scholarly journals Computation of longwave radiative flux and vertical heating rate with 4A-Flux v1.0 as integral part of the radiative transfer code 4A/OP v1.5

2021 ◽  
Author(s):  
Yoann Tellier ◽  
Cyril Crevoisier ◽  
Raymond Armante ◽  
Jean-Louis Dufresne ◽  
Nicolas Meilhac

Abstract. Based on advanced spectroscopic databases, line-by-line and layer-by-layer radiative transfer codes numerically solve the radiative transfer equation with a very high accuracy. Taking advantage of its pre-calculated optical depth look-up table, the fast and accurate radiative transfer model Automatized Atmospheric Absorption Atlas OPerational (4A/OP) calculates the transmission and radiance spectra for a user defined layered atmospheric model. Here we present a module, called 4A-Flux, developed and implemented into 4A/OP in order to include the calculation of the clear-sky longwave radiative flux profiles and heating rate profiles at a very high spectral resolution. Calculations are performed under the assumption of local thermodynamic equilibrium, plane-parallel atmosphere and specular reflection on the surface. The computation takes advantage of pre-tabulated exponential integral functions that are used instead of a classic angular quadrature. Furthermore, the sublayer variation of the Planck function is implemented to better represent the emission of layers with a high optical depth. Thanks to the implementation of 4A-Flux, 4A/OP model have participated in the Radiative Forcing Model Intercomparison Project (RFMIP-IRF) along with other state-of-the-art radiative transfer models. 4A/OP hemispheric flux profiles are compared to other models over the 1800 representative atmospheric situations of RFMIP, yielding an Outgoing Longwave Radiation (OLR) mean difference between 4A/OP and other models of −0.148 W .m−2 and a mean standard deviation of 0.218 W .m−2, showing a good agreement between 4A/OP and other models. 4A/OP is applied to the Thermodynamic Initial Guess Retrieval (TIGR) atmospheric database to analyze the response of the OLR and vertical heating rate to several perturbations of temperature or gas concentration. This work shows that 4A/OP with 4A-Flux module can successfully be used to simulate accurate flux and heating rate profiles and provide useful sensitivity studies including sensitivities to minor trace gases such as HFC134a, HCFC22 and CFC113. We also highlight the interest for the modeling community to extend intercomparison between models to comparisons between spectroscopic databases and modelling to improve the confidence in model simulations.

2021 ◽  
Author(s):  
Filippo Calì Quaglia ◽  
Daniela Meloni ◽  
Alcide Giorgio di Sarra ◽  
Tatiana Di Iorio ◽  
Virginia Ciardini ◽  
...  

<p>Extended and intense wildfires occurred in Northern Canada and, unexpectedly, on the Greenlandic West coast during summer 2017. The thick smoke plume emitted into the atmosphere was transported to the high Arctic, producing one of the largest impacts ever observed in the region. Evidence of Canadian and Greenlandic wildfires was recorded at the Thule High Arctic Atmospheric Observatory (THAAO, 76.5°N, 68.8°W, www.thuleatmos-it.it) by a suite of instruments managed by ENEA, INGV, Univ. of Florence, and NCAR. Ground-based observations of the radiation budget have allowed quantification of the surface radiative forcing at THAAO. </p><p>Excess biomass burning chemical tracers such as CO, HCN, H2CO, C2H6, and NH3 were  measured in the air column above Thule starting from August 19 until August 23. The aerosol optical depth (AOD) reached a peak value of about 0.9 on August 21, while an enhancement of wildfire compounds was  detected in PM10. The measured shortwave radiative forcing was -36.7 W/m2 at 78° solar zenith angle (SZA) for AOD=0.626.</p><p>MODTRAN6.0 radiative transfer model (Berk et al., 2014) was used to estimate the aerosol radiative effect and the heating rate profiles at 78° SZA. Measured temperature profiles, integrated water vapour, surface albedo, spectral AOD and aerosol extinction profiles from CALIOP onboard CALIPSO were used as model input. The peak  aerosol heating rate (+0.5 K/day) was  reached within the aerosol layer between 8 and 12 km, while the maximum radiative effect (-45.4 W/m2) is found at 3 km, below the largest aerosol layer.</p><p>The regional impact of the event that occurred on August 21 was investigated using a combination of atmospheric radiative transfer modelling with measurements of AOD and ground surface albedo from MODIS. The aerosol properties used in the radiative transfer model were constrained by in situ measurements from THAAO. Albedo data over the ocean have been obtained from Jin et al. (2004). Backward trajectories produced through HYSPLIT simulations (Stein et al., 2015) were also employed to trace biomass burning plumes.</p><p>The radiative forcing efficiency (RFE) over land and ocean was derived, finding values spanning from -3 W/m2 to -132 W/m2, depending on surface albedo and solar zenith angle. The fire plume covered a vast portion of the Arctic, with large values of the daily shortwave RF (< -50 W/m2) lasting for a few days. This large amount of aerosol is expected to influence cloud properties in the Arctic, producing significant indirect radiative effects.</p>


2018 ◽  
Vol 10 (10) ◽  
pp. 1632 ◽  
Author(s):  
Bin Yang ◽  
Yuri Knyazikhin ◽  
Donghui Xie ◽  
Haimeng Zhao ◽  
Junqiang Zhang ◽  
...  

