scholarly journals Two Independent Light Dilution Corrections for the SO2 Camera Retrieve Comparable Emission Rates at Masaya Volcano, Nicaragua

2021 ◽  
Vol 13 (5) ◽  
pp. 935
Author(s):  
Matthew Varnam ◽  
Mike Burton ◽  
Ben Esse ◽  
Giuseppe Salerno ◽  
Ryunosuke Kazahaya ◽  
...  

SO2 cameras are able to measure rapid changes in volcanic emission rate but require accurate calibrations and corrections to convert optical depth images into slant column densities. We conducted a test at Masaya volcano of two SO2 camera calibration approaches, calibration cells and co-located spectrometer, and corrected both calibrations for light dilution, a process caused by light scattering between the plume and camera. We demonstrate an advancement on the image-based correction that allows the retrieval of the scattering efficiency across a 2D area of an SO2 camera image. When appropriately corrected for the dilution, we show that our two calibration approaches produce final calculated emission rates that agree with simultaneously measured traverse flux data and each other but highlight that the observed distribution of gas within the image is different. We demonstrate that traverses and SO2 camera techniques, when used together, generate better plume speed estimates for traverses and improved knowledge of wind direction for the camera, producing more reliable emission rates. We suggest combining traverses and the SO2 camera should be adopted where possible.

Author(s):  
Junyao Lyu ◽  
Feng Xiong ◽  
Ningxiao Sun ◽  
Yiheng Li ◽  
Chunjiang Liu ◽  
...  

Volatile organic compound (VOCs) emission is an important cause of photochemical smog and particulate pollution in urban areas, and urban vegetation has been presented as an important source. Different tree species have different emission levels, so adjusting greening species collocation is an effective way to control biogenic VOC pollution. However, there is a lack of measurements of tree species emission in subtropical metropolises, and the factors influencing the species-specific differences need to be further clarified. This study applied an in situ method to investigate the isoprene emission rates of 10 typical tree species in subtropical metropolises. Photosynthesis and related parameters including photosynthetic rate, intercellular CO2 concentration, stomatal conductance, and transpiration rate, which can influence the emission rate of a single species, were also measured. Results showed Salix babylonica always exhibited a high emission level, whereas Elaeocarpus decipiens and Ligustrum lucidum maintained a low level throughout the year. Differences in photosynthetic rate and stomatal CO2 conductance are the key parameters related to isoprene emission among different plants. Through the establishment of emission inventory and determination of key photosynthetic parameters, the results provide a reference for the selection of urban greening species, as well as seasonal pollution control, and help to alleviate VOC pollution caused by urban forests.


2003 ◽  
Vol 447 (1) ◽  
pp. 97-108 ◽  
Author(s):  
S. P. Srinivas ◽  
Joseph A. Bonanno ◽  
Els Larivi�re ◽  
Danny Jans ◽  
Willy Van Driessche

Author(s):  
Juliana Vantellingen ◽  
Sean C. Thomas

Log landings are areas within managed forests used to process and store felled trees prior to transport. Through their construction and use soil is removed or redistributed, compacted, and organic matter contents may be increased by incorporation of wood fragments. The effects of these changes to soil properties on methane (CH<sub>4</sub>) flux is unclear and unstudied. We quantified CH<sub>4</sub> flux rates from year-old landings in Ontario, Canada, and examined spatial variability and relationships to soil properties within these sites. Landings emitted CH<sub>4</sub> throughout the growing season; the average CH<sub>4</sub> emission rate from log landings was 69.2 ± 12.8 nmol m<sup>-2</sup> s<sup>-1</sup> (26.2 ± 4.8 g CH<sub>4</sub> C m<sup>-2</sup> y<sup>-1</sup>), a rate comparable to CH<sub>4</sub>-emitting wetlands. Emission rates were correlated to soil pH, organic matter content and quantities of buried woody debris. These properties led to strong CH<sub>4</sub> emissions, or “hotspots”, in certain areas of landings, particularly where processing of logs occurred and incorporated woody debris into the soil. At the forest level, emissions from landings were estimated to offset ~12% of CH<sub>4</sub> consumption from soils within the harvest area, although making up only ~0.5% of the harvest area. Management practices to avoid or remediate these emissions should be developed as a priority measure in “climate-smart” forestry.


