellite observations and chemistry-transport-modelling has proven to give a good database for assessments and analyses of air pollution. In contrast to sample in-situ measurements, satellite observations provide area-wide coverage ​​of measurements and thus the possibility for an almost gapless mapping of actual air pollutants. For a high temporal resolution, chemistry-transport-models are needed, which calculate concentrations of specific pollutants in continuous time steps. Satellite observations can thus be used to improve model performances.</p><p>There are no direct satellite-measurements of fine particulate matter (PM2.5) but ground-level concentrations of PM2.5 can be derived from optical parameters such as aerosol optical depth (AOD). A wide range of methods for the determination of PM2.5 concentrations from AOD measurements has been developed so far, but it is still a big challenge. In this study a semi-empirical approach based on the physical relationships between meteorological and optical parameters was applied to determine a first-guess of ground-level PM2.5 concentrations for the year 2018 and the larger Germany region. Therefor AOD observations of MODIS (Moderate Resolution Imaging Spectroradiometer) aboard the NASA Aqua satellite were used in a spatial resolution of 3km. First results showed an overestimation of ground-level aerosols and quiet low correlations with in-situ station measurements from the European Environmental Agency (EEA). To improve the results, correction factors were calculated using the coefficients of linear regression between satellite-based and in-situ measured particulate matter concentrations. Spatial and seasonal dependencies were taken into account with it. Correlations between satellite and in-situ measurements could be improved applying this method.</p><p>The MODIS 3km AOD product was found to be a good base for area-wide calculations of ground-level PM2.5 concentrations. First comparisons to the calculated PM2.5 concentrations from chemistry-transport-model POLYPHEMUS/DLR showed significant differences though. Satellite observations will now be used to improve the general model performance, first by helping to find and understand regional and temporal dependencies in the differences. As part of the German project S-VELD funded by the Federal Ministry of Transport and Digital Infrastructure BMVI, it will help for example to adjust the derivation of particle emissions within the model.</p>


Atmosphere ◽  
2021 ◽  
Vol 12 (5) ◽  
pp. 532
Author(s):  
David Olukanni ◽  
David Enetomhe ◽  
Gideon Bamigboye ◽  
Daniel Bassey

Vehicle emissions have become one of the most prevailing air contamination sources, including nitrogen oxides, volatile organic compounds, carbon monoxide and particulate matter (PM). Among other air pollutants, PM limits visible sight distance and poses health risks upon inhalation into the human body. This study focused on assessing PM2.5 concentrations in air at different periods of the day at the highly trafficked grade-separated intersection of Sango-Ota, Ogun State, Nigeria. PM2.5 readings were taken at three at-grade points around the intersection’s roundabout between 10:00 a.m. and 5:00 p.m. for four (4) days using the BR-SMART-126 Portable 4-in-1 air quality monitor. The highest level of PM2.5 obtained on Day 1 (Monday) and Day 4 (Thursday) was about 45.1% and 38.6%, respectively, lower than that of Day 3 (Wednesday). The highest concentrations of PM2.5 were recorded between 11:00 and 13:00 and between 16:00 and 18:00 (up to 217 µg/m3) whereas the lowest levels were recorded between 14:00 and 15:00 (as low as 86 µg/m3). The concentration of PM2.5 at the Sango-Ota intersection is adjudged “very poor” with average hourly concentrations between 97 and 370 µg/m3. Outcomes obtained indicate the need for improved measures to control air quality along major road corridors and at intersections in Ogun State and Nigeria at large.


Atmosphere ◽  
2021 ◽  
Vol 12 (2) ◽  
pp. 267 ◽  
Author(s):  
Shuyi Jiang ◽  
Chuanfeng Zhao ◽  
Hao Fan

Associated with the outbreak of new coronavirus in 2019 (COVID-19), lockdown measures were taken in spring 2020 in China, providing an ideal experiment to investigate the effects of emission controls on air quality. Using the observation data at 56 stations in Hebei province from the China National Environmental Monitoring Center from January 2019 to May 2020, along with the reanalysis meteorology data from ERA5, this study investigates the spatial and temporal variations of six air pollutants, and the clean and pollution events in COVID-19 period. Compared with the same periods in day and month in 2019 (SP19), the concentrations of sulfur dioxide (SO2), nitrogen dioxide (NO2), particulate matter with an aerodynamic diameter of less than 10 μm (PM10), particulate matter with an aerodynamic diameter of less than 2.5 μm (PM2.5), and carbon monoxide (CO) decreased by 39.2%, 38.2%, 42.1%, 39.8%, and 24.8% for lockdown period, respectively; and decreased by 13.7%, 8.9%, 16.8%, 13.4%, and 10.6% for post-lockdown period, respectively. In contrast, ozone (O3) increased by 8.0% and 5.5% for lockdown and post-lockdown periods, respectively. The diurnal variation analysis shows that the air pollutants other than O3 decrease more in the morning time (6:00–10:00 local time) than in the afternoon time (14:00–18:00 local time) during both lockdown and post-lockdown periods compared to SP19, implying the potential contribution from pollution-meteorology interaction. After lockdown period, SO2 and NO2 resumed quickly in most cities other than in Zhangjiakou, which is a city with few industries making it more sensitive to meteorology. The significant improvement of air quality during the lockdown period suggests that the whole air quality is highly dependent on the pollutant emissions, while the relatively weak reduction of pollution events imply that the pollution events are more dependent on adverse weather conditions.


Author(s):  
Marjan Senegačnik ◽  
Davorin Žnidarič ◽  
Drago Vuk

In 2020 the entire world was severely affected by COVID -19 epidemics. Because of preventing of the SARS Cov 2 virus spread there was necessary to introduce considerable restrictions of movement of citizens. This resulted in various negative effects in the field of economy. However, as road traffic is an important source of pollution – particularly of emissions of air pollutants and greenhouse gases it could be expected that these mobility restrictions result in certain positive effects on the environment. The paper will try to estimate the air quality during the period of epidemics when mobility was severely restricted (second half of March and April 2020, second half of October, November and December 2020). The review will be limited to those kinds of pollutants which are particularly related to road traffic (nitrogen oxides, particulate matter, ozone) as well as to carbon dioxide as the most important greenhouse gas.


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