scholarly journals Contrasting trends of mass and optical properties of aerosols over the Northern Hemisphere from 1992 to 2011

2012 ◽  
Vol 12 (19) ◽  
pp. 9387-9398 ◽  
Author(s):  
K. C. Wang ◽  
R. E. Dickinson ◽  
L. Su ◽  
K. E. Trenberth
Keyword(s):  
Human Health ◽  
Atmospheric Aerosols ◽  
Fine Particles ◽  
Light Extinction ◽  
Vehicle Exhaust ◽  
Anthropogenic Aerosol ◽  
Optical Extinction ◽  
Aerosol Emission ◽  
Short Period ◽  
The Us

Abstract. Atmospheric aerosols affect both human health and climate. PMX is the mass concentration of aerosol particles that have aerodynamic diameters less than X μm, PM10 was initially selected to measure the environmental impact of aerosols. Recently, it was realized that fine particles are more hazardous than larger ones and should be measured. Consequently, observational data for PM2.5 have been obtained but only for a much shorter period than that of PM10. Optical extinction of aerosols, the inverse of meteorological visibility, is sensitive to particles less than 1.0 μm. These fine particles only account for a small part of total mass of aerosols although they are very efficient in light extinction. Comparisons are made between PM10 and PM2.5 over the period when the latter is available and with visibility data for a longer period. PM10 has decreased by 44% in Europe from 1992 to 2009, 33% in the US from 1993 to 2010, 10% in Canada from 1994 to 2009, and 26% in China from 2000 to 2011. However, in contrast, aerosol optical extinction has increased 7% in the US, 10% in Canada, and 18% in China during the above study periods. The reduction of optical extinction over Europe of 5% is also much less than the 44% reduction in PM10. Over its short period of record PM2.5 decreased less than PM10. Hence, PM10 is neither a good measure of changes in smaller particles nor of their long-term trends, a result that has important implications for both climate impact and human health effects. The increased fraction of anthropogenic aerosol emission, such as from vehicle exhaust, to total atmospheric aerosols partly explains this contrasting trend of optical and mass properties of aerosols.

scholarly journals Contrasting trends of mass and optical properties of aerosols over the Northern Hemisphere from 1992 to 2011

2012 ◽  
Vol 12 (7) ◽  
pp. 17913-17941
Author(s):  
K. Wang ◽  
R. E. Dickinson ◽  
L. Su ◽  
K. E. Trenberth
Keyword(s):  
Human Health ◽  
Atmospheric Aerosols ◽  
Fine Particles ◽  
Light Extinction ◽  
Vehicle Exhaust ◽  
Anthropogenic Aerosol ◽  
Optical Extinction ◽  
Aerosol Emission ◽  
Short Period ◽  
The Us

Abstract. Atmospheric aerosols impact both human health and climate. PMX is the mass concentration of aerosol particles that have aerodynamic diameters less than X μm, PM10 was initially selected to measure the environmental impact of aerosols. Recently, it was realized that fine particles are more hazardous than larger ones and should be measured. Consequently, observational data for PM2.5 have been obtained but only for a much shorter period than that of PM10. Optical extinction of aerosols, the inverse of meteorological visibility, is sensitive to particles less than 1.0 μm. These fine particles only account for a small part of total mass of aerosols although they are very efficient in light extinction. Comparisons are made between PM10 and PM2.5 over the period when the latter is available and with visibility data for a longer period. PM10 has decreased by 44% in Europe from 1992 to 2009, 33% in the US from 1993 to 2010, 10% in Canada from 1994 to 2009, and 26% in China from 2000 to 2010. However, in contrast, aerosol optical extinction increased 7% in the US, 10% in Canada, and 18% in China during the above study periods. The reduction of optical extinction over Europe of 5% is also much less than the 44% reduction in PM10. Over its short period of record PM2.5 decreased less than PM10. Hence, PM10 is neither a good measure of changes in smaller particles or of their long-term trends, a result that has important implications for both climate impact and human health effects. The increased fraction of anthropogenic aerosol emission, such as vehicle exhaust, to total atmospheric aerosols partly explains this contrasting trend of optical and mass properties of aerosols.

The Long Term Spatial-temporal Distribution of Aerosol Optical Depth and Its Associated Atmospheric Circulation Over Southeast Africa.

