The local and remote atmospheric impacts of Africa’s 21st century aerosol emission trajectory

Author(s):  
Chris Wells ◽  
Apostolos Voulgarakis

<p>Aerosols are a major climate forcer, but their historical effect has the largest uncertainty of any forcing; their mechanisms and impacts are not well understood. Due to their short lifetime, aerosols have large impacts near their emission region, but they also have effects on the climate in remote locations. In recent years, studies have investigated the influences of regional aerosols on global and regional climate, and the mechanisms that lead to remote responses to their inhomogeneous forcing. Using the Shared Socioeconomic Pathway scenarios (SSPs), transient future experiments were performed in UKESM1, testing the effect of African emissions following the SSP3-RCP7.0 scenario as the rest of the world follows SSP1-RCP1.9, relative to a global SSP1-RCP1.9 control. SSP3 sees higher direct anthropogenic aerosol emissions, but lower biomass burning emissions, over Africa. Experiments were performed changing each of these sets of emissions, and both. A further set of experiments additionally accounted for changing future CO<sub>2</sub> concentrations, to investigate the impact of CO<sub>2</sub> on the responses to aerosol perturbations. Impacts on radiation fluxes, temperature, circulation and precipitation are investigated, both over the emission region (Africa), where microphysical effects dominate, and remotely, where dynamical influences become more relevant. </p>

2021 ◽  
Vol 7 (10) ◽  
pp. eabf7133
Author(s):  
J. C. Fyfe ◽  
V. V. Kharin ◽  
N. Swart ◽  
G. M. Flato ◽  
M. Sigmond ◽  
...  

The COVID-19 (coronavirus disease 2019) pandemic has resulted in a marked slowdown in greenhouse gas and aerosol emissions. Although the resulting emission reductions will continue to evolve, this will presumably be temporary. Here, we provide estimates of the potential effect of such short-term emission reductions on global and regional temperature and precipitation by analyzing the response of an Earth System Model to a range of idealized near-term emission pathways not considered in available model intercomparison projects. These estimates reveal the modest impact that temporary emission reductions associated with the COVID-19 pandemic will have on global and regional climate. Our simulations suggest that the impact of carbon dioxide and aerosol emission reductions is actually a temporary enhancement in warming rate. However, our results demonstrate that even large emission reductions applied for a short duration have only a small and likely undetectable impact.


Atmosphere ◽  
2020 ◽  
Vol 11 (10) ◽  
pp. 1095
Author(s):  
Jeongbyn Seo ◽  
Sungbo Shim ◽  
Sang-Hoon Kwon ◽  
Kyung-On Boo ◽  
Yeon-Hee Kim ◽  
...  

As one of the main drivers for climate change, it is important to understand changes in anthropogenic aerosol emissions and evaluate the climate impact. Anthropogenic aerosols have affected global climate while exerting a much larger influence on regional climate by their short lifetime and heterogeneous spatial distribution. In this study, the effective radiative forcing (ERF), which has been accepted as a useful index for quantifying the effect of climate forcing, was evaluated to understand the effects of aerosol on regional climate over a historical period (1850–2014). Eastern United States (EUS), Western European Union (WEU), and Eastern Central China (ECC), are regions that predominantly emit anthropogenic aerosols and were analyzed using Coupled Model Intercomparison Project 6 (CMIP6) simulations implemented within the framework of the Aerosol Chemistry Model Intercomparison Project (AerChemMIP) in the UK’s Earth System Model (UKESM1). In EUS and WEU, where industrialization occurred relatively earlier, the negative ERF seems to have been recovering in recent decades based on the decreasing trend of aerosol emissions. Conversely, the radiative cooling in ECC seems to be strengthened as aerosol emission continuously increases. These aerosol ERFs have been largely attributed to atmospheric rapid adjustments, driven mainly by aerosol-cloud interactions rather than direct effects of aerosol such as scattering and absorption.


