Comparison of Aura MLS Water Vapor Measurements with GFS and NAM Analyses in the Upper Troposphere–Lower Stratosphere

2010 ◽  
Vol 27 (2) ◽  
pp. 274-289 ◽  
Author(s):  
Le Van Thien ◽  
William A. Gallus ◽  
Mark A. Olsen ◽  
Nathaniel Livesey
Keyword(s):  
Water Vapor ◽  
North American ◽  
Lower Stratosphere ◽  
Model Analysis ◽  
Weather Research And Forecasting ◽  
Upper Troposphere ◽  
Mixing Ratios ◽  
Four Seasons ◽  
Gfs Model ◽  
The Tropics

Abstract Water vapor mixing ratios in the upper troposphere and lower stratosphere measured by the Aura Microwave Limb Sounder (MLS) version 2.2 instrument have been compared with Global Forecast System (GFS) analyses at five levels within the 300–100-hPa layer and North American Mesoscale (NAM) model analyses at six levels within the 300–50-hPa layer over the two years of 2005 and 2006 at four analysis times (e.g., 0000, 0600, 1200, and 1800 UTC). Probability density functions of the vapor mixing ratios suggest that both analyses are often moister than Aura MLS values, but NAM model analyses agree somewhat better with Aura MLS measurements than GFS model analyses over the same North American domain at the five common levels. Examining five subsets of the global GFS domain, the GFS model analysis is moister than Aura MLS estimates everywhere but at 150 and 100 hPa in all regions outside of the tropics. NAM model analysis water vapor mixing ratios exceeded the Aura MLS values at all levels from 250 to 150 hPa in all four seasons of both years and some seasons at 100 and 50 hPa. Moist biases in winter and spring of both years were similar at all levels, but these moist biases in summer and fall were smaller in 2005 than in 2006 at all levels. These differences may be due to the change in the NAM from using the Eta Model to using the Weather Research and Forecasting model (WRF) in June 2006.

scholarly journals The efficiency of transport into the stratosphere via the Asian and North American summer monsoon circulations

2019 ◽  
Author(s):  
Xiaolu Yan ◽  
Paul Konopka ◽  
Felix Ploeger ◽  
Aurélien Podglajen ◽  
Jonathon S. Wright ◽  
...  
Keyword(s):  
Summer Monsoon ◽  
North American ◽  
Lower Stratosphere ◽  
Atmospheric Composition ◽  
Transport Pathways ◽  
Transport Efficiency ◽  
Upper Troposphere ◽  
Horizontal Transport ◽  
The Tropics ◽  
K Transport

Abstract. Transport of pollutants into the stratosphere via the Asian summer monsoon (ASM) or North American summer monsoon (NASM) may affect the atmospheric composition and climate both locally and globally. We identify and study the robust characteristics of transport from the ASM and NASM regions to the stratosphere using the Lagrangian chemistry transport model CLaMS as driven by the ERA-Interim and MERRA-2 reanalyses. In particular, we investigate the relative influences of the ASM and NASM on stratospheric composition, the transport pathways by which these influences are effected, and the quantitative contributions and efficiencies of transport from different altitudes in these two monsoon regions to the stratosphere. We release artificial tracers in several vertical layers from the middle troposphere to the lower stratosphere in both ASM and NASM source regions during July and August 2010–2013 and track their evolution until the following summer. We find that the magnitude of transport from the ASM and NASM regions to the tropical stratosphere, and even to the Southern Hemispheric stratosphere, is higher when the tracers are released at the 350–360 K level. For tracers released close to the tropopause (370–380 K), transport is primarily into the Northern Hemispheric stratosphere. Results for different vertical layers or air origin reveal two transport pathways from the upper troposphere over the ASM and NASM regions to the tropical pipe: (i) quasi-horizontal transport to the tropics below the tropopause followed by ascent to the stratosphere via tropical upwelling, and (ii) ascent into the stratosphere inside the ASM/NASM followed by quasi-horizontal transport to the tropical lower stratosphere and tropical pipe. The tropical pathway (i) is faster than the monsoon pathway (ii), particularly in the ascending branch. Ultimately, the abundance of air in the tropical pipe that originates in the ASM upper troposphere (350–360 K, ~ 5 %) is comparable to that of air ascending directly from the tropics ten months after the release of the source tracers. By contrast, the air mass contributions from the ASM to the tropical pipe are about three times larger than the corresponding contribution from the NASM (~ 1.5 %). The transport efficiency into the tropical pipe, normalized by the mass of the domain, is greatest from the ASM region at 370–380 K. Transport from the ASM to the tropical pipe is almost twice as efficient as transport from the NASM or tropics to the tropical pipe. Although the contribution from the NASM to the stratosphere is less than that from either the ASM or the tropics, the transport efficiency from the NASM is comparable to that from the tropics.

