Aerosol influences on radiative heating rates in the Asian tropopause aerosol layer

2021 ◽  
Author(s):  
Jie Gao ◽  
Jonathon Wright
Keyword(s):  
Radiative Transfer ◽  
Radiative Forcing ◽  
Asian Monsoon ◽  
Volcanic Eruptions ◽  
Radiative Heating ◽  
Spatiotemporal Variability ◽  
Radiation Budget ◽  
Aerosol Layer ◽  
Heating Rates ◽  
Aerosol Analysis

<p>The Asian Tropopause Aerosol Layer (ATAL) has emerged over recent decades to play an increasingly prominent role in the upper troposphere and lower stratosphere above the Asian monsoon region. Although the effects of the ATAL on the surface and top-of-atmosphere radiation budget have been examined by several studies, the processes and effects by which the ATAL alters radiative transfer within the tropopause layer have been much less discussed. We have used a conditional composite approach to investigate aerosol mixing ratios and their impacts on radiative heating rates in the Asian monsoon tropopause layer in MERRA-2. We have then subsampled in time based on known volcanic eruptions and the evolution of emission and data assimilation inputs to the MERRA-2 aerosol analysis to isolate the ATAL contribution and compare it to radiative heating signatures in the monsoon anticyclone region after volcanic eruptions. The results indicate that the ATAL impact on radiative heating rates in this region is on the order of 0.1 K/day, similar to that associated with ozone variability in MERRA-2 but weaker than cloud radiative effects at these altitudes. We have validated these results and tested their sensitivity to variations in the vertical structure and composition of ATAL aerosols using offline radiative transfer simulations. The idealized simulations produce similar but slightly stronger responses of radiative heating rates to the ATAL and are in good agreement with previous estimates of the top-of-atmosphere radiative forcing. Although the ATAL perturbations inferred from MERRA-2 are only about 10% of mean heating rates at these levels, their spatial distribution suggests potential implications for both isentropic and diabatic transport within the monsoon anticyclone, which should be examined in future work. Our results are limited by uncertainties in the composition and spatiotemporal variability of the ATAL, and reflect only the conditions in this layer as represented by MERRA-2. Targeted observations and model simulations are needed to adequately constrain the uncertainties, particularly with respect to the relative proportions and contributions of nitrate aerosols, which are not included in the MERRA-2 aerosol analysis.</p>

scholarly journals Impact of the Ambae, Raikoke and Ulawun eruptions in 2018-2019 on the global stratospheric aerosol layer and climate

2020 ◽  
Author(s):  
Corinna Kloss ◽  
Pasquale Sellitto ◽  
Bernard Legras ◽  
Jean-Paul Vernier ◽  
Fabrice Jégou ◽  
...  
Keyword(s):  
Radiative Transfer ◽  
Radiative Forcing ◽  
Volcanic Eruptions ◽  
Stratospheric Aerosol ◽  
Orthogonal Polarization ◽  
Transfer Model ◽  
Aerosol Layer ◽  
The Impact ◽  
Aerosol Plume

<p>Using a combination of satellite, ground-based and in-situ observations, and radiative transfer modelling, we quantify the impact of the most recent moderate volcanic eruptions (Ambae, Vanuatu in July 2018; Raikoke, Russia and Ulawun, New Guinea in June 2019) on the global stratospheric aerosol layer and climate.</p><p>For the Ambae volcano (15°S and 167°E), we use the Stratospheric Aerosol and Gas Experiment III (SAGE III), the Ozone Mapping Profiler Suite (OMPS), the Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) and Himawari geostationary satellite observations of the aerosol plume evolution following the Ambae eruption of July 2018. It is shown that the aerosol plume of the main eruption at Ambae in July 2018 was distributed throughout the global stratosphere within the global large-scale circulation (Brewer-Dobson circulation, BDC), to both hemispheres. Ground-based LiDAR observations in Gadanki, India, as well as in-situ Printed Optical Particle Spectrometer (POPS) measurements acquired during the BATAL campaign confirm a widespread perturbation of the stratospheric aerosol layer due to this eruption. Using the UVSPEC radiative transfer model, we also estimate the radiative forcing of this global stratospheric aerosol perturbation. The climate impact is shown to be comparable to that of the well-known and studied recent moderate stratospheric eruptions from Kasatochi (USA, 2008), Sarychev (Russia, 2009) and Nabro (Eritrea, 2011). Top of the atmosphere radiative forcing values between -0.45 and -0.60 W/m<sup>2</sup>, for the Ambae eruption of July 2018, are found.</p><p>In a similar manner the dispersion of the aerosol plume of the Raikoke (48°N and 153°E) and Ulawun (5°S and 151°E) eruptions of June 2019 is analyzed. As both of those eruptions had a stratospheric impact and happened almost simultaneously, it is challenging to completely distinguish both events. Even though the eruptions occurred very recently, first results show that the aerosol plume of the Raikoke eruption resulted in an increase in aerosol extinction values, double as high as compared to that of the Ambae eruption. However, as the eruption occurred on higher latitudes, the main bulk of Raikoke aerosols was transported towards the northern higher latitude’s in the stratosphere within the BDC, as revealed by OMPS, SAGE III and a new detection algorithm for SO<sub>2</sub> and sulfate aerosol using IASI (Infrared Atmospheric Sounder Interferometer). Even though the Raikoke eruption had a larger impact on the stratospheric aerosol layer, both events (the eruptions at Raikoke and Ambae) have to be considered in stratospheric aerosol budget and climate studies.</p>

