Transport and transformation of atmospheric aerosol across Central Europe with emphasis on anthropogenic sources 

2021 ◽  
Author(s):  
Shubhi Arora ◽  
Radek Lhotka ◽  
Jacub Ondracek ◽  
Petra Pokorna ◽  
Laurent Poulain ◽  
...  
Keyword(s):  
Central Europe ◽  
Atmospheric Aerosol ◽  
State Of The Art ◽  
Chemical Characterization ◽  
Mitigation Strategies ◽  
Receptor Modeling ◽  
Anthropogenic Sources ◽  
Wood Combustion ◽  
Scanning Mobility Particle Sizer ◽  
Transport And Transformation

<p>The trend in PM<sub>10</sub> concentrations in Europe has stagnated over the last two decades, showing only limited annual changes even though there are continued reductions in PM emissions. Possible reasons could be linked to both the aging processes of the particles in the atmosphere and their long-range transport. Therefore, better understanding the multiple origins of the atmospheric aerosol, their sources apportionment at different places are necessary for the development of efficient mitigation strategies. The ultimate objective of the project TRACE is to assess the transport and transformation of atmospheric aerosol across Central Europe with emphasis on anthropogenic sources (including coal and wood combustion) using synergic measurement methods (offline and online) and state-of-the art modelling tools including receptor-oriented models and Chemical transport models. Measurements were performed during winter and summer periods in 2021 simultaneously at three sampling places (Melpitz, DE, Kosetice, CZ, and Frydland, CZ) using state-of-the-art online and offline comprehensive chemical characterization of the atmospheric aerosol. Preliminary results from Scanning Mobility Particle Sizer (SMPS) showed peaks as high as 50 µg/m³ mass concentration during a dust event. Moreover, results from Aerosol Mass Spectrometer (AMS) and receptor modeling (RF) via Positive Matrix Factorization (PMF) from the winter campaign will be presented. </p>

Optical and Chemical Characterization of Aerosols Emitted from Coal, Heavy and Light Fuel Oil, and Small-Scale Wood Combustion

2013 ◽  
Vol 48 (1) ◽  
pp. 827-836 ◽  
Author(s):  
Anna K. Frey ◽  
Karri Saarnio ◽  
Heikki Lamberg ◽  
Fanni Mylläri ◽  
Panu Karjalainen ◽  
...  
Keyword(s):  
Chemical Characterization ◽  
Fuel Oil ◽  
Small Scale ◽  
Wood Combustion

scholarly journals Study of Temporal Variations of Equivalent Black Carbon in a Coastal City in Northwest Spain Using an Atmospheric Aerosol Data Management Software

2021 ◽  
Vol 11 (2) ◽  
pp. 516
Author(s):  
María Piñeiro-Iglesias ◽  
Javier Andrade-Garda ◽  
Sonia Suárez-Garaboa ◽  
Soledad Muniategui-Lorenzo ◽  
Purificación López-Mahía ◽  
...  
Keyword(s):  
Data Management ◽  
Black Carbon ◽  
Light Absorption ◽  
Atmospheric Aerosol ◽  
Urban Areas ◽  
Radiative Properties ◽  
Anthropogenic Sources ◽  
Biomass Combustion ◽  
Management Support ◽  
Diurnal Variability

Light-absorbing carbonaceous aerosols (including black carbon (BC)) pose serious health issues and play significant roles in atmospheric radiative properties. Two-year measurements (2015–2016) of aerosol light absorption, combined with measurements of sub-micrometric particles, were continuously conducted in A Coruña (northwest (NW) Spain) to determine their light absorption properties: absorption coefficients (σabs) and the absorption Ångström exponent (AAE). The mean and standard deviation of equivalent black carbon (eBC) during the period of study were 0.85 ± 0.83 µg m−3, which are lower than other values measured in urban areas of Spain and Europe. High eBC concentrations found in winter are associated with an increase in emissions from anthropogenic sources in combination with lower mixing layer heights and frequent stagnant conditions. The pronounced diurnal variability suggests a strong influence from local sources. AAE had an average value of 1.26 ± 0.22 which implies that both fossil fuel combustion and biomass burning influenced optical aerosol properties. This also highlights biomass combustion in suburban areas, where the use of wood for domestic heating is encouraged, as an important source of eBC. All data treatment was gathered using SCALA© as atmospheric aerosol data management support software program.

