Biomass burning pollution products C2H6, C2H2, HCOOH, and PAN in the Southern hemisphere UTLS region observed by the GLORIA instrument during the SouthTRAC HALO aircraft campaign Sep-Nov 2019

Author(s):  
Felix Friedl-Vallon ◽  
Jörn Ungermann ◽  
Sören Johansson ◽  
Gerald Wetzel ◽  
Markus Geldenhuys ◽  
...  

<p>The Gimballed Limb Observer for Radiance Imaging of the Atmosphere (GLORIA) is an imaging Fourier transform spectrometer (iFTS) using a 2-dimensional detector array to record emission spectra in the mid-infrared region with high spatial resolution. GLORIA has been operated on the High Altitude and Long Range Research Aircraft (HALO) during the SouthTRAC campaign in September-November 2019. The campaign with base in Rio Grande (Tierra del Fuego) consisted of two observational periods, mainly in September and November 2019. Apart from many local flights, between the two phases HALO returned to Germany which allowed us to acquire long-range hemispheric cross-sections.</p><p>Two dimensional distributions of pollution species like C<sub>2</sub>H<sub>6</sub>, C<sub>2</sub>H<sub>2</sub>, HCOOH, and PAN, which are produced as primary and secondary products from biomass burning sources have been derived from the GLORIA observations. We will show that during the hemispheric cross sections as well as during some of the local flights, GLORIA observed pollution plumes with extensions of many kilometres in altitude and hundreds of kilometres horizontally with strongly enhanced concentrations of these species.</p><p>Trajectory analysis as well as comparisons to Microwave Limb Sounder (MLS) satellite observations show that the origin of plumes are mainly fires in South America and Africa, but also first signs of the Australian bush fires have been detected in the UTLS as early as November 2019.</p>

2020 ◽  
Author(s):  
Gerald Wetzel ◽  
Felix Friedl-Vallon ◽  
Norbert Glatthor ◽  
Jens-Uwe Grooß ◽  
Thomas Gulde ◽  
...  

<p>The Gimballed Limb Observer for Radiance Imaging of the Atmosphere (GLORIA) is an imaging Fourier transform spectrometer (iFTS) using a 2-dimensional detector array to record emission spectra in the mid-infrared region with high spatial resolution. GLORIA is operated on high altitude research aircraft, mainly in the limb observational geometry to measure vertical profiles of temperature and atmospheric trace species with high vertical resolution.</p><p>In autumn 2017, the Wave-driven ISentropic Exchange (WISE) aircraft campaign took place from Shannon (Ireland). Sixteen flights with the High Altitude and Long Range Research Aircraft (HALO) were performed between 31 August and 21 October 2017 over the eastern North Atlantic region.</p><p>GLORIA observations were analysed with regard to pollutant species like C<sub>2</sub>H<sub>6</sub>, C<sub>2</sub>H<sub>2</sub>, HCOOH, and PAN, which are produced at distinct source regions near the ground and transported to remote regions due to their atmospheric lifetime of several weeks. Enhanced volume mixing ratios of these molecules were detected along some parts of the flight track in the upper troposphere and lowermost stratosphere (UTLS).</p><p>Measured profiles of these species are compared to simulations from the ECHAM/MESSy Atmospheric Chemistry (EMAC) model and reanalysis data from the Copernicus Atmosphere Monitoring Service (CAMS). Furthermore, emission tracers and back-trajectories from the Chemical Lagrangian Model of the Stratosphere (CLaMS) are used to analyse the source regions of these pollution events.</p>


2012 ◽  
Vol 12 (9) ◽  
pp. 3837-3855 ◽  
Author(s):  
J. S. Fu ◽  
N. C. Hsu ◽  
Y. Gao ◽  
K. Huang ◽  
C. Li ◽  
...  

