scholarly journals Optimal estimation of tropospheric H<sub>2</sub>O and δD with IASI/METOP

2011 ◽  
Vol 11 (21) ◽  
pp. 11207-11220 ◽  
Author(s):  
M. Schneider ◽  
F. Hase

Abstract. We present optimal estimates of tropospheric H2O and δD derived from radiances measured by the instrument IASI (Infrared Atmospheric Sounding Interferometer) flown on EUMETSAT's polar orbiter METOP. We document that the IASI spectra allow for retrieving H2O profiles between the surface and the upper troposphere as well as middle tropospheric δD values. A theoretical error estimation suggests a precision for H2O of better than 35% in the lower troposphere and of better than 15% in the middle and upper troposphere, respectively, whereby surface emissivity and atmospheric temperature uncertainties are the leading error sources. For the middle tropospheric δD values we estimate a precision of 15–20‰ with the measurement noise being the dominating error source. The accuracy of the IASI products is estimated to about 20–10% and 10‰ for lower to upper tropospheric H2O and middle tropospheric δD, respectively. It is limited by systematic uncertainties in the applied spectroscopic parameters and the a priori atmospheric temperature profiles. We compare our IASI products to a large number of near coincident radiosonde in-situ and ground-based FTS (Fourier Transform Spectrometer) remote sensing measurements. The bias and the scatter between the different H2O and δD data sets are consistent with the combined theoretical uncertainties of the involved measurement techniques.

2011 ◽  
Vol 11 (5) ◽  
pp. 16107-16146 ◽  
Author(s):  
M. Schneider ◽  
F. Hase

Abstract. We present an optimal estimation retrieval for tropospheric H2O and δD applying thermal nadir spectra measured by the instrument IASI (Infrared Atmospheric Sounding Interferometer) flown on EUMETSAT's polar orbiter METOP. We document that the IASI spectra allow for retrieving H2O profiles between the surface and the upper troposphere as well as middle tropospheric δD values. A theoretical error estimation suggests a precision for H2O of better than 35 % in the lower troposphere and of better than 15 % in the middle and upper troposphere, respectively, whereby surface emissivity and atmospheric temperature uncertainties are the leading error sources. For the middle tropospheric δD values we estimate a precision of 15–20‰, with the measurement noise being the dominating error source. We compare our IASI products to a large number of quasi coincident radiosonde in-situ and ground-based FTS (Fourier Transform Spectrometer) remote sensing measurements and find no significant bias between the H2O and δD data obtained by the different techniques. Furthermore, the scatter between the different data sets confirms our theoretical precision estimates.


2014 ◽  
Vol 14 (1) ◽  
pp. 103-114 ◽  
Author(s):  
J. X. Warner ◽  
R. Yang ◽  
Z. Wei ◽  
F. Carminati ◽  
A. Tangborn ◽  
...  

Abstract. This study tests a novel methodology to add value to satellite data sets. This methodology, data fusion, is similar to data assimilation, except that the background model-based field is replaced by a satellite data set, in this case AIRS (Atmospheric Infrared Sounder) carbon monoxide (CO) measurements. The observational information comes from CO measurements with lower spatial coverage than AIRS, namely, from TES (Tropospheric Emission Spectrometer) and MLS (Microwave Limb Sounder). We show that combining these data sets with data fusion uses the higher spectral resolution of TES to extend AIRS CO observational sensitivity to the lower troposphere, a region especially important for air quality studies. We also show that combined CO measurements from AIRS and MLS provide enhanced information in the UTLS (upper troposphere/lower stratosphere) region compared to each product individually. The combined AIRS–TES and AIRS–MLS CO products are validated against DACOM (differential absorption mid-IR diode laser spectrometer) in situ CO measurements from the INTEX-B (Intercontinental Chemical Transport Experiment: MILAGRO and Pacific phases) field campaign and in situ data from HIPPO (HIAPER Pole-to-Pole Observations) flights. The data fusion results show improved sensitivities in the lower and upper troposphere (20–30% and above 20%, respectively) as compared with AIRS-only version 5 CO retrievals, and improved daily coverage compared with TES and MLS CO data.


