scholarly journals Global Aerosol Classification Based on Aerosol Robotic Network (AERONET) and Satellite Observation

2021 ◽  
Vol 13 (6) ◽  
pp. 1114
Author(s):  
Jianyu Lin ◽  
Yu Zheng ◽  
Xinyong Shen ◽  
Lizhu Xing ◽  
Huizheng Che
Keyword(s):  
Radiative Forcing ◽  
Temporal Distribution ◽  
Satellite Observation ◽  
Western Africa ◽  
Deep Blue ◽  
Sensing Technology ◽  
Aerosol Classification ◽  
Linear Depolarization Ratio ◽  
Absorbing Aerosols ◽  
Single Scatter

The particle linear depolarization ratio (PLDR) and single scatter albedo (SSA) in 1020 nm from the Aerosol Robotic Network (AERONET) level 2.0 dataset was utilized among 52 stations to identify dust and dust dominated aerosols (DD), pollution dominated mixture (PDM), strongly absorbing aerosols (SA) and weakly absorbing aerosols (WA), investigate their spatial and temporal distribution, net radiative forcing and radiative forcing efficiency in global range, and further compare with VIIRS Deep Blue Production. The conclusion about net radiative forcing suggests that the high values of radiative forcing from dust and dust dominated aerosols, pollution dominated mixture both mainly come from western Africa. Strongly absorbing aerosols in South Africa and India contribute greatly to the net radiative forcing and the regions with relative high values of weakly absorbing aerosols are mainly located at East Asia and India. Lastly, the observation of VIIRS Deep Blue satellite monthly averaged products depicts the characteristics about spatial distribution of four kinds of aerosol well, the result from ground-based observation presents great significant to validate the measurements from remote sensing technology.

scholarly journals Impact of absorbing and non-absorbing aerosols on radiation and low-level clouds over the Southeast Atlantic from co-located satellite observations

2020 ◽  
Author(s):  
Alejandro Baró Pérez ◽  
Abhay Devasthale ◽  
Frida Bender ◽  
Annica M. L. Ekman
Keyword(s):  
Satellite Observation ◽  
Clear Correlation ◽  
Heating Rates ◽  
Cooling Rates ◽  
Thermodynamic Structure ◽  
Aerosol Loading ◽  
Stratocumulus Clouds ◽  
Aerosol Classification ◽  
Absorbing Aerosols ◽  
Aerosol Type

Abstract. We use data derived from instruments onboard the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO) and CloudSat satellites as well as meteorological parameters from reanalysis to explore situations when moist aerosol layers overlie stratocumulus clouds over the Southeast Atlantic during the biomass burning season (June to October). One main goal is to separate and quantify the impacts of aerosol loading, aerosol type, and humidity on the radiative fluxes, including cloud top cooling. To achieve our objectives we split the data into different levels of aerosol and moisture loadings. By using the aerosol classification available from the CALIPSO products, we also separate and compare situations with pristine air, with smoke, and with other (mixed) types of aerosols. We find a substantial number of cases with mixed aerosols above clouds that occur under similar meteorological conditions as the smoke cases. In contrast, the meteorology is substantially different for the pristine situations, making a direct comparison with the aerosol cases ambiguous. The moisture content is enhanced within the aerosol layers, but we do not find a monotonous increase of the relative humidity with increasing aerosol optical depth. Shortwave (SW) heating rates within the moist aerosol plumes increase with increasing aerosol loading and are higher in the smoke cases compared to the mixed cases. However, there is no clear correlation between moisture changes and SW absorption. Cloud top cooling rates tend to decrease with increasing moisture within the overlying aerosol layers, but the influence is relatively weak and confounded by the strong variability of the cooling rates caused by other meteorological factors (most notably cloud top temperature). No clear influence of aerosol type or loading on cloud top cooling rates is detected. We also do not find any correlation between aerosol loading and the thermodynamic structure of the atmosphere nor the cloud top height, i.e. no indication of a semi-direct aerosol effect. This result is consistent with previous studies that examined clearly separated aerosol and cloud layers (in our case at least 0.4 km).

scholarly journals Aerosol Characteristics and Their Impact on the Himalayan Energy Budget