Interpreting remotely-sensed data requires realistic, but simple, models of radiative transfer that occurs within a vegetation canopy. In this paper, an improved version of the stochastic radiative transfer model (SRTM) is proposed by assuming that all photons that have not been specularly reflected enter the leaf interior. The contribution of leaf specular reflection is considered by modifying leaf scattering phase function using Fresnel reflectance. The canopy bidirectional reflectance factor (BRF) estimated from this model is evaluated through comparisons with field-measured maize BRF. The result shows that accounting for leaf specular reflection can provide better performance than that when leaf specular reflection is neglected over a wide range of view zenith angles. The improved version of the SRTM is further adopted to investigate the influence of leaf specular reflection on the canopy radiative regime, with emphases on vertical profiles of mean radiation flux density, canopy absorptance, BRF, and normalized difference vegetation index (NDVI). It is demonstrated that accounting for leaf specular reflection can increase leaf albedo, which consequently increases canopy mean upward/downward mean radiation flux density and canopy nadir BRF and decreases canopy absorptance and canopy nadir NDVI when leaf angles are spherically distributed. The influence is greater for downward/upward radiation flux densities and canopy nadir BRF than that for canopy absorptance and NDVI. The results provide knowledge of leaf specular reflection and canopy radiative regime, and are helpful for forward reflectance simulations and backward inversions. Moreover, polarization measurements are suggested for studies of leaf specular reflection, as leaf specular reflection is closely related to the canopy polarization.


2013 ◽  
Vol 13 (14) ◽  
pp. 7097-7114 ◽  
Author(s):  
L. Zhang ◽  
Q. B. Li ◽  
Y. Gu ◽  
K. N. Liou ◽  
B. Meland

Abstract. Atmospheric mineral dust particles exert significant direct radiative forcings and are important drivers of climate and climate change. We used the GEOS-Chem global three-dimensional chemical transport model (CTM) coupled with the Fu-Liou-Gu (FLG) radiative transfer model (RTM) to investigate the dust radiative forcing and heating rate based on different vertical profiles for April 2006. We attempt to actually quantify the sensitivities of radiative forcing to dust vertical profiles, especially the discrepancies between using realistic and climatological vertical profiles. In these calculations, dust emissions were constrained by observations of aerosol optical depth (AOD). The coupled calculations utilizing a more realistic dust vertical profile simulated by GEOS-Chem minimize the physical inconsistencies between 3-D CTM aerosol fields and the RTM. The use of GEOS-Chem simulated vertical profile of dust extinction, as opposed to the FLG prescribed vertical profile, leads to greater and more spatially heterogeneous changes in the estimated radiative forcing and heating rate produced by dust. Both changes can be attributed to a different vertical structure between dust and non-dust source regions. Values of the dust vertically resolved AOD per grid level (VRAOD) are much larger in the middle troposphere, though smaller at the surface when the GEOS-Chem simulated vertical profile is used, which leads to a much stronger heating rate in the middle troposphere. Compared to the FLG vertical profile, the use of GEOS-Chem vertical profile reduces the solar radiative forcing at the top of atmosphere (TOA) by approximately 0.2–0.25 W m−2 over the African and Asian dust source regions. While the Infrared (IR) radiative forcing decreases 0.2 W m−2 over African dust belt, it increases 0.06 W m−2 over the Asian dust belt when the GEOS-Chem vertical profile is used. Differences in the solar radiative forcing at the surface between the use of the GEOS-Chem and FLG vertical profiles are most significant over the Gobi desert with a value of about 1.1 W m−2. The radiative forcing effect of dust particles is more pronounced at the surface over the Sahara and Gobi deserts by using FLG vertical profile, while it is less significant over the downwind area of Eastern Asia.


2007 ◽  
Vol 20 (17) ◽  
pp. 4459-4475 ◽  
Author(s):  
C. J. Stubenrauch ◽  
F. Eddounia ◽  
J. M. Edwards ◽  
A. Macke

Abstract Combined simultaneous satellite observations are used to evaluate the performance of parameterizations of the microphysical and optical properties of cirrus clouds used for radiative flux computations in climate models. Atmospheric and cirrus properties retrieved from Television and Infrared Observation Satellite (TIROS-N) Operational Vertical Sounder (TOVS) observations are given as input to the radiative transfer model developed for the Met Office climate model to simulate radiative fluxes at the top of the atmosphere (TOA). Simulated cirrus shortwave (SW) albedos are then compared to those retrieved from collocated Scanner for Radiation Budget (ScaRaB) observations. For the retrieval, special care has been given to angular direction models. Three parameterizations of cirrus ice crystal optical properties are represented in the Met Office radiative transfer model. These parameterizations are based on different physical approximations and different hypotheses on crystal habit. One parameterization assumes pristine ice crystals and two ice crystal aggregates. By relating the cirrus ice water path (IWP) retrieved from the effective infrared emissivity to the cirrus SW albedo, differences between the parameterizations are amplified. This study shows that pristine crystals seem to be plausible only for cirrus with IWP less than 30 g m−2. For larger IWP, ice crystal aggregates lead to cirrus SW albedos in better agreement with the observations. The data also indicate that climate models should allow the cirrus effective ice crystal diameter (De) to increase with IWP, especially in the range up to 30 g m−2. For cirrus with IWP less than 20 g m−2, this would lead to SW albedos that are about 0.02 higher than the ones of a constant De of 55 μm.