scholarly journals Measurement of low-ppm mixing ratios of water vapor in the upper troposphere and lower stratosphere using chemical ionization mass spectrometry

2013 ◽  
Vol 6 (1) ◽  
pp. 381-422 ◽  
Author(s):  
T. D. Thornberry ◽  
A. W. Rollins ◽  
R. S. Gao ◽  
L. A. Watts ◽  
S. J. Ciciora ◽  
...  
Keyword(s):  
Water Vapor ◽  
Chemical Ionization ◽  
Lower Stratosphere ◽  
Signal To Noise Ratio ◽  
Ion Source ◽  
Ionization Mass ◽  
Measurement Sensitivity ◽  
Particle Radiation ◽  
Upper Troposphere ◽  
Mixing Ratios

Abstract. A chemical ionization mass spectrometer (CIMS) instrument has been developed for the fast, precise, and accurate measurement of water vapor (H2O) at low mixing ratios in the upper troposphere and lower stratosphere (UT/LS). A low-pressure flow of sample air passes through an ionization volume containing an α-particle radiation source, resulting in a cascade of ion-molecule reactions that produce hydronium ions (H3O+) from ambient H2O. The production of H3O+ ions from ambient H2O depends on pressure and flow through the ion source, which were tightly controlled in order to maintain the measurement sensitivity independent of changes in the airborne sampling environment. The instrument was calibrated every 45 min in flight by introducing a series of H2O mixing ratios between 0.5 and 153 parts per million (ppm) generated by Pt-catalyzed oxidation of H2 standards while overflowing the inlet with dry synthetic air. The CIMS H2O instrument was deployed in an unpressurized payload area aboard the NASA WB-57 high altitude research aircraft during the Mid-latitude Airborne Cirrus Properties Experiment (MACPEX) mission in March and April 2011. The instrument performed successfully during seven flights, measuring H2O mixing ratios below 5 ppm in the lower stratosphere at altitudes up to 17.7 km, and as low as 3.5 ppm near the tropopause. Data were acquired at 10 Hz and reported as 1-s averages. In-flight calibrations demonstrated a typical sensitivity of 2000 Hz ppm−1 at 3 ppm with a signal to noise ratio (2σ, 1-s) greater than 32. The total measurement uncertainty was 9 to 11%, derived from the uncertainty in the in situ calibrations.

scholarly journals The efficiency of transport into the stratosphere via the Asian and North American summer monsoon circulations

2019 ◽  
Vol 19 (24) ◽  
pp. 15629-15649 ◽  
Author(s):  
Xiaolu Yan ◽  
Paul Konopka ◽  
Felix Ploeger ◽  
Aurélien Podglajen ◽  
Jonathon S. Wright ◽  
...  
Keyword(s):  
Summer Monsoon ◽  
North American ◽  
Lower Stratosphere ◽  
Atmospheric Composition ◽  
Transport Pathways ◽  
Air Mass ◽  
Transport Efficiency ◽  
Upper Troposphere ◽  
Horizontal Transport ◽  
The Tropics

