scholarly journals Cross-polar transport and scavenging of Siberian aerosols containing black carbon during the 2012 ACCESS summer campaign

2017 ◽  
Vol 17 (18) ◽  
pp. 10969-10995 ◽  
Author(s):  
Jean-Christophe Raut ◽  
Louis Marelle ◽  
Jerome D. Fast ◽  
Jennie L. Thomas ◽  
Bernadett Weinzierl ◽  
...  
Keyword(s):  
Black Carbon ◽  
Biomass Burning ◽  
Large Scale ◽  
Arctic Region ◽  
Anthropogenic Sources ◽  
The Arctic ◽  
Convective Precipitation ◽  
Svalbard Archipelago ◽  
Wet Removal ◽  
The Arctic Region

Abstract. During the ACCESS airborne campaign in July 2012, extensive boreal forest fires resulted in significant aerosol transport to the Arctic. A 10-day episode combining intense biomass burning over Siberia and low-pressure systems over the Arctic Ocean resulted in efficient transport of plumes containing black carbon (BC) towards the Arctic, mostly in the upper troposphere (6–8 km). A combination of in situ observations (DLR Falcon aircraft), satellite analysis and WRF-Chem simulations is used to understand the vertical and horizontal transport mechanisms of BC with a focus on the role of wet removal. Between the northwestern Norwegian coast and the Svalbard archipelago, the Falcon aircraft sampled plumes with enhanced CO concentrations up to 200 ppbv and BC mixing ratios up to 25 ng kg−1. During transport to the Arctic region, a large fraction of BC particles are scavenged by two wet deposition processes, namely wet removal by large-scale precipitation and removal in wet convective updrafts, with both processes contributing almost equally to the total accumulated deposition of BC. Our results underline that applying a finer horizontal resolution (40 instead of 100 km) improves the model performance, as it significantly reduces the overestimation of BC levels observed at a coarser resolution in the mid-troposphere. According to the simulations at 40 km, the transport efficiency of BC (TEBC) in biomass burning plumes was larger (60 %), because it was impacted by small accumulated precipitation along trajectory (1 mm). In contrast TEBC was small (< 30 %) and accumulated precipitation amounts were larger (5–10 mm) in plumes influenced by urban anthropogenic sources and flaring activities in northern Russia, resulting in transport to lower altitudes. TEBC due to large-scale precipitation is responsible for a sharp meridional gradient in the distribution of BC concentrations. Wet removal in cumulus clouds is the cause of modeled vertical gradient of TEBC, especially in the mid-latitudes, reflecting the distribution of convective precipitation, but is dominated in the Arctic region by the large-scale wet removal associated with the formation of stratocumulus clouds in the planetary boundary layer (PBL) that produce frequent drizzle.

scholarly journals Cross-polar transport and scavenging of Siberian aerosols containing black carbon during the 2012 ACCESS summer campaign

2017 ◽  
Author(s):  
Jean-Christophe Raut ◽  
Louis Marelle ◽  
Jerome D. Fast ◽  
Jennie L. Thomas ◽  
Bernadett Weinzierl ◽  
...  
Keyword(s):  
Black Carbon ◽  
Biomass Burning ◽  
Forest Fires ◽  
Large Scale ◽  
Large Fraction ◽  
Arctic Region ◽  
Horizontal Resolution ◽  
The Arctic ◽  
Svalbard Archipelago ◽  
Wet Removal

Abstract. During the ACCESS airborne campaign in July 2012, extensive boreal forest fires resulted in significant aerosol transport to the Arctic. A 10 day episode combining intense biomass burning over Siberia and low-pressure systems over the Arctic Ocean resulted in efficient transport of plumes containing black carbon (BC) towards the Arctic, mostly in the upper troposphere (6–8 km). A combination of in situ observations (DLR Falcon aircraft), satellite analysis and WRF-Chem simulations are used to understand the vertical and horizontal transport mechanisms of BC with a focus on the role of wet removal. Between the northwestern Norwegian coast and the Svalbard archipelago, the Falcon aircraft sampled plumes with enhanced CO concentrations up to 200 ppbv and BC mixing ratios up to 25 ng kg−1 . During transport to the Arctic region, a large fraction of BC particles are scavenged by two wet deposition processes, namely wet removal by large-scale precipitation and removal in wet convective updrafts, with both processes contributing almost equally to the total accumulated deposition of BC. Our results underline that applying a finer horizontal resolution (40 instead of 100 km) improves the model performance, as it significantly reduces the overestimation of BC levels observed at a coarser resolution in the mid-troposphere. According to the simulations at 40 km, the transport efficiency of BC (TEBC ) in biomass burning plumes is about 60 %, which is impacted by small accumulated precipitation along trajectory (APT) (1 mm). In contrast TEBC is very small (