scholarly journals Stratospheric aerosol radiative forcing simulated by the chemistry climate model EMAC using Aerosol CCI satellite data

2018 ◽  
Vol 18 (17) ◽  
pp. 12845-12857 ◽  
Author(s):  
Christoph Brühl ◽  
Jennifer Schallock ◽  
Klaus Klingmüller ◽  
Charles Robert ◽  
Christine Bingen ◽  
...  
Keyword(s):  
Optical Depth ◽  
Radiative Forcing ◽  
Volcanic Eruptions ◽  
Stratospheric Aerosol ◽  
Radiative Heating ◽  
Aerosol Radiative Forcing ◽  
Tropospheric Aerosol ◽  
Model Aerosol ◽  
Atmospheric Sounding ◽  
Aerosol Radiative

Abstract. This paper presents decadal simulations of stratospheric and tropospheric aerosol and its radiative effects by the chemistry general circulation model EMAC constrained with satellite observations in the framework of the ESA Aerosol CCI project such as GOMOS (Global Ozone Monitoring by Occultation of Stars) and (A)ATSR ((Advanced) Along Track Scanning Radiometer) on the ENVISAT (European Environmental Satellite), IASI (Infrared Atmospheric Sounding Interferometer) on MetOp (Meteorological Operational Satellite), and, additionally, OSIRIS (Optical Spectrograph and InfraRed Imaging System). In contrast to most other studies, the extinctions and optical depths from the model are compared to the observations at the original wavelengths of the satellite instruments covering the range from the UV (ultraviolet) to terrestrial IR (infrared). This avoids conversion artifacts and provides additional constraints for model aerosol and interpretation of the observations. MIPAS (Michelson Interferometer for Passive Atmospheric Sounding) SO2 limb measurements are used to identify plumes of more than 200 volcanic eruptions. These three-dimensional SO2 plumes are added to the model SO2 at the eruption times. The interannual variability in aerosol extinction in the lower stratosphere, and of stratospheric aerosol radiative forcing at the tropopause, is dominated by the volcanoes. To explain the seasonal cycle of the GOMOS and OSIRIS observations, desert dust simulated by a new approach and transported to the lowermost stratosphere by the Asian summer monsoon and tropical convection turns out to be essential. This also applies to the radiative heating by aerosol in the lowermost stratosphere. The existence of wet dust aerosol in the lowermost stratosphere is indicated by the patterns of the wavelength dependence of extinction in observations and simulations. Additional comparison with (A)ATSR total aerosol optical depth at different wavelengths and IASI dust optical depth demonstrates that the model is able to represent stratospheric as well as tropospheric aerosol consistently.

