scholarly journals The impact of large-scale circulation on daily fine particulate matter (PM<sub>2.5</sub>) over major populated regions of China in winter

2021 ◽  
Author(s):  
Zixuan Jia ◽  
Ruth Doherty ◽  
Carlos Ordóñez ◽  
Chaofan Li ◽  
Oliver Wild ◽  
...  
Keyword(s):  
Air Pollution ◽  
Large Scale ◽  
Southern China ◽  
Regional Scale ◽  
Meridional Wind ◽  
River Delta ◽  
Large Scale Circulation ◽  
Siberian High ◽  
Pollution Levels ◽  
The Impact

Abstract. The influence of large-scale circulation on daily PM2.5 variability through its direct effect on key regional meteorological variables is examined over three major populated regions of China: Beijing–Tianjin–Hebei (BTH), the Yangtze River Delta (YRD), and the Pearl River Delta (PRD). In BTH, a shallow East Asian trough curbs northerly cold and dry air from the Siberian High, enhancing PM2.5 pollution levels. Weak southerly winds in eastern and southern China, associated with a weakened Siberian High, suppress horizontal dispersion, contributing to air pollution accumulation over YRD. In PRD, weak southerly winds and precipitation deficits over southern China are conducive to high PM2.5 pollution levels. To account for these dominant large-scale circulation – PM2.5 relationships, we propose three new circulation-based indices for predicting different levels of air pollution based on regional PM2.5 concentrations in each region: a 500 hPa geopotential height-based index for BTH, a sea level pressure-based index for YRD and an 850 hPa meridional wind-based index for PRD. These three indices can effectively distinguish clean days from heavily polluted days in these regions, assuming variation is solely due to meteorology. We also find that including the most important regional meteorological variable in each region improves the performance of the circulation-based indices in predicting daily PM2.5 concentrations on the regional scale. These results are beneficial to understanding and forecasting the occurrence of heavily polluted PM2.5 days in BTH, YRD and PRD from a large-scale perspective.

The impact of large-scale circulation on daily fine particulate matter (PM2.5) in major populated regions of China during winter 

2021 ◽  
Author(s):  
Zixuan Jia ◽  
Ruth Doherty ◽  
Carlos Ordóñez ◽  
Chaofan Li ◽  
Oliver Wild
Keyword(s):  
Particulate Matter ◽  
Relative Humidity ◽  
Large Scale ◽  
Southern China ◽  
East Asian ◽  
River Delta ◽  
Large Scale Circulation ◽  
East Asian Trough ◽  
Siberian High ◽  
Pollution Episodes

&lt;p&gt;With rapid economic growth and urbanization, air pollution episodes with high levels of particulate matter (PM&lt;sub&gt;2.5&lt;/sub&gt;) have become common in China. While emissions of pollutant precursors are important, meteorology also plays a major role in pollution episodes, especially in winter. We examine the influence of the dominant large-scale circulation and the key regional meteorological features on PM&lt;sub&gt;2.5&lt;/sub&gt; over three major regions of China: Beijing&amp;#8211;Tianjin&amp;#8211;Hebei (BTH), the Yangtze River Delta (YRD), and the Pearl River Delta (PRD). The East Asian winter monsoon (EAWM) is primarily studied, including some of its main large-scale components such as the East Asian trough and the Siberian high, as it influences PM&lt;sub&gt;2.5 &lt;/sub&gt;differently in different parts of China. In the BTH region, the shallow East Asian trough curbs the invasion of northerly cold and dry air from the Siberian high which induces high relative humidity and heavy pollution, possibly via relative humidity-promoted aerosol formation and growth. A weak southerly wind in Eastern and Southern China associated with a weakened Siberian high suppresses horizontal dispersion, contributing to pollution accumulation over YRD. In addition, the El Ni&amp;#241;o-Southern Oscillation (ENSO) as the dominant mode of global ocean-atmosphere interaction has a substantial modulation on precipitation over southern China. In the PRD, weak southerly winds and precipitation deficits over southern China are conducive to atmospheric pollution possibly via reduced wet deposition. Furthermore, we construct new circulation-based indices based on the dominant large-scale circulation: a 500 hPa geopotential height-based index for BTH, a sea level pressure-based index for YRD and an 850 hPa meridional wind-based index for PRD. These three indices can effectively distinguish different levels of pollution over BTH, YRD and PRD, respectively. We also show how additional regional meteorological variables can improve the prediction of regional PM&lt;sub&gt;2.5&lt;/sub&gt; concentrations for these three regions. These results are beneficial to understanding and forecasting the occurrence of severely polluted days for BTH, YRD and PRD from a large-scale perspective.&lt;/p&gt;

scholarly journals A Statistical Framework to Identify the Influence of Large-Scale Weather Events on Regional Air Pollution

