Sir John Houghton (30 December 1931 — 15 April 2020) and radiation transfer

2021 ◽  
Author(s):  
Miklos Zagoni

<p>IPCC announced that the WGI contribution to AR6 will be dedicated to the memory of leading climate scientist Sir John Houghton. Sir John died of complications from COVID-19 one year ago. He helped creating the IPCC in 1988, and served as Chair and Co-Chair of WGI from 1988 to 2002. In this presentation we focus on two aspects of his work: radiation transfer and cloud radiative forcing. — His book “The Physics of Atmospheres” (third edition, 2002) says: “The equation of radiative transfer through the slab, which includes both absorption and emission, is sometimes known as Schwarzschild’s equation” (Eq. 2.3, p.11). Introducing a constant Ф net flux (Eq. 2.5) being equal to the outgoing radiation, the black-body function B of the atmosphere is given as a function of Ф and the optical depth as B = Ф(χ* + 1)/2π (Eq. 2.12). He says, “it is easy to show that there must be a temperature discontinuity at the lower boundary”: B<sub>g</sub> – B<sub>0</sub> = Ф/2π (Eq. 2.13). Fig. 2.4 displays the net flux at the boundary as half of the outgoing radiation, independently of the optical depth. He notes: “Such a steep lapse rate will soon be destroyed by the process of convection”, and continues: “Combining (2.12) and (2.13) we find Bg = Ф(χ* + 2)/2π ” (Eq. 2.15, section 2.5 The greenhouse effect). We controlled Eq. (2.13) on 20 years of clear-sky CERES EBAF Ed4.1 global mean data and found it satisfied with a difference of -2.28 Wm<sup>-2</sup>. The validity of this equation casts constraint on the surface net radiation and on the corresponding non-radiative fluxes in the hydrological cycle by connecting them unequivocally to half of the outgoing longwave radiation. We constructed the all-sky version of the equation by separating atmospheric radiation transfer from longwave cloud effect, and found it valid within 2.84 Wm<sup>-2</sup>. We computed Eq. (2.15) with a special optical depth of χ* = 2 for clear-sky; it is justified with a difference of -2.88 Wm<sup>-2</sup>. We also created its all-sky version; the difference is 2.46 Wm<sup>-2</sup>. Altogether, the four equations are satisfied on 20-yr of CERES data with a mean bias of 0.035 Wm<sup>-2</sup>. We show that the four equations together determine a clear-sky and an all-sky greenhouse factor as 1/3 and 0.4. Data from Wild et al. (2018) and IPCC AR5 (2013) show g(clear) = (398 – 267)/398 = 0.33 and g(all) = (398 – 239)/398 = 0.3995. The IPCC reports predict an enhanced greenhouse effect from human emissions. According to the above arithmetic solutions, Earth’s observed greenhouse factors are equal to the theoretical ones without any deviation or enhancement. — The first IPCC report states that cloud radiative forcing is governed by cloud properties as cloud amount, reflectivity, vertical distribution and optical depth. Here we show that the TOA net CRF (= SWCRF + LWCRF) in equilibrium is equivalent to TOA net clear-sky imbalance, hence to determine its magnitude only clear-sky fluxes are needed.</p>

2007 ◽  
Vol 7 (3) ◽  
pp. 7171-7233 ◽  
Author(s):  
P. Stier ◽  
J. H. Seinfeld ◽  
S. Kinne ◽  
O. Boucher

Abstract. We present a comprehensive examination of aerosol absorption with a focus on evaluating the sensitivity of the global distribution of aerosol absorption to key uncertainties in the process representation. For this purpose we extended the comprehensive aerosol-climate model ECHAM5-HAM by effective medium approximations for the calculation of aerosol effective refractive indices, updated black carbon refractive indices, new cloud radiative properties considering the effect of aerosol inclusions, as well as by modules for the calculation of long-wave aerosol radiative properties and instantaneous aerosol forcing. The evaluation of the simulated aerosol absorption optical depth with the AERONET sun-photometer network shows a good agreement in the large scale global patterns. On a regional basis it becomes evident that the update of the BC refractive indices to Bond and Bergstrom (2006) significantly improves the previous underestimation of the aerosol absorption optical depth. In the global annual-mean, absorption acts to reduce the short-wave anthropogenic aerosol top-of-atmosphere (TOA) radiative forcing clear-sky from –0.79 to –0.53 W m−2 (33%) and all-sky from –0.47 to –0.13 W m−2 (72%). Our results confirm that basic assumptions about the BC refractive index play a key role for aerosol absorption and radiative forcing. The effect of the usage of more accurate effective medium approximations is comparably small. We demonstrate that the diversity in the AeroCom land-surface albedo fields contributes to the uncertainty in the simulated anthropogenic aerosol radiative forcings: the usage of an upper versus lower bound of the AeroCom land albedos introduces a global annual-mean TOA forcing range of 0.19 W m−2 (36%) clear-sky and of 0.12 W m−2 (92%) all-sky. The consideration of black carbon inclusions on cloud radiative properties results in a small global annual-mean all-sky absorption of 0.05 W m−2 and a positive TOA forcing perturbation of 0.02 W m−2. The long-wave aerosol radiative effects are small for anthropogenic aerosols but become of relevance for the larger natural dust and sea-salt aerosols.


