scholarly journals Structure Function Analysis of Water Vapor Simulated with a Convection-Permitting Model and Comparison to Airborne Lidar Observations

2017 ◽  
Vol 74 (4) ◽  
pp. 1201-1210
Author(s):  
Tobias Selz ◽  
Lucas Fischer ◽  
George C. Craig

Abstract The spatial scale dependence of midlatitude water vapor variability in the high-resolution limited-area model COSMO is evaluated using diagnostics of scaling behavior. Past analysis of airborne lidar measurements showed that structure function scaling exponents depend on the corresponding airmass characteristics, and that a classification of the troposphere into convective and nonconvective layers led to significantly different power-law behaviors for each of these two regimes. In particular, scaling properties in the convective air mass were characterized by rough and highly intermittent data series, whereas the nonconvective regime was dominated by smoother structures with weaker small-scale variability. This study finds similar results in a model simulation with an even more pronounced distinction between the two air masses. Quantitative scaling diagnostics agree well with measurements in the nonconvective air mass, whereas in the convective air mass the simulation shows a much higher intermittency. Sensitivity analyses were performed using the model data to assess the impact of limitations of the observational dataset, which indicate that analyses of lidar data most likely underestimated the intermittency in convective air masses due to the small samples from single flight tracks, which led to a bias when data with poor fits were rejected. Though the quantitative estimation of intermittency remains uncertain for convective air masses, the ability of the model to capture the dominant weather regime dependence of water vapor scaling properties is encouraging.

2018 ◽  
Vol 18 (4) ◽  
pp. 2973-2983 ◽  
Author(s):  
Christian Rolf ◽  
Bärbel Vogel ◽  
Peter Hoor ◽  
Armin Afchine ◽  
Gebhard Günther ◽  
...  

Abstract. The impact of air masses originating in Asia and influenced by the Asian monsoon anticyclone on the Northern Hemisphere stratosphere is investigated based on in situ measurements. A statistically significant increase in water vapor (H2O) of about 0.5 ppmv (11 %) and methane (CH4) of up to 20 ppbv (1.2 %) in the extratropical stratosphere above a potential temperature of 380 K was detected between August and September 2012 during the HALO aircraft missions Transport and Composition in the UT/LMS (TACTS) and Earth System Model Validation (ESMVal). We investigate the origin of the increased water vapor and methane using the three-dimensional Chemical Lagrangian Model of the Stratosphere (CLaMS). We assign the source of the moist air masses in the Asian region (northern and southern India, eastern China, southeast Asia, and the tropical Pacific) based on tracers of air mass origin used in CLaMS. The water vapor increase is correlated with an increase of the simulated Asian monsoon air mass contribution from about 10 % in August to about 20 % in September, which corresponds to a doubling of the influence from the Asian monsoon region. Additionally, back trajectories starting at the aircraft flight paths are used to differentiate transport from the Asian monsoon anticyclone and other source regions by calculating the Lagrangian cold point (LCP). The geographic location of the LCPs, which indicates the region where the set point of water vapor mixing ratio along these trajectories occurs, can be predominantly attributed to the Asian monsoon region.


Időjárás ◽  
2021 ◽  
Vol 125 (4) ◽  
pp. 571-607
Author(s):  
André Simon ◽  
Martin Belluš ◽  
Katarína Čatlošová ◽  
Mária Derková ◽  
Martin Dian ◽  
...  