2014 ◽  
Vol 14 (23) ◽  
pp. 12613-12629 ◽  
Author(s):  
P. Eriksson ◽  
B. Rydberg ◽  
H. Sagawa ◽  
M. S. Johnston ◽  
Y. Kasai

Abstract. Retrievals of cloud ice mass and humidity from the Superconducting Submillimeter-Wave Limb-Emission Sounder (SMILES) and the Odin-SMR (Sub-Millimetre Radiometer) limb sounder are presented and example applications of the data are given. SMILES data give an unprecedented view of the diurnal variation of cloud ice mass. Mean regional diurnal cycles are reported and compared to some global climate models. Some improvements in the models regarding diurnal timing and relative amplitude were noted, but the models' mean ice mass around 250 hPa is still low compared to the observations. The influence of the ENSO (El Niño–Southern Oscillation) state on the upper troposphere is demonstrated using 12 years of Odin-SMR data. The same retrieval scheme is applied for both sensors, and gives low systematic differences between the two data sets. A special feature of this Bayesian retrieval scheme, of Monte Carlo integration type, is that values are produced for all measurements but for some atmospheric states retrieved values only reflect a priori assumptions. However, this "all-weather" capability allows a direct statistical comparison to model data, in contrast to many other satellite data sets. Another strength of the retrievals is the detailed treatment of "beam filling" that otherwise would cause large systematic biases for these passive cloud ice mass retrievals. The main retrieval inputs are spectra around 635/525 GHz from tangent altitudes below 8/9 km for SMILES/Odin-SMR, respectively. For both sensors, the data cover the upper troposphere between 30° S and 30° N. Humidity is reported as both relative humidity and volume mixing ratio. The vertical coverage of SMILES is restricted to a single layer, while Odin-SMR gives some profiling capability between 300 and 150 hPa. Ice mass is given as the partial ice water path above 260 hPa, but for Odin-SMR ice water content, estimates are also provided. Besides a smaller contrast between most dry and wet cases, the agreement with Aura MLS (Microwave Limb Sounder) humidity data is good. In terms of tropical mean humidity, all three data sets agree within 3.5 %RHi. Mean ice mass is about a factor of 2 lower compared to CloudSat. This deviation is caused by the fact that different particle size distributions are assumed, combined with saturation and a priori influences in the SMILES and Odin-SMR data.


2005 ◽  
Vol 5 (6) ◽  
pp. 1665-1677 ◽  
Author(s):  
A. von Engeln ◽  
G. Nedoluha

Abstract. The Optimal Estimation Method is used to retrieve temperature and water vapor profiles from simulated radio occultation measurements in order to assess how different retrieval schemes may affect the assimilation of this data. High resolution ECMWF global fields are used by a state-of-the-art radio occultation simulator to provide quasi-realistic bending angle and refractivity profiles. Both types of profiles are used in the retrieval process to assess their advantages and disadvantages. The impact of the GPS measurement is expressed as an improvement over the a priori knowledge (taken from a 24h old analysis). Large improvements are found for temperature in the upper troposphere and lower stratosphere. Only very small improvements are found in the lower troposphere, where water vapor is present. Water vapor improvements are only significant between about 1 km to 7 km. No pronounced difference is found between retrievals based upon bending angles or refractivity. Results are compared to idealized retrievals, where the atmosphere is spherically symmetric and instrument noise is not included. Comparing idealized to quasi-realistic calculations shows that the main impact of a ray tracing algorithm can be expected for low latitude water vapor, where the horizontal variability is high. We also address the effect of altitude correlations in the temperature and water vapor. Overall, we find that water vapor and temperature retrievals using bending angle profiles are more CPU intensive than refractivity profiles, but that they do not provide significantly better results.


2013 ◽  
Vol 6 (5) ◽  
pp. 1413-1423 ◽  
Author(s):  
W. W. Verstraeten ◽  
K. F. Boersma ◽  
J. Zörner ◽  
M. A. F. Allaart ◽  
K. W. Bowman ◽  
...  

