scholarly journals Effect of sea breeze circulation on aerosol mixing state and radiative properties in a desert setting

2017 ◽  
Vol 17 (18) ◽  
pp. 11331-11353 ◽  
Author(s):  
Yevgeny Derimian ◽  
Marie Choël ◽  
Yinon Rudich ◽  
Karine Deboudt ◽  
Oleg Dubovik ◽  
...  
Keyword(s):  
Sea Breeze ◽  
Chemical Imaging ◽  
Radiative Properties ◽  
Negev Desert ◽  
Dust Particles ◽  
Hygroscopic Growth ◽  
Inversion Algorithm ◽  
Sensing Applications ◽  
Homogeneity Assumption ◽  
Hygroscopic Particles

Abstract. Chemical composition, microphysical, and optical properties of atmospheric aerosol deep inland in the Negev Desert of Israel are found to be influenced by daily occurrences of sea breeze flow from the Mediterranean Sea. Abrupt increases in aerosol volume concentration and shifts of size distributions towards larger sizes, which are associated with increase in wind speed and atmospheric water content, were systematically recorded during the summertime at a distance of at least 80 km from the coast. Chemical imaging of aerosol samples showed an increased contribution of highly hygroscopic particles during the intrusion of the sea breeze. Besides a significant fraction of marine aerosols, the amount of internally mixed marine and mineral dust particles was also increased during the sea breeze period. The number fraction of marine and internally mixed particles during the sea breeze reached up to 88 % in the PM1–2. 5 and up to 62 % in the PM2. 5–10 size range. Additionally, numerous particles with residuals of liquid coating were observed by SEM/EDX analysis. Ca-rich dust particles that had reacted with anthropogenic nitrates were evidenced by Raman microspectroscopy. The resulting hygroscopic particles can deliquesce at very low relative humidity. Our observations suggest that aerosol hygroscopic growth in the Negev Desert is induced by the daily sea breeze arrival. The varying aerosol microphysical and optical characteristics perturb the solar and thermal infrared radiations. The changes in aerosol properties induced by the sea breeze, relative to the background situation, doubled the shortwave radiative cooling at the surface (from −10 to −20.5 W m−2) and increased by almost 3 times the warming of the atmosphere (from 5 to 14 W m−2), as evaluated for a case study. Given the important value of observed liquid coating of particles, we also examined the possible influence of the particle homogeneity assumption on the retrieval of aerosol microphysical characteristics. The tests suggest that sensitivity to the coating appears if backward scattering and polarimetric measurements are available for the inversion algorithm. This may have an important implication for retrievals of aerosol microphysical properties in remote sensing applications.

scholarly journals Effect of sea breeze circulation on aerosol mixing state and radiative properties in a desert setting

2017 ◽  
Author(s):  
Yevgeny Derimian ◽  
Marie Choël ◽  
Yinon Rudich ◽  
Karine Deboudt ◽  
Oleg Dubovik ◽  
...  
Keyword(s):  
Sea Breeze ◽  
Chemical Imaging ◽  
Radiative Properties ◽  
Negev Desert ◽  
Dust Particles ◽  
Hygroscopic Growth ◽  
Inversion Algorithm ◽  
Sensing Applications ◽  
Homogeneity Assumption ◽  
Hygroscopic Particles

Abstract. Chemical composition, microphysical and optical properties of atmospheric aerosol deep inland in the Negev Desert of Israel were found be influenced by daily occurrences of sea breeze flow from the Mediterranean Sea. Abrupt increases in aerosol volume concentration and shifts of size distributions towards larger sizes, which are associated with increase in wind speed and atmospheric water content, were systematically recorded during the summertime at a distance of at least 80 km from the coast. Chemical imaging of aerosol samples confirmed an increased contribution of highly hygroscopic particles during the intrusion of the sea breeze. Besides a significant fraction of marine aerosols, the amount of internally mixed marine and mineral dust particles was also increased during the sea breeze period. The number fraction of marine and internally mixed particles during the sea breeze reached up to 88 % in the PM1-2.5 and up to 62 % in the PM2.5-10 size range. Additionally, numerous particles with residuals of liquid coating were observed by SEM/EDX analysis. Ca-rich dust particles that had reacted with anthropogenic nitrates were evidenced by Raman microspectroscopy. The resulting hygroscopic particles can deliquesce at very low relative humidity. Our observations suggest that aerosol hygroscopic growth in the Negev Desert is triggered by the daily sea breeze arrival. The varying aerosol microphysical and optical characteristics perturb the solar and thermal infrared radiation. The changes in aerosol properties induced by the sea breeze, relative to the background situation, doubled the shortwave radiative cooling at the surface (from −10 to −20.5 Wm−2) and increased by almost three times the warming of the atmosphere (from 5 to 14 Wm−2), as evaluated for a case study. Given the important value of observed liquid coating of particles, we also examined the possible influence of the particle homogeneity assumption on the retrieval of aerosol microphysical characteristics. The tests suggest that sensitivity to the coating appears if backward scattering and polarimetric measurements are available for the inversion algorithm. This may have an important implication for retrievals of aerosol microphysical properties in remote sensing applications.