Radiative forcing over the Arctic of aerosols from the August 2017 Canadian and Greenlandic wildfires

2021 ◽  
Author(s):  
Filippo Calì Quaglia ◽  
Daniela Meloni ◽  
Alcide Giorgio di Sarra ◽  
Tatiana Di Iorio ◽  
Virginia Ciardini ◽  
...  
Keyword(s):  
Radiative Transfer ◽  
Radiative Forcing ◽  
Solar Zenith Angle ◽  
Surface Albedo ◽  
High Arctic ◽  
The Arctic ◽  
Radiative Transfer Model ◽  
Transfer Model ◽  
Aerosol Layer ◽  
Radiative Effect

<p>Extended and intense wildfires occurred in Northern Canada and, unexpectedly, on the Greenlandic West coast during summer 2017. The thick smoke plume emitted into the atmosphere was transported to the high Arctic, producing one of the largest impacts ever observed in the region. Evidence of Canadian and Greenlandic wildfires was recorded at the Thule High Arctic Atmospheric Observatory (THAAO, 76.5°N, 68.8°W, www.thuleatmos-it.it) by a suite of instruments managed by ENEA, INGV, Univ. of Florence, and NCAR. Ground-based observations of the radiation budget have allowed quantification of the surface radiative forcing at THAAO. </p><p>Excess biomass burning chemical tracers such as CO, HCN, H2CO, C2H6, and NH3 were  measured in the air column above Thule starting from August 19 until August 23. The aerosol optical depth (AOD) reached a peak value of about 0.9 on August 21, while an enhancement of wildfire compounds was  detected in PM10. The measured shortwave radiative forcing was -36.7 W/m2 at 78° solar zenith angle (SZA) for AOD=0.626.</p><p>MODTRAN6.0 radiative transfer model (Berk et al., 2014) was used to estimate the aerosol radiative effect and the heating rate profiles at 78° SZA. Measured temperature profiles, integrated water vapour, surface albedo, spectral AOD and aerosol extinction profiles from CALIOP onboard CALIPSO were used as model input. The peak  aerosol heating rate (+0.5 K/day) was  reached within the aerosol layer between 8 and 12 km, while the maximum radiative effect (-45.4 W/m2) is found at 3 km, below the largest aerosol layer.</p><p>The regional impact of the event that occurred on August 21 was investigated using a combination of atmospheric radiative transfer modelling with measurements of AOD and ground surface albedo from MODIS. The aerosol properties used in the radiative transfer model were constrained by in situ measurements from THAAO. Albedo data over the ocean have been obtained from Jin et al. (2004). Backward trajectories produced through HYSPLIT simulations (Stein et al., 2015) were also employed to trace biomass burning plumes.</p><p>The radiative forcing efficiency (RFE) over land and ocean was derived, finding values spanning from -3 W/m2 to -132 W/m2, depending on surface albedo and solar zenith angle. The fire plume covered a vast portion of the Arctic, with large values of the daily shortwave RF (< -50 W/m2) lasting for a few days. This large amount of aerosol is expected to influence cloud properties in the Arctic, producing significant indirect radiative effects.</p>

scholarly journals Particulate sulfur in the upper troposphere and lowermost stratosphere – sources and climate forcing

2017 ◽  
Vol 17 (18) ◽  
pp. 10937-10953 ◽  
Author(s):  
Bengt G. Martinsson ◽  
Johan Friberg ◽  
Oscar S. Sandvik ◽  
Markus Hermann ◽  
Peter F. J. van Velthoven ◽  
...  
Keyword(s):  
Seasonal Variation ◽  
Radiative Forcing ◽  
Chemical Elements ◽  
Volcanic Eruptions ◽  
Stratospheric Aerosol ◽  
Aerosol Layer ◽  
Pixe Analysis ◽  
Upper Troposphere ◽  
Particulate Sulfur ◽  
Fine Mode

Abstract. This study is based on fine-mode aerosol samples collected in the upper troposphere (UT) and the lowermost stratosphere (LMS) of the Northern Hemisphere extratropics during monthly intercontinental flights at 8.8–12 km altitude of the IAGOS-CARIBIC platform in the time period 1999–2014. The samples were analyzed for a large number of chemical elements using the accelerator-based methods PIXE (particle-induced X-ray emission) and PESA (particle elastic scattering analysis). Here the particulate sulfur concentrations, obtained by PIXE analysis, are investigated. In addition, the satellite-borne lidar aboard CALIPSO is used to study the stratospheric aerosol load. A steep gradient in particulate sulfur concentration extends several kilometers into the LMS, as a result of increasing dilution towards the tropopause of stratospheric, particulate sulfur-rich air. The stratospheric air is diluted with tropospheric air, forming the extratropical transition layer (ExTL). Observed concentrations are related to the distance to the dynamical tropopause. A linear regression methodology handled seasonal variation and impact from volcanism. This was used to convert each data point into stand-alone estimates of a concentration profile and column concentration of particulate sulfur in a 3 km altitude band above the tropopause. We find distinct responses to volcanic eruptions, and that this layer in the LMS has a significant contribution to the stratospheric aerosol optical depth and thus to its radiative forcing. Further, the origin of UT particulate sulfur shows strong seasonal variation. We find that tropospheric sources dominate during the fall as a result of downward transport of the Asian tropopause aerosol layer (ATAL) formed in the Asian monsoon, whereas transport down from the Junge layer is the main source of UT particulate sulfur in the first half of the year. In this latter part of the year, the stratosphere is the clearly dominating source of particulate sulfur in the UT during times of volcanic influence and under background conditions.