Chemical characterization of atmospheric aerosol samples using ion beam techniques

1988 ◽  
Vol 19 (7) ◽  
pp. 1215-1218 ◽  
Author(s):  
Bengt G. Martinsson ◽  
Hans-Christen Hansson
Keyword(s):  
Atmospheric Aerosol ◽  
Ion Beam ◽  
Chemical Characterization

A condensation-growth and impaction method for rapid off-line chemical-characterization of organic submicrometer atmospheric aerosol particles

2003 ◽  
Vol 34 (2) ◽  
pp. 225-242 ◽  
Author(s):  
Berko Sierau ◽  
Frank Stratmann ◽  
Matthias Pelzing ◽  
Christian Neusüß ◽  
Diana Hofmann ◽  
...  
Keyword(s):  
Atmospheric Aerosol ◽  
Aerosol Particles ◽  
Chemical Characterization ◽  
Atmospheric Aerosol Particles ◽  
Condensation Growth

Mutagenic Atmospheric Aerosol Sources Apportioned by Receptor Modeling

2009 ◽  
pp. 187-187-10
Author(s):  
RK Stevens ◽  
CW Lewis ◽  
TG Dzubay ◽  
RE Baumgardner ◽  
RB Zweidinger ◽  
...  
Keyword(s):  
Atmospheric Aerosol ◽  
Receptor Modeling ◽  
Aerosol Sources

scholarly journals Sources and atmospheric dynamics of organic aerosol in New Delhi, India: insights from receptor modeling

2020 ◽  
Vol 20 (2) ◽  
pp. 735-752 ◽  
Author(s):  
Sahil Bhandari ◽  
Shahzad Gani ◽  
Kanan Patel ◽  
Dongyu S. Wang ◽  
Prashant Soni ◽  
...  
Keyword(s):  
Source Apportionment ◽  
Chemical Characterization ◽  
Organic Aerosol ◽  
Receptor Modeling ◽  
World Health ◽  
Aerosol Composition ◽  
Time Resolved ◽  
Online Measurements ◽  
Using Data ◽  
Health Organization

Abstract. Delhi, India, is the second most populated city in the world and routinely experiences some of the highest particulate matter concentrations of any megacity on the planet, posing acute challenges to public health (World Health Organization, 2018). However, the current understanding of the sources and dynamics of PM pollution in Delhi is limited. Measurements at the Delhi Aerosol Supersite (DAS) provide long-term chemical characterization of ambient submicron aerosol in Delhi, with near-continuous online measurements of aerosol composition. Here we report on source apportionment based on positive matrix factorization (PMF), conducted on 15 months of highly time-resolved speciated submicron non-refractory PM1 (NR-PM1) between January 2017 and March 2018. We report on seasonal variability across four seasons of 2017 and interannual variability using data from the two winters and springs of 2017 and 2018. We show that a modified tracer-based organic component analysis provides an opportunity for a real-time source apportionment approach for organics in Delhi. Phase equilibrium modeling of aerosols using the extended aerosol inorganics model (E-AIM) predicts equilibrium gas-phase concentrations and allows evaluation of the importance of the ventilation coefficient (VC) and temperature in controlling primary and secondary organic aerosol. We also find that primary aerosol dominates severe air pollution episodes, and secondary aerosol dominates seasonal averages.

A Study on Methane Emissions and Its Mitigation Strategies in Present Scenario

2016 ◽  
Vol 8 (02) ◽  
pp. 87-92 ◽  
Author(s):  
Virendra Kumar ◽  
Swati SachdevSanjeev Kumar ◽  
Sanjeev Kumar
Keyword(s):  
Carbon Dioxide ◽  
Organic Matter ◽  
Global Warming ◽  
Methane Emission ◽  
Energy Production ◽  
Fossil Fuels ◽  
Mitigation Strategies ◽  
Anthropogenic Sources ◽  
Negative Effects ◽  
Methane Generation

Methane is an important gas of earth's environment. It emits from various naturally as well as anthropogenic sources and responsible for maintaining earth's global temperature favorable for humans and other organisms to live. In recent years many activities of human development led to generation of a large volume of methane which has exhibited catastrophic effect on humans as well as animal lives on earth. Methane poses high global warming potential and has been found second most abounded gas in the environment responsible for global warming of earth after carbon dioxide which is well documented in gigantic body of literature. Methane emission is projected to reach 254 Gg/ year by the year 2025. The sources of methane generation are scattered in nature that includes marshes, paddy crops, landfills and natural anaerobic decomposition of the organic matter present in the environment and digestion in ruminants as well handling and use of fossil fuels. The versatile sources of methane generation are uncontrolled and tough to be tamed. However, its emissions and negative effects could be reduced by effectively and efficiently managing its sources of emission and utilizing generated volume for energy production. This study emphasize on the harmful as well as beneficial aspects of the methane, its utilization and strategies to control emission from various sources.

