scholarly journals Quantifying CO emission rates of industrial point sources from TROPOMI observations

2021 ◽  
Author(s):  
Yuan Tian ◽  
Youwen Sun ◽  
Tobias Borsdorff ◽  
Cheng Liu ◽  
Ting Liu ◽  
...  
Keyword(s):  
Point Source ◽  
Emission Inventory ◽  
Point Sources ◽  
Industrial Park ◽  
Emission Rates ◽  
Environment Policy ◽  
Inversion Methods ◽  
First Time ◽  
Co Emission ◽  
Co Observations

Abstract This work demonstrates for the first time the capability of Tropospheric Monitoring Instrument (TROPOMI) routine operations to quantify CO emission rates down to industrial point sources. We have quantified CO emission rates of four industrial point sources in Asia (i.e., Qianlishan industrial park (39.9°N, 106.9°E), Jiuyuan industrial park (40.7°N, 109.7°E) and Botian industrial park (42.2°N, 125.2°E) in China, and Jindal Factory (15.2°N, 76.7°E) in India) with TROPOMI CO observations from 2017 to 2020. The Qianlishan industrial park is a missing source in emission inventory and we quantify it to be ~14.0 kg/s. Our estimates for other three sources vary over 14.4 to 34.3 kg/s, which are within 37–69% of the inventory values. The plume inversion methods are presented in a manner that can be easily used to other fine-scale emission plumes observed from space. Though only a small number of CO plumes per year for any given industrial point source can be observed in conditions suitable for emission rates estimation, there are many industrial point sources can be captured by a good TROPOMI footprint. This work affirms that a constellation of future CO satellites could monitor individual CO point source emissions to support environment policy.

scholarly journals A very high-resolution global fossil fuel CO<sub>2</sub> emission inventory derived using a point source database and satellite observations of nighttime lights, 1980–2007

2010 ◽  
Vol 10 (7) ◽  
pp. 16307-16344 ◽  
Author(s):  
T. Oda ◽  
S. Maksyutov
Keyword(s):  
High Resolution ◽  
Point Source ◽  
Emission Inventory ◽  
Fossil Fuel ◽  
Population Distribution ◽  
Population Based ◽  
Point Sources ◽  
Satellite Observations ◽  
Source Database ◽  
Nighttime Lights

Abstract. Emissions of CO2 from fossil fuel combustion are a critical quantity that must be accurately given in established flux inversion frameworks. Work with emerging satellite-based inversions requires spatiotemporally-detailed inventories that permit analysis of regional sources and sinks. Conventional approaches for disaggregating national emissions beyond the country and city levels based on population distribution have certain difficulties in their application. We developed a global 1 km×1 km fossil fuel CO2 emission inventory for the years 1980–2007 by combining a worldwide point source database and satellite observations of the global nightlight distribution. In addition to estimating the national emissions using global energy consumption statistics, emissions from point sources were estimated separately and were spatially allocated to exact locations indicated by the point source database. Emissions from other sources were distributed using a special nightlight dataset that had fewer saturated pixels compared with regular nightlight datasets. The resulting spatial distributions differed in several ways from those derived using conventional population-based approaches. Because of the inherent characteristics of the nightlight distribution, source regions corresponding to human settlements and land transportation were well articulated. Our distributions showed good agreement with a high-resolution inventory across the US at spatial resolutions that were adequate for regional flux inversions. The inventory will be incorporated into models for operational flux inversions that use observational data from the Japanese Greenhouse Gases Observing SATellite (GOSAT).

scholarly journals An emission inventory of sulfur from anthropogenic sources in Antarctica

2009 ◽  
Vol 9 (10) ◽  
pp. 3397-3408 ◽  
Author(s):  
S. V. Shirsat ◽  
H. F. Graf
Keyword(s):  
Power Generation ◽  
Fuel Consumption ◽  
Emission Inventory ◽  
Anthropogenic Activities ◽  
Chemical Species ◽  
Point Sources ◽  
Anthropogenic Sources ◽  
Emission Rates ◽  
Mobile Source ◽  
Local Pollution

