scholarly journals Mo:BiVO4 Nanoparticles-Based Optical Modulator and Its Application in a 2-μm Pulsed Laser

Nanomaterials ◽  
2021 ◽  
Vol 11 (12) ◽  
pp. 3243
Author(s):  
Lina Zhao ◽  
Wenyu Zhang ◽  
Ye Yuan ◽  
Luyang Tong ◽  
Jingjing Liu ◽  
...  

Mo:BiVO4 nanoparticles were employed as an optical modulator in a Q-switched all-solid-state Tm:YAP laser for the first time. The nonlinear optical parameters of Mo:BiVO4 nanoparticles in the 2-μm region were characterized by measuring nonlinear transmission. Saturation intensity was 718 MW/cm2, and the modulation depth was 12.3%. A stable pulse sequence was acquired with a 70.08 kHz maximum repetition rate and an 821 ns pulse width. The maximum output average power was 153 mW, corresponding to 2.18 μJ single pulse energy and 2.67 W peak power. Although the response wavelength of Mo:BiVO4 is in visible light region, our experimental results demonstrates that a saturable absorption effect for wavelengths much longer than visible light (2 μm wavelength) is still possible due to sub-bandgap absorption. Therefore, we experimentally proved that Mo:BiVO4 nanoparticles are a great candidate for use as an optical modulator of a 2-μm pulsed laser.

Nanomaterials ◽  
2019 ◽  
Vol 9 (6) ◽  
pp. 865 ◽  
Author(s):  
Tao Wang ◽  
Jin Wang ◽  
Jian Wu ◽  
Pengfei Ma ◽  
Rongtao Su ◽  
...  

In recent years, metal chalcogenide nanomaterials have received much attention in the field of ultrafast lasers due to their unique band-gap characteristic and excellent optical properties. In this work, two-dimensional (2D) indium monosulfide (InS) nanosheets were synthesized through a modified liquid-phase exfoliation method. In addition, a film-type InS-polyvinyl alcohol (PVA) saturable absorber (SA) was prepared as an optical modulator to generate ultrashort pulses. The nonlinear properties of the InS-PVA SA were systematically investigated. The modulation depth and saturation intensity of the InS-SA were 5.7% and 6.79 MW/cm2, respectively. By employing this InS-PVA SA, a stable, passively mode-locked Yb-doped fiber laser was demonstrated. At the fundamental frequency, the laser operated at 1.02 MHz, with a pulse width of 486.7 ps, and the maximum output power was 1.91 mW. By adjusting the polarization states in the cavity, harmonic mode-locked phenomena were also observed. To our knowledge, this is the first time an ultrashort pulse output based on InS has been achieved. The experimental findings indicate that InS is a viable candidate in the field of ultrafast lasers due to its excellent saturable absorption characteristics, which thereby promotes the ultrafast optical applications of InX (X = S, Se, and Te) and expands the category of new SAs.


Nanomaterials ◽  
2019 ◽  
Vol 9 (10) ◽  
pp. 1419 ◽  
Author(s):  
Wang ◽  
Zheng ◽  
Guo ◽  
Chen ◽  
Zhang ◽  
...  

Recently, two-dimensional (2D) materials have been widely studied by researchers due to their exceptional 2D structure and excellent optical characteristics. As one of the typically-layered 2D transition metal dichalcogenide (TMD) semiconductors from group IVB with a bandgap value of 0.9–1.2 eV (bulk to monolayer), the characteristics of zirconium diselenide (ZrSe2) have already been extensively investigated in many fields. However, the nonlinear absorption properties of ZrSe2 in ultra-fast lasers have not been previously demonstrated. In this work, we measured various parameters in order to investigate the characteristics of the nonlinear saturable absorption of ZrSe2. A ZrSe2–polyvinyl alcohol (PVA) film was successfully prepared, which was employed as a saturable absorber (SA) to demonstrate, for the first time, an erbium (Er)-doped passive mode-locking fiber laser with a ring cavity. The saturation intensity of the ZrSe2–PVA film-type SA is 12.72 MW/cm2, while its modulation depth is 2.3%. The stable soliton state with a maximum output power of 11.37 mW and a narrowest monopulse duration of 12.5 ps at a repetition frequency of 21.22 MHz was detected. The experimental results conclusively proved that ZrSe2, with its suitable bandgap value and excellent nonlinear absorption properties, as well as its high damage threshold, should have extensive potential applications within the field of ultra-fast pulse lasers.