Efficient control of dye molecules fluorescence in polydopamine via strong optical coupling in a SPASER nanoparticle

2021 ◽  
Author(s):  
Pavel Melentiev ◽  
Boris Khlebtsov ◽  
Anton Gritchenko ◽  
Denis Kudryavtsev ◽  
Igor Ivanov ◽  
...  
Keyword(s):  
Viral Particle ◽  
Direct Detection ◽  
Fluorescence Emission ◽  
Radiative Properties ◽  
Environment Interaction ◽  
Optical Coupling ◽  
Dye Molecules ◽  
Sensing Applications ◽  
Fluorescence Measurements ◽  
Optical Modes

Abstract One of the main approaches of design and manipulation of the quantum emitters’ radiative properties is based on proper control of optical modes of the surrounding quantum emitter environment, leading to, in its ultimate case, to a strong regime of the emitter - environment interaction. In this Letter, we present the realization of a mesoscopic physical system (Au SPASER nanoparticle with polydopamine shell containing dye molecules Cy 7.5) in which the strong optical coupling regime allows: (i) to get rid of dye molecules quenching, (ii) to suppress photobleaching of dye molecules and (iii) to get a great enhancement of dye molecules fluorescence. We have reduced the rate of fluorescence quenching of dye molecules in PDA by 1000 times and increased the fluorescence emission rate of dye molecules by 30 time, thus preparing bright, nanoscale and biocompatible fluorescent probes suitable for bio-sensing applications. As an example of practical use of the probe, we demonstrate direct detection of single SARS-CoV-2 viral particle via fluorescence measurements of the probes attached to the viral particle through the antibodies.

scholarly journals Chemical aging of atmospheric mineral dust during transatlantic transport

2016 ◽  
Author(s):  
Mohamed Abdelkader ◽  
Swen Metzger ◽  
Benedikt Steil ◽  
Klaus Klingmüller ◽  
Holger Tost ◽  
...  
Keyword(s):  
Atlantic Ocean ◽  
Direct Effect ◽  
Dust Particles ◽  
Hygroscopic Growth ◽  
Aging Effects ◽  
Particle Sedimentation ◽  
Inter Tropical Convergence Zone ◽  
Dust Transport ◽  
Dust Fraction ◽  
The Impact

Abstract. Transatlantic dust transport has many implications for the atmosphere, ocean and climate. We present a modeling study on the impact of the key processes (dust emissions flux, convection and dust aging parameterizations) that control the transatlantic dust transport. Typically, the Inter-Tropical Convergence Zone (ITCZ) acts as a barrier for the meridional dust transport. To characterize the dust outflow over the Atlantic Ocean, we address two regional phenomena: (i) dust interactions with the ITCZ (DIZ) and (ii) the adjacent dust transport over the Atlantic Ocean (DTA). In the DTA zone, the dust loading shows a steep and linear gradient westward over the Atlantic Ocean where particle sedimentation is the dominant removal process, whereas in the DIZ zone cloud interactions and wet deposition predominate. To study the different impacts of aging, we present two case studies that exclude condensation and coagulation, and include dust aging at various levels of complexity. For dust aging, we consider the uptake of inorganic acids on the surface of mineral particles that form salt compounds. Calcium, used as a proxy for the overall chemically reactive dust fraction, drives the dust-related neutralization reactions leading to higher dust aerosol optical depth (AOD). The aged dust particles are transferred to the soluble aerosol modes in the model and are mixed with other species that originate from anthropogenic and natural sources. The neutralization products (salts) take up water vapor from the atmosphere and increase the dust AOD under subsaturated conditions. We define the "direct effect of dust aging" to refer to the increase in AOD as a result of hygroscopic growth. On the other hand, the aged dust is more efficiently removed (wet and dry) because of the increase in particle size and hygroscopicity. This more efficient removal reduces the dust AOD over the DIZ zone. We define this as the "indirect effect of dust aging", complementary to the direct effect that is dominant in the DTA zone. Distinction of the two aging effects helps develop insight into the regional importance of dust–air-pollution interactions.