Abstract. This paper presents first results of a comprehensive emission inventory of chemical species from anthropogenic activities (power generation, vehicles, ships and aircraft) in Antarctica, covering the 2004–2005 period. The inventory is based on estimated emission rates of fuel consumption provided by some of the Antarctic research stations. Since the emission sources have different modes of operation and use a variety of fuel, the emission flux rate of chemical species is calculated by multiplying the fuel consumption value with the density of fuel and appropriate emission factors. A separate inventory is prepared for each anthropogenic emission source in Antarctica. Depending on the type of operation, emission rates of SO2, and BC (Black Carbon, from shipping only) have been calculated using the above technique. However, only results of SO2 emissions from each source are presented here. Emission inventory maps of SO2 depicting the track/path taken by each mobile source are shown. The total annual SO2 is 158 Mg from power generation and vehicle operations, 3873 Mg from ships and 56 Mg from aircraft for 2004–2005 and these values undergo strong seasonality following the human activity in Antarctica. Though these figures are small when compared to the emissions at most other regions of the world, they are an indication that human presence in Antarctica leads to at least local pollution. The sources are mainly line and point sources and thus the local pollution potentially is relatively strong.

scholarly journals Optimal emission control and identification of an unknown pollution source

2021 ◽  
Vol 2090 (1) ◽  
pp. 012142
Author(s):  
David Parra-Guevara ◽  
Yuri N. Skiba
Keyword(s):  
Point Source ◽  
Control Strategies ◽  
Adjoint Operator ◽  
Emission Control ◽  
Point Sources ◽  
Diffusion Reaction ◽  
Open Boundary ◽  
Limited Area ◽  
Monitoring Site ◽  
Emission Rates

Abstract The advection-diffusion-reaction equation is used for describing the dispersion of a quasi-passive contaminant from industrial point sources in a limited area. The conditions established on the open boundary ensure that the problem is correct in the sense of Hadamard, that is, its solution exists, is unique, and is stable to initial perturbations. The Lagrange identity is used to construct the adjoint operator and formulate an adjoint problem. Equivalent direct and adjoint estimates are derived to assess the concentration of the pollutant at monitoring sites of the area. Formulas obtained on the basis of adjoint estimates are useful in analysing the sensitivity of the model to both variations in the intensity of pollution sources and variations in the initial distribution of the pollutant concentration in the area. New optimal emission control strategies based on using the adjoint estimates are developed in order to prevent violations of existing sanitary standards by timely reduction of emission rates of operating sources. Optimal control here lies in minimizing these reductions. In addition, this control is primarily aimed at reducing the intensity of emissions from sources that most pollute the monitoring site. Also, new methods are proposed for identifying the main parameters of an unknown point source that arose as a result of a dangerous incident (accident, explosion, etc.). These methods allow determining the location and intensity of a constant or non-stationary point source, as well as the moment of emission of a pollutant in the case of an instantaneous point source. This helps to quickly assess the scale of the incident and its consequences. Numerical results show the effectiveness of the methods.

scholarly journals An emission inventory of sulfur from anthropogenic sources in Antarctica

2009 ◽  
Vol 9 (1) ◽  
pp. 1907-1937 ◽  
Author(s):  
S. V. Shirsat ◽  
H. F. Graf
Keyword(s):  
Power Generation ◽  
Fuel Consumption ◽  
Emission Inventory ◽  
Anthropogenic Activities ◽  
Chemical Species ◽  
Point Sources ◽  
Anthropogenic Sources ◽  
Emission Rates ◽  
Mobile Source ◽  
Local Pollution

Abstract. This paper presents first results of a comprehensive emission inventory of chemical species from anthropogenic activities (power generation, vehicles, ships and aircraft) in Antarctica, covering the 2004–2005 period. The inventory is based on estimated emission rates of fuel consumption provided by some of the Antarctic research stations. Since the emission sources have different modes of operation and use a variety of fuel, the emission flux rate of chemical species is calculated by multiplying the fuel consumption value with the density of fuel and appropriate emission factors. A separate inventory is prepared for each anthropogenic emission source in Antarctica. Depending on the type of operation, emission rates of SO2, and BC (Black Carbon, from shipping only) have been calculated using the above technique. However, only results of SO2 emissions from each source are presented here. Emission inventory maps of SO2 depicting the track/path taken by each mobile source are shown. The total annual SO2 is 158 Mg from power generation and vehicle operations, 3873 Mg from ships and 56 Mg from aircraft for 2004–2005 and these values undergo strong seasonality following the human activity in Antarctica. Though these figures are small when compared to the emissions at most other regions of the world, they are an indication that human presence in Antarctica leads to at least local pollution. The sources are mainly line and point sources and thus the local pollution potentially is relatively strong.