Molecules ◽  
2021 ◽  
Vol 26 (11) ◽  
pp. 3460
Author(s):  
Jingcheng Shang ◽  
Yizhou Liu ◽  
Shengzhi Zhao ◽  
Yuefeng Zhao ◽  
Yuzhi Song ◽  
...  

We experimentally investigate the formation of various pulses from a thulium–holmium (Tm–Ho)-codoped nonlinear polarization rotation (NPR) mode-locking fiber oscillator. The ultrafast fiber oscillator can simultaneously operate in the noise-like and soliton mode-locking regimes with two different emission wavelengths located around 1947 and 2010 nm, which are believed to be induced from the laser transition of Tm3+ and Ho3+ ions respectively. When the noise-like pulse (NLP) and soliton pulse (SP) co-exist inside the laser oscillator, a maximum output power of 295 mW is achieved with a pulse repetition rate of 19.85-MHz, corresponding to a total single pulse energy of 14.86 nJ. By adjusting the wave plates, the fiber oscillator could also deliver the dual-NLPs or dual-SPs at dual wavelengths, or single NLP and single SP at one wavelength. The highest 61-order harmonic soliton pulse and 33.4-nJ-NLP are also realized respectively with proper design of the fiber cavity.


Author(s):  
Yangyu Liu ◽  
Xue Cao ◽  
AnHua Xian ◽  
Guangmiao Liu ◽  
Wei zhou ◽  
...  

Abstract We demonstrate stable continuous-wave mode-locking (CWML) pulses around 1645nm by employing the home-made Er:YAG ceramic. By using a fiber laser and semiconductor saturable absorber mirror (SESAM) with modulation depth of 1.2%, we get ML pulses with the output average power up to 815 mW, the pulse width shortened as ~4 ps, and the peak power of 1.8 kW. With the SESAM of modulation depth of 2.4%, the second-order harmonic ML pulses were also obtained. As far as we know, this is the first report of CWML from Er3+-doped ceramics and also the shortest pulse duration in Er3+-doped solid-state oscillators.


2000 ◽  
Author(s):  
D. H. Chen ◽  
Z. M. Zhang

Abstract A simplified finite element model is built to study the thermal response of the 193-nm pulsed-laser calorimeter. The nonequivalence between pulsed-laser heating and electrical heating is estimated to be 0.46% at the thermocouple locations by comparing the calibration factors for average-power laser heating and electrical heating. This study should help the development of calibration and measurement standards in pulsed energy measurements for deep ultraviolet excimer lasers that are important for photolithographic and materials processing applications.


2007 ◽  
Vol 60 (10) ◽  
pp. 779 ◽  
Author(s):  
Michael Buback ◽  
Pascal Hesse ◽  
Thomas Junkers ◽  
Thomas Theis ◽  
Philipp Vana

The chain-length dependence of the termination rate coefficient, kt, in methyl acrylate (MA) and dodecyl acrylate (DA) radical polymerization has been determined via the single pulse pulsed-laser polymerization near-infrared reversible addition–fragmentation chain transfer (SP-PLP-NIR-RAFT) technique. Polymerization is induced by a laser SP and the resulting decay in monomer concentration, cM, is monitored via NIR spectroscopy with a time resolution of microseconds. A RAFT agent ensures the correlation of radical chain length and monomer-to-polymer conversion. The obtained rate coefficients for termination of two radicals of approximately the same chain length, i, are represented by power-law expressions, kt(i,i) ∝ i–α. For both monomers, composite model behaviour of kt(i,i) showing two distinct chain length regimes is observed. The exponent αs referring to short chain lengths is close to unity, whereas the exponent αl, which characterizes the chain-length dependency of large radicals, is slightly above the theoretical value for coiled chain-end radicals. The crossover chain length, ic, which separates the two regions, decreases from MA (ic = 30) to DA (ic = 20). The results for MA and DA are consistent with earlier data reported for butyl acrylate. There appears to be a correlation of αs and ic with chain flexibility.