2014 ◽  
Vol 27 (20) ◽  
pp. 7769-7780 ◽  
Author(s):  
Vanda Salgueiro ◽  
Maria João Costa ◽  
Ana Maria Silva ◽  
Daniele Bortoli

Abstract The shortwave cloud radiative forcing is calculated from surface measurements taken in Évora from 2003 to 2010 with a multifilter rotating shadowband radiometer (MFRSR) and with an Eppley black and white pyranometer. A new approach to estimate the clear-sky irradiance based on radiative transfer calculations is also proposed. The daily-mean values of the cloud radiative forcing (absolute and normalized) as well as their monthly and seasonal variabilities are analyzed. The study shows greater variability of radiative forcing during springtime with respect to the other seasons. The mean daily cloudy periods have seasonal variation proportional to the seasonal variation of the cloud radiative forcing, with maximum values also occurring during springtime. The minimum values found for the daily-mean cloud radiative forcing are −139.5 and −198.4 W m−2 for MFRSR and Eppley data, respectively; the normalized values present about 40% of sample amplitude, both for MFRSR and Eppley. In addition, a quantitative relationship between the MFRSR and Eppley cloud radiative forcings applicable to other locations is proposed.


2005 ◽  
Vol 18 (22) ◽  
pp. 4637-4648 ◽  
Author(s):  
Melanie F. Fitzpatrick ◽  
Stephen G. Warren

Abstract Downward solar irradiance at the sea surface, measured on several voyages of an icebreaker in the Southern Ocean, is used to infer transmittance of solar radiation by clouds. Together with surface albedo estimated from coincident hourly sea ice reports, instantaneous cloud radiative forcing and effective cloud optical depth are obtained. Values of “raw cloud transmittance” (trc), the ratio of downward irradiance under cloud to downward irradiance measured under clear sky, vary from 0.1 to 1.0. Over sea ice, few values of trc were observed between 0.8 and 1.0, possibly due to the threshold nature of the aerosol-to-cloud-droplet transition. This sparsely populated region of transmittances is referred to as the Köhler gap. The instantaneous downward shortwave cloud radiative forcing is computed, as well as the time-averaged net forcing. The net forcing at a solar zenith angle of 60° is typically −250 W m−2 over open ocean, but only half this value over sea ice because of the higher surface albedo and less frequent occurrence of clouds. “Effective” optical depths τ (for a radiatively equivalent horizontally homogeneous cloud) are classified by season and surface type. The frequency distributions of τ are well fitted by decaying exponentials, giving a characteristic optical depth of 15 at 47°S, increasing to 24 in the region of maximum cloud cover at 58°S, and decreasing to 11 at 67°S near the coast of Antarctica.


2011 ◽  
Vol 7 (5) ◽  
pp. 3577-3582
Author(s):  
R. Rondanelli ◽  
R. S. Lindzen

Abstract. Goldblatt and Zahnle (2011) raise a number of issues related to the possibility that cirrus clouds can provide a solution to the faint young sun paradox. Here we argue that some of the criticism is not warranted. In particular, the criticism related to cirrus clouds being an "end member" case of possible clouds depends heavily on models that may have an inadequate representation of cirrus clouds. Present climate observations show that thin cirrus clouds (optical depth less than 10) can produce positive cloud radiative forcing. When this forcing is represented in models, resulting cirrus clouds are not necessarily realistic. Therefore, cirrus clouds that have a radiative forcing consistent with present climate observations, can provide a solution to the faint young sun paradox, or at least ease the amount of CO2 or other greenhouse substances needed to provide temperatures above freezing during the Archean.


2016 ◽  
Vol 113 (21) ◽  
pp. 5804-5811 ◽  
Author(s):  
Steven Ghan ◽  
Minghuai Wang ◽  
Shipeng Zhang ◽  
Sylvaine Ferrachat ◽  
Andrew Gettelman ◽  
...  

