scholarly journals Ocean mediation of tropospheric response to reflecting and absorbing aerosols

2015 ◽  
Vol 15 (10) ◽  
pp. 5827-5833 ◽  
Author(s):  
Y. Xu ◽  
S.-P. Xie

Abstract. Radiative forcing by reflecting (e.g., sulfate, SO4) and absorbing (e.g., black carbon, BC) aerosols is distinct: the former cools the planet by reducing solar radiation at the top of the atmosphere and the surface, without largely affecting the atmospheric column, while the latter heats the atmosphere directly. Despite the fundamental difference in forcing, here we show that the structure of the tropospheric response is remarkably similar between the two types of aerosols, featuring a deep vertical structure of temperature change (of opposite sign) at the Northern Hemisphere (NH) mid-latitudes. The deep temperature structure is anchored by the slow response of the ocean, as a large meridional sea surface temperature (SST) gradient drives an anomalous inter-hemispheric Hadley circulation in the tropics and induces atmospheric eddy adjustments at the NH mid-latitudes. The tropospheric warming in response to projected future decline in reflecting aerosols poses additional threats to the stability of mountain glaciers in the NH. Additionally, robust tropospheric response is unique to aerosol forcing and absent in the CO2 response, which can be exploited for climate change attribution.

2015 ◽  
Vol 15 (4) ◽  
pp. 5537-5552 ◽  
Author(s):  
Y. Xu ◽  
S.-P. Xie

Abstract. Radiative forcing by reflecting (e.g., sulfate, SO4) and absorbing (e.g., black carbon, BC) aerosols is distinct: the former cools the planet by reducing solar radiation at the top of the atmosphere and the surface, without largely affecting the atmospheric column, while the latter heats the atmosphere directly. Despite the fundamental difference in forcing, here we show that the structure of the tropospheric response is remarkably similar between the two types of aerosols, featuring a deep vertical structure of temperature change (of opposite sign) in the Northern Hemisphere (NH) mid-latitudes. The deep temperature structure is anchored by the slow response of the ocean, as large meridional sea surface temperature (SST) gradient drives an anomalous inter-hemispheric Hadley circulation in the tropics and induces atmospheric eddy adjustments in the NH mid-latitudes. The robust tropospheric response is unique to aerosol forcing and absent in the CO2 response, which can be exploited for climate change attribution. The tropospheric warming in response to projected future decline in reflecting aerosols poses additional threats to the stability of mountain glaciers in NH.


2014 ◽  
Vol 14 (3) ◽  
pp. 1159-1165 ◽  
Author(s):  
V. S. Manoharan ◽  
R. Kotamarthi ◽  
Y. Feng ◽  
M. P. Cadeddu

Abstract. Each atmospheric aerosol type has distinctive light-absorption characteristics related to its physical/chemical properties. Climate models treat black carbon as the main light-absorbing component of carbonaceous atmospheric aerosols, while absorption by some organic aerosols is also considered, particularly at ultraviolet wavelengths. Most absorbing aerosols are assumed to be < 1 μm in diameter (sub-micron). Here we present results from a recent field study in India, primarily during the post-monsoon season (October–November), suggesting the presence of absorbing aerosols sized 1–10 μm. Absorption due to super-micron-sized particles was nearly 30% greater than that due to smaller particles. Periods of increased absorption by larger particles ranged from a week to a month. Radiative forcing calculations under clear-sky conditions show that super-micron particles account for nearly 44% of the total aerosol forcing. The origin of the large aerosols is unknown, but meteorological conditions indicate that they are of local origin. Such economic and habitation conditions exist throughout much of the developing world. Hence, large absorbing particles could be an important component of the regional-scale atmospheric energy balance.


2011 ◽  
Vol 11 (24) ◽  
pp. 12841-12863 ◽  
Author(s):  
R. Gautam ◽  
N. C. Hsu ◽  
S. C. Tsay ◽  
K. M. Lau ◽  
B. Holben ◽  
...  

