scholarly journals Supplementary material to "Quantifying the impact of synoptic circulations on ozone variations in North China from April–October 2013–2017"

Author(s):  
Jingda Liu ◽  
Lili Wang ◽  
Mingge Li ◽  
Zhiheng Liao ◽  
Yang Sun ◽  
...  
2019 ◽  
Author(s):  
Jingda Liu ◽  
Lili Wang ◽  
Mingge Li ◽  
Zhiheng Liao ◽  
Yang Sun ◽  
...  

Abstract. The ozone variation characteristics and the impact of synoptic and local meteorological factors in North China were analysed quantitively during the warm season from 2013 to 2017 based on multi-city, in-situ ozone and meteorological data, as well as meteorological reanalysis. The domain-averaged maximum daily 8-h running average O3 (MDA8 O3) concentration was 122 ± 11 μg m−3 with an increase rate of 7.88 μg m−3 year−1, and the three most highly-polluted months were June (149 μg m−3), May (138 μg m−3) and July (132 μg m−3), which was closely related to synoptic circulation variations. Twenty-six synoptic circulation types (merged into 5 weather categories) were objectively identified using the Lamb-Jenkinson method. The highly-polluted weather categories included S-W-N directions, LP (low-pressure related circulation patterns) and C (cyclone type), and corresponding domain-averaged MDA8 O3 concentration were 122, 126 and 128 μg m−3, respectively. Based on the frequency and intensity changes of synoptic circulations, 39.2 % of the inter-annual domain-averaged O3 increase from 2013 to 2017 was attributed to synoptic changes, and intensity of synoptic circulations was the dominant factor. Using synoptic classification and local meteorological factors, the segmented synoptic-regression approach was established to evaluate and forecast daily ozone variations on an urban scale. The results showed that this method is practicable in most cities, and that the dominant factors are the maximum temperature, southerly winds, relative humidity in the previous and in the same day, and total cloud cover. Overall, 43–64 % of the day-to-day variability of MDA8 O3 concentrations was due to local meteorological variations in most cities over North China, except for QHD~32 % and ZZ~25 %. Our quantitative exploration on synoptic and local meteorological factors influencing both on inter-annual and day-to-day ozone variations will provide the scientific basis for evaluating emission reduction measures, since the national and local governments have implemented a series of measures to mitigate air pollution in North China in these five years.


Author(s):  
Weiqi Xu ◽  
Chun Chen ◽  
Yanmei Qiu ◽  
Conghui Xie ◽  
Yunle Chen ◽  
...  

Organic aerosol (OA), a large fraction of fine particles, has a large impact on climate radiative forcing and human health, and the impact depends strongly on size distributions. Here we...


2016 ◽  
Author(s):  
X. Long ◽  
X. X. Tie ◽  
J. J. Cao ◽  
R. J. Huang ◽  
T. Feng ◽  
...  

Abstract. Crop field burning (CFB) has important effects on air pollution in China, but it is seldom quantified and reported in a regional scale, which is of great importance for the control strategies of CFB in China, especially in the North China Plain (NCP). With the provincial statistical data and open crop fires captured by satellite (MODIS), we extracted a detailed emission inventory of CFB during a heavy haze event from 6th to 12th October 2014. A regional dynamical and chemical model (WRF-Chem) was applied to investigate the impact of CFB on air pollution in NCP. The model simulations were compared with the in situ measurements of PM2.5 (particular matter with radius less than 2.5 μm) concentrations. The model evaluation shows that the correlation coefficients (R) between measured and calculated values exceeds 0.80 and absolute normalized mean bias (NMB) is no more than 14 %. In addition, the simulated meteorological parameters such as winds and planetary boundary layer height (PBLH) are also in good agreement with observations. The model was intensive used to study (1) the impacts of CFB and (2) the effect of mountains on regional air quality. The results show that the CFB occurred in southern NCP (SNCP) had significant effect on PM2.5 concentrations locally, causing a maximum of 35 % PM2.5 increase in SNCP. Because of south wind condition, the CFB pollution plume is subjective a long transport to northern NCP (NNCP-with several mega cities, including Beijing of the capital city in China), where there are no significant CFB occurrences, causing a maximum of 32 % PM2.5 increase in NNCP. As a result, the heavy haze in Beijing is enhanced by the CFB occurred in SNCP. Further more, there are two major mountains located in the western and northern NCP. Under the south wind condition, these mountains play important roles in enhancing the PM2.5 pollution in NNCP through the blocking and guiding effects. This study suggests that the PM2.5 emissions in SNCP region should be significantly limited in order to reduce the occurrences of heavy haze events in NNCP region, including the Beijing City.