2021 ◽  
Vol 14 (1) ◽  
pp. 179
Author(s):  
Kesar Chand ◽  
Jagdish Chandra Kuniyal ◽  
Shruti Kanga ◽  
Raj Paul Guleria ◽  
Gowhar Meraj ◽  
...  
Keyword(s):  
Solar Radiation ◽  
Radiative Forcing ◽  
Satellite Observation ◽  
Transfer Model ◽  
Hysplit Model ◽  
Aerosol Radiative Forcing ◽  
Alpine Regions ◽  
Himalayan Glaciers ◽  
Moderate Resolution ◽  
Moderate Resolution Imaging Spectroradiometer

The extensive work on the increasing burden of aerosols and resultant climate implications shows a matter of great concern. In this study, we investigate the aerosol optical depth (AOD) variations in the Indian Himalayan Region (IHR) between its plains and alpine regions and the corresponding consequences on the energy balance on the Himalayan glaciers. For this purpose, AOD data from Moderate Resolution Imaging Spectroradiometer (MODIS, MOD-L3), Aerosol Robotic Network (AERONET), India, and Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO) were analyzed. Aerosol radiative forcing (ARF) was assessed using the atmospheric radiation transfer model (RTM) integrated into AERONET inversion code based on the Discrete Ordinate Radiative Transfer (DISORT) module. Further, air mass trajectory over the entire IHR was analyzed using a hybrid Single-Particle Lagrangian Integrated Trajectory (HYSPLIT) model. We estimated that between 2001 and 2015, the monthly average ARF at the surface (ARFSFC), top of the atmosphere (ARFTOA), and atmosphere (ARFATM) were −89.6 ± 18.6 Wm−2, −25.2 ± 6.8 Wm−2, and +64.4 ± 16.5 Wm−2, respectively. We observed that during dust aerosol transport days, the ARFSFC and TOA changed by −112.2 and −40.7 Wm−2, respectively, compared with low aerosol loading days, thereby accounting for the decrease in the solar radiation by 207% reaching the surface. This substantial decrease in the solar radiation reaching the Earth’s surface increases the heating rate in the atmosphere by 3.1-fold, thereby acting as an additional forcing factor for accelerated melting of the snow and glacier resources of the IHR.

scholarly journals A global survey of aerosol-liquid water cloud overlap based on four years of CALIPSO-CALIOP data

2011 ◽  
Vol 11 (3) ◽  
pp. 1143-1154 ◽  
Author(s):  
A. Devasthale ◽  
M. A. Thomas
Keyword(s):  
Liquid Water ◽  
Radiative Forcing ◽  
Feature Detection ◽  
Quality Criteria ◽  
Polar Regions ◽  
Hemispheric Differences ◽  
Aerosol Cloud ◽  
Water Cloud ◽  
Annual Means ◽  
Absorbing Aerosols

Abstract. Simulating the radiative impacts of aerosols located above liquid water clouds presents a significant challenge. In particular, absorbing aerosols, such as smoke, may have significant impact in such situations and even change the sign of net radiative forcing. It is not possible to reliably obtain information on such overlap events from existing passive satellite sensors. However, the CALIOP instrument onboard NASA's CALIPSO satellite allows us to examine these events with unprecedented accuracy. Using four years of collocated CALIPSO 5 km Aerosol and Cloud Layer Version 3 Products (June 2006–May 2010), we quantify, for the first time, the characteristics of overlapping aerosol and water cloud layers globally. We investigate seasonal variability in these characteristics over six latitude bands to understand the hemispheric differences when all aerosol types are included in the analysis (the AAO case). We also investigate frequency of smoke aerosol-cloud overlap (the SAO case). Globally, the frequency is highest during the JJA months in the AAO case, while for the SAO case, it is highest in the SON months. The seasonal mean overlap frequency can regionally exceed 20% in the AAO case and 10% in the SAO case. In about 5–10% cases the vertical distance between aerosol and cloud layers is less than 100 m, while about in 45–60% cases it less than a kilometer in the annual means for different latitudinal bands. In about 70–80% cases, aerosol layers are less than a kilometer thick, while in about 18–22% cases they are 1–2 km thick. The frequency of aerosol layers 2–3 km thick is about 4–5% in the tropical belts during overlap events. Over the regions where high aerosol loadings are present, the overlap frequency can be up to 50% higher when quality criteria on aerosol/cloud feature detection are relaxed. Over the polar regions, more than 50% of the overlapping aerosol layers have optical thickness less than 0.02, but the contribution from the relatively optically thicker aerosol layers increases towards the equatorial regions in both hemispheres. The results suggest that the frequency of occurrence of overlap events is far from being negligible globally.