The paper presented is dedicated to the evaluation of the influence of various improvements to the numerical weather prediction (NWP) systems exploited at the Slovak Hydrometeorological Institute (SHMÚ). The impact was illustrated in a case study with multicell thunderstorms and the results were confronted with the reference analyses from the INCA nowcasting system, regional radar reflectivity data, and METEOSAT satellite imagery. The convective cells evolution was diagnosed in non-hydrostatic dynamics experiments to study weak mesoscale vortices and updrafts. The growth of simulated clouds and evolution of the temperature at their top were compared with the brightness temperature analyzed from satellite imagery. The results obtained indicated the potential for modeling and diagnostics of small-scale structures within the convective cloudiness, which could be related to severe weather. Furthermore, the non-hydrostatic dynamics experiments related to the stability and performance improvement of the time scheme led to the formulation of a new approach to linear operator definition for semi-implicit scheme (in text referred as NHHY). We demonstrate that the execution efficiency has improved by more than 20%. The exploitation of several high resolution measurement types in data assimilation contributed to more precise position of predicted patterns and precipitation representation in the case study. The non-hydrostatic dynamics provided more detailed structures. On the other hand, the potential of a single deterministic forecast of prefrontal heavy precipitation was not as high as provided by the ensemble system. The prediction of a regional ensemble system A-LAEF (ALARO Limited Area Ensemble Forecast) enhanced the localization of precipitation patterns. Though, this was rather due to the simulation of uncertainty in the initial conditions and also because of the stochastic perturbation of physics tendencies. The various physical parameterization setups of A-LAEF members did not exhibit a systematic effect on precipitation forecast in the evaluated case. Moreover, the ensemble system allowed an estimation of uncertainty in a rapidly developing severe weather case, which was high even at very short range.


2013 ◽  
Vol 13 (4) ◽  
pp. 10157-10192 ◽  
Author(s):  
E. L. Yates ◽  
L. T. Iraci ◽  
M. C. Roby ◽  
R. B. Pierce ◽  
M. S. Johnson ◽  
...  

Abstract. Stratosphere-to-troposphere transport (STT) results in air masses of stratospheric origin intruding into the free troposphere. Once in the free troposphere, O3-rich stratospheric air can be transported and mixed with tropospheric air masses, contributing to the tropospheric O3 budget. Evidence of STT can be identified based on the differences in the trace gas composition of the two regions. Because ozone (O3) is present in such large quantities in the stratosphere compared to the troposphere, it is frequently used as a tracer for STT events. This work reports on airborne in situ measurements of O3 and other trace gases during two STT events observed over California, USA. The first, on 14 May 2012, was associated with a cut-off low, and the second, on 5 June 2012, occurred during a post-trough, building ridge event. In each STT event, airborne measurements identified high O3 within a stratospheric intrusion which was observed as low as 3 km above sea level. During both events the stratospheric air mass was characterized by elevated O3 mixing ratios and reduced carbon dioxide (CO2) and water vapor. The reproducible observation of reduced CO2 within the stratospheric air mass supports the use of non-conventional tracers as an additional method for detecting STT. A detailed meteorological analysis of each STT event is presented and observations are interpreted with the Realtime Air Quality Modeling System (RAQMS). The implications of the two STT events are discussed in terms of the impact on the total tropospheric O3 budget and the impact on air quality and policy-making.


2015 ◽  
Vol 15 (2) ◽  
pp. 1703-1746 ◽  
Author(s):  
H. Delattre ◽  
C. Vallet-Coulomb ◽  
C. Sonzogni