Global mapping of seasonal variations in tides from tide gauge and satellite altimeter data

2021 ◽  
Author(s):  
Inger Bij de Vaate ◽  
Henrique Guarneri ◽  
Cornelis Slobbe ◽  
Martin Verlaan
Keyword(s):  
Seasonal Variation ◽  
Sea Level ◽  
Seasonal Variations ◽  
Large Scale ◽  
Arctic Region ◽  
The Arctic ◽  
Altimeter Data ◽  
Tide Gauges ◽  
Tidal Constituents ◽  
The Arctic Region

&lt;p&gt;The existence of seasonal variations in major tides has been recognized since decades. Where Corkan (1934) was the first to describe the seasonal perturbation of the M2 tide, many others have studied seasonal variations in the main tidal constituents since. However, most of these studies are based on sea level observations from tide gauges and are often restricted to coastal and shelf regions. Hence, observed seasonal variations are typically dominated by local processes and the large-scale patterns cannot be clearly distinguished. Moreover, most tide models still perceive tides as annually constant and seasonal variation in tides is ignored in the correction process of satellite altimetry. This results in reduced accuracy of obtained sea level anomalies. &lt;/p&gt;&lt;p&gt;To gain more insight in the large-scale seasonal variations in tides, we supplemented the clustered and sparsely distributed sea level observations from tide gauges by the wealth of data from satellite altimeters. Although altimeter-derived water levels are being widely used to obtain tidal constants, only few of these implementations consider seasonal variation in tides. For that reason, we have set out to explore the opportunities provided by altimeter data for deriving seasonal modulation of the main tidal constituents. Different methods were implemented and compared for the principal tidal constituents and a range of geographical domains, using data from a selection of satellite altimeters. Specific attention was paid to the Arctic region where seasonal variation in tides was expected to be significant as a result of the seasonal sea ice cycle, yet data availability is particularly limited. Our study demonstrates the potential of satellite altimetry for the quantification of seasonal modulation of tides and suggests the seasonal modulation to be considerable. Already for M2 we observed changes in tidal amplitude of the order of decimeters for the Arctic region, and centimeters for lower latitude regions.&lt;/p&gt;&lt;p&gt;&amp;#160;&lt;/p&gt;&lt;div&gt;Corkan, R. H. (1934). An annual perturbation in the range of tide. &lt;em&gt;Proceedings of the Royal Society of London. Series A, Containing Papers of a Mathematical and Physical Character&lt;/em&gt;, &lt;em&gt;144&lt;/em&gt;(853), 537-559.&lt;/div&gt;

scholarly journals Sources of Springtime Surface Black Carbon in the Arctic: An Adjoint Analysis

2017 ◽  
Author(s):  
Ling Qi ◽  
Qinbin Li ◽  
Daven K. Henze ◽  
Hsien-Liang Tseng ◽  
Cenlin He
Keyword(s):  
Natural Gas ◽  
Black Carbon ◽  
Biomass Burning ◽  
Transport Model ◽  
Lower Troposphere ◽  
Anthropogenic Sources ◽  
The Arctic ◽  
Anthropogenic Source ◽  
Gas Flaring ◽  
Arctic Front

