Effects of Reducing PbO Content on the Elastic and Radiation Attenuation Properties of Germanate Glasses: A New Non-toxic Candidate for Shielding Applications

Author(s):  
M.S. Al- Buriahi ◽  
I.O. Olarinoye ◽  
C. Mutuwong ◽  
H. I. Elsaeedy ◽  
Barış Tamer Tonguç

Abstract This work presents a detailed study on the effects of reducing PbO content on the elastic and radiation shielding properties of germanate glasses described by the chemical formula 50GeO2-(50-x)PbO-xZnO, where x between 0 and 50 mol % with step of 10. A theoretical analysis based on Makishima-Mackenzie's theory (MM-theory) was employed to obtain the elastic moduli of the studied glass specimens. Moreover, the Monte Carlo simulations were applied via Geant4 platform to assess the radiation shielding ability of the GeO2-PbO-ZnO glass system by evaluating several fundamental properties such as gamma and neutron transmission factors, total cross sections, effective atomic numbers, 1/e penetration depths, and exposure buildup factors. We found that the bulk elastic modulus increased from 50.751 GPa to 85.389 GPa as the PbO content increased from 50 mol % to 0. The results of the linear attenuation coefficient show that the cross sections of (σ)PE, (σ)CE, and (σ)pp dominates the photon attenuation at 0.15 ≤ E ≤ 0.08; 0.8 < E < 8, and 8 < E < 15 MeV respectively. Moreover, the present glasses have superior photon absorbing capacity compared to ordinary and barite concrete; RS-253-G18 and RS-360 commercial glass shields. This suggests that the GeO2-PbO-ZnO glass system can be used as a non-toxic shielding material in the nuclear facilities.

2020 ◽  
Vol 15 (11) ◽  
pp. 1374-1380
Author(s):  
H. Almohiy ◽  
M. Saad ◽  
Y. M. AbouDeif ◽  
Iwona Grelowska ◽  
M. Reben ◽  
...  

This research reported on the radiation safety characteristics of doped fluorophosphate glasses with heavy rare earth lanthanide (Sm2O3) in the composition 40P2O5/30ZnO/20BaF2/3.8K2TeO3/1.2Al2O3/5.0Nb2O5/30000 ppm Sm2O3 and 40P2O5/30ZnO/20BaF2/3.8K2TeO3/1.2Al2O3/5.0Nb2O5/40000 ppm Sm2O3 in mol%. The parameters for shielding like that mass attenuation coefficient, MAC, linear attenuation coefficient, LAC, tenth value layers, TVL, half-value layers, HVL, effective atomic number, (Zeff), mean free path, MFP, electron density, Neff, electronic cross-sections, ECS, and total atomic cross-sections, ACS, were calculated between 0.015 and 15 MB of preparation glasses. The protection parameters of the current glasses are good in comparison to industrial materials used for nuclear shieldings, such as glass RS 253, ordinary concrete (OC), hematite serpenite (HS), or basalt magnet (BM). From the above mention results, the prepared glasses can be used as radiation safety materials.


2021 ◽  
Vol 0 (0) ◽  
Author(s):  
Canel Eke

Abstract The goal of this study is to examine theoretically radiation absorption properties of zinc alumino bismuth borate (BZnAlBiSm) glasses with chemical formula 60B2O3-9ZnO-(30-x)Al2O3-xBi2O3-1Sm2O3 where x = 5, 10, 15 and 20 mol%. The linear and mass attenuation coefficents of BZnAlBiSm glasses turn out as this trend BZnAlBiSm-1<BZnAlBiSm-2<BZnAlBiSm-3<BZnAlBiSm-4. The BZnAlBiSm-4 with the smallest half value layers, tenth value layers and mean free paths in the examined energy ranges has the superior radiation shielding characteristics among the BZnAlBiSm glasses. The BZnAlBiSm-4 glass has the highest radiation protection efficiency among the BZnAlBiSm glasses. The transmission factors increase as photon energy range enhances from 0.015 to 15 MeV and thickness declines from 2.5 to 0.5 cm. The energy buildup factors and energy absorption buildup factors of BZnAlBiSm glasses reduce from 15 to 1 mfp. Variation of the effective atomic number and effective electron density as a function of photon energy for BZnAlBiSm glasses are similar. The projected ranges of electron, proton, alpha and carbon for the BZnAlBiSm glasses increase as photon energy enlarges. The fast neutron removal cross sections of the BZnAlBiSm glasses vary in order of BZnAlBiSm-4<BZnAlBiSm-3<BZnAlBiSm-2<BZnAlBiSm-1. Thus, it can be concluded that BZnAlBiSm-1 has the highest neutron absorption ability among the BZnAlBiSm glasses.