Abstract. To evaluate the impact of biomass burning from Southeast Asia to East Asia, this study conducted numerical simulations during NASA's 2006 Biomass-burning Aerosols in South-East Asia: Smoke Impact Assessment (BASE-ASIA). Two typical episode periods (27–28 March and 13–14 April) were examined. Two emission inventories, FLAMBE and GFED, were used in the simulations. The influences during two episodes in the source region (Southeast Asia) contributed to the surface CO, O3 and PM2.5 concentrations as high as 400 ppbv, 20 ppbv and 80 μg m−3, respectively. The perturbations with and without biomass burning of the above three species during the intense episodes were in the range of 10 to 60%, 10 to 20% and 30 to 70%, respectively. The impact due to long-range transport could spread over the southeastern parts of East Asia and could reach about 160 to 360 ppbv, 8 to 18 ppbv and 8 to 64 μg m−3 on CO, O3 and PM2.5, respectively; the percentage impact could reach 20 to 50% on CO, 10 to 30% on O3, and as high as 70% on PM2.5. In March, the impact of biomass burning mainly concentrated in Southeast Asia and southern China, while in April the impact becomes slightly broader and even could go up to the Yangtze River Delta region. Two cross-sections at 15° N and 20° N were used to compare the vertical flux of biomass burning. In the source region (Southeast Asia), CO, O3 and PM2.5 concentrations had a strong upward transport from surface to high altitudes. The eastward transport becomes strong from 2 to 8 km in the free troposphere. The subsidence process during the long-range transport contributed 60 to 70%, 20 to 50%, and 80% on CO, O3 and PM2.5, respectively to surface in the downwind area. The study reveals the significant impact of Southeastern Asia biomass burning on the air quality in both local and downwind areas, particularly during biomass burning episodes. This modeling study might provide constraints of lower limit. An additional study is underway for an active biomass burning year to obtain an upper limit and climate effects.


2011 ◽  
Vol 11 (12) ◽  
pp. 32205-32243 ◽  
Author(s):  
J. S. Fu ◽  
N. C. Hsu ◽  
Y. Gao ◽  
K. Huang ◽  
C. Li ◽  
...  

Abstract. To evaluate the impact of biomass burning from Southeast Asia to East Asia, this study conducted numerical simulations during NASA's 2006 Biomass-burning Aerosols in South-East Asia: Smoke Impact Assessment (BASE-ASIA). Two typical episode periods (27–28 March and 13–14 April) were examined. Two emission inventories, FLAMBE and GFED, were used in the simulations. The influences during two episodes in the source region (Southeast Asia) contributed to the surface CO, O3 and PM2.5 concentrations as high as 400 ppbv, 20 ppbv and 80 μg m−3, respectively. The perturbations with and without biomass burning of the above three species during the intense episodes were in the range of 10 to 60%, 10 to 20% and 30 to 70%, respectively. The impact due to long-range transport could spread over the southeastern parts of East Asia and could reach about 160 to 360 ppbv, 8 to 18 ppbv and 8 to 64 μg m−3 on CO, O3 and PM2.5, respectively; the percentage impact could reach 20 to 50% on CO, 10 to 30% on O3, and as high as 70% on PM2.5. In March, the impact of biomass burning was mainly concentrated in Southeast Asia and Southern China, while in April the impact becomes slightly broader, potentially including the Yangtze River Delta region. Two cross-sections at 15° N and 20° N were used to compare the vertical flux of biomass burning. In the source region (Southeast Asia), CO, O3 and PM2.5 concentrations had a strong upward transport from surface to high altitudes. The eastward transport becomes strong from 2 to 8 km in the free troposphere. The subsidence process during the long-range transport contributed 60 to 70%, 20 to 50%, and 80% to CO, O3 and PM2.5, respectively to surface in the downwind area. The study reveals the significant impact of Southeastern Asia biomass burning on the air quality in both local and downwind areas, particularly during biomass burning episodes. This modeling study might provide lower limit constraints. An additional study is underway for an active biomass burning year to obtain an upper limit and climate effects.


2016 ◽  
Author(s):  
Norbert Glatthor ◽  
Michael Höpfner ◽  
Adrian Leyser ◽  
Gabriele P. Stiller ◽  
Thomas von Clarmann ◽  
...  