2011 ◽  
Vol 50 (12) ◽  
pp. 2376-2393 ◽  
Author(s):  
Angadh Singh ◽  
Ahmet Palazoglu
Keyword(s):  
Air Pollution ◽  
Large Scale ◽  
Regional Scale ◽  
Central Valley ◽  
Temporal Patterns ◽  
Pollution Levels ◽  
Statistical Framework ◽  
Weather Events ◽  
The Pacific ◽  
Regional Air Pollution

AbstractRegional air pollution episodes occur as a result of increased emissions and prevalence of conducive meteorological conditions. The frequency of occurrence of such favorable conditions on a regional scale may be influenced by large-scale climatic events like ENSO and the Pacific decadal oscillation (PDO). The scarcity of measurements of criteria pollutants, especially ozone and particulate matter (PM), prior to the last 10–15-yr period, limits the scope of observing the influence of climate variability during recent decades on regional pollution levels. The authors propose a novel statistical framework to utilize available measurements and characterize synoptic influences on regional PM pollution in California’s Central Valley during 1998–2008. The identified target conditions are used to develop a classification scheme to scan historical climate datasets dating back to 1948. The procedure identifies exceedance-conducive days during 1950–98, when no PM2.5 measurements were available. Temporal patterns in seasonal frequency of these identified exceedance-conducive days are investigated for temporal patterns driven by ENSO and PDO.

LARGE-SCALE AIR POLLUTION MODELING IN EUROPE UNDER DIFFERENT CLIMATIC SCENARIOS

2019 ◽  
Vol 01 (02) ◽  
pp. 1950009 ◽  
Author(s):  
ZAHARI ZLATEV ◽  
IVAN DIMOV ◽  
ISTVÁN FARAGÓ ◽  
KRASSIMIR GEORGIEV ◽  
ÁGNES HAVASI
Keyword(s):  
Air Pollution ◽  
High Speed ◽  
Large Scale ◽  
Chemical Species ◽  
Modern Society ◽  
Climatic Changes ◽  
Human Beings ◽  
Pollution Levels ◽  
Pollution Modeling ◽  
The Impact

The treatment of large-scale air pollution models is not only important for modern society, but also an extremely difficult task. Five important physical and chemical processes: (1) horizontal advection, (2) horizontal diffusion, (3) vertical exchange, (4) emission of different pollutants and (5) dry and wet deposition have to be united and handled together. This leads to huge computational problems which have to be treated on modern high-speed parallel architectures by using advanced numerical methods. The computational difficulties are vastly increased when such models are used in the investigation of the impact of climatic changes on high pollution levels that are often exceeding certain critical concentrations and, therefore, are becoming harmful for plants, animals and human beings. There are two major reasons for the great increase in computational difficulties: (a) it is necessary to run the discretized data on fine spatial grid models over very long time-periods consisting of many consecutive years and (b) different scenarios are to be used in order to investigate the sensitivity of the pollution levels to systematic variations of several carefully selected key parameters. How the major difficulties can be resolved is explained here. Furthermore, many results are presented in order to demonstrate the ability of the model to handle successfully the huge computational tasks by using fine space and time discretization and by applying a chemical scheme with many chemical species participating in several hundred chemical reactions. Our results indicate that the climatic changes will often lead to some increases in the pollution levels.

scholarly journals A new indicator on the impact of large-scale circulation on wintertime particulate matter pollution over China

2015 ◽  
Vol 15 (20) ◽  
pp. 11919-11929 ◽  
Author(s):  
B. Jia ◽  
Y. Wang ◽  
Y. Yao ◽  
Y. Xie
Keyword(s):  
Particulate Matter ◽  
Large Scale ◽  
Lower Troposphere ◽  
Circulation Pattern ◽  
Large Scale Circulation ◽  
High Position ◽  
Siberian High ◽  
Modis Aod ◽  
Longitudinal Position ◽  
The Impact