scholarly journals Observational evidence of particle hygroscopic growth in the upper troposphere–lower stratosphere (UTLS) over the Tibetan Plateau

2019 ◽  
Vol 19 (13) ◽  
pp. 8399-8406 ◽  
Author(s):  
Qianshan He ◽  
Jianzhong Ma ◽  
Xiangdong Zheng ◽  
Xiaolu Yan ◽  
Holger Vömel ◽  
...  
Keyword(s):  
Relative Humidity ◽  
Tibetan Plateau ◽  
Lower Stratosphere ◽  
Fine Particles ◽  
Asian Summer Monsoon ◽  
Radiative Properties ◽  
Aerosol Layer ◽  
The Tibetan Plateau ◽  
Hygroscopic Growth ◽  
Upper Troposphere

Abstract. We measured the vertical profiles of backscatter ratio (BSR) using the balloon-borne, lightweight Compact Optical Backscatter AerosoL Detector (COBALD) instruments above Linzhi, located in the southeastern Tibetan Plateau, in the summer of 2014. An enhanced aerosol layer in the upper troposphere–lower stratosphere (UTLS), with BSR (455 nm) > 1.1 and BSR (940 nm) > 1.4, was observed. The color index (CI) of the enhanced aerosol layer, defined as the ratio of aerosol backscatter ratios (ABSRs) at wavelengths of 940 and 455 nm, varied from 4 to 8, indicating the prevalence of fine particles with a mode radius of less than 0.1 µm. We find that unlike the very small particles (mode radius smaller than 0.04 µm) at low relative humidity (RHi < 40 %), the relatively large particles in the aerosol layer were generally very hydrophilic as their size increased dramatically with relative humidity. This result indicates that water vapor can play a very important role in increasing the size of fine particles in the UTLS over the Tibetan Plateau. Our observations provide observation-based evidence supporting the idea that aerosol particle hygroscopic growth is an important factor influencing the radiative properties of the Asian Tropopause Aerosol Layer (ATAL) during the Asian summer monsoon.

scholarly journals Hygroscopicity of Different Types of Aerosol Particles: Case Studies Using Multi-Instrument Data in Megacity Beijing, China

2020 ◽  
Vol 12 (5) ◽  
pp. 785 ◽  
Author(s):  
Tong Wu ◽  
Zhanqing Li ◽  
Jun Chen ◽  
Yuying Wang ◽  
Hao Wu ◽  
...  
Keyword(s):  
Enhancement Factor ◽  
Mineral Dust ◽  
Aerosol Particles ◽  
Dust Aerosol ◽  
Dust Particles ◽  
Chemical Components ◽  
Hygroscopic Growth ◽  
Microphysical Properties ◽  
Fine Mode ◽  
Fine Mode Aerosol

Water uptake by aerosol particles alters its light-scattering characteristics significantly. However, the hygroscopicities of different aerosol particles are not the same due to their different chemical and physical properties. Such differences are explored by making use of extensive measurements concerning aerosol optical and microphysical properties made during a field experiment from December 2018 to March 2019 in Beijing. The aerosol hygroscopic growth was captured by the aerosol optical characteristics obtained from micropulse lidar, aerosol chemical composition, and aerosol particle size distribution information from ground monitoring, together with conventional meteorological measurements. Aerosol hygroscopicity behaves rather distinctly for mineral dust coarse-mode aerosol (Case I) and non-dust fine-mode aerosol (Case II) in terms of the hygroscopic enhancement factor, f β ( R H , λ 532 ) , calculated for the same humidity range. The two types of aerosols were identified by applying the polarization lidar photometer networking method (POLIPHON). The hygroscopicity for non-dust aerosol was much higher than that for dust conditions with the f β ( R H , λ 532 ) being around 1.4 and 3.1, respectively, at the relative humidity of 86% for the two cases identified in this study. To study the effect of dust particles on the hygroscopicity of the overall atmospheric aerosol, the two types of aerosols were identified and separated by applying the polarization lidar photometer networking method in Case I. The hygroscopic enhancement factor of separated non-dust fine-mode particles in Case I had been significantly strengthened, getting closer to that of the total aerosol in Case II. These results were verified by the hygroscopicity parameter, κ (Case I non-dust particles: 0.357 ± 0.024; Case II total: 0.344 ± 0.026), based on the chemical components obtained by an aerosol chemical speciation instrument, both of which showed strong hygroscopicity. It was found that non-dust fine-mode aerosol contributes more during hygroscopic growth and that non-hygroscopic mineral dust aerosol may reduce the total hygroscopicity per unit volume in Beijing.