2021 ◽  
Author(s):  
Matthews Nyasulu ◽  
Md. Mozammel Haque ◽  
Bathsheba Musonda ◽  
Cao Fang
Keyword(s):  
Human Health ◽  
Atmospheric Circulation ◽  
Atmospheric Aerosols ◽  
Crop Residues ◽  
Temporal Distribution ◽  
Western Coast ◽  
High Concentration ◽  
Anthropogenic Aerosols ◽  
Anthropogenic Aerosol

Abstract Recent studies have revealed significant impacts of increased concentration of anthropogenic aerosols in the atmosphere to both climate and human health. Southeast Africa is one of the regions where studies related to atmospheric aerosols remain scant, causing high uncertainty in predicting and understanding the impacts of these aerosols to both climate and human health. The present study therefore has investigated the long term spatial-temporal distribution of atmospheric aerosols, trends, its relationship with cloud properties and the associated atmospheric circulation over the region. High concentration of aerosol has been detected during the dry months of September to November (SON) while low during March to May (MAM) and June-July (JJA) seasons in most areas. Highest 550 was recorded in areas with low elevation such as over Lake Malawi, Zambezi valley and along the western coast of the Indian Ocean. The average of the detected concentration is however low as compared to highly polluted regions of the globe. Statistical analyses revealed insignificant change of AOD550 in most areas between 2002 and 2020 time period. The study has also revealed seasonality of aerosol distribution highly influenced by changes in atmospheric circulation. Burning of biomass during dry months such bush fires and burning of crop residues remain the major source of anthropogenic aerosol concentration over Southeast Africa hence needs to be controlled.

scholarly journals Impact of vehicular emissions on the formation of fine particles in the Sao Paulo Metropolitan Area: a numerical study with the WRF-Chem model

2016 ◽  
Vol 16 (2) ◽  
pp. 777-797 ◽  
Author(s):  
A Vara-Vela ◽  
M. F. Andrade ◽  
P. Kumar ◽  
R. Y. Ynoue ◽  
A. G. Muñoz
Keyword(s):  
Size Distribution ◽  
Metropolitan Area ◽  
Atmospheric Aerosols ◽  
Fine Particles ◽  
Sao Paulo ◽  
Vehicular Emissions ◽  
São Paulo ◽  
Mass Size Distribution ◽  
Mass Size ◽  
The Impact

Abstract. The objective of this work is to evaluate the impact of vehicular emissions on the formation of fine particles (PM2.5;  ≤  2.5 µm in diameter) in the Sao Paulo Metropolitan Area (SPMA) in Brazil, where ethanol is used intensively as a fuel in road vehicles. The Weather Research and Forecasting with Chemistry (WRF-Chem) model, which simulates feedbacks between meteorological variables and chemical species, is used as a photochemical modelling tool to describe the physico-chemical processes leading to the evolution of number and mass size distribution of particles through gas-to-particle conversion. A vehicular emission model based on statistical information of vehicular activity is applied to simulate vehicular emissions over the studied area. The simulation has been performed for a 1-month period (7 August–6 September 2012) to cover the availability of experimental data from the NUANCE-SPS (Narrowing the Uncertainties on Aerosol and Climate Changes in Sao Paulo State) project that aims to characterize emissions of atmospheric aerosols in the SPMA. The availability of experimental measurements of atmospheric aerosols and the application of the WRF-Chem model made it possible to represent some of the most important properties of fine particles in the SPMA such as the mass size distribution and chemical composition, besides allowing us to evaluate its formation potential through the gas-to-particle conversion processes. Results show that the emission of primary gases, mostly from vehicles, led to a production of secondary particles between 20 and 30 % in relation to the total mass concentration of PM2.5 in the downtown SPMA. Each of PM2.5 and primary natural aerosol (dust and sea salt) contributed with 40–50 % of the total PM10 (i.e. those  ≤  10 µm in diameter) concentration. Over 40 % of the formation of fine particles, by mass, was due to the emission of hydrocarbons, mainly aromatics. Furthermore, an increase in the number of small particles impaired the ultraviolet radiation and induced a decrease in ozone formation. The ground-level O3 concentration decreased by about 2 % when the aerosol-radiation feedback is taken into account.