2021 ◽  
pp. petgeo2020-095
Author(s):  
Michael J. Steventon ◽  
Christopher A-L. Jackson ◽  
Howard D. Johnson ◽  
David M. Hodgson ◽  
Sean Kelly ◽  
...  

The geometry, distribution, and rock properties (i.e. porosity and permeability) of turbidite reservoirs, and the processes associated with turbidity current deposition, are relatively well known. However, less attention has been given to the equivalent properties resulting from laminar sediment gravity-flow deposition, with most research limited to cogenetic turbidite-debrites (i.e. transitional flow deposits) or subsurface studies that focus predominantly on seismic-scale mass-transport deposits (MTDs). Thus, we have a limited understanding of the ability of sub-seismic MTDs to act as hydraulic seals and their effect on hydrocarbon production, and/or carbon storage. We investigate the gap between seismically resolvable and sub-seismic MTDs, and transitional flow deposits on long-term reservoir performance in this analysis of a small (<10 km radius submarine fan system), Late Jurassic, sandstone-rich stacked turbidite reservoir (Magnus Field, northern North Sea). We use core, petrophysical logs, pore fluid pressure, quantitative evaluation of minerals by scanning electron microscopy (QEMSCAN), and 3D seismic-reflection datasets to quantify the type and distribution of sedimentary facies and rock properties. Our analysis is supported by a relatively long (c. 37 years) and well-documented production history. We recognise a range of sediment gravity deposits: (i) thick-/thin- bedded, structureless and structured turbidite sandstone, constituting the primary productive reservoir facies (c. porosity = 22%, permeability = 500 mD), (ii) a range of transitional flow deposits, and (iii) heterogeneous mud-rich sandstones interpreted as debrites (c. porosity = <10%, volume of clay = 35%, up to 18 m thick). Results from this study show that over the production timescale of the Magnus Field, debrites act as barriers, compartmentalising the reservoir into two parts (upper and lower reservoir), and transitional flow deposits act as baffles, impacting sweep efficiency during production. Prediction of the rock properties of laminar and transitional flow deposits, and their effect on reservoir distribution, has important implications for: (i) exploration play concepts, particularly in predicting the seal potential of MTDs, (ii) pore pressure prediction within turbidite reservoirs, and (iii) the impact of transitional flow deposits on reservoir quality and sweep efficiency.Supplementary material:https://doi.org/10.6084/m9.figshare.c.5313860


2021 ◽  
Author(s):  
Yang Yang ◽  
Minqiang Zhou ◽  
Ting Wang ◽  
Bo Yao ◽  
Pengfei Han ◽  
...  

Abstract. Atmospheric CO2 mole fractions are observed at Beijing (BJ), Xianghe (XH), and Xinglong (XL) in North China using the Picarro G2301 Cavity Ring-Down Spectroscopy instruments. The measurement system is described comprehensively for the first time. The geo-distances among these three sites are within 200 km, but they have very different surrounding environments: BJ is inside the megacity; XH is in the suburban area; XL is in the countryside on a mountain. The mean and standard deviation of CO2 mole fractions at BJ, XH, and XL between October 2018 and September 2019 are 448.4 ± 12.8 ppm, 436.0 ± 9.2 ppm and 420.6 ± 8.2 ppm, respectively. The seasonal variations of CO2 at these three sites are similar, with a maximum in winter and a minimum in summer, which is dominated by the terrestrial ecosystem. However, the seasonal variations of CO2 at BJ and XH are more affected by human activities as compared to XL. By using CO2 at XL as the background, CO2 enhancements are observed simultaneously at BJ and XH. The diurnal variations of CO2 are driven by the boundary layer height, photosynthesis and human activities at BJ, XH and XL. Moreover, we address the impact of the wind on the CO2 mole fractions at BJ and XL. This study provides an insight into the spatial and temporal variations of CO2 mole fractions in North China.


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