scholarly journals A very high-resolution (1 km×1 km) global fossil fuel CO<sub>2</sub> emission inventory derived using a point source database and satellite observations of nighttime lights

2011 ◽  
Vol 11 (2) ◽  
pp. 543-556 ◽  
Author(s):  
T. Oda ◽  
S. Maksyutov
Keyword(s):  
High Resolution ◽  
Point Source ◽  
Emission Inventory ◽  
Fossil Fuel ◽  
Population Distribution ◽  
Population Based ◽  
Point Sources ◽  
Satellite Observations ◽  
Source Database ◽  
Nighttime Lights

Abstract. Emissions of CO2 from fossil fuel combustion are a critical quantity that must be accurately given in established flux inversion frameworks. Work with emerging satellite-based inversions requires spatiotemporally-detailed inventories that permit analysis of regional natural sources and sinks. Conventional approaches for disaggregating national emissions beyond the country and city levels based on population distribution have certain difficulties in their application. We developed a global 1 km×1 km annual fossil fuel CO2 emission inventory for the years 1980–2007 by combining a worldwide point source database and satellite observations of the global nightlight distribution. In addition to estimating the national emissions using global energy consumption statistics, emissions from point sources were estimated separately and were spatially allocated to exact locations indicated by the point source database. Emissions from other sources were distributed using a special nightlight dataset that had fewer saturated pixels compared with regular nightlight datasets. The resulting spatial distributions differed in several ways from those derived using conventional population-based approaches. Because of the inherent characteristics of the nightlight distribution, source regions corresponding to human settlements and land transportation were well articulated. Our distributions showed good agreement with a high-resolution inventory across the US at spatial resolutions that were adequate for regional flux inversions. The inventory can be extended to the future using updated data, and is expected to be incorporated into models for operational flux inversions that use observational data from the Japanese Greenhouse Gases Observing SATellite (GOSAT).

Sources of Nitrogen and Phosphorus in the Catchment Area of Neusiedlersee/Fertö, Austria/Hungary

1993 ◽  
Vol 28 (3-5) ◽  
pp. 101-110 ◽  
Author(s):  
W. v. d. Emde ◽  
H. Fleckseder ◽  
N. Matsché ◽  
F. Plahl-Wabnegg ◽  
G. Spatzierer ◽  
...  
Keyword(s):  
Point Source ◽  
Catchment Area ◽  
Management Practice ◽  
Water Erosion ◽  
Nonpoint Source ◽  
Point Sources ◽  
Source Control ◽  
Nitrogen And Phosphorus ◽  
Catchment Areas ◽  
The One

Neusiedlersee (in German) / Fertö tó (in Hungarian) is a shallow lake at the Austro-Hungarian border. In the late 1970s, the question arose what to do in order to protect the lake against eutrophication. A preliminary report established the need for point-source control as well as gave first estimates for non-point source inputs. The proposed point-source control was quickly implemented, non-point sources were - among other topics - studied in detail in the period 1982 - 1986. The preliminary work had shown, based on integrated sampling and data from literature, that the aeolic input outweighed the one via water erosion (work was for totP only). In contrast to this, the 1982 - 1986 study showed that (a) water erosion by far dominates over aeolic inputs and (b) the size of nonpoint-source inputs was assessed for the largest catchment area in pronounced detail, whereas additional estimates were undertaken for smaller additional catchment areas. The methods as well as the results are presented in the following. The paper concludes with some remarks on the present management practice of nonpoint-source inputs.

scholarly journals Regional variability in black carbon and carbon monoxide ratio from long-term observations over East Asia: assessment of representativeness for black carbon (BC) and carbon monoxide (CO) emission inventories