scholarly journals Increased absorption by coarse aerosol particles over the Gangetic–Himalayan region

2014 ◽  
Vol 14 (3) ◽  
pp. 1159-1165 ◽  
Author(s):  
V. S. Manoharan ◽  
R. Kotamarthi ◽  
Y. Feng ◽  
M. P. Cadeddu
Keyword(s):  
Atmospheric Aerosols ◽  
Radiative Forcing ◽  
Climate Models ◽  
Monsoon Season ◽  
Regional Scale ◽  
Chemical Properties ◽  
Aerosol Forcing ◽  
Post Monsoon Season ◽  
Absorbing Aerosols ◽  
Coarse Aerosol

Abstract. Each atmospheric aerosol type has distinctive light-absorption characteristics related to its physical/chemical properties. Climate models treat black carbon as the main light-absorbing component of carbonaceous atmospheric aerosols, while absorption by some organic aerosols is also considered, particularly at ultraviolet wavelengths. Most absorbing aerosols are assumed to be < 1 μm in diameter (sub-micron). Here we present results from a recent field study in India, primarily during the post-monsoon season (October–November), suggesting the presence of absorbing aerosols sized 1–10 μm. Absorption due to super-micron-sized particles was nearly 30% greater than that due to smaller particles. Periods of increased absorption by larger particles ranged from a week to a month. Radiative forcing calculations under clear-sky conditions show that super-micron particles account for nearly 44% of the total aerosol forcing. The origin of the large aerosols is unknown, but meteorological conditions indicate that they are of local origin. Such economic and habitation conditions exist throughout much of the developing world. Hence, large absorbing particles could be an important component of the regional-scale atmospheric energy balance.

scholarly journals Impact of brown and clear carbon on light absorption enhancement, single scatter albedo and absorption wavelength dependence of black carbon

2010 ◽  
Vol 10 (9) ◽  
pp. 4207-4220 ◽  
Author(s):  
D. A. Lack ◽  
C. D. Cappa
Keyword(s):  
Black Carbon ◽  
Light Absorption ◽  
Radiative Forcing ◽  
Large Scale ◽  
Wavelength Dependence ◽  
Absorption Enhancement ◽  
Core Shell ◽  
Enhancement Effect ◽  
Visible Radiation ◽  
Single Scatter

Abstract. The presence of clear coatings on atmospheric black carbon (BC) particles is known to enhance the magnitude of light absorption by the BC cores. Based on calculations using core/shell Mie theory, we demonstrate that the enhancement of light absorption (EAbs) by atmospheric black carbon (BC) when it is coated in mildly absorbing material (CBrown) is reduced relative to the enhancement induced by non-absorbing coatings (CClear). This reduction, sensitive to both the CBrown coating thickness and imaginary refractive index (RI), can be up to 50% for 400 nm radiation and 25% averaged across the visible radiation spectrum for reasonable core/shell diameters. The enhanced direct radiative forcing possible due to the enhancement effect of CClear is therefore reduced if the coating is absorbing. Additionally, the need to explicitly treat BC as an internal, as opposed to external, mixture with CBrown is shown to be important to the calculated single scatter albedo only when models treat BC as large spherical cores (>50 nm). For smaller BC cores (or fractal agglomerates) consideration of the BC and CBrown as an external mixture leads to relatively small errors in the particle single scatter albedo of <0.03. It has often been assumed that observation of an absorption Angström exponent (AAE)>1 indicates absorption by a non-BC aerosol. Here, it is shown that BC cores coated in CClear can reasonably have an AAE of up to 1.6, a result that complicates the attribution of observed light absorption to CBrown within ambient particles. However, an AAE<1.6 does not exclude the possibility of CBrown; rather CBrown cannot be confidently assigned unless AAE>1.6. Comparison of these model results to various ambient AAE measurements demonstrates that large-scale attribution of CBrown is a challenging task using current in-situ measurement methods. We suggest that coincident measurements of particle core and shell sizes along with the AAE may be necessary to distinguish absorbing and non-absorbing OC.

scholarly journals Multi-Satellite Retrieval of SSA using OMI-MODIS algorithm

2018 ◽  
Author(s):  
Kruthika Eswaran ◽  
Sreedharan Krishnakumari Satheesh ◽  
Jayaraman Srinivasan
Keyword(s):  
Radiative Forcing ◽  
Single Scattering ◽  
Retrieval Algorithm ◽  
Ozone Monitoring Instrument ◽  
Aerosol Composition ◽  
Aerosol Radiative Forcing ◽  
Aerosol Absorption ◽  
Moderate Resolution Imaging Spectroradiometer ◽  
Absorbing Aerosols ◽  
Aerosol Type