Abstract. Stable isotopes of the water vapor represent a powerful tool for tracing atmospheric vapor origin and mixing processes. Laser spectrometry recently allowed high time resolution measurements, but despite an increasing number of experimental studies, there is still a need for a better understanding of the main drivers of isotopic signal variability at different time scales. We present results of in situ measurements of δ18O and δD during 36 consecutive days in summer 2011 in atmospheric vapor of a Mediterranean coastal wetland exposed to high evapotranspiration (Camargue, Rhône River delta, France). A calibration protocol was tested and instrument stability was analysed over the period. The mean composition of atmospheric vapor during the campaign is δ18O = −14.66‰ and δD = −95.4‰, with δv data plotting clearly above the local meteoric water line, and an average deuterium excess (dv) of 21.9‰. At daily time step, we show a clear separation of isotopic characteristics with respect to the air mass back trajectories, with the Northern air masses providing depleted compositions (δ18O = −15.83‰, δD = −103.5‰) compared to Mediterranean air masses (δ18O = −13.13‰, δD = −86.5‰). There is also a clear separation between dv corresponding to these different air mass origins, but not in the same direction as was previously evidenced from regional rainfall data, with higher dv found for Northern air masses (23.2‰) than for Mediterranean air masses (18.6‰). Based on twenty-four average hourly data, we propose a depiction of typical daily evolution of water vapor isotopic composition. High diurnal variations in dv is attributed to a dominant control of evapotranspiration, over entrainment of free atmosphere. Daily cycles in dv are more pronounced for Mediterranean than for North Atlantic air mass origin and are discussed in terms of local evapotranspiration versus regional signatures. We calculate the composition of the vapor source that produces the day-time increase in dv for the different air mass origins, and propose an atmospheric water and isotopic mass balance.


Atmosphere ◽  
2019 ◽  
Vol 10 (9) ◽  
pp. 537 ◽  
Author(s):  
Fanni Dóra Kelemen ◽  
Cristina Primo ◽  
Hendrik Feldmann ◽  
Bodo Ahrens

A twentieth century-long coupled atmosphere-ocean regional climate simulation with COSMO-CLM (Consortium for Small-Scale Modeling, Climate Limited-area Model) and NEMO (Nucleus for European Modelling of the Ocean) is studied here to evaluate the added value of coupled marginal seas over continental regions. The interactive coupling of the marginal seas, namely the Mediterranean, the North and the Baltic Seas, to the atmosphere in the European region gives a comprehensive modelling system. It is expected to be able to describe the climatological features of this geographically complex area even more precisely than an atmosphere-only climate model. The investigated variables are precipitation and 2 m temperature. Sensitivity studies are used to assess the impact of SST (sea surface temperature) changes over land areas. The different SST values affect the continental precipitation more than the 2 m temperature. The simulated variables are compared to the CRU (Climatic Research Unit) observational data, and also to the HOAPS/GPCC (Hamburg Ocean Atmosphere Parameters and Fluxes from Satellite Data, Global Precipitation Climatology Centre) data. In the coupled simulation, added skill is found primarily during winter over the eastern part of Europe. Our analysis shows that, over this region, the coupled system is dryer than the uncoupled system, both in terms of precipitation and soil moisture, which means a decrease in the bias of the system. Thus, the coupling improves the simulation of precipitation over the eastern part of Europe, due to cooler SST values and in consequence, drier soil.


2013 ◽  
Vol 13 (24) ◽  
pp. 12451-12467 ◽  
Author(s):  
S. J. O'Shea ◽  
G. Allen ◽  
M. W. Gallagher ◽  
S. J.-B. Bauguitte ◽  
S. M. Illingworth ◽  
...  

Abstract. In situ airborne measurements were made over eastern Canada in summer 2011 as part of the BORTAS experiment (Quantifying the impact of BOReal forest fires on Tropospheric oxidants over the Atlantic using Aircraft and Satellites). In this paper we present observations of greenhouse gases (CO2 and CH4) and other biomass burning tracers (CO, HCN and CH3CN), both climatologically and through case studies, as recorded on board the FAAM BAe-146 research aircraft. Vertical profiles of CO2 were generally characterised by depleted boundary layer concentrations relative to the free troposphere, consistent with terrestrial biospheric uptake. In contrast, CH4 concentrations were found to rise with decreasing altitude due to strong local and regional surface sources. BORTAS observations were found to be broadly comparable with both previous measurements in the region during the regional burning season and with reanalysed composition fields from the EU Monitoring Atmospheric Composition and Change (MACC) project. We use coincident tracer–tracer correlations and a Lagrangian trajectory model to characterise and differentiate air mass history of intercepted plumes. In particular, CO, HCN and CH3CN were used to identify air masses that have been recently influenced by biomass burning. Examining individual cases we were able to quantify emissions from biomass burning. Using both near-field (< 1 day) and far-field (> 1 day) sampling, boreal forest fire plumes were identified throughout the troposphere. Fresh plumes from fires in northwestern Ontario yield emission factors for CH4 and CO2 of 8.5 ± 0.9 g (kg dry matter)−1 and 1512 ± 185 g (kg dry matter)−1, respectively. We have also investigated the efficacy of calculating emission factors from far-field sampling, in which there might be expected to be limited mixing with background and other characteristic air masses, and we provide guidance on best practice and limitations in such analysis. We have found that for measurements within plumes that originated from fires in northwestern Ontario 2–4 days upwind, emission factors can be calculated that range between 1618 ± 216 and 1702 ± 173 g (kg dry matter)−1 for CO2 and 1.8 ± 0.2 and 6.1 ± 1 g (kg dry matter)−1 for CH4.


