scholarly journals Significant climate impacts of aerosol changes driven by growth in energy use and advances in emissions control technology

Author(s):  
Alcide Zhao ◽  
Massimo A. Bollasina ◽  
Monica Crippa ◽  
David S. Stevenson

Abstract. Anthropogenic aerosols have increased significantly since the industrial revolution, driven largely by growth in emissions from energy use in sectors including power generation, industry, and transport. Advances in emission control technologies since around 1970, however, have partially counteracted emissions increases from the above sectors. Using the fully-coupled Community Earth System Model, we quantify the effective radiative forcing (ERF) and climate response to 1970–2010 aerosol emission changes associated with the above two policy-relevant emission drivers. Emissions from energy use growth generate a global mean aerosol ERF of −0.31 W m−2, and result in a global mean cooling of −0.35 K and a precipitation reduction of −0.03 mm day−1. By contrast, the avoided emissions from advances in emission control technology, which benefit air quality, generate a global mean ERF of +0.21 W m−2, a global warming of +0.10 K and global mean precipitation increase of +0.01 mm day−1. The total net aerosol impacts on climate are dominated by energy use growth, from Asia in particular. However, technology advances outweigh energy use growth over Europe and North America. Also, the Arctic climate is significantly affected by aerosol emission changes from Europe, North America, and Asia. Various non-linear processes are involved along the pathway from aerosol emissions to radiative forcing and ultimately to climate responses, suggesting that the diagnosed aerosol forcing and effects must be interpreted in the context of experiment designs. Further, the temperature response per unit aerosol ERF varies significantly across many factors, including location and magnitude of emission changes, implying that ERF, and the related metrics, need to be used very carefully for aerosols. Future aerosol emission pathways have large temporal and spatial uncertainties; our findings provide useful information for both assessing and interpreting such uncertainties, and may help inform future climate change impact reduction strategies.

2019 ◽  
Vol 19 (23) ◽  
pp. 14517-14533 ◽  
Author(s):  
Alcide Zhao ◽  
Massimo A. Bollasina ◽  
Monica Crippa ◽  
David S. Stevenson

Abstract. Anthropogenic aerosols have increased significantly since the industrial revolution, driven largely by growth in emissions from energy use in sectors including power generation, industry, and transport. Advances in emission control technologies since around 1970, however, have partially counteracted emissions increases from the above sectors. Using the fully coupled Community Earth System Model, we quantify the effective radiative forcing (ERF) and climate response to 1970–2010 aerosol changes associated with the above two policy-relevant emission drivers. Emissions from energy-use growth generate a global mean aerosol ERF (mean ± 1 standard deviation) of -0.31±0.22 W m−2 and result in a global mean cooling (-0.35±0.17 K) and a precipitation reduction (-0.03±0.02 mm d−1). By contrast, the avoided emissions from advances in emission control technology, which benefit air quality, generate a global mean ERF of +0.21±0.23 W m−2, a global warming of +0.10±0.13 K, and global mean precipitation increase of +0.01±0.02 mm d−1. Despite the relatively small changes in global mean precipitation, these two emission drivers have profound impacts at regional scales, in particular over Asia and Europe. The total net aerosol impacts on climate are dominated by energy-use growth, from Asia in particular. However, technology advances outweigh energy-use growth over Europe and North America. Various non-linear processes are involved along the pathway from aerosol and their precursor emissions to radiative forcing and ultimately to climate responses, suggesting that the diagnosed aerosol forcing and effects must be interpreted in the context of experiment designs. Further, the temperature response per unit aerosol ERF varies significantly across many factors, including location and magnitude of emission changes, implying that ERF, and the related metrics, needs to be used very carefully for aerosols. Future aerosol-related emission pathways have large temporal and spatial uncertainties; our findings provide useful information for both assessing and interpreting such uncertainties, and they may help inform future climate change impact reduction strategies.


