scholarly journals How does the Environment Modulate Aerosol Impacts on Tropical Sea Breeze Convective Systems?

2021 ◽  
Author(s):  
J. Minnie Park ◽  
Susan C. van den Heever

Abstract. This study investigates how the enhanced loading of microphysically and radiatively active aerosol particles impacts tropical sea breeze convection and whether these aerosol impacts are modulated by the multitudinous environments that support these cloud systems. To achieve these goals, we have performed two large numerical model ensembles, each comprised of 130 idealised simulations that represent different initial conditions typical of tropical sea breeze environments. The two ensembles are identical with the exception of the fact that one ensemble is initialised with relatively low aerosol loading or pristine conditions, while the other is initialised with higher aerosol loading or polluted conditions. Six atmospheric and four surface parameters are simultaneously perturbed for the 130 initial conditions. Analysis of the ten-dimensional parameter simulations was facilitated by the use of a statistical emulator and multivariate sensitivity techniques. Comparisons of the clean and polluted ensembles demonstrate that aerosol direct effects reduce the incoming shortwave radiation reaching the surface, as well as the outgoing longwave radiation, within the polluted ensemble. This results in weaker surface fluxes, a reduced ocean-land thermal gradient, and a weaker sea breeze circulation. Consequently, irrespective of the different initial environmental conditions, increasing aerosol concentration decreases the three ingredients necessary for moist convection: moisture, instability, and lift. As reduced surface fluxes and instability inhibit the convective boundary layer development, updraft velocities of the daytime cumulus convection developing ahead of the sea breeze front are robustly reduced in the polluted environments. Furthermore, the variance-based sensitivity analysis reveals that the soil saturation fraction is the most important environmental factor contributing to the updraft velocity variance of this daytime cumulus mode, but that it becomes a less important contributor with enhanced aerosol loading. It is also demonstrated that enhanced aerosol loading results in a weakening of the convection initiated along the sea breeze front. This suppression is particularly robust when the sea breeze-initiated convection is shallower, and hence restricted to warm rain processes. However, when the sea breeze-initiated convection is deep and includes mixed-phase processes, both the sign and magnitude of the convective updraft responses to increased aerosol loading are modulated by the environment. The less favourable convective environment arising from aerosol direct effects also restricts the development of sea breeze-initiated deep convection. While precipitation is ubiquitously suppressed with enhanced aerosol loading, the magnitude of this suppression remains a function of the initial environment. Altogether, our results highlight the importance of evaluating aerosol impacts on convection systems under the wide range of environments supporting such convective development.

2015 ◽  
Vol 72 (9) ◽  
pp. 3378-3388 ◽  
Author(s):  
Usama Anber ◽  
Shuguang Wang ◽  
Adam Sobel

Abstract The effects of turbulent surface fluxes and radiative heating on tropical deep convection are compared in a series of idealized cloud-system-resolving simulations with parameterized large-scale dynamics. Two methods of parameterizing the large-scale dynamics are used: the weak temperature gradient (WTG) approximation and the damped gravity wave (DGW) method. Both surface fluxes and radiative heating are specified, with radiative heating taken as constant in the vertical in the troposphere. All simulations are run to statistical equilibrium. In the precipitating equilibria, which result from sufficiently moist initial conditions, an increment in surface fluxes produces more precipitation than an equal increment of column-integrated radiative heating. This is straightforwardly understood in terms of the column-integrated moist static energy budget with constant normalized gross moist stability. Under both large-scale parameterizations, the gross moist stability does in fact remain close to constant over a wide range of forcings, and the small variations that occur are similar for equal increments of surface flux and radiative heating. With completely dry initial conditions, the WTG simulations exhibit hysteresis, maintaining a dry state with no precipitation for a wide range of net energy inputs to the atmospheric column. The same boundary conditions and forcings admit a rainy state also (for moist initial conditions), and thus multiple equilibria exist under WTG. When the net forcing (surface fluxes minus radiative heating) is increased enough that simulations that begin dry eventually develop precipitation, the dry state persists longer after initialization when the surface fluxes are increased than when radiative heating is increased. The DGW method, however, shows no multiple equilibria in any of the simulations.