Abstract. Extreme particulate matter (PM) air pollution of January 2013 in China was found to be associated with an anomalous eastward extension of the Siberian High (SH). We developed a Siberian High position index (SHPI), which depicts the mean longitudinal position of the SH, as a new indicator of the large-scale circulation pattern that controls wintertime air quality in China. This SHPI explains 58 % (correlation coefficient of 0.76) of the interannual variability of wintertime aerosol optical depth (AOD) retrieved by MODIS over North China (NC) during 2001–2013. By contrast, the intensity-based conventional Siberian High index (SHI) shows essentially no skill in predicting this AOD variability. On the monthly scale, some high-AOD months for NC are accompanied with extremely high SHPIs; notably, extreme PM pollution of January 2013 can be explained by the SHPI value exceeding 2.6 times the standard deviation of the 2001–2013 January mean. When the SH extends eastward, thus higher SHPI, prevailing northwesterly winds over NC are suppressed not only in the lower troposphere but also in the middle troposphere, leading to reduced southward transport of pollution from NC to South China (SC). The SHPI hence exhibits a significantly negative correlation of −0.82 with MODIS AOD over SC during 2001–2013, although the robustness of this correlation depends on that of satellite-derived AOD. The suppressed northwesterly winds during high-SHPI winters also lead to increased relative humidity (RH) over NC. Both the wind and RH changes are responsible for enhanced PM pollution over NC during the high-SHPI winters.

scholarly journals A new indictor on the impact of large-scale circulation on wintertime particulate matter pollution over China

2015 ◽  
Vol 15 (13) ◽  
pp. 19275-19304 ◽  
Author(s):  
B. Jia ◽  
Y. Wang ◽  
Y. Yao ◽  
Y. Xie
Keyword(s):  
Particulate Matter ◽  
Large Scale ◽  
North China ◽  
Lower Troposphere ◽  
Circulation Pattern ◽  
Large Scale Circulation ◽  
High Position ◽  
Siberian High ◽  
Modis Aod ◽  
The Impact

Abstract. Extreme particulate matter (PM) air pollution of January 2013 in China was found to be associated with anomalous large-scale circulation patterns characterized by an eastward extension of the Siberian High (SH). We developed a Siberian High position index (SHPI), which depicts the mean longitudinal position of SH, as a new indicator of the large-scale circulation pattern that controls wintertime air quality in China. This SHPI explains 58 % (correlation coefficient of 0.76) of the interannual variability of wintertime aerosol optical depth (AOD) derived by MODIS over north China (NC) during 2000–2013, whereas the intensity-based conventional Siberian High Index (SHI) shows essentially no skill in predicting the AOD variability. On the monthly scale, some high-AOD months for NC are accompanied with extremely high SHPIs; notably, extreme PM pollution of January 2013 can be explained by the SHPI value exceeding 2.6 standard deviation of the 2000–2013 mean. When the SH extends eastward, thus higher SHPI, prevailing northwesterly winds over NC are suppressed not only in the lower troposphere but also in the middle troposphere, leading to reduced southward transport of pollution from NC to south China (SC). As a consequence, the SHPI exhibits a significantly negative correlation of −0.82 with MODIS AOD over SC during 2000–2013, although the robustness of this correlation depends on that of satellite-derived AOD. The suppressed northwesterly winds during high-SHPI winters also lead to increased relative humidity (RH) over NC. Both the wind and RH changes are responsible for enhanced PM pollution over north China during the high-SHPI winters.

scholarly journals Characteristics of Large-Scale Circulation Affecting the Inter-Annual Precipitation Variability in Northern Sumatra Island during Boreal Summer

Atmosphere ◽  
2021 ◽  
Vol 12 (2) ◽  
pp. 136
Author(s):  
Yahya Darmawan ◽  
Huang-Hsiung Hsu ◽  
Jia-Yuh Yu
Keyword(s):  
Large Scale ◽  
Precipitation Variability ◽  
Specific Humidity ◽  
Boreal Summer ◽  
Moisture Budget ◽  
Large Scale Circulation ◽  
Budget Analysis ◽  
Sumatra Island ◽  
Precipitation Anomalies ◽  
The Impact