2018 ◽  
Vol 36 (5) ◽  
pp. 1471-1481
Author(s):  
Chih-Yu Chiang ◽  
Sunny Wing-Yee Tam ◽  
Tzu-Fang Chang

Abstract. The ISUAL payload onboard the FORMOSAT-2 satellite has often observed airglow bright spots around midnight at equatorial latitudes. Such features had been suggested as the signature of the thermospheric midnight temperature maximum (MTM) effect, which was associated with temperature and meridional neutral winds. This study investigates the influence of neutral temperature and meridional neutral wind on the volume emission rates of the 630.0 nm nightglow. We utilize the SAMI2 model to simulate the charged and neutral species at the 630.0 nm nightglow emission layer under different temperatures with and without the effect of neutral wind. The results show that the neutral wind is more efficient than temperature variation in affecting the nightglow emission rates. For example, based on our estimation, it would require a temperature change of 145 K to produce a change in the integrated emission rate by 9.8 km-photons cm−3 s−1, while it only needs the neutral wind velocity to change by 1.85 m−1 s−1 to cause the same change in the integrated emission rate. However, the emission rate features a local maximum in its variation with the temperature. Two kinds of tendencies can be seen regarding the temperature that corresponds to the turning point, which is named the turning temperature (Tt) in this study: firstly, Tt decreases with the emission rate for the same altitude; secondly, for approximately the same emission rate, Tt increases with the altitude.


2006 ◽  
Vol 33 (7) ◽  
pp. 613 ◽  
Author(s):  
Francis M. Kelliher ◽  
Harry Clark ◽  
Zheng Li ◽  
Paul C. D. Newton ◽  
Anthony J. Parsons ◽  
...  

Keppler et al. (2006, Nature 439, 187–191) showed that plants produce methane (CH4) in aerobic environments, leading Lowe (2006, Nature 439, 148–149) to postulate that in countries such as New Zealand, where grazed pastures have replaced forests, the forests could have produced as much CH4 as the ruminants currently grazing these areas. Estimating CH4 emissions from up to 85 million ruminants in New Zealand is challenging and, for completeness, the capacity of forest and pastoral soils to oxidise CH4 should be included. On average, the CH4 emission rate of grazing ruminants is estimated to be 9.6 ± 2.6 g m–2 year–1 (±standard deviation), six times the corresponding estimate for an indigenous forest canopy (1.6 ± 1.1 g m–2 year–1). The forest’s soil is estimated to oxidise 0.9 ± 0.2 g m–2 year–1 more CH4 than representative soils beneath grazed pasture. Taking into account plant and animal sources and the soil’s oxidative capacity, the net CH4 emission rates of forest and grazed ecosystems are 0.6 ± 1.1 and 9.8 ± 2.6 g m–2 year–1, respectively.


2021 ◽  
Author(s):  
Kang Sun ◽  
Lingbo Li ◽  
Shruti Jagini ◽  
Dan Li

Abstract. The evolving nature of the COVID-19 pandemic necessitates timely estimates of the resultant perturbations to anthropogenic emissions. Here we present a novel framework based on the relationships between observed column abundance and wind speed to rapidly estimate air basin-scale NOx emission rate and apply it at the Po Valley in Italy using OMI and TROPOMI NO2 tropospheric column observations. The NOx chemical lifetime is retrieved together with the emission rate and found to be 15–20 h in winter and 5–6 h in summer. A statistical model is trained using the estimated emission rates before the pandemic to predict the trajectory without COVID-19. Compared with this business-as-usual trajectory, the real 2020 emission rates show two distinctive drops in March (−41 %) and November (−35 %) that correspond to tightened COVID-19 control measures. The temporal variation of pandemic-induced NOx emission changes qualitatively agree with Google and Apple mobility indicators. The overall net NOx emission reduction in 2020 due to the COVID-19 pandemic is estimated to be 21 %.


