scholarly journals Gas-mediated liquid metal printing toward large-scale 2D semiconductors and ultraviolet photodetector

2021 ◽  
Vol 5 (1) ◽  
Author(s):  
Qian Li ◽  
Ju Lin ◽  
Tian-Ying Liu ◽  
Xi-Yu Zhu ◽  
Wen-Hao Yao ◽  
...  
Keyword(s):  
Liquid Metal ◽  
High Performance ◽  
Large Scale ◽  
2D Materials ◽  
Low Cost ◽  
Ambient Air ◽  
Electronic Systems ◽  
Ultraviolet Photodetector ◽  
Metal Printing ◽  
2D Semiconductors

AbstractA gas-mediated fabrication of centimeter-scale two-dimensional (2D) semiconductors and ultraviolet photodetector by a liquid metal-based printing was reported. Various large-scale 2D materials (Ga2O3, In2O3, SnO) were demonstrated to be directly printed at ambient air on different substrates. Such printing represents a generic, fast, clean, and scalable technique to quickly manufacture 2D semiconductors. The electrical properties were explored to quantify the printed 2D films, which were somewhat deficient in previous studies. In particular, to explore and facilitate the advantages of this 2D semiconductor in functional electronic applications, strategies for realizing fully printed Ga2O3/Si heterojunction photodetector via low-temperature and low-cost processes were developed. The device exhibits excellent sensibility and rapid photoresponse times. This work offers feasible way to develop high-performance ultraviolet photodetector for mass production. It also suggests a promising direction for making large-scale 2D photoelectronic and electronic systems and is expected to be extensively useful in the coming time.

scholarly journals Room-Temperature Solution-Processed 0D/1D Bilayer Electrodes for Translucent CsPbBr3 Perovskite Photovoltaics

Nanomaterials ◽  
2021 ◽  
Vol 11 (6) ◽  
pp. 1489
Author(s):  
Bhaskar Parida ◽  
Saemon Yoon ◽  
Dong-Won Kang
Keyword(s):  
Solar Cells ◽  
Indium Tin Oxide ◽  
High Performance ◽  
Room Temperature ◽  
Low Cost ◽  
Perovskite Solar Cells ◽  
Ambient Air ◽  
Plasma Damage ◽  
Temperature Solution ◽  
Ito Nanoparticles

Materials and processing of transparent electrodes (TEs) are key factors to creating high-performance translucent perovskite solar cells. To date, sputtered indium tin oxide (ITO) has been a general option for a rear TE of translucent solar cells. However, it requires a rather high cost due to vacuum process and also typically causes plasma damage to the underlying layer. Therefore, we introduced TE based on ITO nanoparticles (ITO-NPs) by solution processing in ambient air without any heat treatment. As it reveals insufficient conductivity, Ag nanowires (Ag-NWs) are additionally coated. The ITO-NPs/Ag-NW (0D/1D) bilayer TE exhibits a better figure of merit than sputtered ITO. After constructing CsPbBr3 perovskite solar cells, the device with 0D/1D TE offers similar average visible transmission with the cells with sputtered ITO. More interestingly, the power conversion efficiency of 0D/1D TE device was 5.64%, which outperforms the cell (4.14%) made with sputtered-ITO. These impressive findings could open up a new pathway for the development of low-cost, translucent solar cells with quick processing under ambient air at room temperature.

Bifunctional Flexible Fabrics with Excellent Joule Heating and Electromagnetic Interference Shielding Performance Based on Copper Sulfide/Glass Fiber Composite

Nanoscale ◽  
2021 ◽  
Author(s):  
Binguo Liu ◽  
Qi Zhang ◽  
Yuanhui Huang ◽  
Dong Liu ◽  
Wei Pan ◽  
...  
Keyword(s):  
Electromagnetic Interference ◽  
Copper Sulfide ◽  
High Performance ◽  
Fiber Composite ◽  
Low Cost ◽  
Electronic Systems ◽  
Electromagnetic Interference Shielding ◽  
Glass Fiber Composite ◽  
Wearable Electronic ◽  
Sulfide Glass

Flexible and wearable electronic technology is in great demand with the rising of smart electronic systems. Among this, exploring multifunctional with high performance at low cost has attracted extensive attention...

Overview on the Liquid Metal Battery for Grid-Level Large-Scale Energy Storage

2016 ◽  
Vol 723 ◽  
pp. 572-578
Author(s):  
Li Fu ◽  
Qi Chi Le ◽  
Xi Bo Wang ◽  
Xuan Liu ◽  
Wei Tao Jia
Keyword(s):  
Energy Storage ◽  
Liquid Metal ◽  
Large Scale ◽  
Low Cost ◽  
Advantages And Disadvantages ◽  
Comprehensive Comparison ◽  
Development And Utilization ◽  
Working Principle ◽  
Liquid Metal Battery ◽  
Grid Level