This study aims to explore the contrasting characteristics of large-scale circulation that led to the precipitation anomalies over the northern parts of Sumatra Island. Further, the impact of varying the Asian–Australian Monsoon (AAM) was investigated for triggering the precipitation variability over the study area. The moisture budget analysis was applied to quantify the most dominant component that induces precipitation variability during the JJA (June, July, and August) period. Then, the composite analysis and statistical approach were applied to confirm the result of the moisture budget. Using the European Centre for Medium-Range Weather Forecasts (ECMWF) Re-Anaysis Interim (ERA-Interim) from 1981 to 2016, we identified 9 (nine) dry and 6 (six) wet years based on precipitation anomalies, respectively. The dry years (wet years) anomalies over the study area were mostly supported by downward (upward) vertical velocity anomaly instead of other variables such as specific humidity, horizontal velocity, and evaporation. In the dry years (wet years), there is a strengthening (weakening) of the descent motion, which triggers a reduction (increase) of convection over the study area. The overall downward (upward) motion of westerly (easterly) winds appears to suppress (support) the convection and lead to negative (positive) precipitation anomaly in the whole region but with the largest anomaly over northern parts of Sumatra. The AAM variability proven has a significant role in the precipitation variability over the study area. A teleconnection between the AAM and other global circulations implies the precipitation variability over the northern part of Sumatra Island as a regional phenomenon. The large-scale tropical circulation is possibly related to the PWC modulation (Pacific Walker Circulation).

scholarly journals Quantifying the impact of air pollution on the urban population of Brazil

2007 ◽  
Vol 23 (suppl 4) ◽  
pp. S529-S536 ◽  
Author(s):  
Izabel Marcilio ◽  
Nelson Gouveia
Keyword(s):  
Air Pollution ◽  
Urban Population ◽  
Hospital Admissions ◽  
Age Groups ◽  
The Elderly ◽  
Impact Factors ◽  
Pollution Levels ◽  
Time Series Studies ◽  
The Impact ◽  
Respiratory Causes

This study aimed to quantify air pollution impact on morbidity and mortality in the Brazilian urban population using locally generated impact factors. Concentration-response coefficients were used to estimate the number of hospitalizations and deaths attributable to air pollution in seven Brazilian cities. Poisson regression coefficients (beta) were obtained from time-series studies conducted in Brazil. The study included individuals 65 years old and over and children under five. More than 600 deaths a year from respiratory causes in the elderly and 47 in children were attributable to mean air pollution levels, corresponding to 4.9% and 5.5% of all deaths from respiratory causes in these age groups. More than 4,000 hospital admissions for respiratory conditions were also attributable to air pollution. These results quantitatively demonstrate the currently observed contribution of air pollution to mortality and hospitalizations in Brazilian cities. Such assessment is thought to help support the planning of surveillance and control activities for air pollution in these and similar areas.

scholarly journals Impacts of Large-Scale Circulation on Urban Ambient Concentrations of Gaseous Elemental Mercury in New York, USA

2017 ◽  
Author(s):  
Huiting Mao ◽  
Dolly Hall ◽  
Zhuyun Ye ◽  
Ying Zhou ◽  
Dirk Felton ◽  
...  
Keyword(s):  
New York ◽  
North American ◽  
Large Scale ◽  
Measurement Data ◽  
Elemental Mercury ◽  
Urban Site ◽  
Large Scale Circulation ◽  
Gaseous Elemental Mercury ◽  
The North ◽  
The Impact

Abstract. The impact of large-scale circulation on urban gaseous elemental mercury (GEM) was investigated through analysis of 2008–2015 measurement data from an urban site in New York City (NYC), New York, USA. Distinct annual cycles were observed in 2009–2010 with mixing ratios in warm seasons (i.e. spring–summer) 10–20 ppqv (~ 10 %–25 %) higher than in cool seasons (i.e. fall–winter). This annual cycle was disrupted in 2011 by an anomalously strong influence of the North American trough in that warm season and was reproduced in 2014 with annual amplitude enhanced up to ~ 70 ppqv associated with a particularly strong Bermuda High. North American trough axis index (TAI) and intensity index (TII) were used to characterize the effect of the North American trough on NYC GEM especially in winter and summer. The intensity and position of the Bermuda High had a significant impact on GEM in warm seasons supported by a strong correlation (r reaching 0.96, p 

scholarly journals The influence of spatiality on shipping emissions, air quality and potential human exposure in Yangtze River Delta/Shanghai, China

