scholarly journals Amazonian BC Contribution to the Vallunaraju Glacier Surface Melt

2020 ◽  
Author(s):  
Wilmer Sánchez ◽  
Carl Schmitt ◽  
Alexzander Santiago ◽  
Gerles Medina
Keyword(s):  
Black Carbon ◽  
Forest Fires ◽  
Radiative Forcing ◽  
Dry Season ◽  
Decision Makers ◽  
Ablation Zone ◽  
Wet Season ◽  
Glacier Surface ◽  
Glacial Retreat

The role of Black Carbon (BC) as a contributor to glacial retreat is of particular interest to the scientific community and decision makers, due to its impact on snow albedo and glacier melt. In this study, a thermal-optical instrument (LAHM) was used to measure effective Black Carbon (eBC) in a series of surface snow samples collected from the Vallunaraju glacier, Cordillera Blanca, between April 2019 and May 2020. The time series obtained indicates a marked seasonal variability of eBC with maximum concentrations during the dry season and dramatic decrease during the wet season. The concentrations detected ranged between a minimum of 3.73 ng/g and 4.23 ng/g during the wet season and a maximum of 214.13 ng/g and 181.60 ng/g during the dry season, in the accumulation and ablation zone. Using SNICAR model, the reduction of albedo was estimated at 6.36% and 6.60% during the dry season and 0.68% and 0.95% during the wet season, which represents an average radiative forcing of 4.52 ± 1.84 W/m2 and 4.69 ± 1.59 W/m2 in the accumulation zone, and 0.49 ± 0.27 W/m2 and 0.68 ± 0.43 W/m2 in the ablation zone. The melting of snow due to the eBC translates into 80.18 ± 37.30 kg/m2 and 83.16 ± 32.75 kg/m2 during the dry season, and 7.91 ± 4.29 kg/m2 and 10.85 ± 6.62 kg/m2 during the wet season, in the accumulation and ablation zones, respectively. Finally, the HYSPLIT trajectory assessment shows that aerosols predominate in the Amazon rainforest, especially when forest fires are most abundant according to VIIRS images.

scholarly journals Glacier Geometry Changes in the Western Shore of Admiralty Bay, King George Island over the Last Decades

Sensors ◽  
2021 ◽  
Vol 21 (4) ◽  
pp. 1532
Author(s):  
Mariusz Pasik ◽  
Krzysztof Bakuła ◽  
Sebastian Różycki ◽  
Wojciech Ostrowski ◽  
Maria Elżbieta Kowalska ◽  
...  
Keyword(s):  
Protected Area ◽  
Average Rate ◽  
King George Island ◽  
Glacier Surface ◽  
Glacial Retreat ◽  
Glacier Front ◽  
Longitudinal Slope ◽  
Western Shore ◽  
Rapid Temperature

This paper presents changes in the range and thickness of glaciers in Antarctic Specially Protected Area (ASPA) No. 128 on King George Island in the period 1956–2015. The research indicates an intensification of the glacial retreat process over the last two decades, with the rate depending on the type of glacier front. In the period 2001–2015, the average recession rate of the ice cliffs of the Ecology Glacier and the northern part of the Baranowski Glacier was estimated to be approximately 15–25 m a−1 and 10–20 m a−1, respectively. Fronts of Sphinx Glacier and the southern part of the Baranowski Glacier, characterized by a gentle descent onto land, show a significantly lower rate of retreat (up to 5–10 m a−1 1). From 2001 to 2013, the glacier thickness in these areas decreased at an average rate of 1.7–2.5 m a−1 for the Ecology Glacier and the northern part of the Baranowski Glacier and 0.8–2.5 m a−1 for the southern part of the Baranowski Glacier and Sphinx Glacier. The presented deglaciation processes are related to changes of mass balance caused by the rapid temperature increase (1.0 °C since 1948). The work also contains considerations related to the important role of the longitudinal slope of the glacier surface in the connection of the glacier thickness changes and the front recession.

scholarly journals Aerosol characterisation including oxidative potential as a proxy of health impact

2019 ◽  
Vol 29 (2) ◽  
Author(s):  
Miroslav Josipovic ◽  
Catherine Leal-Liousse ◽  
Belinda Crobeddu ◽  
Armelle Baeza-Squiban ◽  
C. Keitumetse Segakweng ◽  
...  
Keyword(s):  
Organic Carbon ◽  
Black Carbon ◽  
Fine Fraction ◽  
Health Impact ◽  
Coarse Fraction ◽  
Dry Season ◽  
Wet Season ◽  
Oxidative Potential ◽  
Ionic Content ◽  
Vaal Triangle

