scholarly journals Increased Northern Hemispheric carbon monoxide burden in the troposphere in 2002 and 2003 detected from the ground and from space

2005 ◽  
Vol 5 (2) ◽  
pp. 563-573 ◽  
Author(s):  
L. N. Yurganov ◽  
P. Duchatelet ◽  
A. V. Dzhola ◽  
D. P. Edwards ◽  
F. Hase ◽  
...  
Keyword(s):  
Carbon Monoxide ◽  
Forest Fires ◽  
Hot Spots ◽  
Ground Level ◽  
The Sun ◽  
Mixing Ratios ◽  
Moderate Resolution ◽  
Northern Hemispheric ◽  
Co Emission ◽  
Total Column

Abstract. Carbon monoxide total column amounts in the atmosphere have been measured in the High Northern Hemisphere (30°-90° N, HNH) between January 2002 and December 2003 using infrared spectrometers of high and moderate resolution and the Sun as a light source. They were compared to ground-level CO mixing ratios and to total column amounts measured from space by the Terra/MOPITT instrument. All these data reveal increased CO abundances in 2002-2003 in comparison to the unperturbed 2000-2001 period. Maximum anomalies were observed in September 2002 and August 2003. Using a simple two-box model, the corresponding annual CO emission anomalies (referenced to 2000-2001 period) have been found equal to 95Tg in 2002 and 130Tg in 2003, thus close to those for 1996 and 1998. A good correlation with hot spots detected by a satellite radiometer allows one to assume strong boreal forest fires, occurred mainly in Russia, as a source of the increased CO burdens.

scholarly journals Increased Northern Hemispheric carbon monoxide burden in the troposphere in 2002 and 2003 detected from the ground and from space

2004 ◽  
Vol 4 (5) ◽  
pp. 4999-5017 ◽  
Author(s):  
L. N. Yurganov ◽  
P. Duchatelet ◽  
A. V. Dzhola ◽  
D. P. Edwards ◽  
F. Hase ◽  
...  
Keyword(s):  
Carbon Monoxide ◽  
Boreal Forest ◽  
Northern Hemisphere ◽  
Forest Fires ◽  
Ground Level ◽  
Mixing Ratios ◽  
Moderate Resolution ◽  
Northern Hemispheric ◽  
Co Emission ◽  
Total Column

Abstract. Carbon monoxide total column amounts in the atmosphere have been measured in the High Northern Hemisphere (30°–90° N, HNH) between January 2002 and December 2003, based on the analysis of infrared solar spectra recorded with spectrometers of high and moderate resolution. They are compared to ground-level CO mixing ratios and to total column amounts measured from space by the Terra/MOPITT instrument. In comparison to the unperturbed 2000–2001 period, all these databases reveal increased CO abundances in 2002–2003 summer-autumn times, with maximum anomalies observed in September 2002 and August 2003. Using a simple two-box model, the corresponding annual CO emission anomalies have been found equal to 98 Tg in 2002 and 142 Tg in 2003, thus close to those for 1996 and 1998. It is most likely that strong boreal forest fires in the HNH induced the increased CO burdens.

scholarly journals Forest Fire in East Nusa Tenggara during 2015-2019: Comparison to Forest Fire in Kalimantan and Sumatera

2021 ◽  
Vol 893 (1) ◽  
pp. 012010
Author(s):  
Sumaryati ◽  
D F Andarini ◽  
N Cholianawati ◽  
A Indrawati
Keyword(s):  
Carbon Monoxide ◽  
Forest Fire ◽  
Forest Fires ◽  
Forest Biomass ◽  
Comparison Method ◽  
Atmospheric Environment ◽  
Annual Average ◽  
Statistical Comparison ◽  
Fire Area ◽  
Total Column