Abstract. In this analysis, Tropospheric Emission Spectrometer (TES) V004 nadir ozone (O3) profiles are validated with more than 4400 coinciding ozonesonde measurements taken across the world from the World Ozone and Ultraviolet Radiation Data Centre (WOUDC) during the period 2005–2010. The TES observation operator was applied to the sonde data to ensure a consistent comparison between TES and ozonesonde data, i.e. without the influence of the a priori O3 profile needed to regulate the retrieval. Generally, TES V004 O3 retrievals are biased high by 2–7 ppbv (7–15%) in the troposphere, consistent with validation results from earlier studies. Because of two degrees of freedom for signal in the troposphere, we can distinguish between upper and lower troposphere mean biases, respectively ranging from −0.4 to +13.3 ppbv for the upper troposphere and +3.9 to +6.0 ppbv for the lower troposphere. Focusing on the 464 hPa retrieval level, broadly representative of the free tropospheric O3, we find differences in the TES biases for the tropics (+3 ppbv, +7%), sub-tropics (+5 ppbv, +11%), and northern (+7 ppbv, +13%) and southern mid-latitudes (+4 ppbv, +10%). The relatively long-term record (6 yr) of TES–ozonesonde comparisons allowed us to quantify temporal variations in TES biases at 464 hPa. We find that there are no discernable biases in each of these latitudinal bands; temporal variations in the bias are typically within the uncertainty of the difference between TES and ozonesondes. Establishing these bias patterns is important in order to make meaningful use of TES O3 data in applications such as model evaluation, trend analysis, or data assimilation.


2013 ◽  
Vol 13 (6) ◽  
pp. 15409-15441
Author(s):  
J. X. Warner ◽  
R. Yang ◽  
Z. Wei ◽  
F. Carminati ◽  
A. Tangborn ◽  
...  

Abstract. This study tests a novel methodology to add value to satellite datasets. This methodology, data fusion, is similar to data assimilation, except that the background model-based field is replaced by a satellite dataset, in this case AIRS (Atmospheric Infrared Sounder) carbon monoxide (CO) measurements. The observational information comes from CO measurements with lower spatial coverage than AIRS, namely, from TES (Tropospheric Emission Spectrometer) and MLS (Microwave Limb Sounder). We show that combining these datasets with data fusion uses the higher spectral resolution of TES to extend AIRS CO observational sensitivity to the lower troposphere, a region especially important for air quality studies. We also show that combined CO measurements from AIRS and MLS provide enhanced information in the UTLS (upper troposphere/lower stratosphere) region compared to each product individually. The combined AIRS/TES and AIRS/MLS CO products are validated against DACOM (differential absorption mid-IR diode laser spectrometer) in situ CO measurements from the INTEX-B (Intercontinental Chemical Transport Experiment: MILAGRO and Pacific phases) field campaign and in situ data from HIPPO (HIAPER Pole-to-Pole Observations) flights. The data fusion results show improved sensitivities in the lower and upper troposphere (20–30% and above 20%, respectively) as compared with AIRS-only retrievals, and improved coverage compared with TES and MLS CO data.


2013 ◽  
Vol 13 (3) ◽  
pp. 7061-7079 ◽  
Author(s):  
J.-B. Renard ◽  
S. N. Tripathi ◽  
M. Michael ◽  
A. Rawal ◽  
G. Berthet ◽  
...  

Abstract. Electrified aerosols have been observed in the lower troposphere and in the mesosphere, but have never been detected in the stratosphere and upper troposphere. We present measurements of aerosols during a balloon flight to an altitude of ~24 km. The measurements were performed with an improved version of the STAC aerosol counter dedicated to the search for charged aerosols. It is found that most of the aerosols are charged in the upper troposphere for altitudes below 10 km and in the stratosphere for altitudes above 20 km. On the contrary, the aerosols seem to be uncharged between 10 km and 20 km. Model calculations are used to quantify the electrification of the aerosols with a stratospheric aerosol-ion model. The percentages of charged aerosols obtained with model calculations are in excellent agreement with the observations below 10 km and above 20 km. On the other hand, the model cannot reproduce the absence of detected electrification in the lower stratosphere, such that a distinct unknown process in this altitude range inhibits electrification. The presence of sporadic transient layers of electrified aerosol in the upper troposphere and in the stratosphere could have significant implications for sprite formation.