2020 ◽  
Author(s):  
Chris Wells ◽  
Apostolos Voulgarakis ◽  
Matt Kasoar

<p>Aerosols are a major climate forcer, but their historical effect has the largest uncertainty of any forcing, and so their mechanisms and impacts must be better understood. Due to their short lifetime, aerosols have large impacts near their emission region, but they also have effects on the climate in remote locations. In recent years, studies have investigated the influences of regional aerosols on global and regional climate, and the mechanisms that lead to remote responses to their inhomogeneous forcing. However, there has been little work on the influence of emissions from the tropics, as the aforementioned studies typically focused only on northern mid-latitude pollution effects. This work uses the new UK Earth System Model (UKESM1) to investigate the atmospheric composition and climate effects of tropical aerosols and aerosol precursor emissions. We performed three idealised perturbation experiments in which a) tropical SO<sub>2</sub> emissions were multiplied by a factor of 10; b) tropical biomass burning carbonaceous aerosol emissions were multiplied by 10; and c) tropical biomass burning carbonaceous aerosol emissions were entirely removed. Impacts on radiation fluxes, temperature, circulation and precipitation are investigated, both over the emission regions, where microphysical effects dominate, and remotely, where dynamical influences become more relevant. Increasing tropical SO<sub>2</sub> emissions causes a global cooling, and the asymmetric forcing (stronger negative forcing in the Northern Hemisphere Tropics) drives a southward shift of the intertropical convergence zone (ITCZ). The experiment with the large increase in tropical biomass burning organic carbon (OC) and black carbon (BC) features a net warming globally, and a local cooling in locations where the aerosol load increases the most, since OC and BC reduce radiation at the surface locally, causing cooling. However, whereas OC scatters radiation with a negative forcing, BC has a warming effect since it reduces the planetary albedo, and this warming wins out on the global scale. The forcing is asymmetric, but changes sign between seasons as biomass burning in Africa shifts across the Equator, driving a more complex response of the ITCZ. The removal of biomass burning OC and BC leads to opposite effects to the 10x increase, but with a smaller magnitude, and with dynamical changes playing a more important role than microphysical ones, relative to the larger perturbations. Using the Shared Socioeconomic Pathway scenarios (SSPs), transient future experiments have also been performed, testing the effect of Africa following a relatively more polluting route (SSP3-RCP7.0) to the rest of the world (SSP1-RCP1.9), relative to a global SSP1-RCP1.9 control. Preliminary results from this analysis will also be presented.</p>


2020 ◽  
Vol 20 (24) ◽  
pp. 16023-16040
Author(s):  
Kine Onsum Moseid ◽  
Michael Schulz ◽  
Trude Storelvmo ◽  
Ingeborg Rian Julsrud ◽  
Dirk Olivié ◽  
...  

Abstract. Anthropogenic aerosol emissions have increased considerably over the last century, but climate effects and quantification of the emissions are highly uncertain as one goes back in time. This uncertainty is partly due to a lack of observations in the pre-satellite era, making the observations we do have before 1990 additionally valuable. Aerosols suspended in the atmosphere scatter and absorb incoming solar radiation and thereby alter the Earth's surface energy balance. Previous studies show that Earth system models (ESMs) do not adequately represent surface energy fluxes over the historical era. We investigated global and regional aerosol effects over the time period 1961–2014 by looking at surface downwelling shortwave radiation (SDSR). We used observations from ground stations as well as multiple experiments from eight ESMs participating in the Coupled Model Intercomparison Project Version 6 (CMIP6). Our results show that this subset of models reproduces the observed transient SDSR well in Europe but poorly in China. We suggest that this may be attributed to missing emissions of sulfur dioxide in China, sulfur dioxide being a precursor to sulfate, which is a highly reflective aerosol and responsible for more reflective clouds. The emissions of sulfur dioxide used in the models do not show a temporal pattern that could explain observed SDSR evolution over China. The results from various aerosol emission perturbation experiments from DAMIP, RFMIP and AerChemMIP show that only simulations containing anthropogenic aerosol emissions show dimming, even if the dimming is underestimated. Simulated clear-sky and all-sky SDSR do not differ greatly, suggesting that cloud cover changes are not a dominant cause of the biased SDSR evolution in the simulations. Therefore we suggest that the discrepancy between modeled and observed SDSR evolution is partly caused by erroneous aerosol and aerosol precursor emission inventories. This is an important finding as it may help interpret whether ESMs reproduce the historical climate evolution for the right or wrong reason.