Author(s):  
S. Golladay

The theory of multiple scattering has been worked out by Groves and comparisons have been made between predicted and observed signals for thick specimens observed in a STEM under conditions where phase contrast effects are unimportant. Independent measurements of the collection efficiencies of the two STEM detectors, calculations of the ratio σe/σi = R, where σe, σi are the total cross sections for elastic and inelastic scattering respectively, and a model of the unknown mass distribution are needed for these comparisons. In this paper an extension of this work will be described which allows the determination of the required efficiencies, R, and the unknown mass distribution from the data without additional measurements or models. Essential to the analysis is the fact that in a STEM two or more signal measurements can be made simultaneously at each image point.


Materials ◽  
2021 ◽  
Vol 14 (5) ◽  
pp. 1158
Author(s):  
Huseyin O. Tekin ◽  
Shams A. M. Issa ◽  
Gokhan Kilic ◽  
Hesham M. H. Zakaly ◽  
Mohamed M. Abuzaid ◽  
...  

In the current study, promising glass composites based on vanadium pentoxide (V2O5)-doped zinc borate (ZnB) were investigated in terms of their nuclear-radiation-shielding dynamics. The mass and linear attenuation coefficient, half-value layer, mean free path, tenth-value layer, effective atomic number, exposure-buildup factor, and energy-absorption-buildup factor were deeply simulated by using MCNPX code, Phy-X PSD code, and WinXcom to study the validation of ZBV1, ZBV2, ZBV3, and ZBV4 based on (100−x)(0.6ZnO-0.4B2O3)(x)(V2O5) (x = 1, 2, 3, 4 mol%) samples against ionizing radiation. The results showed that attenuation competencies of the studied glasses slightly changed while increasing the V2O5 content from 1 mol% to 4 mol%. The domination of ZnO concentration in the composition compared to B2O3 makes ZnO substitution with V2O5 more dominant, leading to a decrease in density. Since density has a significant role in the attenuation of gamma rays, a negative effect was observed. It can be concluded that the aforementioned substitution can negatively affect the shielding competencies of studied glasses.


2021 ◽  
Vol 2021 (1) ◽  
Author(s):  
Roman N. Lee ◽  
Alexey A. Lyubyakin ◽  
Vyacheslav A. Stotsky

Abstract Using modern multiloop calculation methods, we derive the analytical expressions for the total cross sections of the processes e−γ →$$ {e}^{-}X\overline{X} $$ e − X X ¯ with X = μ, γ or e at arbitrary energies. For the first two processes our results are expressed via classical polylogarithms. The cross section of e−γ → e−e−e+ is represented as a one-fold integral of complete elliptic integral K and logarithms. Using our results, we calculate the threshold and high-energy asymptotics and compare them with available results.


2006 ◽  
Vol 39 (6) ◽  
pp. 1337-1344 ◽  
Author(s):  
J Beale ◽  
S Armitage ◽  
G Laricchia

2021 ◽  
Vol 196 ◽  
pp. 110566
Author(s):  
Jamila S. Alzahrani ◽  
Miysoon A. Alothman ◽  
Canel Eke ◽  
Hanan Al-Ghamdi ◽  
Dalal Abdulldh Aloraini ◽  
...  

Sign in / Sign up

Export Citation Format

Share Document