2017 ◽  
Vol 2017 ◽  
pp. 1-9 ◽  
Author(s):  
Shuqing Chen ◽  
Zhiqiang Xie ◽  
Junmin Liu ◽  
Yanliang He ◽  
Yao Cai ◽  
...  

By using optical heterodyne technique, we demonstrated the stable emission of sub-terahertz wave with the frequency ranging from 88 GHz to 101 GHz, which can operate as microwave source for nonlinear response measurement system. Mutual frequency beating of two well-separated sideband signals at a 0.1 THz photo-detector (PD) allows for the generation of sub-terahertz signal. Based on this approach, we have achieved the radiation of 0.1 THz wave with power up to 4 mW. By transmittance measurement, two-dimensional nanomaterial topological insulator (TI: Bi2Te3) shows saturable absorption behaviors with normalized modulation depth of 47% at 0.1 THz. Our results show that optical heterodyne technique could be developed as an effective microwave source generation for nonlinear measurement at sub-terahertz, even terahertz band.


2018 ◽  
Vol 2018 ◽  
pp. 1-7
Author(s):  
Xinyue Guo ◽  
Shuangshuang Li ◽  
Yang Guo

With the rapid development of light-emitting diode, visible light communication (VLC) has become a candidate technology for the next generation of high-speed indoor wireless communication. In this paper, we investigate the performance of the 32-quadrature amplitude modulation (32-QAM) constellation shaping schemes for the first time, where two special circular constellations, named Circular (4, 11, 17) and Circular (1, 5, 11, 15), and a triangular constellation are proposed based on the Shannon’s criterion. Theoretical analysis indicates that the triangular constellation scheme has the largest minimum Euclidian distance while the Circular (4, 11, 17) scheme achieves the lowest peak-to-average power ratio (PAPR). Experimental results show that the bit error rate performance is finally decided by the value of PAPR in the VLC system due to the serious nonlinearity of the LED, where the Circular (4, 11, 17) scheme always performs best under the 7% preforward error correction threshold of 3.8 × 10−3 with 62.5Mb/s transmission data rate and 1-meter transmission distance.


Nanomaterials ◽  
2021 ◽  
Vol 11 (8) ◽  
pp. 2078
Author(s):  
Qianqian Shi ◽  
Guodong Zhang ◽  
Yuheng Wang ◽  
Yu Lan ◽  
Jiang Wang ◽  
...  

Vanadium pentoxide (V2O5) is the most stable phase among many transition metal vanadium oxides, and has already been widely used in many fields. In this study, the morphological, structural, and optical responses of V2O5 film to ultrafast laser irradiation was investigated. The third-order nonlinear optical properties of V2O5 film were measured by common Z-scan technique, and the results showed that V2O5 film has self-defocusing and saturable absorption characteristics. The third-order nonlinear absorption coefficient and nonlinear refractive index were calculated to be −338 cm/GW and −3.62 × 10−12 cm2/W, respectively. The tunable saturated absorption with modulation depth ranging from 13.8% to 29.3% was realized through controlling the thickness of vanadium pentoxide film. V2O5 film was irradiated by ultrafast laser with variable pulse energy, and the morphological and structural responses of the V2O5 to the laser with different energy densities were investigated. The irreversible morphological and structural responses of V2O5 films to ultrafast laser irradiation was analyzed using the phase-contrast microscope and Raman spectrum. The chemical structure change from V2O5 to V6O13 was considered the main reason for refractive index modification.


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