Abstract. We quantify source contributions to springtime (April 2008) surface black carbon (BC) in the Arctic by interpreting surface observations of BC at five receptor sites (Denali, Barrow, Alert, Zeppelin, and Summit) using a global chemical transport model (GEOS-Chem) and its adjoint. Contributions to BC at Barrow, Alert, and Zeppelin are dominated by Asian anthropogenic sources (40–43 %) before April 18 and by Siberian open biomass burning emissions (29–41 %) afterward. In contrast, Summit, a mostly free tropospheric site, has predominantly an Asian anthropogenic source contribution (24–68 %, with an average of 45 %). We compute the adjoint sensitivity of BC concentrations at the five sites during a pollution episode (April 20–25) to global emissions from March 1 to April 25. The associated contributions are the combined results of these sensitivities and BC emissions. Local and regional anthropogenic sources in Alaska are the largest anthropogenic sources of BC at Denali (63 %), and natural gas flaring emissions in the Western Extreme North of Russia (WENR) are the largest anthropogenic sources of BC at Zeppelin (26 %) and Alert (13 %). We find that long-range transport of emissions from Beijing-Tianjin-Hebei (also known as Jing-Jin-Ji), the biggest urbanized region in Northern China, contribute significantly (~ 10 %) to surface BC across the Arctic. On average it takes ~ 12 days for Asian anthropogenic emissions and Siberian biomass burning emissions to reach Arctic lower troposphere, supporting earlier studies. Natural gas flaring emissions from the WENR reach Zeppelin in about a week. We find that episodic, direct transport events dominate BC at Denali (87 %), a site outside the Arctic front, a strong transport barrier. The relative contribution of direct transport to surface BC within the Arctic front is much smaller (~ 50 % at Barrow and Zeppelin and ~ 10 % at Alert). The large contributions from Asian anthropogenic sources are predominately in the form of ‘chronic’ pollution (~ 40 % at Barrow and 65 % at Alert and 57 % at Zeppelin) on 1–2 month timescales. As such, it is likely that previous studies using 5- or 10-day trajectory analyses strongly underestimated the contribution from Asia to surface BC in the Arctic. Both finer temporal resolution of biomass burning emissions and accounting for the Wegener-Bergeron-Findeisen (WBF) process in wet scavenging improve the source attribution estimates.

scholarly journals Arctic black carbon during PAMARCMiP 2018 and previous aircraft experiments in spring

2021 ◽  
Author(s):  
Sho Ohata ◽  
Makoto Koike ◽  
Atsushi Yoshida ◽  
Nobuhiro Moteki ◽  
Kouji Adachi ◽  
...  
Keyword(s):  
Numerical Model ◽  
Black Carbon ◽  
Biomass Burning ◽  
Base Station ◽  
Anthropogenic Sources ◽  
The Arctic ◽  
Core Diameter ◽  
Model Simulations ◽  
Anthropogenic Contributions ◽  
Mass Concentrations

Abstract. Vertical profiles of the mass concentration of black carbon (BC) were measured at altitudes up to 5 km during the PAMARCMiP aircraft-based field experiment conducted around the Northern Greenland Sea (Fram Strait) during March and April 2018, with operation base Station Nord (81.6° N, 16.7° W). Median BC mass concentrations in individual altitude ranges were 7–18 ng m–3 at standard temperature and pressure at altitudes below 4.5 km. These concentrations were systematically lower than previous observations in the Arctic in spring conducted by ARCTAS-A in 2008 and NETCARE in 2015 and similar to those observed during HIPPO3 in 2010. Column amounts of BC for altitudes below 5 km in the Arctic (> 66.5° N, COLBC), observed during the ARCTAS-A and NETCARE experiments were higher by factors of 4.2 and 2.7, respectively, than those of the PAMARCMiP experiment. These differences could not be explained solely by the different locations of the experiments. The year-to-year variation of COLBC values generally corresponded to that of biomass burning activities in northern high latitudes over western and eastern Eurasia. Furthermore, numerical model simulations estimated the year-to-year variation of contributions from anthropogenic sources to be smaller than 30–40 %. These results suggest that the year-to-year variation of biomass burning activities likely affected BC amounts in the Arctic troposphere in spring, at least in the years examined in this study. The year-to-year variations in BC mass concentrations were also observed at the surface at high Arctic sites Ny-Ålesund and Barrow, although their magnitudes were slightly lower than those in COLBC. Numerical model simulations in general successfully reproduced the observed COLBC values for PAMARCMiP and HIPPO3 (within a factor of 2), whereas they markedly underestimated the values for ARCTAS-A and NETCARE by factors of 3.7–5.8 and 3.3–5.0, respectively. Because anthropogenic contributions account for nearly all of the COLBC (82–98 %) in PAMARCMiP and HIPPO3, the good agreements between the observations and calculations for these two experiments suggest that anthropogenic contributions were generally well reproduced. However, the significant underestimations of COLBC for ARCTAS-A and NETCARE suggest that biomass burning contributions were underestimated. In this study, we also investigated plumes with enhanced BC mass concentrations, which were affected by biomass burning emissions, observed at 5 km altitude. Interestingly, the mass-averaged diameter of BC (core) and the shell-to-core diameter ratio of BC-containing particles in the plumes were generally not very different from those in other air sampled, which were considered to be mostly aged anthropogenic BC. These observations provide useful bases to evaluate numerical model simulations of the BC radiative effect in the Arctic region in spring.