scholarly journals On the Origin of Carbonaceous Particles in American Cities: Results of Radiocarbon “Dating” and Chemical Characterization

Radiocarbon ◽  
1983 ◽  
Vol 25 (2) ◽  
pp. 603-614 ◽  
Author(s):  
L A Currie ◽  
G A Klouda ◽  
R E Continetti ◽  
I R Kaplan ◽  
W W Wong ◽  
...  
Keyword(s):  
Los Angeles ◽  
Power Plants ◽  
Fine Particles ◽  
Chemical Characterization ◽  
Receptor Modeling ◽  
Organic Chemical ◽  
Dispersion Modeling ◽  
Radiation Balance ◽  
Statistical Characterization ◽  
Carbonaceous Particles

During the past three years radiocarbon assay has emerged as a primary tool in the quantitative assignment of sources of urban and rural particulate pollution. Its use in several major field studies has come about because of its excellent (fossil/biogenic) discriminating power, because of advances in 14C measurements of small samples, and because of the increased significance of carbonaceous particles in the atmosphere. The problem is especially important in the cities, where increased concentrations of fine particles lead to pollution episodes characterized by poor visibility and changes in the radiation balance (absorption, scattering), and immediate and possibly long-term health effects. Efforts in source apportionment in such affected areas have been based on emissions inventories, dispersion modeling, and receptor modeling – ie, chemical and physical (and statistical) characterization of particles collected at designated receptor sites. It is in the last category that 14C has become quite effective in helping to resolve particle sources. Results are presented for studies carried out in Los Angeles, Denver, and Houston which incorporated 14C measurements, inorganic and organic chemical characterization, and receptor modeling. The 14C data indicated wide ranging contributions of biogenic and fossil carbon sources – eg, <10% to 60% contemporary (biogenic) in Houston – depending on meteorological, biological, and anthropological activity. The combined (chemical, isotopic, statistical) data point to sources such as vehicles, wood combustion, power plants, and vegetation.

Size and chemical characterization of atmospheric aerosol and savanna fire samples in Southern Africa

2000 ◽  
Vol 31 ◽  
pp. 186-187 ◽  
Author(s):  
X.D. Liu ◽  
S.P. Dong ◽  
P. Van Espen ◽  
F. Adams ◽  
J. Cafmeyer ◽  
...  
Keyword(s):  
Southern Africa ◽  
Atmospheric Aerosol ◽  
Chemical Characterization

Assessing the Risk of Persistent Drought Using Climate Model Simulations and Paleoclimate Data

2014 ◽  
Vol 27 (20) ◽  
pp. 7529-7549 ◽  
Author(s):  
Toby R. Ault ◽  
Julia E. Cole ◽  
Jonathan T. Overpeck ◽  
Gregory T. Pederson ◽  
David M. Meko
Keyword(s):  
Climate Models ◽  
Climate Model ◽  
State Of The Art ◽  
Global Climate ◽  
Global Climate Models ◽  
Mitigation Strategies ◽  
Drought Risk ◽  
Climate Model Simulations ◽  
Projected Changes ◽  
Paleoclimate Data

Abstract Projected changes in global rainfall patterns will likely alter water supplies and ecosystems in semiarid regions during the coming century. Instrumental and paleoclimate data indicate that natural hydroclimate fluctuations tend to be more energetic at low (multidecadal to multicentury) than at high (interannual) frequencies. State-of-the-art global climate models do not capture this characteristic of hydroclimate variability, suggesting that the models underestimate the risk of future persistent droughts. Methods are developed here for assessing the risk of such events in the coming century using climate model projections as well as observational (paleoclimate) information. Where instrumental and paleoclimate data are reliable, these methods may provide a more complete view of prolonged drought risk. In the U.S. Southwest, for instance, state-of-the-art climate model projections suggest the risk of a decade-scale megadrought in the coming century is less than 50%; the analysis herein suggests that the risk is at least 80%, and may be higher than 90% in certain areas. The likelihood of longer-lived events (&gt;35 yr) is between 20% and 50%, and the risk of an unprecedented 50-yr megadrought is nonnegligible under the most severe warming scenario (5%–10%). These findings are important to consider as adaptation and mitigation strategies are developed to cope with regional impacts of climate change, where population growth is high and multidecadal megadrought—worse than anything seen during the last 2000 years—would pose unprecedented challenges to water resources in the region.

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