A large number of processes are involved in the chain from emissions of aerosol precursor gases and primary particles to impacts on cloud radiative forcing. Those processes are manifest in a number of relationships that can be expressed as factors dlnX/dlnY driving aerosol effects on cloud radiative forcing. These factors include the relationships between cloud condensation nuclei (CCN) concentration and emissions, droplet number and CCN concentration, cloud fraction and droplet number, cloud optical depth and droplet number, and cloud radiative forcing and cloud optical depth. The relationship between cloud optical depth and droplet number can be further decomposed into the sum of two terms involving the relationship of droplet effective radius and cloud liquid water path with droplet number. These relationships can be constrained using observations of recent spatial and temporal variability of these quantities. However, we are most interested in the radiative forcing since the preindustrial era. Because few relevant measurements are available from that era, relationships from recent variability have been assumed to be applicable to the preindustrial to present-day change. Our analysis of Aerosol Comparisons between Observations and Models (AeroCom) model simulations suggests that estimates of relationships from recent variability are poor constraints on relationships from anthropogenic change for some terms, with even the sign of some relationships differing in many regions. Proxies connecting recent spatial/temporal variability to anthropogenic change, or sustained measurements in regions where emissions have changed, are needed to constrain estimates of anthropogenic aerosol impacts on cloud radiative forcing.


2014 ◽  
Vol 14 (4) ◽  
pp. 2185-2201 ◽  
Author(s):  
R. S. Park ◽  
S. Lee ◽  
S.-K. Shin ◽  
C. H. Song

Abstract. This study focused on the contribution of ammonium nitrate (NH4NO3) to aerosol optical depth (AOD) and direct radiative forcing (DRF) by aerosols over an East Asian domain. In order to evaluate the contribution, chemistry-transport model (CTM)-estimated AOD was combined with satellite-retrieved AOD, utilizing a data assimilation technique, over East Asia for the entire year of 2006. Using the assimilated AOD and CTM-estimated aerosol optical properties, the DRF by aerosols was estimated over East Asia via a radiative transfer model (RTM). Both assimilated AOD and estimated DRF values showed relatively good agreements with AOD and DRF by aerosols from AERONET. Based on these results, the contributions of NH4NO3 to AOD and DRF by aerosols (ΦAOD and ΦDRF) were estimated for the four seasons of 2006 over East Asia. Both ΦAOD and ΦDRF showed seasonal variations over East Asia within the ranges between 4.7% (summer) and 31.3% (winter) and between 4.7% (summer) and 30.7% (winter), respectively, under clear-sky conditions, showing annual average contributions of 15.6% and 15.3%. Under all-sky conditions, ΦDRF varied between 3.6% (summer) and 24.5% (winter), showing annual average contribution of 12.1% over East Asia. These annual average contributions of NH4NO3 to AOD and DRF are almost comparable to the annual average mass fractions of NH4NO3 in PM2.5 and PM10 (17.0% and 14.0%, respectively). ΦAOD and ΦDRF were even larger in the locations where NH3 and NOx emission rates are strong, such as the central East China (CEC) region and Sichuan Basin. For example, under clear-sky conditions, both ΦAOD and ΦDRF over the CEC region range between 6.9% (summer) and 47.9% (winter) and between 6.7% (summer) and 47.5% (winter), respectively. Based on this analysis, it was concluded that both ΦAOD and ΦDRF cannot be ignored in East Asian air quality and radiative forcing studies, particularly during winter.


2005 ◽  
Vol 18 (20) ◽  
pp. 4235-4252 ◽  
Author(s):  
Michael S. Town ◽  
Von P. Walden ◽  
Stephen G. Warren

Abstract Annual cycles of downwelling broadband infrared radiative flux and spectral downwelling infrared flux were determined using data collected at the South Pole during 2001. Clear-sky conditions are identified by comparing radiance ratios of observed and simulated spectra. Clear-sky fluxes are in the range of 110–125 W m−2 during summer (December–January) and 60–80 W m−2 during winter (April–September). The variability is due to day-to-day variations in temperature, strength of the surface-based temperature inversion, atmospheric humidity, and the presence of “diamond dust” (near-surface ice crystals). The persistent presence of diamond dust under clear skies during the winter is evident in monthly averages of clear-sky radiance. About two-thirds of the clear-sky flux is due to water vapor, and one-third is due to CO2, both in summer and winter. The seasonal constancy of this approximately 2:1 ratio is investigated through radiative transfer modeling. Precipitable water vapor (PWV) amounts were calculated to investigate the H2O/CO2 flux ratio. Monthly mean PWV during 2001 varied from 1.6 mm during summer to 0.4 mm during winter. Earlier published estimates of PWV at the South Pole are similar for winter, but are 50% lower for summer. Possible reasons for low earlier estimates of summertime PWV are that they are based either on inaccurate hygristor technology or on an invalid assumption that the humidity was limited by saturation with respect to ice. The average fractional cloud cover derived from the spectral infrared data is consistent with visual observations in summer. However, the wintertime average is 0.3–0.5 greater than that obtained from visual observations. The annual mean of longwave downwelling cloud radiative forcing (LDCRF) for 2001 is about 23 W m−2 with no apparent seasonal cycle. This is about half that of the global mean LDCRF; the low value is attributed to the small optical depths and low temperatures of Antarctic clouds.