scholarly journals Transport of the 2017 Canadian wildfire plume to the tropics via the Asian monsoon circulation

2019 ◽  
Vol 19 (21) ◽  
pp. 13547-13567 ◽  
Author(s):  
Corinna Kloss ◽  
Gwenaël Berthet ◽  
Pasquale Sellitto ◽  
Felix Ploeger ◽  
Silvia Bucci ◽  
...  
Keyword(s):  
Radiative Forcing ◽  
Asian Monsoon ◽  
Regional Climate ◽  
Climate Impact ◽  
Monsoon Circulation ◽  
Aerosol Layer ◽  
Fire Plume ◽  
Monsoon Area ◽  
The Tropics ◽  
The Impact

Abstract. We show that a fire plume injected into the lower stratosphere at high northern latitudes during the Canadian wildfire event in August 2017 partly reached the tropics. The transport to the tropics was mediated by the anticyclonic flow of the Asian monsoon circulation. The fire plume reached the Asian monsoon area in late August/early September, when the Asian monsoon anticyclone (AMA) was still in place. While there is no evidence of mixing into the center of the AMA, we show that a substantial part of the fire plume is entrained into the anticyclonic flow at the AMA edge and is transported from the extratropics to the tropics, and possibly the Southern Hemisphere particularly following the north–south flow on the eastern side of the AMA. In the tropics the fire plume is lifted by ∼5 km in 7 months. Inside the AMA we find evidence of the Asian tropopause aerosol layer (ATAL) in August, doubling background aerosol conditions with a calculated top of the atmosphere shortwave radiative forcing of −0.05 W m−2. The regional climate impact of the fire signal in the wider Asian monsoon area in September exceeds the impact of the ATAL by a factor of 2–4 and compares to that of a plume coming from an advected moderate volcanic eruption. The stratospheric, trans-continental transport of this plume to the tropics and the related regional climate impact point to the importance of long-range dynamical interconnections of pollution sources.

scholarly journals The Interactive Stratospheric Aerosol Model Intercomparison Project (ISA-MIP): motivation and experimental design

2018 ◽  
Vol 11 (7) ◽  
pp. 2581-2608 ◽  
Author(s):  
Claudia Timmreck ◽  
Graham W. Mann ◽  
Valentina Aquila ◽  
Rene Hommel ◽  
Lindsay A. Lee ◽  
...  
Keyword(s):  
Radiative Forcing ◽  
Volcanic Eruptions ◽  
Stratospheric Aerosol ◽  
Transport Processes ◽  
Aerosol Layer ◽  
Model Intercomparison ◽  
Aerosol Model ◽  
Model Experiments ◽  
Aerosol Forcing ◽  
Intercomparison Project

Abstract. The Stratospheric Sulfur and its Role in Climate (SSiRC) Interactive Stratospheric Aerosol Model Intercomparison Project (ISA-MIP) explores uncertainties in the processes that connect volcanic emission of sulfur gas species and the radiative forcing associated with the resulting enhancement of the stratospheric aerosol layer. The central aim of ISA-MIP is to constrain and improve interactive stratospheric aerosol models and reduce uncertainties in the stratospheric aerosol forcing by comparing results of standardized model experiments with a range of observations. In this paper we present four co-ordinated inter-model experiments designed to investigate key processes which influence the formation and temporal development of stratospheric aerosol in different time periods of the observational record. The Background (BG) experiment will focus on microphysics and transport processes under volcanically quiescent conditions, when the stratospheric aerosol is controlled by the transport of aerosols and their precursors from the troposphere to the stratosphere. The Transient Aerosol Record (TAR) experiment will explore the role of small- to moderate-magnitude volcanic eruptions, anthropogenic sulfur emissions, and transport processes over the period 1998–2012 and their role in the warming hiatus. Two further experiments will investigate the stratospheric sulfate aerosol evolution after major volcanic eruptions. The Historical Eruptions SO2 Emission Assessment (HErSEA) experiment will focus on the uncertainty in the initial emission of recent large-magnitude volcanic eruptions, while the Pinatubo Emulation in Multiple models (PoEMS) experiment will provide a comprehensive uncertainty analysis of the radiative forcing from the 1991 Mt Pinatubo eruption.

