Detecting halfmetallic electronic structures of spintronic materials in a magnetic field
Abstract Band-gap engineering is one of the fundamental techniques in semiconductor technology and also applicable in the next generation spintronics using the spin degrees of freedom. To fully utilize the spintronic material, it is essential to optimize the spin-dependent electronic structures in the operando conditions by applying the magnetic and/or electric fields. Here we present a new spectroscopic technique to probe the spin-polarized electronic structures by using magnetic circular dichroism (MCD) in the resonant inelastic soft X-ray scattering (RIXS) under an external magnetic field. Thanks to the spin-selective dipole-allowed transitions in the RIXS-MCD, we have successfully demonstrated the direct evidence of the perfectly spin-polarized electronic structures for the prototypical halfmetallic Heusller alloy, Co2MnSi. The RIXS-MCD is a promising tool to probe the spin-dependent carriers and band-gap with element specific way induced in the buried magnetic layers under the operando conditions.