2011 ◽  
Vol 11 (3) ◽  
pp. 931-954 ◽  
Author(s):  
Y. Lei ◽  
Q. Zhang ◽  
K. B. He ◽  
D. G. Streets

Abstract. An inventory of anthropogenic primary aerosol emissions in China was developed for 1990–2005 using a technology-based approach. Taking into account changes in the technology penetration within industry sectors and improvements in emission controls driven by stricter emission standards, a dynamic methodology was derived and implemented to estimate inter-annual emission factors. Emission factors of PM2.5 decreased by 7%–69% from 1990 to 2005 in different industry sectors of China, and emission factors of TSP decreased by 18%–80% as well, with the measures of controlling PM emissions implemented. As a result, emissions of PM2.5 and TSP in 2005 were 11.0 Tg and 29.7 Tg, respectively, less than what they would have been without the adoption of these measures. Emissions of PM2.5, PM10 and TSP presented similar trends: they increased in the first six years of 1990s and decreased until 2000, then increased again in the following years. Emissions of TSP peaked (35.5 Tg) in 1996, while the peak of PM10 (18.8 Tg) and PM2.5 (12.7 Tg) emissions occurred in 2005. Although various emission trends were identified across sectors, the cement industry and biofuel combustion in the residential sector were consistently the largest sources of PM2.5 emissions, accounting for 53%–62% of emissions over the study period. The non-metallic mineral product industry, including the cement, lime and brick industries, accounted for 54%–63% of national TSP emissions. There were no significant trends of BC and OC emissions until 2000, but the increase after 2000 brought the peaks of BC (1.51 Tg) and OC (3.19 Tg) emissions in 2005. Although significant improvements in the estimation of primary aerosols are presented here, there still exist large uncertainties. More accurate and detailed activity information and emission factors based on local tests are essential to further improve emission estimates, this especially being so for the brick and coke industries, as well as for coal-burning stoves and biofuel usage in the residential sector.


2020 ◽  
Author(s):  
Kine Onsum Moseid ◽  
Michael Schulz ◽  
Trude Storelvmo ◽  
Ingeborg Rian Julsrud ◽  
Dirk Olivié ◽  
...  

<p>Anthropogenic aerosol emissions have increased considerably over the last century, but climate effects and quantification of the emissions are highly uncertain as one goes back in time. This uncertainty is partly due to a lack of observations in the pre-satellite era, and previous studies show that Earth system models (ESMs) do not adequately represent surface energy fluxes over the historical era. We investigated global and regional aerosol effects over the time period 1961-2014 by looking at surface downwelling shortwave radiation (SDSR).<br>We used observations from ground stations as well as multiple experiments from five ESMs participating in the Coupled Model Intercomparison Project Version 6 (<em>CMIP6</em>). Our results show that this subset of models reproduces the observed transient SDSR well in Europe, but poorly in China. <br>The models do not reproduce the observed trend reversal in SDSR in China in the late 1980s, which is attributed to a change in the emission of SO<sub>2</sub> in this region. The emissions of SO<sub>2</sub> show no sign of a trend reversal that could explain the observed SDSR evolution over China, and neither do other aerosols relevant to SDSR. The results from various aerosol emission perturbation experiments from <em>DAMIP</em>, <em>RFMIP</em> and <em>AerChemMIP</em> suggest that its likely, that aerosol effects are responsible for the dimming signal, although not its full amplitude. Simulated cloud cover changes in the different models are not correlated with observed changes over China.  Therefore we suggest that the discrepancy between modeled and observed SDSR evolution is partly caused by erroneous aerosol and aerosol precursor emission inventories. This is an important finding as it may help interpreting whether ESMs reproduce the historical climate evolution for the right or wrong reason.</p>


2018 ◽  
Vol 31 (20) ◽  
pp. 8381-8399 ◽  
Author(s):  
S. Undorf ◽  
M. A. Bollasina ◽  
G. C. Hegerl

The impact of North American and European (NAEU) anthropogenic aerosol emissions on Eurasian summer climate during the twentieth century is studied using historical single- and all-forcing (including anthropogenic aerosols, greenhouse gases, and natural forcings) simulations from phase 5 of the Coupled Model Intercomparison Project (CMIP5). Intermodel agreement on significant linear trends during a period of increasing NAEU sulfate emissions (1900–74) reveals robust features of NAEU aerosol impact, supported by opposite changes during the subsequent period of decreasing emissions. Regionally, these include a large-scale cooling and associated anticyclonic circulation, as well as a narrowing of the diurnal temperature range (DTR) over Eurasian midlatitudes. Remotely, NAEU aerosols induce a drying over the western African and northern Indian monsoon regions and a strengthening and southward shift of the subtropical jet consistent with the pattern of temperature change. Over Europe, the temporal variations of observed temperature, pressure, and DTR tend to agree better with simulations that include aerosols. Throughout the twentieth century, aerosols are estimated to explain more than a third of the simulated interdecadal forced variability of European near-surface temperature and more than half between 1940 and 1970. These results highlight the substantial aerosol impact on Eurasian climate, already identifiable in the first half of the twentieth century. This may be relevant for understanding future patterns of change related to further emission reductions.