Abstract East Nusa Tenggara is one of the provinces in Indonesia that has big forest fires following some provinces in Kalimantan and Sumatra. However, forest fires in East Nusa Tenggara have less attention in forest fires discussion in Indonesia. This study aims to analyze forest fires in East Nusa Tenggara and their impact on reducing visibility and increasing carbon monoxide (CO) from 2015 to 2019. In this study, hotspot, forest fire area, Oceanic Niño Index, visibility, and CO total column data were used to analyze the forest fires using a statistical comparison method in East Nusa Tenggara, Kalimantan, and Sumatra. The result shows that the number of hotspots in East Nusa Tenggara less than in Kalimantan and Sumatra for the same forest fire area. The forest fires in East Nusa Tenggara do not harm the atmospheric environment significantly. East Nusa Tenggara dominantly consists of savanna areas with no peatland, hence, the forest biomass burning produces less smoke and CO. Furthermore, the forest fire in East Nusa Tenggara has not an impact on decreasing visibility and increasing CO total column, in contrast, visibility in Sumatra and Kalimantan has fallen to 6 km from the annual average, and CO total column rise three times of normal condition during peak fire.

scholarly journals Atmospheric hydrogen variations and traffic emissions at an urban site in Finland

2009 ◽  
Vol 9 (19) ◽  
pp. 7387-7396 ◽  
Author(s):  
T. Aalto ◽  
M. Lallo ◽  
J. Hatakka ◽  
T. Laurila
Keyword(s):  
Carbon Monoxide ◽  
Traffic Flow ◽  
Road Traffic ◽  
Urban Site ◽  
High Carbon ◽  
Traffic Emission ◽  
High Hydrogen ◽  
Mixing Ratios ◽  
One Year ◽  
Co Emission

Abstract. Atmospheric hydrogen (H2) mixing ratios were observed over a one year period from summer 2007 to 2008 in Helsinki, Finland. Relatively stable background values of hydrogen were occasionally observed at the site, with minimum in October and maximum between March and May. High hydrogen mixing ratios occurred simultaneously with high carbon monoxide (CO) values and coincided with high traffic flow periods. Carbon monoxide and radon (222Rn) were continuously monitored at the same site and they were used in estimation of the hydrogen emissions from traffic. The morning rush hour slope of ΔH2/ΔCO was in average 0.43±0.03 ppb (H2)/ppb (CO). After correction due to soil deposition of H2 the slope was 0.49±0.07 ppb (H2)/ppb (CO). Using this slope and CO emission statistics, a road traffic emission of about 260 t (H2)/year was estimated for Helsinki in 2007.

scholarly journals Impact of spaceborne carbon monoxide observations from the S-5P platform on tropospheric composition analyses and forecasts

2017 ◽  
Vol 17 (2) ◽  
pp. 1081-1103 ◽  
Author(s):  
Rachid Abida ◽  
Jean-Luc Attié ◽  
Laaziz El Amraoui ◽  
Philippe Ricaud ◽  
William Lahoz ◽  
...  
Keyword(s):  
Carbon Monoxide ◽  
Forest Fires ◽  
Weather Conditions ◽  
Emission Sources ◽  
Simulation Experiments ◽  
Northern Summer ◽  
Free Model ◽  
Comparison Of The Results ◽  
The Impact ◽  
Total Column

Abstract. We use the technique of Observing System Simulation Experiments (OSSEs) to quantify the impact of spaceborne carbon monoxide (CO) total column observations from the Sentinel-5 Precursor (S-5P) platform on tropospheric analyses and forecasts. We focus on Europe for the period of northern summer 2003, when there was a severe heat wave episode associated with extremely hot and dry weather conditions. We describe different elements of the OSSE: (i) the nature run (NR), i.e., the truth; (ii) the CO synthetic observations; (iii) the assimilation run (AR), where we assimilate the observations of interest; (iv) the control run (CR), in this study a free model run without assimilation; and (v) efforts to establish the fidelity of the OSSE results. Comparison of the results from AR and the CR, against the NR, shows that CO total column observations from S-5P provide a significant benefit (at the 99 % confidence level) at the surface, with the largest benefit occurring over land in regions far away from emission sources. Furthermore, the S-5P CO total column observations are able to capture phenomena such as the forest fires that occurred in Portugal during northern summer 2003. These results provide evidence of the benefit of S-5P observations for monitoring processes contributing to atmospheric pollution.

scholarly journals Atmospheric hydrogen variations and traffic emissions at an urban site in Finland

2009 ◽  
Vol 9 (3) ◽  
pp. 13917-13942 ◽  
Author(s):  
T. Aalto ◽  
M. Lallo ◽  
J. Hatakka ◽  
T. Laurila
Keyword(s):  
Carbon Monoxide ◽  
Traffic Flow ◽  
Road Traffic ◽  
Urban Site ◽  
High Carbon ◽  
Traffic Emission ◽  
High Hydrogen ◽  
Mixing Ratios ◽  
One Year ◽  
Co Emission