Abstract. Transport of pollutants into the stratosphere via the Asian summer monsoon (ASM) or North American summer monsoon (NASM) may affect the atmospheric composition and climate both locally and globally. We identify and study the robust characteristics of transport from the ASM and NASM regions to the stratosphere using the Lagrangian chemistry transport model CLaMS driven by both the ERA-Interim and MERRA-2 reanalyses. In particular, we quantify the relative influences of the ASM and NASM on stratospheric composition and investigate the transport pathways and efficiencies of transport of air masses originating at different altitudes in these two monsoon regions to the stratosphere. We release artificial tracers in several vertical layers from the middle troposphere to the lower stratosphere in both ASM and NASM source regions during July and August 2010–2013 and track their evolution until the following summer. We find that more air mass is transported from the ASM and NASM regions to the tropical stratosphere, and even to the southern hemispheric stratosphere, when the tracers are released clearly below the tropopause (350–360 K) than when they are released close to the tropopause (370–380 K). For tracers released close to the tropopause (370–380 K), transport is primarily into the northern hemispheric lower stratosphere. Results for different vertical layers of air origin reveal two transport pathways from the upper troposphere over the ASM and NASM regions to the tropical pipe: (i) quasi-horizontal transport to the tropics below the tropopause followed by ascent to the stratosphere via tropical upwelling, and (ii) ascent into the stratosphere inside the ASM/NASM followed by quasi-horizontal transport to the tropical lower stratosphere and further to the tropical pipe. Overall, the tropical pathway (i) is faster than the monsoon pathway (ii), particularly in the ascending branch. The abundance of air in the tropical pipe that originates in the ASM upper troposphere (350–360 K) is comparable to the abundance of air ascending directly from the tropics to the tropical pipe 10 months after (the following early summer) the release of the source tracers. The air mass contributions from the ASM to the tropical pipe are about 3 times larger than the corresponding contributions from the NASM. The transport efficiency into the tropical pipe, the air mass fraction inside this destination region normalized by the mass of the domain of origin, is greatest from the ASM region at 370–380 K. Although the contribution from the NASM to the stratosphere is less than that from either the ASM or the tropics, the transport efficiency from the NASM is comparable to that from the tropics.

scholarly journals Measurement of low-ppm mixing ratios of water vapor in the upper troposphere and lower stratosphere using chemical ionization mass spectrometry

2013 ◽  
Vol 6 (6) ◽  
pp. 1461-1475 ◽  
Author(s):  
T. D. Thornberry ◽  
A. W. Rollins ◽  
R. S. Gao ◽  
L. A. Watts ◽  
S. J. Ciciora ◽  
...  
Keyword(s):  
Water Vapor ◽  
Chemical Ionization ◽  
Lower Stratosphere ◽  
Signal To Noise Ratio ◽  
Ion Source ◽  
Ionization Mass ◽  
Measurement Sensitivity ◽  
Particle Radiation ◽  
Upper Troposphere ◽  
Mixing Ratios

Abstract. A chemical ionization mass spectrometer (CIMS) instrument has been developed for the fast, precise, and accurate measurement of water vapor (H2O) at low mixing ratios in the upper troposphere and lower stratosphere (UT/LS). A low-pressure flow of sample air passes through an ionization volume containing an α-particle radiation source, resulting in a cascade of ion-molecule reactions that produce hydronium ions (H3O+) from ambient H2O. The production of H3O+ ions from ambient H2O depends on pressure and flow through the ion source, which were tightly controlled in order to maintain the measurement sensitivity independent of changes in the airborne sampling environment. The instrument was calibrated every 45 min in flight by introducing a series of H2O mixing ratios between 0.5 and 153 parts per million (ppm, 10−6 mol mol−1) generated by Pt-catalyzed oxidation of H2 standards while overflowing the inlet with dry synthetic air. The CIMS H2O instrument was deployed in an unpressurized payload area aboard the NASA WB-57F high-altitude research aircraft during the Mid-latitude Airborne Cirrus Properties Experiment (MACPEX) mission in March and April 2011. The instrument performed successfully during seven flights, measuring H2O mixing ratios below 5 ppm in the lower stratosphere at altitudes up to 17.7 km, and as low as 3.5 ppm near the tropopause. Data were acquired at 10 Hz and reported as 1 s averages. In-flight calibrations demonstrated a typical sensitivity of 2000 Hz ppm−1 at 3 ppm with a signal to noise ratio (2 σ, 1 s) greater than 32. The total measurement uncertainty was 9 to 11%, derived from the uncertainty in the in situ calibrations.

scholarly journals Effect of tropical cyclones on the Stratosphere-Troposphere Exchange observed using satellite observations over north Indian Ocean

2016 ◽  
Author(s):  
M. Venkat Ratnam ◽  
S. Ravindra Babu ◽  
S. S. Das ◽  
Ghouse Basha ◽  
B. V. Krishnamurthy ◽  
...  
Keyword(s):  
Water Vapor ◽  
Indian Ocean ◽  
Tropical Cyclones ◽  
Lower Stratosphere ◽  
North Indian Ocean ◽  
Satellite Observations ◽  
Upper Troposphere ◽  
North West ◽  
The North ◽  
The Impact