In recent years, the development and utilization of renewable generation have attracted more and more attention, and the grid puts forward higher requirements to the energy storage technology, especially for security, stability and reliability. The liquid metal battery (LMB) consists of two liquid metal electrodes and a molten salt electrolyte, which will be segregated into three liquid layers naturally. Being low-cost and long-life, it is regarded as the best choice for grid-level large-scale energy storage. This paper describes the main structure and working principle of the LMB, analyzes the advantages and disadvantages of the LMB when compared with the traditional batteries, and explores the feasibility and economy when it is used as a kind of large-scale energy storage applied in the power grid. The paper also makes a comprehensive comparison on the performance of several LMBs, and points out the LMB’s research and development in the future.

scholarly journals Process Design Kit and Design Automation for Flexible Hybrid Electronics

2019 ◽  
Vol 16 (3) ◽  
pp. 117-123
Author(s):  
Tsung-Ching Huang ◽  
Ting Lei ◽  
Leilai Shao ◽  
Sridhar Sivapurapu ◽  
Madhavan Swaminathan ◽  
...  
Keyword(s):  
Process Design ◽  
Design Automation ◽  
High Performance ◽  
Large Scale ◽  
Low Cost ◽  
Thin Film Transistor ◽  
Solution Process ◽  
Oxide Semiconductor ◽  
Wearable Electronics ◽  
Wide Range

Abstract High-performance low-cost flexible hybrid electronics (FHE) are desirable for applications such as internet of things and wearable electronics. Carbon nanotube (CNT) thin-film transistor (TFT) is a promising candidate for high-performance FHE because of its high carrier mobility, superior mechanical flexibility, and material compatibility with low-cost printing and solution processes. Flexible sensors and peripheral CNT-TFT circuits, such as decoders, drivers, and sense amplifiers, can be printed and hybrid-integrated with thinned (<50 μm) silicon chips on soft, thin, and flexible substrates for a wide range of applications, from flexible displays to wearable medical devices. Here, we report (1) a process design kit (PDK) to enable FHE design automation for large-scale FHE circuits and (2) solution process-proven intellectual property blocks for TFT circuits design, including Pseudo-Complementary Metal-Oxide-Semiconductor (Pseudo-CMOS) flexible digital logic and analog amplifiers. The FHE-PDK is fully compatible with popular silicon design tools for design and simulation of hybrid-integrated flexible circuits.

Recent progress in zinc-based redox flow batteries: a review

2021 ◽  
Author(s):  
Guixiang Wang ◽  
Haitao Zou ◽  
Xiaobo Zhu ◽  
Mei Ding ◽  
Chuankun Jia
Keyword(s):  
High Performance ◽  
Large Scale ◽  
Electrode Materials ◽  
Low Cost ◽  
Ion Selectivity ◽  
Commercial Application ◽  
Environmental Friendliness ◽  
Membrane Materials ◽  
Redox Flow Batteries ◽  
Flow Batteries

Abstract Zinc-based redox flow batteries (ZRFBs) have been considered as ones of the most promising large-scale energy storage technologies owing to their low cost, high safety, and environmental friendliness. However, their commercial application is still hindered by a few key problems. First, the hydrogen evolution and zinc dendrite formation cause poor cycling life, of which needs to ameliorated or overcome by finding suitable anolytes. Second, the stability and energy density of catholytes are unsatisfactory due to oxidation, corrosion, and low electrolyte concentration. Meanwhile, highly catalytic electrode materials remain to be explored and the ion selectivity and cost efficiency of membrane materials demands further improvement. In this review, we summarize different types of ZRFBs according to their electrolyte environments including ZRFBs using neutral, acidic, and alkaline electrolytes, then highlight the advances of key materials including electrode and membrane materials for ZRFBs, and finally discuss the challenges and perspectives for the future development of high-performance ZRFBs.

Day-to-day variations in paddy-residue burning and residential heating emissions control aerosol pollution peaks in rural north-west India

2021 ◽  
Author(s):  
Harshita Pawar ◽  
Baerbel Sinha
Keyword(s):  
Air Quality ◽  
Large Scale ◽  
Learning Algorithm ◽  
Low Cost ◽  
Winter Season ◽  
Ambient Air ◽  
Rural Site ◽  
North West ◽  
Daily Average ◽  
Residential Heating

<p>November onwards, the poor air quality over north-west India is blamed on the large-scale paddy residue burning in Punjab and Haryana. However, the emission strength of this source remains poorly constrained due to the lack of ground-based measurements within the rural source regions. In this study, we report the particulate matter (PM) levels at Nadampur, a rural site in the Sangrur district of Punjab that witnesses rampant paddy residue burning, using the Airveda low-cost PM sensors from October to December 2019. The raw PM measurements from the sensor were corrected using the Random Forest machine learning algorithm. The daily average PM<sub>10</sub> and PM<sub>2.5</sub> mass concentration at Nadampur correlated well  (r > 0.7) with the daily sum of VIIRS fire counts. Agricultural activities, including paddy residue burning and harvesting operations, contributed less than 40% to the overall PM loading, even in the peak burning period at Nadampur. We show that the increased residential heating emissions in the winter season have a profound and currently neglected impact on ambient air quality. A dip in the daily average temperature by 1 ºC increased the daily emission of PM<sub>10</sub> by 6.3 tonnes and that of PM<sub>2.5</sub> by 5.8 tonnes. Overall, paddy harvest, local and regional paddy residue burning, residential heating emissions, ventilation, and wet scavenging could explain 79% of the variations in PM<sub>10</sub> and 85% of the variations in PM<sub>2.5</sub>. Day to day variations in PM emissions from residential heating in response to the ambient temperature must be incorporated into emission inventories and models for accurate air quality forecasts.</p>