scholarly journals Heterogeneous ice nucleation on dust particles sourced from nine deserts worldwide – Part 2: Deposition nucleation and condensation freezing

2019 ◽  
Vol 19 (2) ◽  
pp. 1059-1076 ◽  
Author(s):  
Yvonne Boose ◽  
Philipp Baloh ◽  
Michael Plötze ◽  
Johannes Ofner ◽  
Hinrich Grothe ◽  
...  
Keyword(s):  
Active Sites ◽  
Mineral Dust ◽  
Atmospheric Transport ◽  
Chemical Imaging ◽  
Ice Nucleation ◽  
Dust Particles ◽  
Full Potential ◽  
Nucleation Behavior ◽  
Crystal Water ◽  
Desert Dust

Abstract. Mineral dust particles from deserts are amongst the most common ice nucleating particles in the atmosphere. The mineralogy of desert dust differs depending on the source region and can further fractionate during the dust emission processes. Mineralogy to a large extent explains the ice nucleation behavior of desert aerosol, but not entirely. Apart from pure mineral dust, desert aerosol particles often exhibit a coating or are mixed with small amounts of biological material. Aging on the ground or during atmospheric transport can deactivate nucleation sites, thus strong ice nucleating minerals may not exhibit their full potential. In the partner paper of this work, it was shown that mineralogy determines most but not all of the ice nucleation behavior in the immersion mode found for desert dust. In this study, the influence of semi-volatile organic compounds and the presence of crystal water on the ice nucleation behavior of desert aerosol is investigated. This work focuses on the deposition and condensation ice nucleation modes at temperatures between 238 and 242 K of 18 dust samples sourced from nine deserts worldwide. Chemical imaging of the particles' surface is used to determine the cause of the observed differences in ice nucleation. It is found that, while the ice nucleation ability of the majority of the dust samples is dominated by their quartz and feldspar content, in one carbonaceous sample it is mostly caused by organic matter, potentially cellulose and/or proteins. In contrast, the ice nucleation ability of an airborne Saharan sample is found to be diminished, likely by semi-volatile species covering ice nucleation active sites of the minerals. This study shows that in addition to mineralogy, other factors such as organics and crystal water content can alter the ice nucleation behavior of desert aerosol during atmospheric transport in various ways.

scholarly journals The spatial distribution of mineral dust and its shortwave radiative forcing over North Africa: modeling sensitivities to dust emissions and aerosol size treatments

2010 ◽  
Vol 10 (18) ◽  
pp. 8821-8838 ◽  
Author(s):  
C. Zhao ◽  
X. Liu ◽  
L. R. Leung ◽  
B. Johnson ◽  
S. A. McFarlane ◽  
...  
Keyword(s):  
North Africa ◽  
Radiative Forcing ◽  
Mineral Dust ◽  
Regional Climate ◽  
Dust Emission ◽  
Radiative Properties ◽  
Lower Atmosphere ◽  
Dust Particles ◽  
Dust Emissions ◽  
Sahel Region