scholarly journals Constraints on aerosol processes in climate models from vertically-resolved aircraft observations of black carbon

2013 ◽  
Vol 13 (1) ◽  
pp. 437-473 ◽  
Author(s):  
Z. Kipling ◽  
P. Stier ◽  
J. P. Schwarz ◽  
A. E. Perring ◽  
J. R. Spackman ◽  
...  
Keyword(s):  
Vertical Distribution ◽  
Black Carbon ◽  
Biomass Burning ◽  
Large Scale ◽  
Climate Models ◽  
Convective Transport ◽  
Convective Precipitation ◽  
Scale Model ◽  
Modest Improvement ◽  
Order Of Magnitude

Abstract. Evaluation of the aerosol schemes in current climate models is dependent upon the available observational data. In-situ observations from flight campaigns can provide valuable data about the vertical distribution of aerosol that is difficult to obtain from satellite or ground-based platforms, although they are localised in space and time. Using single-particle soot-photometer (SP2) measurements from the HIAPER Pole-to-Pole Observations (HIPPO) campaign, which consists of many vertical profiles over a large region of the Pacific, we evaluate the meridional and vertical distribution of black carbon (BC) aerosol simulated by the HadGEM3-UKCA and ECHAM5-HAM2 models. Both models show a similar pattern of overestimating the BC column burden compared to that derived from the observations, in many areas by an order of magnitude. However, by sampling the simulated BC mass mixing ratio along the flight track and comparing to the observations, we show that this discrepancy has a rather different vertical structure in the two models. Using this methodology, we conduct sensitivity tests on two specific elements of the models: biomass-burning emissions and scavenging by convective precipitation. We show that, by coupling the convective scavenging more tightly with convective transport, both the column burden and vertical distribution of BC in HadGEM3–UKCA are significantly improved with respect to the observations, demonstrating the importance of a realistic representation of this process. In contrast, updating from GFED2 to GFED3.1 biomass-burning emissions makes a more modest improvement in both models, which is not statistically significant. We also demonstrate the important role that nudged simulations (where the large-scale model dynamics are continuously relaxed towards a reanalysis) can play in this type of evaluation, allowing statistically significant differences between configurations of the aerosol scheme to be seen where the differences between the corresponding free-running simulations would not be significant.

scholarly journals SEISMICITY of the ARCTIC in 2015

2021 ◽  
pp. 210-216
Author(s):  
A. Morozov ◽  
G. Avetisov ◽  
G. Antonovskaya ◽  
V. Asming ◽  
S. Baranov ◽  
...  
Keyword(s):  
Seismic Station ◽  
Arctic Region ◽  
The Arctic ◽  
Earthquake Catalog ◽  
Svalbard Archipelago ◽  
Ocean Ridges ◽  
The North ◽  
Franz Josef Land ◽  
Barents And Kara Seas ◽  
The Arctic Region

The article provides an overview and analysis of seismicity within the boundaries of the Arctic region for 2015, a description of seismic station networks, and processing methods. The catalog of earthquakes in the Arctic region was compiled on the basis of catalogs of several organizations and seismological centers. In total, 334 earthquakes are included in the earthquake catalog. Most of the earthquakes that occurred in 2015, including all the strongest earthquakes, were located within the mid-ocean ridges of Mon, Knipovich and Gakkel. In the offshore territories, most of the earthquakes were confined to the Svalbard archipelago, in particular, to the seismically active zone in the Sturfjord strait. The renewal of instrumental seismological observations in 2011 (station ZFI) on Alexandra Land Island in the Franz Josef Land archipelago made it possible to record weak earthquakes in the north of the shelf of the Barents and Kara Seas. For twelve earthquakes, the focal mechanism parameters are presented according to the Global CMT catalog.

scholarly journals Wildfires in Northern Eurasia affect the budget of black carbon in the Arctic. A 12-year retrospective synopsis (2002–2013).