2019 ◽  
Vol 32 (23) ◽  
pp. 8335-8354 ◽  
Author(s):  
Claire Scannell ◽  
Ben B. B. Booth ◽  
Nick J. Dunstone ◽  
David P. Rowell ◽  
Dan J. Bernie ◽  
...  

Abstract Past changes in global industrial aerosol emissions have played a significant role in historical shifts in African rainfall, and yet assessment of the impact on African rainfall of near-term (10–40 yr) potential aerosol emission pathways remains largely unexplored. While existing literature links future aerosol declines to a northward shift of Sahel rainfall, existing climate projections rely on RCP scenarios that do not explore the range of air quality drivers. Here we present projections from two emission scenarios that better envelop the range of potential aerosol emissions. More aggressive emission cuts result in northward shifts of the tropical rainbands whose signal can emerge from expected internal variability on short, 10–20-yr time horizons. We also show for the first time that this northward shift also impacts East Africa, with evidence of delays to both onset and withdrawal of the short rains. However, comparisons of rainfall impacts across models suggest that only certain aspects of both the West and East African model responses may be robust, given model uncertainties. This work motivates the need for wider exploration of air quality scenarios in the climate science community to assess the robustness of these projected changes and to provide evidence to underpin climate adaptation in Africa. In particular, revised estimates of emission impacts of legislated measures every 5–10 years would have a value in providing near-term climate adaptation information for African stakeholders.


2011 ◽  
Vol 8 (2) ◽  
pp. 387-414 ◽  
Author(s):  
N. Mahowald ◽  
K. Lindsay ◽  
D. Rothenberg ◽  
S. C. Doney ◽  
J. K. Moore ◽  
...  

Abstract. Coupled-carbon-climate simulations are an essential tool for predicting the impact of human activity onto the climate and biogeochemistry. Here we incorporate prognostic desert dust and anthropogenic aerosols into the CCSM3.1 coupled carbon-climate model and explore the resulting interactions with climate and biogeochemical dynamics through a series of transient anthropogenic simulations (20th and 21st centuries) and sensitivity studies. The inclusion of prognostic aerosols into this model has a small net global cooling effect on climate but does not significantly impact the globally averaged carbon cycle; we argue that this is likely to be because the CCSM3.1 model has a small climate feedback onto the carbon cycle. We propose a mechanism for including desert dust and anthropogenic aerosols into a simple carbon-climate feedback analysis to explain the results of our and previous studies. Inclusion of aerosols has statistically significant impacts on regional climate and biogeochemistry, in particular through the effects on the ocean nitrogen cycle and primary productivity of altered iron inputs from desert dust deposition.


2020 ◽  
Author(s):  
Laura Wilcox ◽  
Zhen Liu ◽  
Bjørn Samset ◽  
Ed Hawkins ◽  
Marianne Lund ◽  
...  

<div> <div> <div> <p>There is large uncertainty in future aerosol emissions scenarios explored in the Shared Socioeconomic Pathways (SSPs), with plausible pathways spanning a range of possibilities from large global reductions in emissions to 2050 to moderate global increases over the same period. Diversity in emissions across the pathways is particularly large over Asia. CMIP6 models indicate that rapid anthropogenic aerosol and precursor emission reductions between the present day and the 2050s lead to enhanced increases in global and Asian summer monsoon precipitation relative to scenarios with weak air quality policies. However, the effects of aerosol reductions don’t persist in precipitation to the end of the 21st century, when response to greenhouse gases dominates differences across the SSPs. The relative magnitude and spatial distribution of aerosol changes is particularly important for South Asian summer monsoon precipitation changes. Precipitation increases here are initially suppressed in SSPs 2-4.5 and 5-8.5 relative to SSP 1-1.9 and 3-7.0 when the impact of East Asian emission decreases is counteracted by that due to continued increases in South Asian emissions.</p> </div> </div> </div>


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