2007 ◽  
Vol 20 (5) ◽  
pp. 843-855 ◽  
Author(s):  
J. A. Kettleborough ◽  
B. B. B. Booth ◽  
P. A. Stott ◽  
M. R. Allen

Abstract A method for estimating uncertainty in future climate change is discussed in detail and applied to predictions of global mean temperature change. The method uses optimal fingerprinting to make estimates of uncertainty in model simulations of twentieth-century warming. These estimates are then projected forward in time using a linear, compact relationship between twentieth-century warming and twenty-first-century warming. This relationship is established from a large ensemble of energy balance models. By varying the energy balance model parameters an estimate is made of the error associated with using the linear relationship in forecasts of twentieth-century global mean temperature. Including this error has very little impact on the forecasts. There is a 50% chance that the global mean temperature change between 1995 and 2035 will be greater than 1.5 K for the Special Report on Emissions Scenarios (SRES) A1FI scenario. Under SRES B2 the same threshold is not exceeded until 2055. These results should be relatively robust to model developments for a given radiative forcing history.


2016 ◽  
Author(s):  
Marianne T. Lund ◽  
Terje K. Berntsen ◽  
Bjørn H. Samset

Abstract. Despite recent improvements, significant uncertainties in global modeling of black carbon (BC) aerosols persist, posing important challenges for the design and evaluation of effective climate mitigation strategies targeted at BC emission reductions. Here we investigate the sensitivity of BC concentrations in the chemistry-transport model OsloCTM2 with the microphysical aerosol parameterization M7 (OsloCTM2-M7) to parameters controlling aerosol aging and scavenging. We focus on Arctic surface concentrations and remote region BC vertical profiles, and introduce a novel treatment of condensation of nitric acid on BC. The OsloCTM2-M7 underestimates annual averaged BC surface concentrations, with a mean normalized bias of −0.55. The seasonal cycle and magnitude of Arctic BC surface concentrations is improved compared to previous OsloCTM2 studies, but model-measurement discrepancies during spring remain. High-altitude BC over the Pacific is overestimated compared with measurements from the HIPPO campaigns. We find that a shorter global BC lifetime improves the agreement with HIPPO, in line with other recent studies. Several processes can achieve this, including allowing for convective scavenging of hydrophobic BC and reducing the amount of soluble material required for aging. Simultaneously, the concentrations in the Arctic are reduced, resulting in poorer agreement with measurements in part of the region. A first step towards inclusion of aging by nitrate in OsloCTM2-M7 is made by allowing for condensation of nitric acid on BC. This results in a faster aging and reduced lifetime, and in turn to a better agreement with the HIPPO measurements. On the other hand, model-measurement discrepancies in the Arctic are exacerbated. Work to further improve this parameterization is needed. The impact on global mean radiative forcing (RF) and surface temperature response (TS) in our experiments is estimated. Compared to the baseline, decreases in global mean direct RF on the order of 10–30 % of the total pre-industrial to present BC direct RF is estimated for the experiments that result in the largest changes in BC concentrations. We show that globally tuning parameters related to BC aging and scavenging can improve the representation of BC vertical profiles in the OsloCTM2-M7 compared with observations. Our results also show that such improvements can result from changes in several processes and often depend on assumptions about uncertain parameters such as the BC ice nucleating efficiency and the change in hygroscopicity with aging. It is also important to be aware of potential tradeoffs in model performance between different regions. Other important sources of uncertainty, particularly for Arctic BC, such as model resolution has not been investigated here. Our results underline the importance of more observations and experimental data to improve process understanding and thus further constrain models.


2011 ◽  
Vol 11 (14) ◽  
pp. 6809-6836 ◽  
Author(s):  
R. B. Skeie ◽  
T. Berntsen ◽  
G. Myhre ◽  
C. A. Pedersen ◽  
J. Ström ◽  
...  

Abstract. The distribution of black carbon (BC) in the atmosphere and the deposition of BC on snow surfaces since pre-industrial time until present are modelled with the Oslo CTM2 model. The model results are compared with observations including recent measurements of BC in snow in the Arctic. The global mean burden of BC from fossil fuel and biofuel sources increased during two periods. The first period, until 1920, is related to increases in emissions in North America and Europe, and the last period after 1970 are related mainly to increasing emissions in East Asia. Although the global burden of BC from fossil fuel and biofuel increases, in the Arctic the maximum atmospheric BC burden as well as in the snow was reached in 1960s, with a slight reduction thereafter. The global mean burden of BC from open biomass burning sources has not changed significantly since 1900. With current inventories of emissions from open biomass sources, the modelled burden of BC in snow and in the atmosphere north of 65° N is small compared to the BC burden of fossil fuel and biofuel origin. From the concentration changes radiative forcing time series due to the direct aerosol effect as well as the snow-albedo effect is calculated for BC from fossil fuel and biofuel. The calculated radiative forcing in 2000 for the direct aerosol effect is 0.35 W m−2 and for the snow-albedo effect 0.016 W m−2 in this study. Due to a southward shift in the emissions there is an increase in the lifetime of BC as well as an increase in normalized radiative forcing, giving a change in forcing per unit of emissions of 26 % since 1950.