2016 ◽  
Author(s):  
N. Evangeliou ◽  
Y. Balkanski ◽  
W. M. Hao ◽  
A. Petkov ◽  
R. P. Silverstein ◽  
...  
Keyword(s):  
Black Carbon ◽  
Northern Hemisphere ◽  
Biomass Burning ◽  
Emission Inventory ◽  
Atmospheric Composition ◽  
Anthropogenic Sources ◽  
The Arctic ◽  
Northern Eurasia ◽  
Fire Emissions ◽  
Vegetation Fires

Abstract. In recent decades much attention has been given to the Arctic environment, where climate change is happening rapidly. Black carbon (BC) has been shown to be a major component of Arctic pollution that also affects the radiative balance. In the present study, we focused on how vegetation fires that occurred in Northern Eurasia during the period of 2002–2013 influenced the budget of BC in the Arctic. For simulating the transport of fire emissions from Northern Eurasia to the Arctic, we adopted BC fire emission estimates developed independently by GFED3 (Global Fire Emissions Database) and FEI-NE (Fire Emission Inventory – Northern Eurasia). Both datasets were based on fire locations and burned areas detected by MODIS (MODerate resolution Imaging Spectroradiometer) instruments on NASA's (National Aeronautics and Space Administration) Terra and Aqua satellites. Anthropogenic sources of BC were estimated using the MACCity (Monitoring Atmospheric Composition &amp; Climate/megaCITY – Zoom for the ENvironment) emission inventory. During the 12-year period, an average area of 250,000 km2 yr−1 was burned in Northern Eurasia and the global emissions of BC ranged between 8.0 and 9.5 Tg yr−1. For the BC emitted in the Northern Hemisphere, about 70 % originated from anthropogenic sources and the rest from biomass burning (BB). Using the FEI-NE inventory, we found that 102 ± 29 kt yr−1 BC from biomass burning was deposited on the Arctic (defined here as the area north of 67º N) during the 12 years simulated, which was twice as much as when using MACCity inventory (56 ± 8 kt yr−1). The annual mass of BC deposited in the Arctic from all sources (FEI-NE in Northern Eurasia, MACCity elsewhere) is significantly higher by about 37 % in 2009 to 181 % in 2012, compared to the BC deposited using just the MACCity emission inventory. Deposition of BC in the Arctic from BB sources in the Northern Hemisphere thus represents 68 % of the BC deposited from all BC sources (the remaining being due to anthropogenic sources). Northern Eurasian vegetation fires (FEI-NE) contributed 85 % (79–91 %) to the BC deposited over the Arctic from all BB sources in the Northern Hemisphere. Arctic total BC burden showed strong seasonal variations, with highest values during the Arctic Haze season. High winter–spring values of BC burden were caused by transport of BC mainly from anthropogenic sources in Europe, whereas the peak in summer was mainly due to the fire emissions in Northern Eurasia. BC particles emitted from fires in lower latitudes (35° N–40° N) were found to remain the longest in the atmosphere due to the high release altitudes of smoke plumes, exhibit tropospheric transport resulting in a high summer peak of burden, and grow by condensation processes. In regards to the geographic contribution on the deposition of BC, we estimated that about 46 % of the BC deposited over the Arctic from vegetation fires in Northern Eurasia originated from Siberia, 6 % from Kazakhstan, 5 % from Europe, and about 1 % from Mongolia. The remaining 42 % originated from other areas in Northern Eurasia. For spring and summer, we computed that 42 % of the BC released from Northern Eurasian vegetation fires was deposited over the Arctic (annual average: 17 %). Vegetation fires in Northern Eurasia contributed to 14 % to 57 % of BC surface concentrations at the Arctic stations (Alert, Barrow, Zeppelin, Villum, and Tiksi), with fires in Siberia contributing the largest share. However, anthropogenic sources in the Northern Hemisphere remain essential, contributing 29 % to 54 % to the surface concentrations at the Arctic monitoring stations. The rest originated from North American fires.

scholarly journals FLEXPART v10.1 simulation of source contributions to Arctic black carbon

2020 ◽  
Vol 20 (3) ◽  
pp. 1641-1656 ◽  
Author(s):  
Chunmao Zhu ◽  
Yugo Kanaya ◽  
Masayuki Takigawa ◽  
Kohei Ikeda ◽  
Hiroshi Tanimoto ◽  
...  
Keyword(s):  
Black Carbon ◽  
Biomass Burning ◽  
Anthropogenic Sources ◽  
The Arctic ◽  
Anthropogenic Emissions ◽  
High Altitudes ◽  
Arctic Environment ◽  
Gas Flaring ◽  
Rapid Changes ◽  
Arctic Surface