Abstract. Tropical cyclones play an important role in modifying the tropopause structure and dynamics as well as stratosphere-troposphere exchange (STE) process in the Upper Troposphere and Lower Stratosphere (UTLS) region. In the present study, the impact of cyclones that occurred over the North Indian Ocean during 2007–2013 on the STE process is quantified using satellite observations. Tropopause characteristics during cyclones are obtained from the Global Positioning System (GPS) Radio Occultation (RO) measurements and ozone and water vapor concentrations in UTLS region are obtained from Aura-Microwave Limb Sounder (MLS) satellite observations. The effect of cyclones on the tropopause parameters is observed to be more prominent within 500 km from the centre of cyclone. In our earlier study we have observed decrease (increase) in the tropopause altitude (temperature) up to 0.6 km (3 K) and the convective outflow level increased up to 2 km. This change leads to a total increase in the tropical tropopause layer (TTL) thickness of 3 km within the 500 km from the centre of cyclone. Interestingly, an enhancement in the ozone mixing ratio in the upper troposphere is clearly noticed within 500 km from cyclone centre whereas the enhancement in the water vapor in the lower stratosphere is more significant on south-east side extending from 500–1000 km away from the cyclone centre. We estimated the cross-tropopause mass flux for different intensities of cyclones and found that the mean flux from stratosphere to troposphere for cyclonic stroms is 0.05 ± 0.29 × 10−3 kg m−2 and for very severe cyclonic stroms it is 0.5 ± 1.07 × 10−3 kg m−2. More downward flux is noticed in the north-west and south-west side of the cyclone centre. These results indicate that the cyclones have significant impact in effecting the tropopause structure, ozone and water vapour budget and consequentially the STE in the UTLS region.

scholarly journals A statistical analysis of the influence of deep convection on water vapor variability in the tropical upper troposphere

2009 ◽  
Vol 9 (15) ◽  
pp. 5847-5864 ◽  
Author(s):  
J. S. Wright ◽  
R. Fu ◽  
A. J. Heymsfield
Keyword(s):  
Water Vapor ◽  
Deep Convection ◽  
Tropical Rainfall Measuring Mission ◽  
Upper Troposphere ◽  
Ambient Relative Humidity ◽  
Wide Range ◽  
Ice Water Content ◽  
The Tropics ◽  
Ice Water ◽  
Tropical Upper Troposphere

Abstract. The factors that control the influence of deep convective detrainment on water vapor in the tropical upper troposphere are examined using observations from multiple satellites in conjunction with a trajectory model. Deep convection is confirmed to act primarily as a moisture source to the upper troposphere, modulated by the ambient relative humidity (RH). Convective detrainment provides strong moistening at low RH and offsets drying due to subsidence across a wide range of RH. Strong day-to-day moistening and drying takes place most frequently in relatively dry transition zones, where between 0.01% and 0.1% of Tropical Rainfall Measuring Mission Precipitation Radar observations indicate active convection. Many of these strong moistening events in the tropics can be directly attributed to detrainment from recent tropical convection, while others in the subtropics appear to be related to stratosphere-troposphere exchange. The temporal and spatial limits of the convective source are estimated to be about 36–48 h and 600–1500 km, respectively, consistent with the lifetimes of detrainment cirrus clouds. Larger amounts of detrained ice are associated with enhanced upper tropospheric moistening in both absolute and relative terms. In particular, an increase in ice water content of approximately 400% corresponds to a 10–90% increase in the likelihood of moistening and a 30–50% increase in the magnitude of moistening.

Manifestation of the Pacific Decadal Oscillation in the stationary planetary waves activity

2021 ◽  
Author(s):  
Daria Sobaeva ◽  
Yulia Zyulyaeva ◽  
Sergey Gulev
Keyword(s):  
Pacific Decadal Oscillation ◽  
North American ◽  
Lower Stratosphere ◽  
El Nino ◽  
Planetary Waves ◽  
Positive Phase ◽  
Negative Phase ◽  
Middle Troposphere ◽  
The Pacific ◽  
The Tropics