2020 ◽  
Author(s):  
Srinath Krishnan ◽  
Annica Ekman ◽  
Hans-Christen Hansson ◽  
Ilona Riipinen

<p><span>Modeling studies have shown that changes in sulphate aerosol emissions from both Europe and North America can have an impact on remote Arctic climate. The bulk of this response is driven by atmospheric changes, rather than through changes in meridional ocean heat transport. However, these simulations have focused on the Arctic response from an equilibrium perspective; i.e. the simulations are run for 200 years and the analyses are based on means of the last 50 years. While these simulations are useful to analyze the extent of contribution of mid-latitude aerosol emission changes, they cannot be used to investigate the mechanistic processes that initiate and drive the high-latitude response. We approach this problem by conducting two sets of initial condition ensemble simulations with >30 members for each set and focus our analysis on the first 30 years. Having a large number of ensemble members improves the signal-noise ratio and allows us to distinguish the model response to emission changes from internal variability. In the first set of simulations (control set), the aerosol emissions are set to year 2000. In the second set of simulations (perturbed set), we increase the European sulphate aerosol emissions to seven times the year 2000 value. We compare the two sets of simulations to evaluate the dynamical response of the atmosphere to the change in aerosol emissions. One of the key parameters that link the mid- and high-latitudes in the equilibrium response is the change in sea-ice area in the sub-polar latitudes. Reduced sea-ice coverage and greater open ocean area with lower mid-latitude aerosol emissions leads to increased ocean-atmosphere energy exchange and impacts the atmospheric meridional heat and energy budgets in the Arctic. We present the extent and seasonality of sea-ice changes for the first 30 years of our ensemble simulations and discuss their implications in the context of the mechanistical links between the mid- and high-latitudes.</span></p><p> </p>


2011 ◽  
Vol 11 (3) ◽  
pp. 7469-7534 ◽  
Author(s):  
R. B. Skeie ◽  
T. Berntsen ◽  
G. Myhre ◽  
C. A. Pedersen ◽  
J. Ström ◽  
...  

Abstract. The distribution of black carbon (BC) in the atmosphere and the deposition of BC on snow surfaces since pre-industrial time until present are modelled with the Oslo CTM2 model. The model results are compared with observations including recent measurements of BC in snow in the Arctic. The global mean burden of BC from fossil fuel and biofuel sources increased during two periods. The first period, until 1920, is related to increases in emissions in North America and Europe, and the last period after 1970 are related mainly to increasing emissions in East Asia. Although the global burden of BC from fossil fuel and biofuel increases, in the Arctic the maximum atmospheric BC burden as well as in the snow was reached in 1960s, with a slight reduction thereafter. The global mean burden of BC from open biomass burning sources has not changed significantly since 1900. With current inventories of emissions from open biomass sources, the modelled burden of BC in snow and in the atmosphere north of 65° N is small compared to the BC burden of fossil fuel and biofuel origin. From the concentration changes radiative forcing time series due to the direct aerosol effect as well as the snow-albedo effect is calculated for BC from fossil fuel and biofuel. The calculated radiative forcing in 2000 for the direct aerosol effect is 0.35 W m−2 and for the snow-albedo effect 0.016 W m−2. Due to a southward shift in the emissions there is an increase in the lifetime of BC as well as an increase in normalized radiative forcing, giving a change in forcing per unit of emissions of 26% since 1950.


2012 ◽  
Vol 12 (8) ◽  
pp. 21105-21210 ◽  
Author(s):  
D. T. Shindell ◽  
J.-F. Lamarque ◽  
M. Schulz ◽  
M. Flanner ◽  
C. Jiao ◽  
...  