Abstract. Single scattering albedo (SSA) represents a unique identification of aerosol type and aerosol radiative forcing. However, SSA retrievals are highly uncertain due cloud contamination and aerosol composition. Recent improvement in the SSA retrieval algorithm has combined the superior cloud masking technique of Moderate Resolution Imaging Spectroradiometer (MODIS) and the better sensitivity of Ozone Monitoring Instrument (OMI) to aerosol absorption. The combined OMI-MODIS algorithm has been validated over a small spatial and temporal scale only. The present study validates the algorithm over global oceans for the period 2008–2012. The geographical heterogeneity in the aerosol type and concentration over the Atlantic Ocean, the Arabian Sea and the Bay of Bengal was useful to delineate the effect of aerosol type on the retrieval algorithm. We also noted that OMI overestimates SSA when absorbing aerosols were present closer to the surface. We attribute this overestimation to data discontinuity in the aerosol height climatology derived from Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) satellite. OMI uses pre-defined aerosol heights over regions where CALIPSO climatology is not present leading to overestimation of SSA. The importance of aerosol height was also studied using the Santa Barbara DISORT radiative transfer (SBDART) model. The results from the joint retrieval were validated with ground-based measurements and it was seen that OMI-MODIS SSA retrievals were better constrained than OMI only retrieval.

scholarly journals Pre-monsoon aerosol characteristics over the Indo-Gangetic Basin: implications to climatic impact

2011 ◽  
Vol 29 (5) ◽  
pp. 789-804 ◽  
Author(s):  
A. K. Srivastava ◽  
S. Tiwari ◽  
P. C. S. Devara ◽  
D. S. Bisht ◽  
Manoj K. Srivastava ◽  
...  
Keyword(s):  
Radiative Forcing ◽  
Geographical Location ◽  
Dust Particles ◽  
Radiative Transfer Model ◽  
Transfer Model ◽  
Climatic Impact ◽  
Surface Cooling ◽  
Monsoon Period ◽  
Aerosol Radiative Forcing ◽  
Absorbing Aerosols

Abstract. Sun/sky radiometer observations over the Indo-Gangetic Basin (IGB) region during pre-monsoon (from April–June 2009) have been processed to analyze various aerosol characteristics in the central and eastern IGB region, represented by Kanpur and Gandhi College, respectively, and their impacts on climate in terms of radiative forcing. Monthly mean aerosol optical depth (AOD at 500 nm) and corresponding Angstrom Exponent (AE at 440–870 nm, given within the brackets) was observed to be about 0.50 (0.49) and 0.51 (0.65) in April, 0.65 (0.74) and 0.67 (0.91) in May and 0.69 (0.45) and 0.77 (0.71) in June at Kanpur and Gandhi College, respectively. Results show a positive gradient in AOD and AE from central to eastern IGB region with the advancement of the pre-monsoon, which may be caused due to diverse geographical location of the stations having different meteorological conditions and emission sources. Relatively lower SSA was observed at the eastern IGB (0.89) than the central IGB (0.92) region during the period, which suggests relative dominance of absorbing aerosols at the eastern IGB as compared to central IGB region. The absorbing aerosol optical properties over the station suggest that the atmospheric absorption over central IGB region is mainly due to dominance of coarse-mode dust particles; however, absorption over eastern IGB region is mainly due to dominance of fine-particle pollution. The derived properties from sun/sky radiometer during pre-monsoon period are used in a radiative-transfer model to estimate aerosol radiative forcing at the top-of-the atmosphere (TOA) and at the surface over the IGB region. Relatively large TOA and surface cooling was observed at the eastern IGB as compared to the central IGB region. This translates into large heating of the atmosphere ranging from 0.45 to 0.55 K day−1 at Kanpur and from 0.45 to 0.59 K day−1 at Gandhi College.

scholarly journals Shortwave radiative forcing and efficiency of key aerosol types using AERONET data

2012 ◽  
Vol 12 (11) ◽  
pp. 5129-5145 ◽  
Author(s):  
O. E. García ◽  
J. P. Díaz ◽  
F. J. Expósito ◽  
A. M. Díaz ◽  
O. Dubovik ◽  
...  
Keyword(s):  
Biomass Burning ◽  
Atmospheric Aerosols ◽  
Radiative Forcing ◽  
Mineral Dust ◽  
High Surface ◽  
Global Scale ◽  
Free Troposphere ◽  
Anthropogenic Aerosols ◽  
Radiative Balance ◽  
Absorbing Aerosols