Abstract. We examine the distribution of aerosols and associated optical/radiative properties in the Gangetic-Himalayan region from simultaneous radiometric measurements over the Indo-Gangetic Plains (IGP) and the foothill/southern slopes of the Himalayas during the 2009 pre-monsoon season. Enhanced dust transport extending from the Southwest Asian arid regions into the IGP, results in seasonal mean (April–June) aerosol optical depths of over 0.6 – highest over Southern Asia. The influence of dust loading is greater over the Western IGP as suggested by pronounced coarse mode peak in aerosol size distribution and spectral single scattering albedo (SSA). Transported dust in the IGP, driven by prevailing westerly airmass, is found to be more absorbing (SSA550 nm<0.9) than the near-desert region in Northwestern (NW) India suggesting mixing with carbonaceous aerosols in the IGP. On the contrary, significantly reduced dust transport is observed over eastern IGP and foothill/elevated Himalayan slopes in Nepal where strongly absorbing haze is prevalent, as indicated by lower SSA (0.85–0.9 at 440–1020 nm), suggesting presence of more absorbing aerosols compared to IGP. Additionally, our observations show a distinct diurnal pattern of aerosols with characteristic large afternoon peak, from foothill to elevated mountain locations, associated with increased upslope transport of pollutants – that likely represent large-scale lifting of absorbing aerosols along the elevated slopes during pre-monsoon season. In terms of radiative impact of aerosols, over the source region of NW India, diurnal mean reduction in solar radiation fluxes was estimated to be 19–23 Wm−2 at surface (12–15% of the surface solar insolation). Furthermore, based on limited observations of aerosol optical properties during the pre-monsoon period and comparison of our radiative forcing estimates with published literature, there exists a general spatial heterogeneity in the regional aerosol forcing, associated with the absorbing aerosol distribution over northern India, with both diurnal mean surface forcing and forcing efficiency over the IGP exceeding that over Northwestern India. Finally, the role of the seasonal progressive buildup of aerosol loading and water vapor is investigated in the observed net aerosol radiative effect over Northwestern India. The radiative impact of water vapor is found to amplify the net regional aerosol radiative forcing suggesting that the two exert forcing in tandem leading to enhanced surface cooling. It is suggested that water vapor contribution should be taken into account while assessing aerosol forcing impact for this region and other seasonally similar environments.


2014 ◽  
Vol 27 (18) ◽  
pp. 6960-6977 ◽  
Author(s):  
Leon D. Rotstayn ◽  
Emily L. Plymin ◽  
Mark A. Collier ◽  
Olivier Boucher ◽  
Jean-Louis Dufresne ◽  
...  

Abstract The effects of declining anthropogenic aerosols in representative concentration pathway 4.5 (RCP4.5) are assessed in four models from phase 5 the Coupled Model Intercomparison Project (CMIP5), with a focus on annual, zonal-mean atmospheric temperature structure and zonal winds. For each model, the effect of declining aerosols is diagnosed from the difference between a projection forced by RCP4.5 for 2006–2100 and another that has identical forcing, except that anthropogenic aerosols are fixed at early twenty-first-century levels. The response to declining aerosols is interpreted in terms of the meridional structure of aerosol radiative forcing, which peaks near 40°N and vanishes at the South Pole. Increasing greenhouse gases cause amplified warming in the tropical upper troposphere and strengthening midlatitude jets in both hemispheres. However, for declining aerosols the vertically averaged tropospheric temperature response peaks near 40°N, rather than in the tropics. This implies that for declining aerosols the tropospheric meridional temperature gradient generally increases in the Southern Hemisphere (SH), but in the Northern Hemisphere (NH) it decreases in the tropics and subtropics. Consistent with thermal wind balance, the NH jet then strengthens on its poleward side and weakens on its equatorward side, whereas the SH jet strengthens more than the NH jet. The asymmetric response of the jets is thus consistent with the meridional structure of aerosol radiative forcing and the associated tropospheric warming: in the NH the latitude of maximum warming is roughly collocated with the jet, whereas in the SH warming is strongest in the tropics and weakest at high latitudes.