This study aimed to characterise aerosols sampled in the vicinity of a major industrialised area, i.e. the Vaal Triangle. It included thedetermination of oxidative potential as a predictive indicator of particle toxicity. Aerosol samples were collated through the cascadefiltering during an eight-month period (12 h over three days in one week). Three size fractions were analysed for organic carbon(OC), black carbon (BC) and oxidative potential (OP), while ionic content was presented as monthly and seasonal concentrations. Thecontinuous measurement of black carbon by an optical attenuation instrument was collated concurrently with cascade filtering. Thecarbonaceous content was low compared to the ionic one. Within the carbonaceous concentrations, the organic carbon was higherthan concentrations of black carbon in both seasons in the ultra-fine fraction; the opposite was the case for the fine fraction, whilethe coarse fraction concentrations of organic carbon in the dry season had higher concentrations than black carbon in the wet seasonand organic carbon in the wet season. The OP tended to increase as the size was decreasing for wet season aerosols, whereas, forthe dry season, the highest OP was exerted by the fine fraction. The ultrafine fraction was the one showing the most contrasting OPbetween the two seasons. Continuous monitoring indicated that the higher BC concentrations were recorded in the dry/winter partof the year, with the daily pattern of concentrations being typically bimodal, having both the morning and evening peaks in bothseasons. Within the ionic content, the dominance of sulphate, nitrate and ammonium was evident. Multiple linear correlations wereperformed between all determined compounds. Strong correlations of carboxylic acids with other organic compounds were revealed.These acids point to emissions of VOC, both anthropogenic and biogenic. Since they were equally present in both seasons, a mixtureof sources was responsible, both present in the wider area and throughout the year.

Spatial and temporal heterogeneity in aerosol radiative effects over ecological area in south China: Composition and transmission implications

2020 ◽  
Author(s):  
Ma Yining ◽  
Xin Jinyuan
Keyword(s):  
Organic Carbon ◽  
Radiative Forcing ◽  
Dry Season ◽  
Water Soluble ◽  
Chemical Components ◽  
Radiative Effects ◽  
Wet Season ◽  
Cooling Effects ◽  
Ecological Region ◽  
Aerosol Radiative

<p><strong>Abstract:</strong> Ecological region in southern China has been perennially affected by monsoon climate and anthropogenic emissions, resulting in complex aerosol components and frequent long-range transport. In this study, a Santa Barbara DISORT Atmospheric Radiative Transfer (SBDART) model is applied to estimate aerosol radiative forcing (ARF) and multiple aerosol observation datasets is used to estimate the aerosol chemical components and optical properties. The aerosol loading and the radiative effects in the ecological region exhibited strong seasonal changes. The average major components (NH<sub>4</sub><sup>+</sup>, NO<sub>3</sub><sup>−</sup>, SO<sub>4</sub><sup>2−</sup>) in Total water soluble ionic (TWSI) ,organic carbon (OC) concentration, the ratio of organic carbon to element carbon (OC/EC) and biogenic secondary organic aerosol (BSOA) tracers were 3.20±1.22 μg·m<sup>-3</sup>, 2.19±1.39 μg·m<sup>-3</sup>, 3.17 and 74.00±35.23 ng·m<sup>-3 </sup>in the dry season and 2.22±0.91 μg·m<sup>-3</sup>, 3.14±1.62 μg·m<sup>-3</sup>, 7.13 and 186.34±113.82 ng·m<sup>-3</sup> in the wet season, respectively. The average radiative forcing at the top of atmosphere (TOA) is -11.73±11.36 W/m<sup>2</sup> and -0.41±10.08 W/m<sup>2</sup> in dry and wet season. When the aerosol single scattering albedo (SSA) less than 0.9, the retrieve frequency in wet season reached account for 75%. The increase of OC and BSOA transformed by forests in the wet season weaken the cooling effects. However, the dry season is mainly composed of anthropogenic inorganic aerosols, which enhances the scattering effect. The aerosol observation baseline also verified the seasonal variation of ARF in the ecological region. Driven by multiple factors such as meteorological conditions, emission sources, and the mixed state of particulate matter, the transport patterns of air masses in ecological area exhibits completely opposite affects to ARF.</p>

scholarly journals Origin of water-soluble organic aerosols at the Maïdo high-altitude observatory, Réunion Island in the tropical Indian Ocean

2021 ◽  
Author(s):  
Sharmine Akter Simu ◽  
Yuzo Miyazaki ◽  
Eri Tachibana ◽  
Henning Finkenzeller ◽  
Jérôme Brioude ◽  
...  
Keyword(s):  
Indian Ocean ◽  
High Altitude ◽  
Radiative Forcing ◽  
Numerical Models ◽  
Stable Carbon Isotope ◽  
Organic Aerosols ◽  
Dry Season ◽  
Water Soluble ◽  
Spatial And Temporal Variation ◽  
Wet Season