Abstract. We present a global OCS data set covering the period June 2002 to April 2012, derived from FTIR limb emission spectra measured with the Michelson Interferometer for Passive Atmospheric Sounding (MIPAS) on the ENVISAT satellite. The vertical resolution is 4–5 km in the height region 6–15 km and 15 km at 40 km altitude. The total estimated error amounts to 40–50 pptv between 10 and 20 km and to 120 pptv at 40 km altitude. MIPAS OCS data show no systematic bias with respect to balloon observations, with deviations mostly below ±50 pptv. However, they are systematically higher than the OCS volume mixing ratios of the ACE-FTS instrument on SCISAT, with maximum deviations of up to 100 pptv in the altitude region 13–16 km. The data set of MIPAS OCS exhibits only moderate interannual variations and low interhemispheric differences. Average concentrations at 10 km altitude range from 480 pptv at high latitudes to 500–510 pptv in the tropics and at northern mid-latitudes. Seasonal variations at 10 km altitude amount up to 35 pptv in the northern and up to 15 pptv in the southern hemisphere. Northern hemispheric OCS abundances at 10 km altitude peak in June in the tropics and around October at high latitudes, while the respective southern hemispheric maxima were observed in July and in November. Global OCS distributions at 250 hPa (~ 10–11 km) show enhanced values at low latitudes, peaking during boreal summer above the western Pacific and the Indian Ocean, which indicates oceanic release. Further, a region of depleted OCS amounts extending from Brazil to central and southern Africa was detected at this altitude, which is most pronounced in austral summer. This depletion is related to seasonally varying vegetative uptake by the tropical forests. Typical signatures of biomass burning like the southern hemispheric biomass burning plume are not visible in MIPAS data, indicating that this process is only a minor source of tropospheric OCS. At the 150 hPa level (~ 13–14 km) enhanced amounts of OCS were also observed inside the Asian Monsoon Anticyclone, but this enhancement is not especially outstanding as compared to other low latitude regions at the same altitude. At the 80 hPa level (~ 17–18 km) equatorward transport of mid-latitude air masses containing lower OCS amounts around the summertime anticyclones was observed. A significant trend could not be detected in tropospheric MIPAS OCS amounts, which points to globally balanced sources and sinks.


2019 ◽  
Vol 244 ◽  
pp. 414-422 ◽  
Author(s):  
Katsushige Uranishi ◽  
Fumikazu Ikemori ◽  
Hikari Shimadera ◽  
Akira Kondo ◽  
Seiji Sugata

2016 ◽  
Vol 16 (18) ◽  
pp. 12329-12345 ◽  
Author(s):  
Jessie M. Creamean ◽  
Paul J. Neiman ◽  
Timothy Coleman ◽  
Christoph J. Senff ◽  
Guillaume Kirgis ◽  
...  

Abstract. Biomass burning plumes containing aerosols from forest fires can be transported long distances, which can ultimately impact climate and air quality in regions far from the source. Interestingly, these fires can inject aerosols other than smoke into the atmosphere, which very few studies have evidenced. Here, we demonstrate a set of case studies of long-range transport of mineral dust aerosols in addition to smoke from numerous fires (including predominantly forest fires and a few grass/shrub fires) in the Pacific Northwest to Colorado, US. These aerosols were detected in Boulder, Colorado, along the Front Range using beta-ray attenuation and energy-dispersive X-ray fluorescence spectroscopy, and corroborated with satellite-borne lidar observations of smoke and dust. Further, we examined the transport pathways of these aerosols using air mass trajectory analysis and regional- and synoptic-scale meteorological dynamics. Three separate events with poor air quality and increased mass concentrations of metals from biomass burning (S and K) and minerals (Al, Si, Ca, Fe, and Ti) occurred due to the introduction of smoke and dust from regional- and synoptic-scale winds. Cleaner time periods with good air quality and lesser concentrations of biomass burning and mineral metals between the haze events were due to the advection of smoke and dust away from the region. Dust and smoke present in biomass burning haze can have diverse impacts on visibility, health, cloud formation, and surface radiation. Thus, it is important to understand how aerosol populations can be influenced by long-range-transported aerosols, particularly those emitted from large source contributors such as wildfires.


Author(s):  
Hervé Petetin ◽  
Bastien Sauvage ◽  
Mark Parrington ◽  
Hannah Clark ◽  
Alain Fontaine ◽  
...  