Author(s):  
B. Müller

AbstractModels of neutrino-driven core-collapse supernova explosions have matured considerably in recent years. Explosions of low-mass progenitors can routinely be simulated in 1D, 2D, and 3D. Nucleosynthesis calculations indicate that these supernovae could be contributors of some lighter neutron-rich elements beyond iron. The explosion mechanism of more massive stars remains under investigation, although first 3D models of neutrino-driven explosions employing multi-group neutrino transport have become available. Together with earlier 2D models and more simplified 3D simulations, these have elucidated the interplay between neutrino heating and hydrodynamic instabilities in the post-shock region that is essential for shock revival. However, some physical ingredients may still need to be added/improved before simulations can robustly explain supernova explosions over a wide range of progenitors. Solutions recently suggested in the literature include uncertainties in the neutrino rates, rotation, and seed perturbations from convective shell burning. We review the implications of 3D simulations of shell burning in supernova progenitors for the ‘perturbations-aided neutrino-driven mechanism,’ whose efficacy is illustrated by the first successful multi-group neutrino hydrodynamics simulation of an 18 solar mass progenitor with 3D initial conditions. We conclude with speculations about the impact of 3D effects on the structure of massive stars through convective boundary mixing.


2016 ◽  
Vol 16 (12) ◽  
pp. 7725-7741 ◽  
Author(s):  
Luping Su ◽  
Edward G. Patton ◽  
Jordi Vilà-Guerau de Arellano ◽  
Alex B. Guenther ◽  
Lisa Kaser ◽  
...  

Abstract. The emission, dispersion, and photochemistry of isoprene (C5H8) and related chemical species in the convective boundary layer (CBL) during sunlit daytime were studied over a mixed forest in the southeastern United States by combining ground-based and aircraft observations. Fluxes of isoprene and monoterpenes were quantified at the top of the forest canopy using a high-resolution proton transfer reaction time-of-flight mass spectrometer (PTR-TOF-MS). Snapshot (∼  2 min sampling duration) vertical profiles of isoprene, methyl vinyl ketone (MVK) + methacrolein (MACR), and monoterpenes were collected from aircraft every hour in the CBL (100–1000 m). Both ground-based and airborne collected volatile organic compound (VOC) data are used to constrain the initial conditions of a mixed-layer chemistry model (MXLCH), which is applied to examine the chemical evolution of the O3–NOx–HOx–VOC system and how it is affected by boundary layer dynamics in the CBL. The chemical loss rate of isoprene (∼  1 h) is similar to the turbulent mixing timescale (0.1–0.5 h), which indicates that isoprene concentrations are equally dependent on both photooxidation and boundary layer dynamics. Analysis of a model-derived concentration budget suggests that diurnal evolution of isoprene inside the CBL is mainly controlled by surface emissions and chemical loss; the diurnal evolution of O3 is dominated by entrainment. The NO to HO2 ratio (NO : HO2) is used as an indicator of anthropogenic impact on the CBL chemical composition and spans a wide range (1–163). The fate of hydroxyl-substituted isoprene peroxyl radical (HOC5H8OO·; ISOPOO) is strongly affected by NO : HO2, shifting from NO-dominant to NO–HO2-balanced conditions from early morning to noontime. This chemical regime change is reflected in the diurnal evolution of isoprene hydroxynitrates (ISOPN) and isoprene hydroxy hydroperoxides (ISOPOOH).


2019 ◽  
Vol 19 (15) ◽  
pp. 10191-10203 ◽  
Author(s):  
Franziska Glassmeier ◽  
Fabian Hoffmann ◽  
Jill S. Johnson ◽  
Takanobu Yamaguchi ◽  
Ken S. Carslaw ◽  
...  

Abstract. The climatic relevance of aerosol–cloud interactions depends on the sensitivity of the radiative effect of clouds to cloud droplet number N, and liquid water path LWP. We derive the dependence of cloud fraction CF, cloud albedo AC, and the relative cloud radiative effect rCRE=CF⋅AC on N and LWP from 159 large-eddy simulations of nocturnal stratocumulus. These simulations vary in their initial conditions for temperature, moisture, boundary-layer height, and aerosol concentration but share boundary conditions for surface fluxes and subsidence. Our approach is based on Gaussian-process emulation, a statistical technique related to machine learning. We succeed in building emulators that accurately predict simulated values of CF, AC, and rCRE for given values of N and LWP. Emulator-derived susceptibilities ∂ln⁡rCRE/∂ln⁡N and ∂ln⁡rCRE/∂ln⁡LWP cover the nondrizzling, fully overcast regime as well as the drizzling regime with broken cloud cover. Theoretical results, which are limited to the nondrizzling regime, are reproduced. The susceptibility ∂ln⁡rCRE/∂ln⁡N captures the strong sensitivity of the cloud radiative effect to cloud fraction, while the susceptibility ∂ln⁡rCRE/∂ln⁡LWP describes the influence of cloud amount on cloud albedo irrespective of cloud fraction. Our emulation-based approach provides a powerful tool for summarizing complex data in a simple framework that captures the sensitivities of cloud-field properties over a wide range of states.