Abstract. The shortwave radiative forcing (ΔF) and the radiative forcing efficiency (ΔFeff) of natural and anthropogenic aerosols have been analyzed using estimates of radiation both at the Top (TOA) and at the Bottom Of Atmosphere (BOA) modeled based on AERONET aerosol retrievals. Six main types of atmospheric aerosols have been compared (desert mineral dust, biomass burning, urban-industrial, continental background, oceanic and free troposphere) in similar observational conditions (i.e., for solar zenith angles between 55° and 65°) in order to compare the nearly same solar geometry. The instantaneous ΔF averages obtained vary from −122 ± 37 Wm−2 (aerosol optical depth, AOD, at 0.55 μm, 0.85 ± 0.45) at the BOA for the mixture of desert mineral dust and biomass burning aerosols in West Africa and −42 ± 22 Wm−2 (AOD = 0.9 ± 0.5) at the TOA for the pure mineral dust also in this region up to −6 ± 3 Wm−2 and −4 ± 2 Wm−2 (AOD = 0.03 ± 0.02) at the BOA and the TOA, respectively, for free troposphere conditions. This last result may be taken as reference on a global scale. Furthermore, we observe that the more absorbing aerosols are overall more efficient at the BOA in contrast to at the TOA, where they backscatter less solar energy into the space. The analysis of the radiative balance at the TOA shows that, together with the amount of aerosols and their absorptive capacity, it is essential to consider the surface albedo of the region on which they are. Thus, we document that in regions with high surface reflectivity (deserts and snow conditions) atmospheric aerosols lead to a warming of the Earth-atmosphere system.

scholarly journals Radiative forcing by light-absorbing aerosols of pyrogenetic iron oxides

2018 ◽  
Vol 8 (1) ◽  
Author(s):  
Akinori Ito ◽  
Guangxing Lin ◽  
Joyce E. Penner
Keyword(s):  
Iron Oxides ◽  
Radiative Forcing ◽  
Absorbing Aerosols

scholarly journals Scattering and Radiative Properties of Morphologically Complex Carbonaceous Aerosols: A Systematic Modeling Study

2018 ◽  
Vol 10 (10) ◽  
pp. 1634 ◽  
Author(s):  
Li Liu ◽  
Michael Mishchenko
Keyword(s):  
Black Carbon ◽  
Radiative Forcing ◽  
Accurate Estimate ◽  
Coating Material ◽  
Radiative Properties ◽  
Absorption Enhancement ◽  
Carbonaceous Aerosols ◽  
Carbonaceous Particles ◽  
Full Characterization ◽  
Linear Depolarization Ratio

This paper provides a thorough modeling-based overview of the scattering and radiative properties of a wide variety of morphologically complex carbonaceous aerosols. Using the numerically-exact superposition T-matrix method, we examine the absorption enhancement, absorption Ångström exponent (AAE), backscattering linear depolarization ratio (LDR), and scattering matrix elements of black-carbon aerosols with 11 different model morphologies ranging from bare soot to completely embedded soot–sulfate and soot–brown carbon mixtures. Our size-averaged results show that fluffy soot particles absorb more light than compact bare-soot clusters. For the same amount of absorbing material, the absorption cross section of internally mixed soot can be more than twice that of bare soot. Absorption increases as soot accumulates more coating material and can become saturated. The absorption enhancement is affected by particle size, morphology, wavelength, and the amount of coating. We refute the conventional belief that all carbonaceous aerosols have AAEs close to 1.0. Although LDRs caused by bare soot and certain carbonaceous particles are rather weak, LDRs generated by other soot-containing aerosols can reproduce strong depolarization measured by Burton et al. for aged smoke. We demonstrate that multi-wavelength LDR measurements can be used to identify the presence of morphologically complex carbonaceous particles, although additional observations can be needed for full characterization. Our results show that optical constants of the host/coating material can significantly influence the scattering and absorption properties of soot-containing aerosols to the extent of changing the sign of linear polarization. We conclude that for an accurate estimate of black-carbon radiative forcing, one must take into account the complex morphologies of carbonaceous aerosols in remote sensing studies as well as in atmospheric radiation computations.

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