<p><strong>Abstract.</strong> This study investigates the role of biomass burning and long-range transport in the anomalies of carbon monoxide (CO) regularly observed along the tropospheric vertical profiles measured in the framework of IAGOS. Considering the high interannual variability of biomass burning emissions and the episodic nature of pollution long-range transport, one strength of this study is the amount of data taken into account, namely 30,000 vertical profiles at 9 clusters of airports in Europe, North America, Asia, India and southern Africa over the period 2002&amp;ndash;2017. </p> <p> As a preliminary, a brief overview of the spatio-temporal variability, latitudinal distribution, interannual variability and trends of biomass burning CO emissions from 14 regions is provided. The distribution of CO mixing ratios at different levels of the troposphere is also provided based on the entire IAGOS database (125 million CO observations). </p> <p> This study focuses on the free troposphere (altitudes above 2<span class="thinspace"></span>km) where the long-range transport of pollution is favoured. Anomalies at a given airport cluster are here defined as departures from the local seasonally-averaged climatological vertical profile. The intensity of these anomalies varies significantly depending on the airport, with maximum (minimum) CO anomalies of 110&amp;ndash;150 (48)<span class="thinspace"></span>ppbv in Asia (Europe). Looking at the seasonal variation of the frequency of occurrence, the 25<span class="thinspace"></span>% strongest CO anomalies appears reasonably well distributed along the year, in contrast to the 5<span class="thinspace"></span>% or 1<span class="thinspace"></span>% strongest anomalies that exhibit a strong seasonality with for instance more frequent anomalies during summertime in northern United-States, during winter/spring in Japan, during spring in South-east China, during the non-monsoon seasons in south-east Asia and south India, and during summer/fall at Windhoek, Namibia. Depending on the location, these strong anomalies are observed in different parts of the free troposphere. </p> <p> In order to investigate the role of biomass burning emissions in these anomalies, we used the SOFT-IO v1.0 IAGOS added-value products that consist of FLEXPART 20-days backward simulations along all IAGOS aircraft trajectories, coupled with anthropogenic (MACCity) and biomass burning (GFAS) CO emission inventories and vertical injections. SOFT-IO estimates the contribution (in ppbv) of the recent (less than 20 days) primary worldwide CO emissions, tagged per source region. Biomass burning emissions are found to play an important role in the strongest CO anomalies observed at most airport clusters. The regional tags indicate a large contribution from boreal regions at airport clusters in Europe and North America during summer season. In both Japan and south India, the anthropogenic emissions dominate all along the year, except for the strongest summertime anomalies observed in Japan that are due to Siberian fires. The strongest CO anomalies at airport clusters located in south-east Asia are induced by fires burning during spring in south-east Asia and during fall in equatorial Asia. In southern Africa, the Windhoek airport was mainly impacted by fires in southern hemisphere Africa and South America. </p> <p> To our knowledge, no other studies have used such a large dataset of in situ vertical profiles for deriving a climatology of the impact of biomass burning versus anthropogenic emissions on the strongest CO anomalies observed in the troposphere, in combination with information on the source regions. This study therefore provides both qualitative and quantitative information for interpreting the highly variable CO vertical distribution in several regions of interest.</p>


2016 ◽  
Vol 9 (5) ◽  
pp. 2015-2042 ◽  
Author(s):  
Florian Ewald ◽  
Tobias Kölling ◽  
Andreas Baumgartner ◽  
Tobias Zinner ◽  
Bernhard Mayer

Abstract. The new spectrometer of the Munich Aerosol Cloud Scanner (specMACS) is a multipurpose hyperspectral cloud and sky imager designated, but is not limited to investigations of cloud–aerosol interactions in Earth's atmosphere. With its high spectral and spatial resolution, the instrument is designed to measure solar radiation in the visible and shortwave infrared region that is reflected from, or transmitted through clouds and aerosol layers. It is based on two hyperspectral cameras that measure in the solar spectral range between 400 and 2500 nm with a spectral bandwidth between 2.5 and 12.0 nm. The instrument was operated in ground-based campaigns as well as aboard the German High Altitude LOng Range (HALO) research aircraft, e.g., during the ACRIDICON-CHUVA campaign in Brazil during summer 2014. This paper describes the specMACS instrument hardware and software design and characterizes the instrument performance. During the laboratory characterization of the instrument, the radiometric response as well as the spatial and spectral resolution was assessed. Since the instrument is primarily intended for retrievals of atmospheric quantities by inversion of radiative models using measured radiances, a focus is placed on the determination of its radiometric response. Radiometric characterization was possible for both spectrometers, with an absolute accuracy of 3 % at their respective central wavelength regions. First measurements are presented which demonstrate the wide applicability of the instrument. They show that key demands are met regarding the radiometric and spectral accuracy which is required for the intended remote sensing techniques.