2019 ◽  
Author(s):  
Franziska Glassmeier ◽  
Fabian Hoffmann ◽  
Jill S. Johnson ◽  
Takanobu Yamaguchi ◽  
Ken S. Carslaw ◽  
...  

Abstract. The climatic relevance of aerosol-cloud interactions depends on the sensitivity of the radiative effect of clouds to cloud droplet number N and liquid water path LWP. We derive the dependence of cloud fraction CF, cloud albedo AC and the relative cloud radiative effect rCRE = CF · AC on N and LWP from 159 large-eddy simulations of nocturnal stratocumulus. These simulations vary in their initial conditions for temperature, moisture, boundary-layer height and aerosol concentration but share boundary conditions for surface fluxes and subsidence. Our approach is based on Gaussian process emulation, a statistical technique related to machine learning. We succeed in building emulators that accurately predict simulated values of CF, AC and rCRE for given values of N and LWP. Emulator-derived susceptibilities ∂ ln rCRE/∂ ln N and ∂ ln rCRE/∂ ln LWP cover the non-drizzling, fully-overcast regime as well as the drizzling regime with broken cloud cover. Theoretical results, which are limited to the non-drizzling regime, are reproduced. The susceptibility ∂ ln rCRE/∂ ln N captures the strong sensitivity of the cloud radiative effect to cloud fraction, while the susceptibility ∂ ln rCRE/∂ ln LWP describes the influence of cloud amount on cloud albedo irrespective of cloud fraction. Our emulation-based approach provides a powerful tool for summarizing complex data in a simple framework that captures the sensitivities of cloud field properties over a wide range of states.


1999 ◽  
Vol 17 (2) ◽  
pp. 242-256 ◽  
Author(s):  
V. Pavan ◽  
N. Hall ◽  
P. Valdes ◽  
M. Blackburn

Abstract. A primitive equation model is used to study the sensitivity of baroclinic wave life cycles to the initial latitude-height distribution of humidity. Diabatic heating is parametrized only as a consequence of condensation in regions of large-scale ascent. Experiments are performed in which the initial relative humidity is a simple function of model level, and in some cases latitude bands are specified which are initially relatively dry. It is found that the presence of moisture can either increase or decrease the peak eddy kinetic energy of the developing wave, depending on the initial moisture distribution. A relative abundance of moisture at mid-latitudes tends to weaken the wave, while a relative abundance at low latitudes tends to strengthen it. This sensitivity exists because competing processes are at work. These processes are described in terms of energy box diagnostics. The most realistic case lies on the cusp of this sensitivity. Further physical parametrizations are then added, including surface fluxes and upright moist convection. These have the effect of increasing wave amplitude, but the sensitivity to initial conditions of relative humidity remains. Finally, 'control' and 'doubled CO2' life cycles are performed, with initial conditions taken from the time-mean zonal-mean output of equilibrium GCM experiments. The attenuation of the wave resulting from reduced baroclinicity is more pronounced than any effect due to changes in initial moisture.Key words. Meteorology and atmospheric dynamics (climatology; convective processes; synoptic-scale meteorology)


2012 ◽  
Vol 25 (20) ◽  
pp. 6885-6904 ◽  
Author(s):  
Isabelle Tobin ◽  
Sandrine Bony ◽  
Remy Roca

Abstract Tropical deep convection exhibits complex organization over a wide range of scales. This study investigates the relationships between the spatial organization of deep convection and the large-scale atmospheric state. By using several satellite datasets and reanalyses, and by defining a simple diagnostic of convective aggregation, relationships between the degree of convective aggregation and the amount of water vapor, turbulent surface fluxes, and radiation are highlighted above tropical oceans. When deep convection is more aggregated, the middle and upper troposphere are drier in the convection-free environment, turbulent surface fluxes are enhanced, and the low-level and midlevel cloudiness is reduced in the environment. Humidity and cloudiness changes lead to a large increase in outgoing longwave radiation. Cloud changes also result in reduced reflected shortwave radiation. Owing to these opposing effects, the sensitivity of the radiative budget at the top of the atmosphere to convective aggregation turns out to be weak, but the distribution of radiative heating throughout the troposphere is affected. These results suggest that feedbacks between convective aggregation and the large-scale atmospheric state might influence large-scale dynamics and the transports of water and energy and, thus, play a role in the climate variability and change. These observational findings are qualitatively consistent with previous cloud-resolving model results, except for the effects on cloudiness and reflected shortwave radiation. The proposed methodology may be useful for assessing the representation of convective aggregation and its interaction with the large-scale atmospheric state in various numerical models.