scholarly journals The impact of volcanic eruptions of different magnitude on stratospheric water vapor in the tropics

2021 ◽  
Vol 21 (8) ◽  
pp. 6565-6591
Author(s):  
Clarissa Alicia Kroll ◽  
Sally Dacie ◽  
Alon Azoulay ◽  
Hauke Schmidt ◽  
Claudia Timmreck
Keyword(s):  
Water Vapor ◽  
Radiative Forcing ◽  
Volcanic Eruptions ◽  
Aerosol Layer ◽  
Power Functions ◽  
Max Planck ◽  
Point Temperature ◽  
Stratospheric Water Vapor ◽  
Cold Point ◽  
The Impact

Abstract. Increasing the temperature of the tropical cold-point region through heating by volcanic aerosols results in increases in the entry value of stratospheric water vapor (SWV) and subsequent changes in the atmospheric energy budget. We analyze tropical volcanic eruptions of different strengths with sulfur (S) injections ranging from 2.5 Tg S up to 40 Tg S using EVAens, the 100-member ensemble of the Max Planck Institute – Earth System Model in its low-resolution configuration (MPI-ESM-LR) with artificial volcanic forcing generated by the Easy Volcanic Aerosol (EVA) tool. Significant increases in SWV are found for the mean over all ensemble members from 2.5 Tg S onward ranging between [5, 160] %. However, for single ensemble members, the standard deviation between the control run members (0 Tg S) is larger than SWV increase of single ensemble members for eruption strengths up to 20 Tg S. A historical simulation using observation-based forcing files of the Mt. Pinatubo eruption, which was estimated to have emitted (7.5±2.5) Tg S, returns SWV increases slightly higher than the 10 Tg S EVAens simulations due to differences in the aerosol profile shape. An additional amplification of the tape recorder signal is also apparent, which is not present in the 10 Tg S run. These differences underline that it is not only the eruption volume but also the aerosol layer shape and location with respect to the cold point that have to be considered for post-eruption SWV increases. The additional tropical clear-sky SWV forcing for the different eruption strengths amounts to [0.02, 0.65] W m−2, ranging between [2.5, 4] % of the aerosol radiative forcing in the 10 Tg S scenario. The monthly cold-point temperature increases leading to the SWV increase are not linear with respect to aerosol optical depth (AOD) nor is the corresponding SWV forcing, among others, due to hysteresis effects, seasonal dependencies, aerosol profile heights and feedbacks. However, knowledge of the cold-point temperature increase allows for an estimation of SWV increases of 12 % per Kelvin increase in mean cold-point temperature. For yearly averages, power functions are fitted to the cold-point warming and SWV forcing with increasing AOD.

scholarly journals Stratospheric aerosol radiative forcing simulated by the chemistry climate model EMAC using aerosol CCI satellite data

2018 ◽  
Author(s):  
Christoph Brühl ◽  
Jennifer Schallock ◽  
Klaus Klingmüller ◽  
Charles Robert ◽  
Christine Bingen ◽  
...  
Keyword(s):  
Optical Depth ◽  
Radiative Forcing ◽  
General Circulation ◽  
Asian Summer Monsoon ◽  
Michelson Interferometer ◽  
Circulation Model ◽  
Volcanic Eruptions ◽  
Radiative Heating ◽  
Tropospheric Aerosol ◽  
Atmospheric Sounding

Abstract. This paper presents decadal simulations of stratospheric and tropospheric aerosol by the chemistry general circulation model EMAC constrained with satellite observations in the framework of the ESA-Aerosol-CCI project like GOMOS (Global Ozone Monitoring by Occultation of Stars) and (A)ATSR ((Advanced) Along Track Scanning Radiometer) on ENVISAT (European Environmental Satellite), and IASI (Infrared Atmospheric Sounding Interferometer) on Metop (Meteorological Operational Satellite). The EMAC simulations with modal interactive aerosol and observations by GOMOS show that sulfate particles from about 230 volcanic eruptions identified mostly from MIPAS (Michelson Interferometer for Passive Atmospheric Sounding) SO2 limb measurements dominate the interannual variability of aerosol extinction in the lower stratosphere, and of radiative forcing at the tropopause. To explain the observations, desert dust and organic and black carbon, transported to the lowermost stratosphere by the Asian summer monsoon and tropical convection, are also important. This holds also for radiative heating by aerosol in the lowermost stratosphere. Comparison with (A)ATSR total aerosol optical depth at different wavelengths and IASI dust optical depth shows that the model is able to represent stratospheric and tropospheric aerosol in a consistent way.