Abstract. The tropical and subtropical Indian Ocean (IO) is expected to be a significant source of water-soluble organic aerosols (WSOAs), which are important factors relevant to cloud condensation nuclei and ice nuclei of aerosol particles. Current atmospheric numerical models significantly underestimate the budget of organic aerosols and their precursors, especially over tropical oceans. This is primarily due to poor knowledge of sources and the paucity of observations of these parameters considering spatial and temporal variation over the tropical open ocean. To evaluate the contribution of sources to WSOA as well as their formation processes, submicrometer aerosol sampling was conducted at the high-altitude Maïdo observatory (21.1° S, 55.4° E, 2,160 m a.s.l), located on the remote island of La Réunion in the southwest IO. The aerosol samples were continuously collected during local daytime and nighttime, which corresponded to the ambient conditions of the marine boundary layer (MBL) and free troposphere (FT), respectively, from March 15 to May 24, 2018. Chemical analysis showed that organic matter was the dominant component of submicrometer water-soluble aerosol (~45 ± 17 %) during the wet season (March 15–April 23), whereas sulfate dominated (~77 ± 17 %) during the dry season (April 24–May 24). Measurements of the stable carbon isotope ratio of water-soluble organic carbon (WSOC) suggested that marine sources contributed significantly to the observed WSOC mass in both the MBL and the FT in the wet season, whereas a mixture of marine and terrestrial sources contributed to WSOC in the dry season. The distinct seasonal changes in the dominant source of WSOC were also supported by Lagrangian trajectory analysis. Positive matrix factorization analysis suggested that marine secondary OA dominantly contributed to the observed WSOC mass (~70 %) during the wet season, whereas mixtures of marine and terrestrial sources contributed during the dry season in both MBL and FT. Overall, this study demonstrates that the effect of marine secondary sources is likely important up to the FT in the wet season, which may be responsible for cloud formation as well as direct radiative forcing over oceanic regions.

scholarly journals Amplification of black carbon light absorption induced by atmospheric aging: temporal variation at seasonal and diel scales in urban Guangzhou

2019 ◽  
Author(s):  
Jia Yin Sun ◽  
Cheng Wu ◽  
Dui Wu ◽  
Chunlei Cheng ◽  
Mei Li ◽  
...  
Keyword(s):  
Optical Properties ◽  
Organic Carbon ◽  
Black Carbon ◽  
Light Absorption ◽  
Dry Season ◽  
Diurnal Fluctuation ◽  
Absorption Enhancement ◽  
Wet Season ◽  
Diurnal Variability ◽  
The Impact

Abstract. Black carbon (BC) is an important climate forcer in the atmosphere. Amplification of light absorption can occur by coatings on BC aerosols, an effect that remains one of the major sources of uncertainties for accessing the radiative forcing of BC. In this study, the absorption enhancement factor (Eabs) was quantified by the minimum R squared (MRS) method using elemental carbon (EC) as the tracer. Two field campaigns were conducted in urban Guangzhou at the Jinan university super site during both wet season (July 31–September 10, 2017) and dry season (November 15, 2017–January 15, 2018) to explore the temporal dynamics of BC optical properties. The average concentration of EC was 1.94 ± 0.93 and 2.81 ± 2.01 μgC m−3 in the wet and dry seasons, respectively. Mass absorption efficiency at 520 nm by primary aerosols (MAEp520) determined by MRS exhibit a strong seasonality (8.6 m2g−1 in the wet season and 16.8 m2g−1 in the dry season). Eabs520 was higher in the wet season (1.51 ± 0.50) and lower in the dry season (1.29 ± 0.28). Absorption Ångström exponent (AAE470-660) in the dry season (1.46 ± 0.12) were higher than that in the wet season (1.37 ± 0.10). Collective evidence showed that the active biomass burning (BB) in dry season effectively altered optical properties of BC, leading to elevated MAE, MAEp and AAE in dry season comparing to those in wet season. Diurnal Eabs520 was positively correlated with AAE470-660 (R2 = 0.71) and negatively correlated with the AE33 aerosol loading compensation parameter (k) (R2 = 0.74) in the wet season, but these correlations were significantly weaker in the dry season, which may be related to the impact of BB. This result suggests that lensing effect was dominating the AAE diurnal variability during the wet season. The effect of secondary processing on Eabs diurnal dynamic were also investigated. The Eabs520 exhibit a clear dependency on secondary organic carbon to organic carbon ratio (SOC/OC). Eabs520 correlated well with nitrate, implying that gas-particle partitioning of semi-volatile compounds may potentially play an important role in steering the diurnal fluctuation of Eabs520. In dry season, the diurnal variability of Eabs520 was associated with photochemical aging as evidenced by the good correlation (R2 = 0.69) between oxidant concentrations (Ox=O3+NO2) and Eabs520.