2021 ◽  
Author(s):  
Alexander J. Winkler ◽  
Ranga B. Myneni ◽  
Markus Reichstein ◽  
Victor Brovkin

&lt;div&gt; &lt;div&gt; &lt;div&gt; &lt;p&gt;The prevailing understanding of the carbon-cycle response to anthropogenic CO&lt;sub&gt;2 &lt;/sub&gt;emissions suggests that it depends only on the magnitude of this forcing, not on its timing. However, a recent study (Winkler &lt;em&gt;et al&lt;/em&gt;., &lt;em&gt;Earth System Dynamics&lt;/em&gt;, 2019) demonstrated that the same magnitude of CO&lt;sub&gt;2 &lt;/sub&gt;forcing causes considerably different responses in various Earth system models when realized following different temporal trajectories. Because the modeling community focuses on concentration-driven runs that do not represent a fully-coupled carbon-cycle-climate continuum, and the experimental setups are mainly limited to exponential forcing timelines, the effect of different temporal trajectories of CO&lt;sub&gt;2 &lt;/sub&gt;emissions in the system is under-explored. Together, this could lead to an incomplete notion of the carbon-cycle response to anthropogenic CO&lt;sub&gt;2 &lt;/sub&gt;emissions.&lt;/p&gt; &lt;p&gt;We use the latest CMIP6 version of the Max-Planck-Institute Earth System Model (MPI-ESM1.2) with a fully-coupled carbon cycle to investigate the effect of emission timing in form of four drastically different pathways. All pathways emit an identical total of 1200 Pg C over 200 years, which is about the IPCC estimate to stay below 2 &amp;#176;K of warming, and the approximate amount needed to double the atmospheric CO&lt;sub&gt;2 &lt;/sub&gt;concentration. The four pathways differ only in their CO&lt;sub&gt;2 &lt;/sub&gt;emission rates, which include a constant, a negative parabolic (ramp-up/ramp-down), a linearly decreasing, and an exponentially increasing emission trajectory. These experiments are idealized, but designed not to exceed the observed maximum emission rates, and thus can be placed in the context of the observed system.&lt;/p&gt; &lt;p&gt;We find that the resulting atmospheric CO&lt;sub&gt;2 &lt;/sub&gt;concentration, after all the carbon has been emitted, can vary as much as 100 ppm between the different pathways. The simulations show that for pathways, where the system is exposed to higher rates of CO&lt;sub&gt;2 &lt;/sub&gt;emissions early in the forcing timeline, there is considerably less excess CO&lt;sub&gt;2 &lt;/sub&gt;in the atmosphere at the end. These pathways also show an airborne fraction approaching zero in the final decades of the simulation. At this point, the carbon sinks have reached a strength that removes more carbon from the atmosphere than is emitted. In contrast, the exponentially increasing pathway with high CO&lt;sub&gt;2 &lt;/sub&gt;emission rates in the last decades of the simulation, the pathway usually studied, shows a fairly stable airborne fraction. We propose a new general framework to estimate the atmospheric growth rate of CO&lt;sub&gt;2 &lt;/sub&gt;not only as a function of the emission rate, but also include the aspect of time the system has been exposed to excess CO&lt;sub&gt;2 &lt;/sub&gt;in the atmosphere. As a result, the transient temperature response is a function not only of the cumulative CO&lt;sub&gt;2 &lt;/sub&gt;emissions, but also of the time the system was exposed to the excess CO&lt;sub&gt;2&lt;/sub&gt;. We also apply this framework to other Earth system models and observational records of CO&lt;sub&gt;2 &lt;/sub&gt;concentration and emissions.&lt;/p&gt; &lt;/div&gt; &lt;/div&gt; &lt;/div&gt;&lt;div&gt; &lt;div&gt; &lt;div&gt; &lt;p&gt;The Earth system is currently in a phase of increasing, nearly exponential CO&lt;sub&gt;2 &lt;/sub&gt;forcing. The impact of excess CO&lt;sub&gt;2 &lt;/sub&gt;exposure time could become apparent as we approach the point of maximum CO&lt;sub&gt;2 &lt;/sub&gt;emission rate, affecting the achievability of the climate targets.&lt;/p&gt; &lt;/div&gt; &lt;/div&gt; &lt;/div&gt;