2018 ◽  
Author(s):  
Junlan Feng ◽  
Yan Zhang ◽  
Shanshan Li ◽  
Jingbo Mao ◽  
Allison P. Patton ◽  
...  
Keyword(s):  
Air Quality ◽  
Yangtze River ◽  
Human Exposure ◽  
Regional Scale ◽  
Yangtze River Delta ◽  
River Delta ◽  
Population Exposure ◽  
Inland Water ◽  
The Yrd ◽  
The Impact

Abstract. The Yangtze River Delta (YRD) and the megacity of Shanghai are host to one of the busiest port clusters in the world, the region also suffers from high levels of air pollution. The goal of this study was to estimate the contributions of shipping to emissions, air quality, and population exposure and characterize their dependence on the geographic spatiality of ship lanes from the regional scale to city scale for 2015. The WRF-CMAQ model was used to simulate the influence of coastal and inland-water shipping, in port emissions, shipping-related cargo transport on air quality and, population-weighted concentrations, a measure of human exposure. Our results showed that the impact of shipping on air quality in the YRD was attributable primarily to shipping emissions within 12 NM of shore, but emissions coming from the coastal area of 24 to 96 NM still contributed substantially to ship-related PM2.5 concentrations in YRD. The overall contribution of ships to PM2.5 concentration in YRD could reach to 4.62 μg/m3 in summer when monsoon winds transport shipping emissions onshore. In Shanghai city, inland-water going ships were major contributors (40–80 %) to the shipping impact on urban air quality. Given the proximity of inland-water ships to urban populations of Shanghai, the emissions of inland-water ships contributed more to population-weighted concentrations. These research results provide scientific evidence to inform policies for controlling future shipping emissions; in particular, stricter standards could be considered for the ships on inland rivers and other waterways close to residential regions.

scholarly journals The Impact of COVID-19 on NO2 and PM2.5 Levels and Their Associations with Human Mobility Patterns in Singapore

2021 ◽  
Author(s):  
Yangyang Li ◽  
Yihan Zhu ◽  
Jia Yu Karen Tan ◽  
Hoong Chen Teo ◽  
Andrea Law ◽  
...  
Keyword(s):  
Air Pollution ◽  
East Coast ◽  
Human Mobility ◽  
Regional Scale ◽  
Air Pollutant ◽  
Pollution Level ◽  
The South ◽  
High Association ◽  
Pollutant Level ◽  
The Impact

AbstractThe decline in NO2 and PM2.5 pollutant levels were observed during COVID-19 around the world, especially during lockdowns. Previous studies explained such observed decline with the decrease in human mobility, whilst overlooking the meteorological changes (e.g., rainfall, wind speed) that could mediate air pollution level simultaneously. This pitfall could potentially lead to over-or under-estimation of the effect of COVID-19 on air pollution. Consequently, this study aims to re-evaluate the impact of COVID-19 on NO2 and PM2.5 pollutant level in Singapore, by incorporating the effect of meteorological parameters in predicting NO2 and PM2.5 baseline in 2020 using machine learning methods. The results found that NO2 and PM2.5 declined by a maximum of 38% and 36%, respectively, during lockdown period. As two proxies for change in human mobility, taxi availability and carpark availability were found to increase and decrease by a maximum of 12.6% and 9.8%, respectively, in 2020 from 2019 during lockdown. To investigate how human mobility influenced air pollutant level, two correlation analyses were conducted: one between PM2.5 and carpark availability changes at regional scale and the other between NO2 and taxi availability changes at a spatial resolution of 0.01°. The NO2 variation was found to be more associated with the change in human mobility, with the correlation coefficients vary spatially across Singapore. A cluster of stronger correlations were found in the South and East Coast of Singapore. Contrarily, PM2.5 and carpark availability had a weak correlation, which could be due to the limit of regional analyses. Drawing to the wider context, the high association between human mobility and NO2 in the South and East Coast area can provide insights into future NO2 reduction policy in Singapore.Graphical Abstract

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