Abstract. Atmospheric hydrogen (H2) mixing ratios were observed over one year period from summer 2007 to 2008 in Helsinki, Finland. Relatively stable background values of hydrogen were occasionally observed at the site, with minimum in October and maximum between March and May. High hydrogen mixing ratios occurred simultaneously with high carbon monoxide (CO) values and coincided with high traffic flow periods. Carbon monoxide and radon (222Rn) were continuously monitored at the same site and they were used in estimation of the hydrogen emissions from traffic. The morning rush hour slope of ΔH2/ΔCO was in average 0.43±0.03 ppb (H2)/ppb(CO). After correction due to soil deposition of H2 the slope was 0.49±0.07 ppb (H2)/ppb(CO). Using this slope and CO emission statistics, a road traffic emission of about 260 t (H2)/year was estimated for Helsinki in 2007.

scholarly journals Impact of data quality and surface-to-column representativeness on the PM<sub>2.5</sub> / satellite AOD relationship for the contiguous United States

2014 ◽  
Vol 14 (12) ◽  
pp. 6049-6062 ◽  
Author(s):  
T. D. Toth ◽  
J. Zhang ◽  
J. R. Campbell ◽  
E. J. Hyer ◽  
J. S. Reid ◽  
...  
Keyword(s):  
United States ◽  
Data Quality ◽  
Ground Level ◽  
Dry Mass ◽  
Orthogonal Polarization ◽  
Data Sets ◽  
Moderate Resolution ◽  
Resolution Imaging ◽  
Moderate Resolution Imaging Spectroradiometer ◽  
Total Column

Abstract. Satellite-derived aerosol optical depth (AOD) observations have been used to estimate particulate matter smaller than 2.5 μm (PM2.5). However, such a relationship could be affected by the representativeness of satellite-derived AOD to surface aerosol particle mass concentration and satellite AOD data quality. Using purely measurement-based methods, we have explored the impacts of data quality and representativeness on the AOD-inferred PM2.5 / AOD relationship for the contiguous United States (CONUS). This is done through temporally and spatially collocated data sets of PM2.5 and AOD retrievals from Aqua/Terra Moderate Resolution Imaging Spectroradiometer (MODIS), Multi-angle Imaging Spectroradiometer (MISR), and Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP). These analyses show that improving data quality of satellite AOD, such as done with data assimilation-grade retrievals, increases their correlation with PM2.5. However, overall correlation is relatively low across the CONUS. Also, integrated extinction observed within 500 m above ground level (a.g.l.), as measured by CALIOP, is not well representative of the total column AOD. Surface aerosol in the eastern CONUS is better correlated with total column AOD than in the western CONUS. The best correlation values are found for estimated dry mass CALIOP extinction at 200–300 m a.g.l. and PM2.5, but additional work is needed to address the ability of using actively sensed AOD as a proxy for PM2.5 concentrations.

scholarly journals Satellite-Observed Variations and Trends in Carbon Monoxide over Asia and Their Sensitivities to Biomass Burning

2020 ◽  
Vol 12 (5) ◽  
pp. 830 ◽  
Author(s):  
Xun Zhang ◽  
Jane Liu ◽  
Han Han ◽  
Yongguang Zhang ◽  
Zhe Jiang ◽  
...  
Keyword(s):  
Carbon Monoxide ◽  
Biomass Burning ◽  
Interannual Variation ◽  
Correlation Coefficients ◽  
Temporal Variations ◽  
South Siberia ◽  
Moderate Resolution ◽  
Moderate Resolution Imaging Spectroradiometer ◽  
Annual Means ◽  
Total Column