Abstract. A primary goal of the Atmospheric Chemistry and Climate Model Intercomparison Project (ACCMIP) was to characterize the short-lived drivers of preindustrial to 2100 climate change in the current generation of climate models. Here we evaluate historical and future radiative forcing in the 10 ACCMIP models that included aerosols, 8 of which also participated in the Coupled Model Intercomparison Project phase 5 (CMIP5). The models generally reproduce present-day climatological total aerosol optical depth (AOD) relatively well. They have quite different contributions from various aerosol components to this total, however, and most appear to underestimate AOD over East Asia. The models generally capture 1980–2000 AOD trends fairly well, though they underpredict AOD increases over the Yellow/Eastern Sea. They appear to strongly underestimate absorbing AOD, especially in East Asia, South and Southeast Asia, South America and Southern Hemisphere Africa. We examined both the conventional direct radiative forcing at the tropopause (RF) and the forcing including rapid adjustments (adjusted forcing; AF, including direct and indirect effects). The models' calculated all aerosol all-sky 1850 to 2000 global mean annual average RF ranges from −0.06 to −0.49 W m−2, with a mean of −0.26 W m−2 and a median of −0.27 W m−2. Adjusting for missing aerosol components in some models brings the range to −0.12 to −0.62 W m−2, with a mean of −0.39 W m−2. Screening the models based on their ability to capture spatial patterns and magnitudes of AOD and AOD trends yields a quality-controlled mean of −0.42 W m−2 and range of −0.33 to −0.50 W m−2 (accounting for missing components). The CMIP5 subset of ACCMIP models spans −0.06 to −0.49 W m−2, suggesting some CMIP5 simulations likely have too little aerosol RF. A substantial, but not well quantified, contribution to historical aerosol RF may come from climate feedbacks (35 to −58 %). The mean aerosol AF during this period is −1.12 W m−2 (median value −1.16 W m−2, range −0.72 to −1.44 W m−2), indicating that adjustments to aerosols, which include cloud, water vapor and temperature, lead to stronger forcing than the aerosol direct RF. Both negative aerosol RF and AF are greatest over and near Europe, South and East Asia and North America during 1850 to 2000. AF, however, is positive over both polar regions, the Sahara, and the Karakoram. Annual average AF is stronger than 0.5 W m−2 over parts of the Arctic and more than 1.5 W m−2 during boreal summer. Examination of the regional pattern of RF and AF shows that the multi-model spread relative to the mean of AF is typically the same or smaller than that for RF over areas with substantial forcing. Historical aerosol RF peaks in nearly all models around 1980, declining thereafter. Aerosol RF declines greatly in most models over the 21st century and is only weakly sensitive to the particular Representative Concentration Pathway (RCP). One model, however, shows approximate stabilization at current RF levels under RCP 8.5, while two others show increasingly negative RF due to the influence of nitrate aerosols (which are not included in most models). Aerosol AF, in contrast, continues to become more negative during 1980 to 2000 despite the turnaround in RF. Total anthropogenic composition forcing (RF due to well-mixed greenhouse gases (WMGHGs) and ozone plus aerosol AF) shows substantial masking of greenhouse forcing by aerosols towards the end of the 20{th} century and in the early 21st century at the global scale. Regionally, net forcing is negative over most industrialized and biomass burning regions through 1980, but remains strongly negative only over East and Southeast Asia by 2000 and only over a very small part of Southeast Asia by 2030 (under RCP8.5). Net forcing is strongly positive by 1980 over the Sahara, Arabian peninsula, the Arctic, Southern Hemisphere South America, Australia and most of the oceans. Both the magnitude of and area covered by positive forcing expand steadily thereafter. There is no clear relationship between aerosol AF and climate sensitivity in the CMIP5 subset of ACCMIP models. There is a clear link between the strength of aerosol+ozone forcing and the global mean historical climate response to anthropogenic non-WMGHG forcing (ANWF). The models show ~20–35% greater climate sensitivity to ANWF than to WMGHG forcing, at least in part due to geographic differences in climate sensitivity. These lead to ~50% more warming in the Northern Hemisphere in response to increasing WMGHGs. This interhemispheric asymmetry is enhanced for ANWF by an additional 10–30%. At smaller spatial scales, response to ANWF and WMGHGs show distinct differences.