2015 ◽  
Vol 15 (21) ◽  
pp. 31621-31663 ◽  
Author(s):  
L. Su ◽  
E. G. Patton ◽  
J. Vilà-Guerau de Arellano ◽  
A. B. Guenther ◽  
L. Kaser ◽  
...  

Abstract. The emission, dispersion and photochemistry of isoprene (C5H8) and related chemical species in the convective boundary layer (CBL) during sunlit daytime was studied over a mixed forest in the Southeast United States by combining ground-based and aircraft observations. Fluxes of isoprene and monoterpenes were quantified at the top of the forest canopy using a high resolution Proton Transfer Reaction Time of Flight Mass Spectrometer (PTR-TOF-MS). Snapshot (~ 2 min sampling duration) vertical profiles of isoprene, methyl vinyl ketone (MVK) + methacrolein (MACR), and monoterpenes were collected from aircraft every hour in the CBL (100–1000 m). Both ground-based and airborne collected volatile organic compound (VOC) data are used to constrain the initial conditions of a mixed layer chemistry model (MXLCH), which is applied to examine the chemical evolution of the O3-NOx-HOx-VOC system and how it is affected by boundary layer dynamics in the CBL. The chemical loss rate of isoprene (~ 1 h) is similar to the turbulent mixing time scale (0.1–0.5 h), which indicates that isoprene concentrations are equally dependent on both photo-oxidation and boundary layer dynamics. Analysis of a model-derived concentration budget suggests that diurnal evolution of isoprene inside the CBL is mainly controlled by surface emissions and chemical loss. The NO to HO2 ratio (NO : HO2) is used as an indicator of anthropogenic impact on the CBL chemical composition, and spans a wide range (1–163). The fate of hydroxyl-substituted isoprene peroxyl radical (HOC5H8OO·; ISOPOO) is strongly affected by NO : HO2, shifting from NO-dominant to NO-HO2-balanced condition from early morning to noontime. This chemical regime change is reflected in the diurnal evolution of isoprene hydroxynitrates (ISOPN) and isoprene hydroxy hydroperoxides (ISOPOOH).


Author(s):  
Alyssa T Brooks ◽  
Hannah K Allen ◽  
Louise Thornton ◽  
Tracy Trevorrow

Abstract Health behavior researchers should refocus and retool as it becomes increasingly clear that the challenges of the COVID-19 pandemic surpass the direct effects of COVID-19 and include unique, drastic, and ubiquitous consequences for health behavior. The circumstances of the pandemic have created a natural experiment, allowing researchers focusing on a wide range of health behaviors and populations with the opportunity to use previously collected and future data to study: (a) changes in health behavior prepandemic and postpandemic, (b) health behavior prevalence and needs amidst the pandemic, and (c) the effects of the pandemic on short- and long-term health behavior. Our field is particularly challenged as we attempt to consider biopsychosocial, political, and environmental factors that affect health and health behavior. These realities, while daunting, should call us to action to refocus and retool our research, prevention, and intervention efforts


2021 ◽  
Vol 11 (1) ◽  
Author(s):  
R. Mendes ◽  
J. C. B. da Silva ◽  
J. M. Magalhaes ◽  
B. St-Denis ◽  
D. Bourgault ◽  
...  

AbstractInternal waves (IWs) in the ocean span across a wide range of time and spatial scales and are now acknowledged as important sources of turbulence and mixing, with the largest observations having 200 m in amplitude and vertical velocities close to 0.5 m s−1. Their origin is mostly tidal, but an increasing number of non-tidal generation mechanisms have also been observed. For instance, river plumes provide horizontally propagating density fronts, which were observed to generate IWs when transitioning from supercritical to subcritical flow. In this study, satellite imagery and autonomous underwater measurements are combined with numerical modeling to investigate IW generation from an initial subcritical density front originating at the Douro River plume (western Iberian coast). These unprecedented results may have important implications in near-shore dynamics since that suggest that rivers of moderate flow may play an important role in IW generation between fresh riverine and coastal waters.


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