2002 ◽  
Vol 20 (12) ◽  
pp. 2105-2109 ◽  
Author(s):  
S. K. Satheesh

Abstract. It is now clearly understood that atmospheric aerosols have a significant impact on climate due to their important role in modifying the incoming solar and outgoing infrared radiation. The question of whether aerosol cools (negative forcing) or warms (positive forcing) the planet depends on the relative dominance of absorbing aerosols. Recent investigations over the tropical Indian Ocean have shown that, irrespective of the comparatively small percentage contribution in optical depth ( ~ 11%), soot has an important role in the overall radiative forcing. However, when the amount of absorbing aerosols such as soot are significant, aerosol optical depth and chemical composition are not the only determinants of aerosol climate effects, but the altitude of the aerosol layer and the altitude and type of clouds are also important. In this paper, the aerosol forcing in the presence of clouds and the effect of different surface types (ocean, soil, vegetation, and different combinations of soil and vegetation) are examined based on model simulations, demonstrating that aerosol forcing changes sign from negative (cooling) to positive (warming) when reflection from below (either due to land or clouds) is high.Key words. Atmospheric composition and structure (aerosols and particles) History of Geophysics (atmospheric sciences) Hydrology (anthropogenic effects)


2013 ◽  
Vol 13 (7) ◽  
pp. 19837-19852
Author(s):  
V. S. Manoharan ◽  
R. Kotamarthi ◽  
Y. Feng ◽  
M. P. Cadeddu

Abstract. Each atmospheric aerosol type has distinctive light-absorption characteristics related to its physical/chemical properties. Climate models treat black carbon as the light-absorbing component of all carbonaceous atmospheric aerosols. Most absorbing aerosols are assumed to be <1 μm in diameter (sub-micron). Here we present results from a recent field study in India, primarily during the post-monsoon season (October–November), suggesting the presence of absorbing aerosols sized 1–10 μm. Absorption due to super-micron-sized particles was nearly 30% greater than that due to smaller particles. Periods of increased absorption by larger particles ranged from a week to a month. Radiative forcing calculations under clear-sky conditions show that super-micron particles account for nearly 44% of the total aerosol-forcing. The origin of the large aerosols is unknown, but meteorological conditions indicate that they are of local origin. Such economic and habitation conditions exist throughout much of the developing world. Hence, large absorbing particles could be an important component of the regional-scale atmospheric-energy balance.


2021 ◽  
Vol 13 (6) ◽  
pp. 1114
Author(s):  
Jianyu Lin ◽  
Yu Zheng ◽  
Xinyong Shen ◽  
Lizhu Xing ◽  
Huizheng Che

The particle linear depolarization ratio (PLDR) and single scatter albedo (SSA) in 1020 nm from the Aerosol Robotic Network (AERONET) level 2.0 dataset was utilized among 52 stations to identify dust and dust dominated aerosols (DD), pollution dominated mixture (PDM), strongly absorbing aerosols (SA) and weakly absorbing aerosols (WA), investigate their spatial and temporal distribution, net radiative forcing and radiative forcing efficiency in global range, and further compare with VIIRS Deep Blue Production. The conclusion about net radiative forcing suggests that the high values of radiative forcing from dust and dust dominated aerosols, pollution dominated mixture both mainly come from western Africa. Strongly absorbing aerosols in South Africa and India contribute greatly to the net radiative forcing and the regions with relative high values of weakly absorbing aerosols are mainly located at East Asia and India. Lastly, the observation of VIIRS Deep Blue satellite monthly averaged products depicts the characteristics about spatial distribution of four kinds of aerosol well, the result from ground-based observation presents great significant to validate the measurements from remote sensing technology.


2021 ◽  
Author(s):  
Matthew Kasoar ◽  
Douglas Hamilton ◽  
Daniela Dalmonech ◽  
Stijn Hantson ◽  
Gitta Lasslop ◽  
...  