scholarly journals Snow-darkening versus direct radiative effects of mineral dust aerosol on the Indian summer monsoon onset: role of temperature change over dust sources

2019 ◽  
Vol 19 (3) ◽  
pp. 1605-1622 ◽  
Author(s):  
Zhengguo Shi ◽  
Xiaoning Xie ◽  
Xinzhou Li ◽  
Liu Yang ◽  
Xiaoxun Xie ◽  
...  
Keyword(s):  
Tibetan Plateau ◽  
Central Asia ◽  
Black Carbon ◽  
Summer Monsoon ◽  
Indian Summer Monsoon ◽  
Radiative Forcing ◽  
Indian Monsoon ◽  
Indian Subcontinent ◽  
Direct Radiative Forcing

Abstract. Atmospheric absorptive aerosols exert complicated effects on the climate system, two of which are through their direct radiative forcing and snow-darkening forcing. Compared to black carbon, the snow-darkening effect of dust on climate has been scarcely explored till now. When depositing in snow, dust can reduce the albedo of snow by darkening it and increasing the snowmelt. In this study, the snow-darkening effect of dust, as well as the direct radiative effect, on the Indian summer monsoon are evaluated by atmospheric general circulation model experiments. The results show that the snow-darkening and direct radiative forcing of dust both have significant impacts on the onset of the Indian monsoon, but they are distinctly opposite. The snow-darkening effect of dust weakens the Indian monsoon precipitation during May and June, opposite to black carbon. The surface temperature over central Asia and the western Tibetan Plateau becomes warmer due to the dust-induced decrease in snow cover, which leads to a local low-level cyclonic anomaly as well as an anticyclonic anomaly over the Indian subcontinent and Arabian Sea. This circulation pattern allows air currents penetrating into the Indian subcontinent more from central Asia but less from the Indian Ocean. In contrast, the direct radiative forcing of dust warms the low troposphere over the Arabian Peninsula, which intensifies moisture convergence and precipitation over the Indian monsoon region. The upper tropospheric atmospheric circulation over Asia is also sensitive to both effects. Compared to previous studies which emphasized the temperature over the Tibetan Plateau, our results further highlight an important role of surface/low tropospheric temperature changes over dust source areas, which can also significantly modify the response of summer monsoon. Thus, links between the climatic impact of dust and complicated thermal conditions over Asia are of importance and need to be clarified accurately.

scholarly journals Anthropogenic aerosol radiative forcing in Asia derived from regional models with atmospheric and aerosol data assimilation

2010 ◽  
Vol 10 (13) ◽  
pp. 6007-6024 ◽  
Author(s):  
C. E. Chung ◽  
V. Ramanathan ◽  
G. Carmichael ◽  
S. Kulkarni ◽  
Y. Tang ◽  
...  
Keyword(s):  
Interannual Variability ◽  
Radiative Forcing ◽  
Dry Season ◽  
Heating Rates ◽  
Wet Season ◽  
Aerosol Chemistry ◽  
Anthropogenic Aerosol ◽  
Anthropogenic Forcing ◽  
Aerosol Radiative Forcing ◽  
Aerosol Forcing

Abstract. An estimate of monthly 3-D aerosol solar heating rates and surface solar fluxes in Asia from 2001 to 2004 is described here. This product stems from an Asian aerosol assimilation project, in which a) the PNNL regional model bounded by the NCEP reanalyses was used to provide meteorology, b) MODIS and AERONET data were integrated for aerosol observations, c) the Iowa aerosol/chemistry model STEM-2K1 used the PNNL meteorology and assimilated aerosol observations, and d) 3-D (X-Y-Z) aerosol simulations from the STEM-2K1 were used in the Scripps Monte-Carlo Aerosol Cloud Radiation (MACR) model to produce total and anthropogenic aerosol direct solar forcing for average cloudy skies. The MACR model and STEM-2K1 both used the PNNL model resolution of 0.45°×0.4° in the horizontal and of 23 layers in the troposphere. The 2001–2004 averaged anthropogenic all-sky aerosol forcing is −1.3 Wm−2 (TOA), +7.3 Wm−2 (atmosphere) and −8.6 Wm−2 (surface) averaged in Asia (60–138° E and Equator–45° N). In the absence of AERONET SSA assimilation, absorbing aerosol concentration (especially BC aerosol) is much smaller, giving −2.3 Wm−2 (TOA), +4.5 Wm−2 (atmosphere) and −6.8 Wm−2 (surface), averaged in Asia. In the vertical, monthly forcing is mainly concentrated below 600 hPa with maximum around 800 hPa. Seasonally, low-level forcing is far larger in dry season than in wet season in South Asia, whereas the wet season forcing exceeds the dry season forcing in East Asia. The anthropogenic forcing in the present study is similar to that in Chung et al. (2005) in overall magnitude but the former offers fine-scale features and simulated vertical profiles. The interannual variability of the computed anthropogenic forcing is significant and extremely large over major emission outflow areas. Given the interannual variability, the present study's estimate is within the implicated range of the 1999 INDOEX result.