2019 ◽  
Vol 28 (03) ◽  
pp. 1950013
Author(s):  
Saeed Soheyli ◽  
Morteza Khalil Khalili ◽  
Ghazaaleh Ashrafi

Whereas there is a slight information on the pre-saddle neutron emission rate and neutron multiplicity, as well as it is impossible to separate the pre-saddle and saddle to scission neutron contributions experimentally, the theoretical studies of pre-saddle neutron emission rate and neutron multiplicity are of great importance. In the present work, the calculations of pre-saddle neutron multiplicity are performed using the analysis of fission fragment angular anisotropy data for [Formula: see text] and [Formula: see text] reaction systems. The obtained results show that the pre-saddle neutron multiplicity decreases by increasing the initial excitation energy and it has found to be characterized by a nonlinear behavior. Through the analysis of pre-saddle neutron multiplicity and pre-saddle transition time by means of the neutron clock method, the pre-saddle neutron emission rate is calculated for the first time. The findings of this study show that the pre-scission neutron emission rate is lower than the pre-saddle neutron emission rate.


2014 ◽  
Vol 5 (2) ◽  
pp. 409-422 ◽  
Author(s):  
T. Herrington ◽  
K. Zickfeld

Abstract. Recent studies have identified an approximately proportional relationship between global warming and cumulative carbon emissions, yet the robustness of this relationship has not been tested over a broad range of cumulative emissions and emission rates. This study explores the path dependence of the climate and carbon cycle response using an Earth system model of intermediate complexity forced with 24 idealized emissions scenarios across five cumulative emission groups (1275–5275 Gt C) with varying rates of emission. We find the century-scale climate and carbon cycle response after cessation of emissions to be approximately independent of emission pathway for all cumulative emission levels considered. The ratio of global mean temperature change to cumulative emissions – referred to as the transient climate response to cumulative carbon emissions (TCRE) – is found to be constant for cumulative emissions lower than ∼1500 Gt C but to decline with higher cumulative emissions. The TCRE is also found to decrease with increasing emission rate. The response of Arctic sea ice is found to be approximately proportional to cumulative emissions, while the response of the Atlantic Meridional Overturning Circulation does not scale linearly with cumulative emissions, as its peak response is strongly dependent on emission rate. Ocean carbon uptake weakens with increasing cumulative emissions, while land carbon uptake displays non-monotonic behavior, increasing up to a cumulative emission threshold of ∼2000 Gt C and then declining.


2011 ◽  
Vol 354-355 ◽  
pp. 231-235 ◽  
Author(s):  
Xue Jiao Xiao ◽  
Bao Qing Deng ◽  
Peng Zhang ◽  
Yun Lin Zang ◽  
Meng Ling Zhu ◽  
...  

This study aimed to investigate the influence of the paint film thickness on formaldehyde emission rates. A small-scale environmental chamber was set up to test the formaldehyde emission from wood lacquer with different thicknesses. In all experiments, the temperature, the airflow rate and the relative humidity were the same, which were set to 23 °C, 1000 L/s, 45 %, respectively. The emission rates of formaldehyde were calculated through the double exponential decay model. Results showed that the peak concentration was dependent of the paint film thickness. The thicker the film thickness was, the slower the emission rate was.


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