&lt;p&gt;The CMIP6 Shared Socioeconomic Pathway (SSP) scenarios include projections of future changes in anthropogenic biomass-burning.&amp;#160; Globally, they assume a decrease in total fire emissions over the next century under all scenarios.&amp;#160; However, fire regimes and emissions are expected to additionally change with future climate, and the methodology used to project fire emissions in the SSP scenarios is opaque.&lt;/p&gt;&lt;p&gt;We aim to provide a more traceable estimate of future fire emissions under CMIP6 scenarios and evaluate the impacts for aerosol radiative forcing. &amp;#160;We utilise interactive wildfire emissions from four independent land-surface models (CLM5, JSBACH3.2, LPJ-GUESS, and ISBA-CTRIP) used within CMIP6 ESMs, and two different machine-learning methods (a random forest, and a generalised additive model) trained on historical data, to predict year 2100 biomass-burning aerosol emissions consistent with the CMIP6-modelled climate for three different scenarios: SSP126, SSP370, and SSP585.&amp;#160; This multi-method approach provides future fire emissions integrating information from observations, projections of climate, socioeconomic parameters and changes in vegetation distribution and fuel loads.&lt;/p&gt;&lt;p&gt;Our analysis shows a robust increase in fire emissions for large areas of the extra-tropics until the end of this century for all methods.&amp;#160; Although this pattern was present to an extent in the original SSP projections, both the interactive fire models and machine-learning methods predict substantially higher increases in extra-tropical emissions in 2100 than the corresponding SSP datasets.&amp;#160; Within the tropics the signal is mixed. Increases in emissions are largely driven by the temperature changes, while in some tropical areas reductions in fire emissions are driven by human factors and changes in precipitation, with the largest reductions in Africa. The machine-learning methods show a stronger reduction in the tropics than the interactive fire models, however overall there is strong agreement between both the models and the machine-learning methods.&lt;/p&gt;&lt;p&gt;We then use additional nudged atmospheric simulations with two state-of-the-art composition-climate models, UKESM1 and CESM2, to diagnose the impact of these updated fire emissions on aerosol burden and radiative forcing, compared with the original SSP prescribed emissions.&amp;#160; We provide estimates of future fire radiative forcing, compared to modern-day, under these CMIP6 scenarios which span both the severity of climate change in 2100, and the rate of reduction of other aerosol species.&lt;/p&gt;


2013 ◽  
Vol 13 (10) ◽  
pp. 5227-5241 ◽  
Author(s):  
M. G. Tosca ◽  
J. T. Randerson ◽  
C. S. Zender

Abstract. Each year landscape fires across the globe emit black and organic carbon smoke particles that can last in the atmosphere for days to weeks. We characterized the climate response to these aerosols using an Earth system model. We used remote sensing observations of aerosol optical depth (AOD) and simulations from the Community Atmosphere Model, version 5 (CAM5) to optimize satellite-derived smoke emissions for high biomass burning regions. Subsequent global simulations using the adjusted fire emissions produced AODs that were in closer agreement with surface and space-based measurements. We then used CAM5, which included radiative aerosol effects, to evaluate the climate response to the fire-aerosol forcing. We conducted two 52 yr simulations, one with four sets of monthly cycling 1997–2009 fire emissions and one without. Fire emissions increased global mean annual AOD by 10% (+0.02) and decreased net all-sky surface radiation by 1% (1.3 W m−2). Elevated AODs reduced global surface temperatures by 0.13 &amp;pm; 0.01 °C. Though global precipitation declined only slightly, patterns of precipitation changed, with large reductions near the Equator offset by smaller increases north and south of the intertropical convergence zone (ITCZ). A combination of increased tropospheric heating and reduced surface temperatures increased equatorial subsidence and weakened the Hadley circulation. As a consequence, precipitation decreased over tropical forests in South America, Africa and equatorial Asia. These results are consistent with the observed correlation between global temperatures and the strength of the Hadley circulation and studies linking tropospheric heating from black carbon aerosols with tropical expansion.


2011 ◽  
Vol 11 (3) ◽  
pp. 9057-9081
Author(s):  
T. Kurtén ◽  
L. Zhou ◽  
R. Makkonen ◽  
J. Merikanto ◽  
P. Räisänen ◽  
...  

Abstract. The release of vast quantities of methane into the atmosphere as a result of clathrate destabilization is a potential mechanism for rapid amplification of global warming. Previous studies have calculated the enhanced warming based mainly on the radiative effect of the methane itself, with smaller contributions from the associated carbon dioxide or ozone increases. Here, we study the effect of strongly elevated methane (CH4) levels on oxidant and aerosol particle concentrations using a combination of chemistry-transport and general circulation models. A 10-fold increase in methane concentrations is predicted to significantly decrease hydroxyl radical (OH) concentrations, while moderately increasing ozone (O3). These changes lead to a 70% increase in the atmospheric lifetime of methane, and an 18% decrease in global mean cloud droplet number concentrations (CDNC). The CDNC change causes a radiative forcing that is comparable in magnitude to the longwave radiative forcing ("enhanced greenhouse effect") of the added methane. Together, the indirect CH4-O3 and CH4-OH-aerosol forcings could more than double the warming effect of large methane increases. Our findings may help explain the anomalously large temperature changes associated with historic methane releases.


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