Abstract. A fully coupled meteorology-chemistry-aerosol model (WRF-Chem) is applied to simulate mineral dust and its shortwave (SW) radiative forcing over North Africa. Two dust emission schemes (GOCART and DUSTRAN) and two aerosol models (MADE/SORGAM and MOSAIC) are adopted in simulations to investigate the modeling sensitivities to dust emissions and aerosol size treatments. The modeled size distribution and spatial variability of mineral dust and its radiative properties are evaluated using measurements (ground-based, aircraft, and satellites) during the AMMA SOP0 campaign from 6 January to 3 February of 2006 (the SOP0 period) over North Africa. Two dust emission schemes generally simulate similar spatial distributions and temporal evolutions of dust emissions. Simulations using the GOCART scheme with different initial (emitted) dust size distributions require ~40% difference in total emitted dust mass to produce similar SW radiative forcing of dust over the Sahel region. The modal approach of MADE/SORGAM retains 25% more fine dust particles (radius<1.25 μm) but 8% less coarse dust particles (radius>1.25 μm) than the sectional approach of MOSAIC in simulations using the same size-resolved dust emissions. Consequently, MADE/SORGAM simulates 11% higher AOD, up to 13% lower SW dust heating rate, and 15% larger (more negative) SW dust radiative forcing at the surface than MOSAIC over the Sahel region. In the daytime of the SOP0 period, the model simulations show that the mineral dust heats the lower atmosphere with an average rate of 0.8 ± 0.5 K day−1 over the Niamey vicinity and 0.5 ± 0.2 K day−1 over North Africa and reduces the downwelling SW radiation at the surface by up to 58 W m−2 with an average of 22 W m−2 over North Africa. This highlights the importance of including dust radiative impact in understanding the regional climate of North Africa. When compared to the available measurements, the WRF-Chem simulations can generally capture the measured features of mineral dust and its radiative properties over North Africa, suggesting that the model is suitable for more extensive simulations of dust impact on regional climate over North Africa.

The SANDEE campaign: Electrical effects during sand transport by aeolian processes in the Negev desert and implications for Mars

2020 ◽  
Author(s):  
Itzhak Katra ◽  
Yoav Yair
Keyword(s):  
Wind Tunnel ◽  
Electric Field ◽  
Field Experiments ◽  
Negev Desert ◽  
Energy Output ◽  
Dust Particles ◽  
Sand Transport ◽  
Solar Panels ◽  
Aeolian Processes ◽  
Airborne Dust

&lt;p&gt;The electrification of mineral sand/dust particles during aeolian processes is a well-documented phenomenon both in natural settings and in laboratory experiments. When in motion, small airborne dust particles collide with other suspended particles or impact the surface through the kinetic energy they acquire from the ambient wind. Field experiments will be conducted in conjunction with the AMEDEE-2020 Analog Mars Mission, planned for November 2020 in the Ramon Crater in southern Israel and led by the Austrian Space Forum. During SANDEE, we will deploy a portable wind-tunnel (Katra et al., 2016) at the site, and record particle movements in conditions that simulate sand storms of varying speeds. We will use local Negev desert, as well as Mars-simulant, soil samples that will be placed inside the wind-tunnel. We will measure particles' dynamic, mineralogical and electrical characteristics as they are blown by wind inside the tunnel. &amp;#160;A JCI 114 portable electric field detector will be used to to measure the amplification of the ambient electric field during sand movement. A vertical array of traps oriented along the wind direction will be used for sampling particles, in order to calculate the related sand fluxes and to analyze particle characteristics. The experiment will be repeated at night under dark conditions, in order to observe if light is emitted from electrified dust, due to corona discharges.&lt;/p&gt;&lt;p&gt;We expect that SANDEE will help decipher wind-speed/aerosol/electrical charge relationships. These have practical implications for future Mars landers, because airborne sand particles are likely to interfere with communications and also to impede the energy output of solar panels due to the electrical adhesion of charged aerosol.&lt;/p&gt;

scholarly journals Effects of relative humidity on aerosol light scattering in the Arctic

2010 ◽  
Vol 10 (8) ◽  
pp. 3875-3890 ◽  
Author(s):  
P. Zieger ◽  
R. Fierz-Schmidhauser ◽  
M. Gysel ◽  
J. Ström ◽  
S. Henne ◽  
...  
Keyword(s):  
Standard Deviation ◽  
Light Scattering ◽  
Relative Humidity ◽  
Aerosol Particles ◽  
Aerosol Size Distribution ◽  
Hygroscopic Growth ◽  
Scattering Coefficients ◽  
Dry Conditions ◽  
Hygroscopic Particles