2020 ◽  
Vol 20 (1) ◽  
pp. 83-98 ◽  
Author(s):  
Yongjoo Choi ◽  
Yugo Kanaya ◽  
Seung-Myung Park ◽  
Atsushi Matsuki ◽  
Yasuhiro Sadanaga ◽  
...  
Keyword(s):  
Carbon Monoxide ◽  
South Korea ◽  
East Asia ◽  
Black Carbon ◽  
North Korea ◽  
Northeast China ◽  
Emission Inventory ◽  
East China ◽  
Co Emission

Abstract. The black carbon (BC) and carbon monoxide (CO) emission ratios were estimated and compiled from long-term, harmonized observations of the ΔBC∕ΔCO ratios under conditions unaffected by wet deposition at four sites in East Asia, including two sites in South Korea (Baengnyeong and Gosan) and two sites in Japan (Noto and Fukuoka). Extended spatio-temporal coverage enabled estimation of the full seasonality and elucidation of the emission ratio in North Korea for the first time. The estimated ratios were used to validate the Regional Emission inventory in ASia (REAS) version 2.1 based on six study domains (“East China”, “North China”, “Northeast China”, South Korea, North Korea, and Japan). We found that the ΔBC∕ΔCO ratios from four sites converged into a narrow range (6.2–7.9 ng m−3 ppb−1), suggesting consistency in the results from independent observations and similarity in source profiles over the regions. The BC∕CO ratios from the REAS emission inventory (7.7 ng m−3 ppb−1 for East China – 23.2 ng m−3 ppb−1 for South Korea) were overestimated by factors of 1.1 for East China to 3.0 for South Korea, whereas the ratio for North Korea (3.7 ng m−3 ppb−1 from REAS) was underestimated by a factor of 2.0, most likely due to inaccurate emissions from the road transportation sector. Seasonal variation in the BC∕CO ratio from REAS was found to be the highest in winter (China and North Korea) or summer (South Korea and Japan), whereas the measured ΔBC∕ΔCO ratio was the highest in spring in all source regions, indicating the need for further characterization of the seasonality when creating a bottom-up emission inventory. At levels of administrative districts, overestimation in Seoul, the southwestern regions of South Korea, and Northeast China was noticeable, and underestimation was mainly observed in the western regions in North Korea, including Pyongyang. These diagnoses are useful for identifying regions where revisions in the inventory are necessary, providing guidance for the refinement of BC and CO emission rate estimates over East Asia.

scholarly journals TNO-MACC_II emission inventory; a multi-year (2003–2009) consistent high-resolution European emission inventory for air quality modelling

2014 ◽  
Vol 14 (20) ◽  
pp. 10963-10976 ◽  
Author(s):  
J. J. P. Kuenen ◽  
A. J. H. Visschedijk ◽  
M. Jozwicka ◽  
H. A. C. Denier van der Gon
Keyword(s):  
Particulate Matter ◽  
Air Quality ◽  
High Resolution ◽  
Emission Inventory ◽  
Point Sources ◽  
Air Quality Modelling ◽  
Emission Data ◽  
Data Set ◽  
Spatially Distributed ◽  
Reported Data

Abstract. Emissions to air are reported by countries to EMEP. The emissions data are used for country compliance checking with EU emission ceilings and associated emission reductions. The emissions data are also necessary as input for air quality modelling. The quality of these "official" emissions varies across Europe. As alternative to these official emissions, a spatially explicit high-resolution emission inventory (7 × 7 km) for UNECE-Europe for all years between 2003 and 2009 for the main air pollutants was made. The primary goal was to supply air quality modellers with the input they need. The inventory was constructed by using the reported emission national totals by sector where the quality is sufficient. The reported data were analysed by sector in detail, and completed with alternative emission estimates as needed. This resulted in a complete emission inventory for all countries. For particulate matter, for each source emissions have been split in coarse and fine particulate matter, and further disaggregated to EC, OC, SO4, Na and other minerals using fractions based on the literature. Doing this at the most detailed sectoral level in the database implies that a consistent set was obtained across Europe. This allows better comparisons with observational data which can, through feedback, help to further identify uncertain sources and/or support emission inventory improvements for this highly uncertain pollutant. The resulting emission data set was spatially distributed consistently across all countries by using proxy parameters. Point sources were spatially distributed using the specific location of the point source. The spatial distribution for the point sources was made year-specific. The TNO-MACC_II is an update of the TNO-MACC emission data set. Major updates included the time extension towards 2009, use of the latest available reported data (including updates and corrections made until early 2012) and updates in distribution maps.