2012 ◽  
Vol 12 (8) ◽  
pp. 3761-3782 ◽  
Author(s):  
J.-M. Diesch ◽  
F. Drewnick ◽  
S. R. Zorn ◽  
S.-L. von der Weiden-Reinmüller ◽  
M. Martinez ◽  
...  

Abstract. Measurements of the ambient aerosol were performed at the Southern coast of Spain, within the framework of the DOMINO (Diel Oxidant Mechanisms In relation to Nitrogen Oxides) project. The field campaign took place from 20 November until 9 December 2008 at the atmospheric research station "El Arenosillo" (37°5'47.76" N, 6°44'6.94" W). As the monitoring station is located at the interface between a natural park, industrial cities (Huelva, Seville) and the Atlantic Ocean, a variety of physical and chemical parameters of aerosols and gas phase could be characterized in dependency on the origin of air masses. Backwards trajectories were examined and compared with local meteorology to classify characteristic air mass types for several source regions. Aerosol number and mass as well as polycyclic aromatic hydrocarbons and black carbon concentrations were measured in PM1 and size distributions were registered covering a size range from 7 nm up to 32 μm. The chemical composition of the non-refractory submicron aerosol (NR-PM1) was measured by means of an Aerosol Mass Spectrometer (Aerodyne HR-ToF-AMS). Gas phase analyzers monitored various trace gases (O3, SO2, NO, NO2, CO2) and a weather station provided meteorological parameters. Lowest average submicron particle mass and number concentrations were found in air masses arriving from the Atlantic Ocean with values around 2 μg m−3 and 1000 cm−3. These mass concentrations were about two to four times lower than the values recorded in air masses of continental and urban origins. For some species PM1-fractions in marine air were significantly larger than in air masses originating from Huelva, a closely located city with extensive industrial activities. The largest fraction of sulfate (54%) was detected in marine air masses and was to a high degree not neutralized. In addition, small concentrations of methanesulfonic acid (MSA), a product of biogenic dimethyl sulfate (DMS) emissions, could be identified in the particle phase. In all air masses passing the continent the organic aerosol fraction dominated the total NR-PM1. For this reason, using Positive Matrix Factorization (PMF) four organic aerosol (OA) classes that can be associated with various aerosol sources and components were identified: a highly-oxygenated OA is the major component (43% OA) while semi-volatile OA accounts for 23%. A hydrocarbon-like OA mainly resulting from industries, traffic and shipping emissions as well as particles from wood burning emissions also contribute to total OA and depend on the air mass origin. A significant variability of ozone was observed that depends on the impact of different air mass types and solar radiation.


2021 ◽  
Vol 14 (4) ◽  
pp. 2827-2840
Author(s):  
David R. Thompson ◽  
Brian H. Kahn ◽  
Philip G. Brodrick ◽  
Matthew D. Lebsock ◽  
Mark Richardson ◽  
...  