Three-Dimensional MoS2/Graphene Hybrid Aerogel as Free-Standing, High-Performance Electrode for Supercapacitor

NANO ◽  
2020 ◽  
Vol 15 (05) ◽  
pp. 2050062
Author(s):  
Zhaolei Meng ◽  
Xiaojian He ◽  
Song Han ◽  
Zijian Hu
Keyword(s):  
Porous Structure ◽  
Surface Area ◽  
High Performance ◽  
Large Scale ◽  
Low Cost ◽  
Hydrothermal Process ◽  
Three Dimensional ◽  
Rate Capability ◽  
Free Standing ◽  
Hybrid Aerogel

Carbon materials are generally employed as supercapacitor electrodes due to their low- cost, high-chemical stability and environmental friendliness. However, the design of carbon structures with large surface area and controllable porous structure remains a daunt challenge. In this work, a three-dimensional (3D) hybrid aerogel with different contents of MoS2 nanosheets in 3D graphene aerogel (MoS2-GA) was synthesized through a facial hydrothermal process. The influences of MoS2 content on microstructure and subsequently on electrochemical properties of MoS2-GA are systematically investigated and an optimized mass ratio with MoS2: GA of 1:2 is chosen to achieve high mechanical robustness and outstanding electrochemical performance in the hybrid structure. Due to the large specific surface area, porous structure and continuous charge transfer network, such MoS2-GA electrodes exhibit high specific capacitance, good rate capability and excellent cyclic stability, showing great potential in large-scale and low-cost fabrication of high-performance supercapacitors.

Epitaxial growth of large-scale In2S3 nanoflakes and the construction of a high performance In2S3/Si photodetector

2019 ◽  
Vol 7 (39) ◽  
pp. 12104-12113 ◽  
Author(s):  
Jianting Lu ◽  
Zhaoqiang Zheng ◽  
Wei Gao ◽  
Jiandong Yao ◽  
Yu Zhao ◽  
...  
Keyword(s):  
Epitaxial Growth ◽  
Material Properties ◽  
High Performance ◽  
Large Scale ◽  
2D Materials

MoS2-like layered 2D materials have attracted attention worldwide due to their intriguing material properties.

scholarly journals Low-cost, large-scale, one-pot synthesis of C/Ni3(NO3)2(OH)4 composites for high performance supercapacitor

2018 ◽  
Vol 217 ◽  
pp. 291-299 ◽  
Author(s):  
Yingyuan Zhao ◽  
Nian Jiang ◽  
Xu Zhang ◽  
Jing Guo ◽  
Yanqiang Li ◽  
...  
Keyword(s):  
High Performance ◽  
Large Scale ◽  
Low Cost ◽  
One Pot ◽  
One Pot Synthesis

scholarly journals Towards High Performance Chemical Vapour Deposition V2O5 Cathodes for Batteries Employing Aqueous Media

Molecules ◽  
2020 ◽  
Vol 25 (23) ◽  
pp. 5558
Author(s):  
Dimitra Vernardou ◽  
Charalampos Drosos ◽  
Andreas Kafizas ◽  
Martyn E. Pemble ◽  
Emmanouel Koudoumas
Keyword(s):  
Energy Storage ◽  
High Performance ◽  
Large Scale ◽  
Electrode Materials ◽  
Low Cost ◽  
Aqueous Media ◽  
Chemical Vapour ◽  
Cost Effective ◽  
Scale Production ◽  
Environmentally Safe

The need for clean and efficient energy storage has become the center of attention due to the eminent global energy crisis and growing ecological concerns. A key component in this effort is the ultra-high performance battery, which will play a major role in the energy industry. To meet the demands in portable electronic devices, electric vehicles, and large-scale energy storage systems, it is necessary to prepare advanced batteries with high safety, fast charge ratios, and discharge capabilities at a low cost. Cathode materials play a significant role in determining the performance of batteries. Among the possible electrode materials is vanadium pentoxide, which will be discussed in this review, due to its low cost and high theoretical capacity. Additionally, aqueous electrolytes, which are environmentally safe, provide an alternative approach compared to organic media for safe, cost-effective, and scalable energy storage. In this review, we will reveal the industrial potential of competitive methods to grow cathodes with excellent stability and enhanced electrochemical performance in aqueous media and lay the foundation for the large-scale production of electrode materials.

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