2020 ◽  
Vol 20 (4) ◽  
pp. 2221-2261 ◽  
Author(s):  
Olexandr Lednyts'kyy ◽  
Christian von Savigny

Abstract. Electronically excited states of molecular and atomic oxygen (six O2 and two O) were implemented in the proposed Multiple Airglow Chemistry (MAC) model as minor species coupled with each other as well as with the ground states of O2 and O to represent the photochemistry in the upper mesosphere and lower thermosphere (MLT) region. The MAC model combines chemical processes of well-known photochemical models related to identified O2 and O species and some additional processes. Concentrations of excited O2 and O species were retrieved using the MAC model on the basis of the multiple nightglow emissions measured in situ during the Energy Transfer in the Oxygen Nightglow (ETON) rocket campaign. The proposed retrieval procedure to obtain the concentrations of these minor species in the MLT region is implemented by avoiding a priori data sets. Unknown and poorly constrained reaction rates were tuned, and the reaction rates of the well-known models were updated with the MAC model by comparing in situ and evaluated emission profiles as well as in situ and retrieved O concentration profiles. As a result, precursors of O2 and O species responsible for the transitions considered in the MAC model are identified and validated.


Author(s):  
Andrew C. Kren ◽  
Richard A. Anthes

AbstractThis study estimates the random error variances and standard deviations (STDs) for four data sets: Global Hawk (GH) dropsondes (DROP), the High-Altitude Monolithic Microwave Integrated Circuit Sounding Radiometer (HAMSR) aboard the GH, the European Centre for Medium-Range Weather Forecasts (ECMWF) ERA5 reanalysis, and the Hurricane Weather Research and Forecasting (HWRF) model, using the three-cornered hat (3CH) method. These estimates are made during the 2016 Sensing Hazards with Operational Unmanned Technology (SHOUT) season in the environment of four tropical cyclones from August to October. For temperature and specific and relative humidity, the ERA5, HWRF, and DROP data sets all have similar magnitudes of errors, with ERA5 having the smallest. The error STDs of temperature and specific humidity are less than 0.8 K and 1.0 g kg-1 over most of the troposphere, while relative humidity error STDs increase from less than 5% near the surface to between 10 and 20% in the upper troposphere. The HAMSR bias-corrected data have larger errors, with estimated error STDs of temperature and specific humidity in the lower troposphere between 1.5 and 2.0 K and 1.5 and 2.5 g kg-1. HAMSR’s relative humidity error STD increases from approximately 10% in the lower troposphere to 30% in the upper troposphere. The 3CH method error estimates are generally consistent with prior independent estimates of errors and uncertainties for the HAMSR and dropsonde data sets, although they are somewhat larger, likely due to the inclusion of representativeness errors (differences associated with different spatial and temporal scales represented by the data).


2005 ◽  
Vol 5 (11) ◽  
pp. 2901-2914 ◽  
Author(s):  
B. Barret ◽  
S. Turquety ◽  
D. Hurtmans ◽  
C. Clerbaux ◽  
J. Hadji-Lazaro ◽  
...  

Abstract. This paper presents the first global distributions of CO vertical profiles retrieved from a thermal infrared FTS working in the nadir geometry. It is based on the exploitation of the high resolution and high quality spectra measured by the Interferometric Monitor of Greenhouse gases (IMG) which flew onboard the Japanese ADEOS platform in 1996-1997. The retrievals are performed with an algorithm based on the Optimal Estimation Method (OEM) and are characterized in terms of vertical sensitivity and error budget. It is found that most of the IMG measurements contain between 1.5 and 2.2 independent pieces of information about the vertical distribution of CO from the lower troposphere to the upper troposphere-lower stratosphere (UTLS). The retrievals are validated against coincident NOAA/CMDL in situ surface measurements and NDSC/FTIR total columns measurements. The retrieved global distributions of CO are also found to be in good agreement with the distributions modeled by the GEOS-CHEM 3D CTM, highlighting the ability of IMG to capture the horizontal as well as the vertical structure of the CO distributions.


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