2021 ◽  
Vol 21 (1) ◽  
pp. 357-392
Author(s):  
Igor B. Konovalov ◽  
Nikolai A. Golovushkin ◽  
Matthias Beekmann ◽  
Meinrat O. Andreae

Abstract. Long-range transport of biomass burning (BB) aerosol from regions affected by wildfires is known to have a significant impact on the radiative balance and air quality in receptor regions. However, the changes that occur in the optical properties of BB aerosol during long-range transport events are insufficiently understood, limiting the adequacy of representations of the aerosol processes in chemistry transport and climate models. Here we introduce a framework to infer and interpret changes in the optical properties of BB aerosol from satellite observations of multiple BB plumes. Our framework includes (1) a procedure for analysis of available satellite retrievals of the absorption and extinction aerosol optical depths (AAOD and AOD) and single-scattering albedo (SSA) as a function of the BB aerosol photochemical age and (2) a representation of the AAOD and AOD evolution with a chemistry transport model (CTM) involving a simplified volatility basis set (VBS) scheme with a few adjustable parameters. We apply this framework to analyze a large-scale outflow of BB smoke plumes from Siberia toward Europe that occurred in July 2016. We use AAOD and SSA data derived from OMI (Ozone Monitoring Instrument) satellite measurements in the near-UV range along with 550 nm AOD and carbon monoxide (CO) columns retrieved from MODIS (Moderate Resolution Imaging Spectroradiometer) and IASI (Infrared Atmospheric Sounding Interferometer) satellite observations, respectively, to infer changes in the optical properties of Siberian BB aerosol due to its atmospheric aging and to get insights into the processes underlying these changes. Using the satellite data in combination with simulated data from the CHIMERE CTM, we evaluate the enhancement ratios (EnRs) that allow isolating AAOD and AOD changes due to oxidation and gas–particle partitioning processes from those due to other processes, including transport, deposition, and wet scavenging. The behavior of EnRs for AAOD and AOD is then characterized using nonlinear trend analysis. It is found that the EnR for AOD strongly increases (by about a factor of 2) during the first 20–30 h of the analyzed evolution period, whereas the EnR for AAOD does not exhibit a statistically significant increase during this period. The increase in AOD is accompanied by a statistically significant enhancement of SSA. Further BB aerosol aging (up to several days) is associated with a strong decrease in EnRs for both AAOD and AOD. Our VBS simulations constrained by the observations are found to be more consistent with satellite observations of strongly aged BB plumes than “tracer” simulations in which atmospheric transformations of BB organic aerosol were disregarded. The simulation results indicate that the upward trends in EnR for AOD and in SSA are mainly due to atmospheric processing of secondary organic aerosol (SOA), leading to an increase in the mass scattering efficiency of BB aerosol. Evaporation and chemical fragmentation of the SOA species, part of which is assumed to be absorptive (to contain brown carbon), are identified as likely reasons for the subsequent decrease in the EnR for both AAOD and AOD. Hence, our analysis reveals that the long-range transport of smoke plumes from Siberian fires is associated with major changes in BB aerosol optical properties and chemical composition. Overall, this study demonstrates the feasibility of using available satellite observations for evaluating and improving representations in atmospheric models of the BB aerosol aging processes in different regions of the world at much larger temporal scales than those typically addressed in aerosol chamber experiments.


2014 ◽  
Vol 7 (5) ◽  
pp. 4623-4657
Author(s):  
M. Mech ◽  
E. Orlandi ◽  
S. Crewell ◽  
F. Ament ◽  
L. Hirsch ◽  
...  

Abstract. An advanced package of microwave remote sensing instrumentation has been developed for the operation on the new German High Altitude LOng range research aircraft (HALO). The HALO Microwave Package, HAMP, consists of two nadir looking instruments: a cloud radar at 36 GHz and a suite of passive microwave radiometers with 26 frequencies in different bands between 22.24 and 183.31 ± 12.5 GHz. We present a description of HAMP's instrumentation together with an illustration of its potential. To demonstrate this potential synthetic measurements for the implemented passive microwave frequencies and the cloud radar based on cloud resolving and radiative transfer model calculations were performed. These illustrate the advantage of HAMP's chosen frequency coverage, which allows for improved detection of hydrometeors both via the emission and scattering of radiation. Regression algorithms compare HAMP retrieval with standard satellite instruments from polar orbiters and show its advantages particularly for the lower atmosphere with a reduced root mean square error by 5 and 15% for temperature and humidity, respectively. HAMP's main advantage is the high spatial resolution of about 1 km which is illustrated by first measurements from test flights. Together these qualities make it an exciting tool for gaining better understanding of cloud processes, testing retrieval algorithms, defining future satellite instrument specifications, and validating platforms after they have been placed in orbit.


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