<p>Strong quasi-decadal oscillations of the stratospheric polar vortex (SPV) intensity are in phase with the Pacific decadal oscillation (PDO). A stronger SPV is observed during the positive phase of the PDO, and during the negative phase, the intensity of the SPV is below the mean climate values. The SPV intensity anomalies, formed by the planetary waves and zonal mean flow interaction, lead to the weakening/intensification of the vortex.</p><p>This research aimed to obtain the differences in the characteristics and the spatial propagation pattern of the planetary waves in the middle troposphere and lower stratosphere during different PDO phases. We analyzed composite periods of years when the PDO index has extremely high and low values. Two periods were constructed for both positive and negative phases, the first consisting of years with El-Nino/La-Nina events and the second without prominent sea surface temperature anomalies in the tropics. </p><p>During the wintertime in the Northern Hemisphere (December-February), wave 2 with two ridges (Siberian and North American Highs) and two troughs (Icelandic and Aleutian Lows) dominates in the middle troposphere, along with wave 1 dominating in the lower stratosphere. In the middle troposphere, at the positive phase ​​of the PDO, the amplitude of wave 2 is higher than in years with negative values of the PDO index. The differences in the Aleutian Low and the North American High intensity between the two phases are significant at the 97.5% level. In the lower stratosphere, the wave amplitude is lower at the negative phase ​​of the PDO, but we can also talk about a slight shift of the wave phase to the east. The regions of the heavy rains in the tropics during El-Nino events are the planetary waves source. They propagate from low to high latitudes, which results in modifying the characteristics and locations of the intensification of the stationary planetary waves in mid-latitudes.</p>

Water-vapor Measurements in the Lower Stratosphere

1974 ◽  
Vol 52 (8) ◽  
pp. 1527-1531 ◽  
Author(s):  
H. J. Mastenbrook
Keyword(s):  
Water Vapor ◽  
Lower Stratosphere ◽  
Marked Decrease ◽  
Vapor Concentration ◽  
Water Vapor Concentration ◽  
Mixing Ratio ◽  
Stratospheric Water Vapor ◽  
Mixing Ratios ◽  
Natural Concentration ◽  
General Range

Nearly 10 years of water-vapor measurements to heights of 30 km provide a basis for assessing the natural concentration of stratospheric water vapor and its variability. The measurements which began in 1964 have been made at monthly intervals from the mid-latitude location of Washington, D.C, using a balloon-borne frost-point hygrometer. The observations show the mixing ratio of water-vapor mass to air mass in the stratosphere to be in the general range of 1 to 4 p.p.m. with a modal concentration between 2 and 3 p.p.m. An annual cycle of mixing ratio is evident for the low stratosphere. A trend of water-vapor increase observed during the first 6 years does not persist beyond 1969 or 1970. The 6 year increase was followed by a marked decrease in 1971, with mixing ratios remaining generally below 3 p.p.m. thereafter. The measurements of recent years suggest that the series of observations may have begun during a period of low water-vapor concentration in the stratosphere.

scholarly journals Retrieval of water vapor vertical distributions in the upper troposphere and the lower stratosphere from SCIAMACHY limb measurements

2011 ◽  
Vol 4 (5) ◽  
pp. 933-954 ◽  
Author(s):  
A. Rozanov ◽  
K. Weigel ◽  
H. Bovensmann ◽  
S. Dhomse ◽  
K.-U. Eichmann ◽  
...  
Keyword(s):  
Water Vapor ◽  
Solar Radiation ◽  
Lower Stratosphere ◽  
Water Vapor Content ◽  
Retrieval Algorithm ◽  
Altitude Range ◽  
Upper Troposphere ◽  
Vertical Distributions ◽  
First Results ◽  
Scanning Imaging

Abstract. This study describes the retrieval of water vapor vertical distributions in the upper troposphere and lower stratosphere (UTLS) altitude range from space-borne observations of the scattered solar light made in limb viewing geometry. First results using measurements from SCIAMACHY (Scanning Imaging Absorption spectroMeter for Atmospheric CHartographY) aboard ENVISAT (Environmental Satellite) are presented here. In previous publications, the retrieval of water vapor vertical distributions has been achieved exploiting either the emitted radiance leaving the atmosphere or the transmitted solar radiation. In this study, the scattered solar radiation is used as a new source of information on the water vapor content in the UTLS region. A recently developed retrieval algorithm utilizes the differential absorption structure of the water vapor in 1353–1410 nm spectral range and yields the water vapor content in the 11–25 km altitude range. In this study, the retrieval algorithm is successfully applied to SCIAMACHY limb measurements and the resulting water vapor profiles are compared to in situ balloon-borne observations. The results from both satellite and balloon-borne instruments are found to agree typically within 10 %.

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