Water quality modeling in the watershed-based approach for waste load allocations

1998 ◽  
Vol 38 (10) ◽  
pp. 165-172 ◽  
Author(s):  
Ruochuan Gu ◽  
Mei Dong
Keyword(s):  
Water Quality ◽  
Point Source ◽  
Water Quality Modeling ◽  
Point Sources ◽  
Low Flow ◽  
Quality Analysis ◽  
Management Approach ◽  
Water Quality Control ◽  
Quality Modeling ◽  
Waste Load

The conventional method for waste load allocations (WLA) employs spatial-differentiation, considering individual point sources, and temporal-integration, using a constant flow, typically 7Q10 low flow. This paper presents a watershed-based seasonal management approach, in which non-point source as well as point sources are incorporated, seasonal design flows are used for water quality analysis, and WLA are performend in a watershed scale. The strategy for surface water quality modeling in the watershed-based approach is described. The concept of seasonal discharge management is discussed and suggested for the watershed-based approach. A case study using the method for the Des Moines River, Iowa, USA is conducted. Modeling considerations and procedure are presented. The significance of non-point source pollutant load and its impact on water quality of the river is evaluated by analyzing field data. A water quality model is selected and validated against field measurements. The model is applied to projections of future water quality situations under different watershed management and water quality control scenarios with respect to river flow and pollutant loading rate.

scholarly journals Presence of Pathogens and Indicator Microbes at a Non-Point Source Subtropical Recreational Marine Beach

2009 ◽  
Vol 76 (3) ◽  
pp. 724-732 ◽  
Author(s):  
Amir M. Abdelzaher ◽  
Mary E. Wright ◽  
Cristina Ortega ◽  
Helena M. Solo-Gabriele ◽  
Gary Miller ◽  
...  
Keyword(s):  
Point Source ◽  
High Tide ◽  
South Florida ◽  
Point Sources ◽  
Fecal Coliforms ◽  
Health Concern ◽  
Ocean Water ◽  
Solar Insolation ◽  
Sources Of Pollution ◽  
Water Detection

ABSTRACT Swimming in ocean water, including ocean water at beaches not impacted by known point sources of pollution, is an increasing health concern. This study was an initial evaluation of the presence of indicator microbes and pathogens and the association among the indicator microbes, pathogens, and environmental conditions at a subtropical, recreational marine beach in south Florida impacted by non-point sources of pollution. Twelve water and eight sand samples were collected during four sampling events at high or low tide under elevated or reduced solar insolation conditions. The analyses performed included analyses of fecal indicator bacteria (FIB) (fecal coliforms, Escherichia coli, enterococci, and Clostridium perfringens), human-associated microbial source tracking (MST) markers (human polyomaviruses [HPyVs] and Enterococcus faecium esp gene), and pathogens (Vibrio vulnificus, Staphylococcus aureus, enterovirus, norovirus, hepatitis A virus, Cryptosporidium spp., and Giardia spp.). The enterococcus concentrations in water and sand determined by quantitative PCR were greater than the concentrations determined by membrane filtration measurement. The FIB concentrations in water were below the recreational water quality standards for three of the four sampling events, when pathogens and MST markers were also generally undetectable. The FIB levels exceeded regulatory guidelines during one event, and this was accompanied by detection of HPyVs and pathogens, including detection of the autochthonous bacterium V. vulnificus in sand and water, detection of the allochthonous protozoans Giardia spp. in water, and detection of Cryptosporidium spp. in sand samples. The elevated microbial levels were detected at high tide and under low-solar-insolation conditions. Additional sampling should be conducted to further explore the relationships between tidal and solar insolation conditions and between indicator microbes and pathogens in subtropical recreational marine waters impacted by non-point source pollution.

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