2012 ◽  
Vol 51 (7) ◽  
pp. 1391-1406 ◽  
Author(s):  
U. Schumann ◽  
B. Mayer ◽  
K. Graf ◽  
H. Mannstein

AbstractA new parameterized analytical model is presented to compute the instantaneous radiative forcing (RF) at the top of the atmosphere (TOA) produced by an additional thin contrail cirrus layer (called “contrail” below). The model calculates the RF using as input the outgoing longwave radiation and reflected solar radiation values at TOA for a contrail-free atmosphere, so that the model is applicable for both cloud-free and cloudy ambient atmospheres. Additional input includes the contrail temperature, contrail optical depth (at 550 nm), effective particle radius, particle habit, solar zenith angle, and the optical depth of cirrus above the contrail layer. The model parameters (5 for longwave and 10 for shortwave) are determined from least squares fits to calculations from the “libRadtran” radiative transfer model over a wide range of atmospheric and surface conditions. The correlation coefficient between model and calculations is larger than 98%. The analytical model is compared with published results, including a 1-yr simulation of global RF, and is found to agree well with previous studies. The fast analytical model is part of a larger modeling system to simulate contrail life cycles (“CoCiP”) and can allow for the rapid simulation of contrail cirrus RF over a wide range of meteorological conditions and for a given size-dependent habit mixture. Ambient clouds are shown to have large local impact on the net RF of contrails. Net RF of contrails may both increase and decrease and even change sign in the presence of higher-level cirrus, depending on solar zenith angle.


1995 ◽  
Vol 13 (4) ◽  
pp. 413-418 ◽  
Author(s):  
J. P. F. Fortuin ◽  
R. van Dorland ◽  
W. M. F. Wauben ◽  
H. Kelder

Abstract. With a radiative transfer model, assessments are made of the radiative forcing in northern mid-latitudes due to aircraft emissions up to 1990. Considered are the direct climate effects from the major combustion products carbon dioxide, nitrogen dioxide, water vapor and sulphur dioxide, as well as the indirect effect of ozone production from NOx emissions. Our study indicates a local radiative forcing at the tropopause which should be negative in summer (–0.5 to 0.0 W/m2) and either negative or positive in winter (–0.3 to 0.2 W/m2). To these values the indirect effect of contrails has to be added, which for the North Atlantic Flight Corridor covers the range –0.2 to 0.3 W/m2 in summer and 0.0 to 0.3 W/m2 in winter. Apart from optically dense non-aged contrails during summer, negative forcings are due to solar screening by sulphate aerosols. The major positive contributions come from contrails, stratospheric water vapor in winter and ozone in summer. The direct effect of NO2 is negligible and the contribution of CO2 is relatively small.


2013 ◽  
Vol 52 (3) ◽  
pp. 710-726 ◽  
Author(s):  
Chenxi Wang ◽  
Ping Yang ◽  
Steven Platnick ◽  
Andrew K. Heidinger ◽  
Bryan A. Baum ◽  
...  

AbstractA computationally efficient high-spectral-resolution cloudy-sky radiative transfer model (HRTM) in the thermal infrared region (700–1300 cm−1, 0.1 cm−1 spectral resolution) is advanced for simulating the upwelling radiance at the top of atmosphere and for retrieving cloud properties. A precomputed transmittance database is generated for simulating the absorption contributed by up to seven major atmospheric absorptive gases (H2O, CO2, O3, O2, CH4, CO, and N2O) by using a rigorous line-by-line radiative transfer model (LBLRTM). Both the line absorption of individual gases and continuum absorption are included in the database. A high-spectral-resolution ice particle bulk scattering properties database is employed to simulate the radiation transfer within a vertically nonisothermal ice cloud layer. Inherent to HRTM are sensor spectral response functions that couple with high-spectral-resolution measurements in the thermal infrared regions from instruments such as the Atmospheric Infrared Sounder (AIRS) and Infrared Atmospheric Sounding Interferometer. When compared with the LBLRTM and the discrete ordinates radiative transfer model (DISORT), the root-mean-square error of HRTM-simulated single-layer cloud brightness temperatures in the thermal infrared window region is generally smaller than 0.2 K. An ice cloud optical property retrieval scheme is developed using collocated AIRS and Moderate Resolution Imaging Spectroradiometer (MODIS) data. A retrieval method is proposed to take advantage of the high-spectral-resolution instrument. On the basis of the forward model and retrieval method, a case study is presented for the simultaneous retrieval of ice cloud optical thickness τ and effective particle size Deff that includes a cloud-top-altitude self-adjustment approach to improve consistency with simulations.


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