2018 ◽  
Vol 18 (20) ◽  
pp. 14867-14887 ◽  
Author(s):  
Daniele Visioni ◽  
Giovanni Pitari ◽  
Glauco di Genova ◽  
Simone Tilmes ◽  
Irene Cionni

Abstract. Aside from the direct surface cooling that sulfate geoengineering (SG) would produce, investigations of the possible side effects of this method are still ongoing, such as the exploration of the effect that SG may have on upper tropospheric cirrus cloudiness. The goal of the present study is to better understand the SG thermodynamical effects on the freezing mechanisms leading to ice particle formation. This is undertaken by comparing SG model simulations against a Representative Concentration Pathway 4.5 (RCP4.5) reference case. In the first case, the aerosol-driven surface cooling is included and coupled to the stratospheric warming resulting from the aerosol absorption of terrestrial and solar near-infrared radiation. In a second SG perturbed case, the surface temperatures are kept unchanged with respect to the reference RCP4.5 case. When combined, surface cooling and lower stratospheric warming tend to stabilize the atmosphere, which decreases the turbulence and updraft velocities (−10 % in our modeling study). The net effect is an induced cirrus thinning, which may then produce a significant indirect negative radiative forcing (RF). This RF would go in the same direction as the direct effect of solar radiation scattering by aerosols, and would consequently influence the amount of sulfur needed to counteract the positive RF due to greenhouse gases. In our study, given an 8 Tg-SO2 yr−1 equatorial injection into the lower stratosphere, an all-sky net tropopause RF of −1.46 W m−2 is calculated, of which −0.3 W m−2 (20 %) is from the indirect effect on cirrus thinning (6 % reduction in ice optical depth). When surface cooling is ignored, the ice optical depth reduction is lowered to 3 %, with an all-sky net tropopause RF of −1.4 W m−2, of which −0.14 W m−2 (10 %) is from cirrus thinning. Relative to the clear-sky net tropopause RF due to SG aerosols (−2.1 W m−2), the cumulative effect of the background clouds and cirrus thinning accounts for +0.6 W m−2, due to the partial compensation of large positive shortwave (+1.6 W m−2) and negative longwave adjustments (−1.0 W m−2). When surface cooling is ignored, the net cloud adjustment becomes +0.8 W m−2, with the shortwave contribution (+1.5 W m−2) almost twice as much as that of the longwave (−0.7 W m−2). This highlights the importance of including all of the dynamical feedbacks of SG aerosols.


2018 ◽  
Author(s):  
Daniele Visioni ◽  
Giovanni Pitari ◽  
Glauco di Genova

Abstract. Aside from the direct surface cooling sulfate geoengineering (SG) would produce, the investigation on possible side-effects of this method is still ongoing, as for instance on upper tropospheric cirrus cloudiness. Goal of the present study is to better understand the SG thermo-dynamical effects on the homogeneous freezing ice formation process. This is done by comparing SG model simulations against a RCP4.5 reference case: in one case the aerosol-driven surface cooling is included and coupled to the stratospheric warming resulting from aerosol absorption of longwave radiation. In a second SG perturbed case, surface temperatures are kept unchanged with respect to the reference RCP4.5 case. Surface cooling and lower stratospheric warming, together, tend to stabilize the atmosphere, thus decreasing turbulence and water vapor updraft velocities (−10 % in our modeling study). The net effect is an induced cirrus thinning, which may then produce a significant indirect negative radiative forcing (RF). This would go in the same direction as the direct effect of solar radiation scattering by the aerosols, thus influencing the amount of sulfur needed to counteract the positive RF due to greenhouse gases. In our study, given a 8 Tg-SO2 equatorial injection in the lower stratosphere, an all-sky net tropopause RF of −2.13 W/m2 is calculated, of which −0.96 W/m2 (45 %) from the indirect effect on cirrus thinning (7.5 % reduction in ice optical depth). When the surface cooling is ignored, the ice optical depth reduction is lowered to 5 %, with an all-sky net tropopause RF of −1.45 W/m2, of which −0.21 W/m2 (14 %) from cirrus thinning. Relatively to the clear-sky net tropopause RF due to SG aerosols (−2.06 W/m2), the cumulative effect of background clouds and cirrus thinning accounts for −0.07 W/m2, due to close compensation of large positive shortwave (+1.85 W/m2) and negative longwave adjustments (−1.92 W/m2). When the surface cooling is ignored, the net cloud adjustment becomes +0.71 W/m2, with the shortwave contribution (+1.97 W/m2) significantly larger in magnitude than the longwave one (−1.26 W/m2). This highlights the importance of including all dynamical feedbacks of SG aerosols.


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