Aerosol Properties and Processes: A Path from Field and Laboratory Measurements to Global Climate Models

2007 ◽  
Vol 88 (7) ◽  
pp. 1059-1084 ◽  
Author(s):  
Steven J. Ghan ◽  
Stephen E. Schwartz

Aerosol particles in the lower atmosphere exert a substantial influence on climate and climate change through a variety of complex mechanisms. Consequently, there is a need to represent these influences in global climate models, and models have begun to include representations of these influences. However, the present treatment of aerosols in global climate models is highly simplified, omitting many processes and feedbacks that are thought to be climatically important. Thus, there is need for substantial improvement. Here we describe the strategy of the U.S. Department of Energy for improving representation of the properties, processes, and effects of tropospheric aerosols in global climate models. The strategy begins with a foundation of field and laboratory measurements that provide the basis for modules describing specific aerosol properties and processes. These modules are then integrated into regional aerosol models, which are evaluated by comparison with field measurements. Issues of scale are then addressed so that the modules can be applied to global aerosol models, which are evaluated by comparison with satellite retrievals and other observations. Finally, the validated set of modules is applied in global climate models for multicentury simulations. This strategy is expected to be applied to successive generations of global climate models.

2017 ◽  
Vol 17 (7) ◽  
pp. 4451-4475 ◽  
Author(s):  
Ilissa B. Ocko ◽  
Paul A. Ginoux

Abstract. Anthropogenic aerosols are a key factor governing Earth's climate and play a central role in human-caused climate change. However, because of aerosols' complex physical, optical, and dynamical properties, aerosols are one of the most uncertain aspects of climate modeling. Fortunately, aerosol measurement networks over the past few decades have led to the establishment of long-term observations for numerous locations worldwide. Further, the availability of datasets from several different measurement techniques (such as ground-based and satellite instruments) can help scientists increasingly improve modeling efforts. This study explores the value of evaluating several model-simulated aerosol properties with data from spatially collocated instruments. We compare aerosol optical depth (AOD; total, scattering, and absorption), single-scattering albedo (SSA), Ångström exponent (α), and extinction vertical profiles in two prominent global climate models (Geophysical Fluid Dynamics Laboratory, GFDL, CM2.1 and CM3) to seasonal observations from collocated instruments (AErosol RObotic NETwork, AERONET, and Cloud–Aerosol Lidar with Orthogonal Polarization, CALIOP) at seven polluted and biomass burning regions worldwide. We find that a multi-parameter evaluation provides key insights on model biases, data from collocated instruments can reveal underlying aerosol-governing physics, column properties wash out important vertical distinctions, and improved models does not mean all aspects are improved. We conclude that it is important to make use of all available data (parameters and instruments) when evaluating aerosol properties derived by models.


Hadmérnök ◽  
2019 ◽  
Vol 14 (1) ◽  
pp. 99-107
Author(s):  
László Földi ◽  
László Halász

Defining the term of climate, we investigate the role of natural causes and effects of human activities in climate change. The temperature of the Earth is determined by the balance between the amount of radiation energy received from the Sun and that emitted from the surface of the Earth towards the outer space. Greenhouse gases in the atmosphere, including water vapor, carbon dioxide, methane and nitrous oxides, act to make the surface much warmer, because they absorb and emit heat energy in all directions (including downwards), keeping Earth’s surface and lower atmosphere warm. The primary cause of climate change is the burning of fossil fuels, such as oil and coal, which emits greenhouse gases into the atmosphere – primarily carbon dioxide. We give a review about the activity of the Intergovernmental Panel on Climate Change and the United Nations Climate Change Conferences. Shortly investigate the different global climate models and some regional climate models. Finally discuss the results of regional climate model simulations for the Carpathian Basin.


2016 ◽  
Author(s):  
Ilissa B. Ocko ◽  
Paul A. Ginoux

Abstract. Anthropogenic aerosols are a key factor governing Earth’s climate, and play a central role in human-caused climate change. However, because of aerosols’ complex physical, optical, and dynamical properties, aerosols are one of the most uncertain aspects of climate modeling. Fortunately, aerosol measurement networks over the past few decades have led to the establishment of long-term observations for numerous locations worldwide. Further, the availability of datasets from several different measurement techniques (such as ground-based and satellite instruments) can help scientists increasingly improve modeling efforts. This study explores the value of evaluating several model-simulated aerosol properties with data from collocated instruments. We compare optical depth (total, scattering, and absorption), single scattering albedo, Ångström exponent, and extinction vertical profiles in two prominent global climate models to seasonal observations from collocated instruments (AERONET and CALIOP) at seven polluted and biomass burning regions worldwide. We find that models may accurately reproduce one variable while totally failing at another; data from collocated instruments can reveal underlying aerosol-governing physics; column properties may wash out important vertical distinctions; and "improved" models does not mean all aspects are improved. We conclude that it is important to make use of all available data (parameters and instruments) when evaluating aerosol properties derived by models.


2019 ◽  
Author(s):  
Matthieu Riva ◽  
Yuzhi Chen ◽  
Zhang, Yue ◽  
Ziying Lei ◽  
Nicole Olson ◽  
...  