Sounding-Based Thermodynamic Budgets for DYNAMO

2015 ◽  
Vol 72 (2) ◽  
pp. 598-622 ◽  
Author(s):  
Richard H. Johnson ◽  
Paul E. Ciesielski ◽  
James H. Ruppert ◽  
Masaki Katsumata
Keyword(s):  
Radiative Forcing ◽  
Deep Convection ◽  
Active Phase ◽  
Life Cycles ◽  
Radiative Heating ◽  
Convective Heating ◽  
Madden Julian Oscillation ◽  
Heating Rates ◽  
Gross Moist Stability ◽  
Cumulus Congestus

Abstract The Dynamics of the Madden–Julian Oscillation (DYNAMO) field campaign, conducted over the Indian Ocean from October 2011 to March 2012, was designed to study the initiation of the Madden–Julian oscillation (MJO). Two prominent MJOs occurred in the experimental domain during the special observing period in October and November. Data from a northern and a southern sounding array (NSA and SSA, respectively) have been used to investigate the apparent heat sources and sinks (Q1 and Q2) and radiative heating rates QR throughout the life cycles of the two MJO events. The MJO signal was far stronger in the NSA than the SSA. Time series of Q1, Q2, and the vertical eddy flux of moist static energy reveal an evolution of cloud systems for both MJOs consistent with prior studies: shallow, nonprecipitating cumulus during the suppressed phase, followed by cumulus congestus, then deep convection during the active phase, and finally stratiform precipitation. However, the duration of these phases was shorter for the November MJO than for the October event. The profiles of Q1 and Q2 for the two arrays indicate a greater stratiform rain fraction for the NSA than the SSA—a finding supported by TRMM measurements. Surface rainfall rates and net tropospheric QR determined as residuals from the budgets show good agreement with satellite-based estimates. The cloud radiative forcing was approximately 20% of the column-integrated convective heating and of the same amplitude as the normalized gross moist stability, leaving open the possibility of radiative–convective instability for the two MJOs.

scholarly journals On the Approximation of Local and Linear Radiative Damping in the Middle Atmosphere

2010 ◽  
Vol 67 (6) ◽  
pp. 2070-2085 ◽  
Author(s):  
Peter Hitchcock ◽  
Theodore G. Shepherd ◽  
Shigeo Yoden
Keyword(s):  
Climate Model ◽  
Middle Atmosphere ◽  
Mechanistic Modeling ◽  
Radiative Heating ◽  
Spatiotemporal Variability ◽  
Quadratic Term ◽  
Heating Rates ◽  
Temperature State ◽  
Large Fluctuations ◽  
Damping Rate

Abstract The validity of approximating radiative heating rates in the middle atmosphere by a local linear relaxation to a reference temperature state (i.e., “Newtonian cooling”) is investigated. Using radiative heating rate and temperature output from a chemistry–climate model with realistic spatiotemporal variability and realistic chemical and radiative parameterizations, it is found that a linear regression model can capture more than 80% of the variance in longwave heating rates throughout most of the stratosphere and mesosphere, provided that the damping rate is allowed to vary with height, latitude, and season. The linear model describes departures from the climatological mean, not from radiative equilibrium. Photochemical damping rates in the upper stratosphere are similarly diagnosed. Three important exceptions, however, are found. The approximation of linearity breaks down near the edges of the polar vortices in both hemispheres. This nonlinearity can be well captured by including a quadratic term. The use of a scale-independent damping rate is not well justified in the lower tropical stratosphere because of the presence of a broad spectrum of vertical scales. The local assumption fails entirely during the breakup of the Antarctic vortex, where large fluctuations in temperature near the top of the vortex influence longwave heating rates within the quiescent region below. These results are relevant for mechanistic modeling studies of the middle atmosphere, particularly those investigating the final Antarctic warming.

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