Abstract. Aerosol particles experience hygroscopic growth in the ambient atmosphere. Their optical properties – especially the aerosol light scattering – are therefore strongly dependent on the ambient relative humidity (RH). In-situ light scattering measurements of long-term observations are usually performed under dry conditions (RH>30–40%). The knowledge of this RH effect is of eminent importance for climate forcing calculations or for the comparison of remote sensing with in-situ measurements. This study combines measurements and model calculations to describe the RH effect on aerosol light scattering for the first time for aerosol particles present in summer and fall in the high Arctic. For this purpose, a field campaign was carried out from July to October 2008 at the Zeppelin station in Ny-Ålesund, Svalbard. The aerosol light scattering coefficient σsp(λ) was measured at three distinct wavelengths (λ=450, 550, and 700 nm) at dry and at various, predefined RH conditions between 20% and 95% with a recently developed humidified nephelometer (WetNeph) and with a second nephelometer measuring at dry conditions with an average RH<10% (DryNeph). In addition, the aerosol size distribution and the aerosol absorption coefficient were measured. The scattering enhancement factor f(RH, λ) is the key parameter to describe the RH effect on σsp(λ) and is defined as the RH dependent σsp(RH, λ) divided by the corresponding dry σsp(RHdry, λ). During our campaign the average f(RH=85%, λ=550 nm) was 3.24±0.63 (mean ± standard deviation), and no clear wavelength dependence of f(RH, λ) was observed. This means that the ambient scattering coefficients at RH=85% were on average about three times higher than the dry measured in-situ scattering coefficients. The RH dependency of the recorded f(RH, λ) can be well described by an empirical one-parameter equation. We used a simplified method to retrieve an apparent hygroscopic growth factor g(RH), defined as the aerosol particle diameter at a certain RH divided by the dry diameter, using the WetNeph, the DryNeph, the aerosol size distribution measurements and Mie theory. With this approach we found, on average, g(RH=85%) values to be 1.61±0.12 (mean±standard deviation). No clear seasonal shift of f(RH, λ) was observed during the 3-month period, while aerosol properties (size and chemical composition) clearly changed with time. While the beginning of the campaign was mainly characterized by smaller and less hygroscopic particles, the end was dominated by larger and more hygroscopic particles. This suggests that compensating effects of hygroscopicity and size determined the temporal stability of f(RH, λ). During sea salt influenced periods, distinct deliquescence transitions were observed. At the end we present a method on how to transfer the dry in-situ measured aerosol scattering coefficients to ambient values for the aerosol measured during summer and fall at this location.

Comprehensive Study of Optical, Physical, Chemical, and Radiative Properties of Total Columnar Atmospheric Aerosols over China: An Overview of Sun–Sky Radiometer Observation Network (SONET) Measurements

2018 ◽  
Vol 99 (4) ◽  
pp. 739-755 ◽  
Author(s):  
Z. Q. Li ◽  
H. Xu ◽  
K. T. Li ◽  
D. H. Li ◽  
Y. S. Xie ◽  
...  
Keyword(s):  
Aerosol Optical Depth ◽  
Optical Depth ◽  
Atmospheric Aerosol ◽  
Radiative Properties ◽  
Dust Particles ◽  
Aerosol Composition ◽  
Strong Light ◽  
Observation Network ◽  
Fine Mode ◽  
Cooling Effects

AbstractAn overview of Sun–Sky Radiometer Observation Network (SONET) measurements in China is presented. Based on observations at 16 distributed SONET sites in China, atmospheric aerosol parameters are acquired via standardization processes of operational measurement, maintenance, calibration, inversion, and quality control implemented since 2010. A climatology study is performed focusing on total columnar atmospheric aerosol characteristics, including optical (aerosol optical depth, ÅngstrÖm exponent, fine-mode fraction, single-scattering albedo), physical (volume particle size distribution), chemical composition (black carbon; brown carbon; fine-mode scattering component, coarse-mode component; and aerosol water), and radiative properties (aerosol radiative forcing and efficiency). Data analyses show that aerosol optical depth is low in the west but high in the east of China. Aerosol composition also shows significant spatial and temporal variations, leading to noticeable diversities in optical and physical property patterns. In west and north China, aerosols are generally affected by dust particles, while monsoon climate and human activities impose remarkable influences on aerosols in east and south China. Aerosols in China exhibit strong light-scattering capability and result in significant radiative cooling effects.

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