Abstract. The Arctic environment is undergoing rapid changes such as faster warming than the global average and exceptional melting of glaciers in Greenland. Black carbon (BC) particles, which are a short-lived climate pollutant, are one cause of Arctic warming and glacier melting. However, the sources of BC particles are still uncertain. We simulated the potential emission sensitivity of atmospheric BC present over the Arctic (north of 66∘ N) using the FLEXPART (FLEXible PARTicle) Lagrangian transport model (version 10.1). This version includes a new aerosol wet removal scheme, which better represents particle-scavenging processes than older versions did. Arctic BC at the surface (0–500 m) and high altitudes (4750–5250 m) is sensitive to emissions in high latitude (north of 60∘ N) and mid-latitude (30–60∘ N) regions, respectively. Geospatial sources of Arctic BC were quantified, with a focus on emissions from anthropogenic activities (including domestic biofuel burning) and open biomass burning (including agricultural burning in the open field) in 2010. We found that anthropogenic sources contributed 82 % and 83 % of annual Arctic BC at the surface and high altitudes, respectively. Arctic surface BC comes predominantly from anthropogenic emissions in Russia (56 %), with gas flaring from the Yamalo-Nenets Autonomous Okrug and Komi Republic being the main source (31 % of Arctic surface BC). These results highlight the need for regulations to control BC emissions from gas flaring to mitigate the rapid changes in the Arctic environment. In summer, combined open biomass burning in Siberia, Alaska, and Canada contributes 56 %–85 % (75 % on average) and 40 %–72 % (57 %) of Arctic BC at the surface and high altitudes, respectively. A large fraction (40 %) of BC in the Arctic at high altitudes comes from anthropogenic emissions in East Asia, which suggests that the rapidly growing economies of developing countries could have a non-negligible effect on the Arctic. To our knowledge, this is the first year-round evaluation of Arctic BC sources that has been performed using the new wet deposition scheme in FLEXPART. The study provides a scientific basis for actions to mitigate the rapidly changing Arctic environment.

scholarly journals Sources of springtime surface black carbon in the Arctic: an adjoint analysis for April 2008

2017 ◽  
Vol 17 (15) ◽  
pp. 9697-9716 ◽  
Author(s):  
Ling Qi ◽  
Qinbin Li ◽  
Daven K. Henze ◽  
Hsien-Liang Tseng ◽  
Cenlin He
Keyword(s):  
Natural Gas ◽  
Black Carbon ◽  
Biomass Burning ◽  
Transport Model ◽  
Lower Troposphere ◽  
Anthropogenic Sources ◽  
The Arctic ◽  
Anthropogenic Source ◽  
Chemical Transport Model ◽  
Gas Flaring

Abstract. We quantify source contributions to springtime (April 2008) surface black carbon (BC) in the Arctic by interpreting surface observations of BC at five receptor sites (Denali, Barrow, Alert, Zeppelin, and Summit) using a global chemical transport model (GEOS-Chem) and its adjoint. Contributions to BC at Barrow, Alert, and Zeppelin are dominated by Asian anthropogenic sources (40–43 %) before 18 April and by Siberian open biomass burning emissions (29–41 %) afterward. In contrast, Summit, a mostly free tropospheric site, has predominantly an Asian anthropogenic source contribution (24–68 %, with an average of 45 %). We compute the adjoint sensitivity of BC concentrations at the five sites during a pollution episode (20–25 April) to global emissions from 1 March to 25 April. The associated contributions are the combined results of these sensitivities and BC emissions. Local and regional anthropogenic sources in Alaska are the largest anthropogenic sources of BC at Denali (63 % of total anthropogenic contributions), and natural gas flaring emissions in the western extreme north of Russia (WENR) are the largest anthropogenic sources of BC at Zeppelin (26 %) and Alert (13 %). We find that long-range transport of emissions from Beijing–Tianjin–Hebei (also known as Jing–Jin–Ji), the biggest urbanized region in northern China, contribute significantly (∼ 10 %) to surface BC across the Arctic. On average, it takes ∼ 12 days for Asian anthropogenic emissions and Siberian biomass burning emissions to reach the Arctic lower troposphere, supporting earlier studies. Natural gas flaring emissions from the WENR reach Zeppelin in about a week. We find that episodic transport events dominate BC at Denali (87 %), a site outside the Arctic front, which is a strong transport barrier. The relative contribution of these events to surface BC within the polar dome is much smaller (∼ 50 % at Barrow and Zeppelin and ∼ 10 % at Alert). The large contributions from Asian anthropogenic sources are predominately in the form of chronic pollution (∼ 40 % at Barrow, 65 % at Alert, and 57 % at Zeppelin) on about a 1-month timescale. As such, it is likely that previous studies using 5- or 10-day trajectory analyses strongly underestimated the contribution from Asia to surface BC in the Arctic.

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