<div>Acid-driven multiphase chemistry of isoprene epoxydiols (IEPOX), a key isoprene oxidation product, with inorganic sulfate aerosol yields substantial amounts of secondary organic aerosol (SOA) through the formation of organosulfur. The extent and implications of inorganic-to-organic sulfate conversion, however, are unknown. Herein, we reveal that extensive consumption of inorganic sulfate occurs, which increases with the IEPOX-to-inorganic sulfate ratio (IEPOX:Sulf<sub>inorg</sub>), as determined by laboratory and field measurements. We further demonstrate that organosulfur greatly modifies critical aerosol properties, such as acidity, morphology, viscosity, and phase state. These new mechanistic insights reveal that changes in SO<sub>2</sub> emissions, especially in isoprene-dominated environments, will significantly alter biogenic SOA physicochemical properties. Consequently, IEPOX:Sulf<sub>inorg</sub> will play a central role in understanding historical climate and determining future impacts of biogenic SOA on global climate and air quality.</div>


2011 ◽  
Author(s):  
Enrico Scoccimarro ◽  
Silvio Gualdi ◽  
Antonella Sanna ◽  
Edoardo Bucchignani ◽  
Myriam Montesarchio

2021 ◽  
Vol 4 (1) ◽  
Author(s):  
Mateusz Taszarek ◽  
John T. Allen ◽  
Mattia Marchio ◽  
Harold E. Brooks

AbstractGlobally, thunderstorms are responsible for a significant fraction of rainfall, and in the mid-latitudes often produce extreme weather, including large hail, tornadoes and damaging winds. Despite this importance, how the global frequency of thunderstorms and their accompanying hazards has changed over the past 4 decades remains unclear. Large-scale diagnostics applied to global climate models have suggested that the frequency of thunderstorms and their intensity is likely to increase in the future. Here, we show that according to ERA5 convective available potential energy (CAPE) and convective precipitation (CP) have decreased over the tropics and subtropics with simultaneous increases in 0–6 km wind shear (BS06). Conversely, rawinsonde observations paint a different picture across the mid-latitudes with increasing CAPE and significant decreases to BS06. Differing trends and disagreement between ERA5 and rawinsondes observed over some regions suggest that results should be interpreted with caution, especially for CAPE and CP across tropics where uncertainty is the highest and reliable long-term rawinsonde observations are missing.


2021 ◽  
Vol 11 (1) ◽  
Author(s):  
Lennart Quante ◽  
Sven N. Willner ◽  
Robin Middelanis ◽  
Anders Levermann

AbstractDue to climate change the frequency and character of precipitation are changing as the hydrological cycle intensifies. With regards to snowfall, global warming has two opposing influences; increasing humidity enables intense snowfall, whereas higher temperatures decrease the likelihood of snowfall. Here we show an intensification of extreme snowfall across large areas of the Northern Hemisphere under future warming. This is robust across an ensemble of global climate models when they are bias-corrected with observational data. While mean daily snowfall decreases, both the 99th and the 99.9th percentiles of daily snowfall increase in many regions in the next decades, especially for Northern America and Asia. Additionally, the average intensity of snowfall events exceeding these percentiles as experienced historically increases in many regions. This is likely to pose a challenge to municipalities in mid to high latitudes. Overall, extreme snowfall events are likely to become an increasingly important impact of climate change in the next decades, even if they will become rarer, but not necessarily less intense, in the second half of the century.


Water ◽  
2021 ◽  
Vol 13 (13) ◽  
pp. 1819
Author(s):  
Eleni S. Bekri ◽  
Polychronis Economou ◽  
Panayotis C. Yannopoulos ◽  
Alexander C. Demetracopoulos

Freshwater resources are limited and seasonally and spatially unevenly distributed. Thus, in water resources management plans, storage reservoirs play a vital role in safeguarding drinking, irrigation, hydropower and livestock water supply. In the last decades, the dams’ negative effects, such as fragmentation of water flow and sediment transport, are considered in decision-making, for achieving an optimal balance between human needs and healthy riverine and coastal ecosystems. Currently, operation of existing reservoirs is challenged by increasing water demand, climate change effects and active storage reduction due to sediment deposition, jeopardizing their supply capacity. This paper proposes a methodological framework to reassess supply capacity and management resilience for an existing reservoir under these challenges. Future projections are derived by plausible climate scenarios and global climate models and by stochastic simulation of historic data. An alternative basic reservoir management scenario with a very low exceedance probability is derived. Excess water volumes are investigated under a probabilistic prism for enabling multiple-purpose water demands. Finally, this method is showcased to the Ladhon Reservoir (Greece). The probable total benefit from water allocated to the various water uses is estimated to assist decision makers in examining the tradeoffs between the probable additional benefit and risk of exceedance.


2021 ◽  
Vol 12 (1) ◽  
Author(s):  
Jun Yang ◽  
Maigeng Zhou ◽  
Zhoupeng Ren ◽  
Mengmeng Li ◽  
Boguang Wang ◽  
...  

AbstractRecent studies have reported a variety of health consequences of climate change. However, the vulnerability of individuals and cities to climate change remains to be evaluated. We project the excess cause-, age-, region-, and education-specific mortality attributable to future high temperatures in 161 Chinese districts/counties using 28 global climate models (GCMs) under two representative concentration pathways (RCPs). To assess the influence of population ageing on the projection of future heat-related mortality, we further project the age-specific effect estimates under five shared socioeconomic pathways (SSPs). Heat-related excess mortality is projected to increase from 1.9% (95% eCI: 0.2–3.3%) in the 2010s to 2.4% (0.4–4.1%) in the 2030 s and 5.5% (0.5–9.9%) in the 2090 s under RCP8.5, with corresponding relative changes of 0.5% (0.0–1.2%) and 3.6% (−0.5–7.5%). The projected slopes are steeper in southern, eastern, central and northern China. People with cardiorespiratory diseases, females, the elderly and those with low educational attainment could be more affected. Population ageing amplifies future heat-related excess deaths 2.3- to 5.8-fold under different SSPs, particularly for the northeast region. Our findings can help guide public health responses to ameliorate the risk of climate change.


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