2018 ◽  
Author(s):  
Anna Lewinschal ◽  
Annica M. L. Ekman ◽  
Hans-Christen Hansson ◽  
Maria Sand ◽  
Terje K. Berntsen ◽  
...  

Abstract. Short-lived anthropogenic climate forcers, such as sulphate aerosols, affect both climate and air quality. Despite being short-lived, these forcers do not affect temperatures only locally; regions far away from the emission sources are also affected. Climate metrics are often used e.g. in a policy context to compare the climate impact of different anthropogenic forcing agents. These metrics typically relate a forcing change in a certain region with a temperature change in another region and thus often require a separate model to convert emission changes to radiative forcing changes. In this study, we used a coupled Earth System Model (NorESM) to calculate emission-to-temperature-response metrics for sulphur dioxide (SO2) emission changes in four different policy-relevant regions: Europe, North America, East Asia and South Asia. We first increased the SO2 emissions in each individual region by an amount giving approximately the same global average radiative forcing change (−0.45 W m−2). The global mean temperature change per unit sulphur emission compared to the control experiment was independent of emission region and equal to ∼ 0.006 K/TgSyr−1. On a regional scale, the Arctic showed the largest temperature response in all experiments. The second largest temperature change occurred in the region of the imposed emission increase, except when South Asian emissions were changed; in this experiment, the temperature response was approximately the same in South Asia and East Asia. We also examined the non-linearity of the temperature response by removing all anthropogenic SO2 emissions over Europe in one experiment. In this case, the temperature response (both global and regional) was twice of that in the corresponding experiment with a European emission increase. This nonlinearity in the temperature response is one of many uncertainties associated with the use of simplified climate metrics.


2017 ◽  
Vol 17 (4) ◽  
pp. 2709-2720 ◽  
Author(s):  
Gunnar Myhre ◽  
Wenche Aas ◽  
Ribu Cherian ◽  
William Collins ◽  
Greg Faluvegi ◽  
...  

Abstract. Over the past few decades, the geographical distribution of emissions of substances that alter the atmospheric energy balance has changed due to economic growth and air pollution regulations. Here, we show the resulting changes to aerosol and ozone abundances and their radiative forcing using recently updated emission data for the period 1990–2015, as simulated by seven global atmospheric composition models. The models broadly reproduce large-scale changes in surface aerosol and ozone based on observations (e.g. −1 to −3 % yr−1 in aerosols over the USA and Europe). The global mean radiative forcing due to ozone and aerosol changes over the 1990–2015 period increased by +0.17 ± 0.08 W m−2, with approximately one-third due to ozone. This increase is more strongly positive than that reported in IPCC AR5. The main reasons for the increased positive radiative forcing of aerosols over this period are the substantial reduction of global mean SO2 emissions, which is stronger in the new emission inventory compared to that used in the IPCC analysis, and higher black carbon emissions.


Climate ◽  
2018 ◽  
Vol 6 (4) ◽  
pp. 85 ◽  
Author(s):  
Sergei Soldatenko

In this paper, we apply the optimal control theory to obtain the analytic solutions of the two-component globally averaged energy balance model in order to estimate the influence of solar radiation management (SRM) operations on the global mean surface temperature in the 21st century. It is assumed that SRM is executed via injection of sulfur aerosols into the stratosphere to limit the global temperature increase in the year 2100 by 1.5 °C and keeping global temperature over the specified period (2020–2100) within 2 °C as required by the Paris climate agreement. The radiative forcing produced by the rise in the atmospheric concentrations of greenhouse gases is defined by the Representative Concentration Pathways and the 1pctCO2 (1% per year CO2 increase) scenario. The goal of SRM is formulated in terms of extremal problem, which entails finding a control function (the albedo of aerosol layer) that minimizes the amount of aerosols injected into the upper atmosphere to satisfy the Paris climate target. For each climate change scenario, the optimal albedo of the aerosol layer and the corresponding global mean surface temperature changes were obtained. In addition, the aerosol emission rates required to create an aerosol cloud with optimal optical properties were calculated.


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