Abstract. The subgrid spatial variability of water vapor is an important geophysical parameter for modeling tropical convention and cloud processes in atmospheric models. This study maps sub-kilometer spatial structures in total atmospheric column water vapor with visible to shortwave infrared (VSWIR) imaging spectroscopy. We describe our inversion approach and validate its accuracy with coincident measurements by airborne imaging spectrometers and the AERONET ground-based observation network. Next, data from NASA's AVIRIS-NG spectrometer enable the highest-resolution measurement to date of water vapor's spatial variability and scaling properties. We find second-order structure function scaling exponents consistent with prior studies of convective atmospheres. Airborne lidar data show that this total column measurement provides information about variability in the lower troposphere. We conclude by discussing the implications of these measurements and paths toward future campaigns to build upon these results.


Author(s):  
I. McRae ◽  
L. Zheng ◽  
S. Bourke ◽  
N. Cherbuin ◽  
K.J. Anstey

Background: Assessment of cost-effectiveness of interventions to address modifiable risk factors associated with dementia requires estimates of long-term impacts of these interventions which are rarely directly available and must be estimated using a range of assumptions. OBJECTIVES: To test the cost-effectiveness of dementia prevention measures using a methodology which transparently addresses the many assumptions required to use data from short-term studies, and which readily incorporates sensitivity analyses. DESIGN: We explore an approach to estimating cost-effective prices which uses aggregate data including estimated lifetime costs of dementia, both financial and quality of life, and incorporates a range of assumptions regarding sustainability of short- term gains and other parameters. SETTING: The approach is addressed in the context of the theoretical reduction in a range of risk factors, and in the context of a specific small-scale trial of an internet-based intervention augmented with diet and physical activity consultations. MEASUREMENTS: The principal outcomes were prices per unit of interventions at which interventions were cost-effective or cost-saving. RESULTS: Taking a societal perspective, a notional intervention reducing a range of dementia risk-factors by 5% was cost-effective at $A460 per person with higher risk groups at $2,148 per person. The on-line program costing $825 per person was cost-effective at $1,850 per person even if program effect diminished by 75% over time. CONCLUSIONS: Interventions to address risk factors for dementia are likely to be cost-effective if appropriately designed, but confirmation of this conclusion requires longer term follow-up of trials to measure the impact and sustainability of short-term gains.


2011 ◽  
Vol 4 (3) ◽  
pp. 2469-2544 ◽  
Author(s):  
T. A. M. Pugh ◽  
M. Cain ◽  
J. Methven ◽  
O. Wild ◽  
S. R. Arnold ◽  
...  

Abstract. A Lagrangian model of photochemistry and mixing is described (CiTTyCAT, stemming from the Cambridge Tropospheric Trajectory model of Chemistry And Transport), which is suitable for transport and chemistry studies throughout the troposphere. Over the last five years, the model has been developed in parallel at several different institutions and here those developments have been incorporated into one "community" model and documented for the first time. The key photochemical developments include a new scheme for biogenic volatile organic compounds and updated emissions schemes. The key physical development is to evolve composition following an ensemble of trajectories within neighbouring air-masses, including a simple scheme for mixing between them via an evolving "background profile", both within the boundary layer and free troposphere. The model runs along trajectories pre-calculated using winds and temperature from meteorological analyses. In addition, boundary layer height and precipitation rates, output from the analysis model, are interpolated to trajectory points and used as inputs to the mixing and wet deposition schemes. The model is most suitable in regimes when the effects of small-scale turbulent mixing are slow relative to advection by the resolved winds so that coherent air-masses form with distinct composition and strong gradients between them. Such air-masses can persist for many days while stretching, folding and thinning. Lagrangian models offer a useful framework for picking apart the processes of air-mass evolution over inter-continental distances, without being hindered by the numerical diffusion inherent to global Eulerian models. The model, including different box and trajectory modes, is described and some output for each of the modes is presented for evaluation. The model is available for download from a Subversion-controlled repository by contacting the corresponding authors.


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