As the carbon monoxide (CO) total column over Asia is among the highest in the world, it is important to characterize its variations in space and time. Using Measurements of Pollution in the Troposphere (MOPITT) and Atmospheric InfraRed Sounder (AIRS) satellite data, the variations and trends in CO total column over Asia and its seven subregions during 2003–2017 are investigated in this study. The CO total column in Asia is higher in spring and winter than in summer and autumn. The seasonal maximum and minimum are in spring and summer respectively in the regional mean over Asia, varying between land and oceans, as well as among the subregions. The CO total column in Asia shows strong interannual variation, with a regional mean coefficient of variation of 5.8% in MOPITT data. From 2003 to 2017, the annual mean of CO total column over Asia decreased significantly at a rate of (0.58 ± 0.15)% per year (or −(0.11 ± 0.03) × 1017 molecules cm−2 per year) in MOPITT data, resulting from significant CO decreases in winter, summer, and spring. In most of the subregions, significant decreasing trends in CO total column are also observed, more obviously over areas with high CO total column, including eastern regions of China and the Sichuan Basin. The regional decreasing trends in these areas are over 1% per year. Over the entire Asia, and in fire-prone subregions including South Siberia, Indo-China Peninsula, and Indonesia, we found significant correlations between the MOPITT CO total column and the fire counts from the Moderate Resolution Imaging Spectroradiometer (MODIS). The variations in MODIS fire counts may explain 58%, 60%, 36%, and 71% of the interannual variation in CO total column in Asia and these three subregions, respectively. Over different land cover types, the variations in biomass burning may explain 62%, 52%, and 31% of the interannual variation in CO total column, respectively, over the forest, grassland, and shrubland in Asia. Extremes in CO total column in Asia can be largely explained by the extreme fire events, such as the fires over Siberia in 2003 and 2012 and over Indonesia in 2006 and 2015. The significant decreasing trends in MODIS fire counts inside and outside Asia suggest that global biomass burning may be a driver for the decreasing trend in CO total column in Asia, especially in spring. In general, the variations and trends in CO total column over Asia detected by AIRS are similar to but smaller than those by MOPITT. The two datasets show similar spatial and temporal variations in CO total column over Asia, with correlation coefficients of 0.86–0.98 in the annual means. This study shows that the interannual variation in atmospheric CO in Asia is sensitive to biomass burning, while the decreasing trend in atmospheric CO over Asia coincides with the decreasing trend in MODIS fire counts from 2003 to 2017.

scholarly journals Impact of Spaceborne Carbon Monoxide Observations from the S-5P platform on Tropospheric Composition Analyses and Forecasts

2016 ◽  
Author(s):  
R. Abida ◽  
J.-L. Attié ◽  
L. El Amraoui ◽  
P. Ricaud ◽  
W. Lahoz ◽  
...  
Keyword(s):  
Carbon Monoxide ◽  
Forest Fires ◽  
System Simulation ◽  
Weather Conditions ◽  
Simulation Experiments ◽  
Northern Summer ◽  
Free Model ◽  
Comparison Of The Results ◽  
The Impact ◽  
Total Column

Abstract. We use the technique of Observing System Simulation Experiments (OSSEs) to quantify the impact of spaceborne carbon monoxide (CO) total column observations from the Sentinel-5 Precursor (S-5P) platform on tropospheric analyses and forecasts. We focus on Europe for the period of northern summer 2003, when there was a severe heat wave episode associated with extremely hot and dry weather conditions. We describe different elements of the OSSE: (i) the Nature Run (NR), i.e., the "Truth"; ii) the CO synthetic observations; (iii) the assimilation run (AR), where we assimilate the observations of interest; (iv) the control run (CR), in this study a free model run without assimilation; and (v) efforts to establish the fidelity of the OSSE results. Comparison of the results from AR and the CR, against the NR, shows that CO total column observations from S-5P provide a significant benefit (at the 99 % confidence level) at the surface, with the largest benefit occurring over land in remote regions. Furthermore, the S-5P CO total column observations are able to capture phenomena such as the forest fires that occurred in Portugal during summer 2003. These results provide evidence of the benefit of S-5P observations for monitoring processes contributing to atmospheric pollution.

scholarly journals Regional variability in black carbon and carbon monoxide ratio from long-term observations over East Asia: assessment of representativeness for black carbon (BC) and carbon monoxide (CO) emission inventories

2020 ◽  
Vol 20 (1) ◽  
pp. 83-98 ◽  
Author(s):  
Yongjoo Choi ◽  
Yugo Kanaya ◽  
Seung-Myung Park ◽  
Atsushi Matsuki ◽  
Yasuhiro Sadanaga ◽  
...  
Keyword(s):  
Carbon Monoxide ◽  
South Korea ◽  
East Asia ◽  
Black Carbon ◽  
North Korea ◽  
Northeast China ◽  
Emission Inventory ◽  
East China ◽  
Co Emission