scholarly journals Black Carbon Emissions from the Siberian Fires 2019: Modelling of the Atmospheric Transport and Possible Impact on the Radiation Balance in the Arctic Region

Atmosphere ◽  
2021 ◽  
Vol 12 (7) ◽  
pp. 814
Author(s):  
Sergey Kostrykin ◽  
Anastasia Revokatova ◽  
Alexey Chernenkov ◽  
Veronika Ginzburg ◽  
Polina Polumieva ◽  
...  
Keyword(s):  
Black Carbon ◽  
Forest Fires ◽  
Radiative Forcing ◽  
Climate Model ◽  
Arctic Region ◽  
The Arctic ◽  
Radiation Balance ◽  
Climatic Effects ◽  
Fire Emissions ◽  
Trajectory Model

The work is devoted to the study of the climatic effects of black carbon (BC) transferred from forest fires to the Arctic zone. The HYSPLIT (The Hybrid Single-Particle Lagrangian Integrated Trajectory model) trajectory model was used to initially assess the potential for particle transport from fires. The results of the trajectory analysis of the 2019 fires showed that the probability of the transfer of particles to the Arctic ranges from 1% to 10%, and in some cases increases to 20%. Detailed studies of the possible influence of BC ejected as a result of fires became possible by using the climate model of the INMCM5 (Institute of Numerical Mathematics Climate Model). The results of the numerical experiments have shown that the maximum concentration of BC in the Arctic atmosphere is observed in July and August and is associated with emissions from fires. The deposition of BC in the Arctic increases by about 1.5–2 times in the same months, in comparison with simulation without forest fire emissions. This caused an average decrease in solar radiation forcing of 0.3–0.4 Wt/m2 and an increase in atmospheric radiation heating of up to 5–6 Wt/m2. To assess the radiation forcing from BC contaminated snow, we used the dependences of the change in the snow albedo on the snow depth, and the albedo of the underlying surface for a given amount of BC fallen on the snow. These dependences were constructed on the basis of the SNICAR (Snow, Ice, and Aerosol Radiative) model. According to our calculations, the direct radiative forcing from BC in the atmosphere with a clear sky is a maximum of 4–5 W/m2 in July and August.

scholarly journals Non-structural carbohydrates mediate seasonal water stress across Amazon forests

2021 ◽  
Vol 12 (1) ◽  
Author(s):  
Caroline Signori-Müller ◽  
Rafael S. Oliveira ◽  
Fernanda de Vasconcellos Barros ◽  
Julia Valentim Tavares ◽  
Martin Gilpin ◽  
...  
Keyword(s):  
Water Stress ◽  
Tree Species ◽  
Tree Mortality ◽  
Soluble Sugar ◽  
Dry Season ◽  
Future Climate Change ◽  
Wet Season ◽  
Dry Conditions ◽  
Almost All

AbstractNon-structural carbohydrates (NSC) are major substrates for plant metabolism and have been implicated in mediating drought-induced tree mortality. Despite their significance, NSC dynamics in tropical forests remain little studied. We present leaf and branch NSC data for 82 Amazon canopy tree species in six sites spanning a broad precipitation gradient. During the wet season, total NSC (NSCT) concentrations in both organs were remarkably similar across communities. However, NSCT and its soluble sugar (SS) and starch components varied much more across sites during the dry season. Notably, the proportion of leaf NSCT in the form of SS (SS:NSCT) increased greatly in the dry season in almost all species in the driest sites, implying an important role of SS in mediating water stress in these sites. This adjustment of leaf NSC balance was not observed in tree species less-adapted to water deficit, even under exceptionally dry conditions. Thus, leaf carbon metabolism may help to explain floristic sorting across water availability gradients in Amazonia and enable better prediction of forest responses to future climate change.

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