Abstract. The black carbon (BC) and carbon monoxide (CO) emission ratios were estimated and compiled from long-term, harmonized observations of the ΔBC∕ΔCO ratios under conditions unaffected by wet deposition at four sites in East Asia, including two sites in South Korea (Baengnyeong and Gosan) and two sites in Japan (Noto and Fukuoka). Extended spatio-temporal coverage enabled estimation of the full seasonality and elucidation of the emission ratio in North Korea for the first time. The estimated ratios were used to validate the Regional Emission inventory in ASia (REAS) version 2.1 based on six study domains (“East China”, “North China”, “Northeast China”, South Korea, North Korea, and Japan). We found that the ΔBC∕ΔCO ratios from four sites converged into a narrow range (6.2–7.9 ng m−3 ppb−1), suggesting consistency in the results from independent observations and similarity in source profiles over the regions. The BC∕CO ratios from the REAS emission inventory (7.7 ng m−3 ppb−1 for East China – 23.2 ng m−3 ppb−1 for South Korea) were overestimated by factors of 1.1 for East China to 3.0 for South Korea, whereas the ratio for North Korea (3.7 ng m−3 ppb−1 from REAS) was underestimated by a factor of 2.0, most likely due to inaccurate emissions from the road transportation sector. Seasonal variation in the BC∕CO ratio from REAS was found to be the highest in winter (China and North Korea) or summer (South Korea and Japan), whereas the measured ΔBC∕ΔCO ratio was the highest in spring in all source regions, indicating the need for further characterization of the seasonality when creating a bottom-up emission inventory. At levels of administrative districts, overestimation in Seoul, the southwestern regions of South Korea, and Northeast China was noticeable, and underestimation was mainly observed in the western regions in North Korea, including Pyongyang. These diagnoses are useful for identifying regions where revisions in the inventory are necessary, providing guidance for the refinement of BC and CO emission rate estimates over East Asia.

scholarly journals The influence of typhoons on atmospheric composition deduced from IAGOS measurements over Taipei

2020 ◽  
Vol 20 (6) ◽  
pp. 3945-3963
Author(s):  
Frank Roux ◽  
Hannah Clark ◽  
Kuo-Ying Wang ◽  
Susanne Rohs ◽  
Bastien Sauvage ◽  
...  
Keyword(s):  
Carbon Monoxide ◽  
Relative Humidity ◽  
Tropical Cyclones ◽  
Marine Boundary Layer ◽  
Chemical Species ◽  
Atmospheric Composition ◽  
Commercial Aircraft ◽  
Regular Feature ◽  
Mixing Ratios ◽  
The Vertical Distribution

Abstract. The research infrastructure IAGOS (In-Service Aircraft for a Global Observing System) equips commercial aircraft with instruments to monitor the composition of the atmosphere during flights around the world. In this article, we use data from two China Airlines aircraft based in Taipei (Taiwan) which provided daily measurements of ozone, carbon monoxide and water vapour throughout the summer of 2016. We present time series, from the surface to the upper troposphere, of ozone, carbon monoxide and relative humidity near Taipei, focusing on periods influenced by the passage of typhoons. We examine landing and take-off profiles in the vicinity of tropical cyclones using ERA-5 reanalyses to elucidate the origin of the anomalies in the vertical distribution of these chemical species. Results indicate a high ozone content in the upper- to middle-troposphere track of the storms. The high ozone mixing ratios are generally correlated with potential vorticity and anti-correlated with relative humidity, suggesting stratospheric origin. These results suggest that tropical cyclones participate in transporting air from the stratosphere to troposphere and that such transport could be a regular feature of typhoons. After the typhoons passed Taiwan, the tropospheric column was filled with substantially lower ozone mixing ratios due to the rapid uplift of marine boundary layer air. At the same time, the relative humidity increased, and carbon monoxide mixing ratios fell. Locally, therefore, the passage of typhoons has a positive effect on air quality at the surface, cleansing the atmosphere and reducing the mixing ratios of pollutants such as CO and O3.

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