The local and remote atmospheric impacts of Africa’s 21st century aerosol emission trajectory

2021 ◽  
Author(s):  
Chris Wells ◽  
Apostolos Voulgarakis
Keyword(s):  
Regional Climate ◽  
Emission Region ◽  
Anthropogenic Aerosol ◽  
Remote Locations ◽  
Aerosol Emission ◽  
Radiation Fluxes ◽  
The World ◽  
Aerosol Emissions ◽  
The Impact ◽  
Lower Biomass

<p>Aerosols are a major climate forcer, but their historical effect has the largest uncertainty of any forcing; their mechanisms and impacts are not well understood. Due to their short lifetime, aerosols have large impacts near their emission region, but they also have effects on the climate in remote locations. In recent years, studies have investigated the influences of regional aerosols on global and regional climate, and the mechanisms that lead to remote responses to their inhomogeneous forcing. Using the Shared Socioeconomic Pathway scenarios (SSPs), transient future experiments were performed in UKESM1, testing the effect of African emissions following the SSP3-RCP7.0 scenario as the rest of the world follows SSP1-RCP1.9, relative to a global SSP1-RCP1.9 control. SSP3 sees higher direct anthropogenic aerosol emissions, but lower biomass burning emissions, over Africa. Experiments were performed changing each of these sets of emissions, and both. A further set of experiments additionally accounted for changing future CO<sub>2</sub> concentrations, to investigate the impact of CO<sub>2</sub> on the responses to aerosol perturbations. Impacts on radiation fluxes, temperature, circulation and precipitation are investigated, both over the emission region (Africa), where microphysical effects dominate, and remotely, where dynamical influences become more relevant. </p>

Back to the Future: Reducing Atmospheric Particulate Matter Levels to Improve Human Health

2021 ◽  
Author(s):  
Spyros Pandis
Keyword(s):  
Particulate Matter ◽  
Atmospheric Aerosols ◽  
Atmospheric Chemistry ◽  
Control Strategy ◽  
Atmospheric Particulate Matter ◽  
Anthropogenic Emissions ◽  
The Us ◽  
Negative Impacts ◽  
Predictive Understanding ◽  
Physical And Chemical

<p>The human development of our planet has a variety of negative impacts on the composition of its atmosphere at every scale – locally, regionally, and even globally. One of these dramatic changes has been the increase in the mass concentrations of sub-micrometer particles by one to sometimes two orders of magnitude over populated areas in the Northern Hemisphere. These atmospheric aerosols can cause serious health problems, reduce visibility, contribute to acidic deposition and material damage, but are also cooling the planet by reflecting sunlight back to space. Atmospheric chemistry occurs within a fabric of complicated atmospheric dynamics and physics. This interplay often results in nonlinear and often counterintuitive changes of the system when anthropogenic emissions change. A major goal of our research has been to gain a predictive understanding of the physical and chemical processes that govern the dynamics, size, and chemical composition of atmospheric aerosols.</p><p>To illustrate the advances in the experimental techniques and theoretical tools in atmospheric aerosol science, we will go back to the beginning of the 21<sup>st</sup> century and we will revisit the design a particulate matter control strategy for the Eastern US based on the data, knowledge, and tools available at that time. We will then look at the effects of the parts of this control strategy that have been materialized and their effects on public health using the current understanding. Finally, we will look forward in ways of further improving air quality in the US and Europe.</p>

scholarly journals Comparison of in situ and columnar aerosol spectral measurements during TexAQS-GoMACCS 2006: testing parameterizations for estimating aerosol fine mode properties

2009 ◽  
Vol 9 (4) ◽  
pp. 17465-17494
Author(s):  
D. B. Atkinson ◽  
P. Massoli ◽  
N. T. O'Neill ◽  
P. K. Quinn ◽  
S. Brooks ◽  
...  
Keyword(s):  
Gulf Of Mexico ◽  
Atmospheric Aerosols ◽  
Regional Scale ◽  
Atmospheric Composition ◽  
Light Extinction ◽  
Large Area ◽  
Light Extinction Coefficient ◽  
Spectral Models ◽  
Fine Mode

Abstract. During the 2006 Texas Air Quality Study and Gulf of Mexico Atmospheric Composition and Climate Study (TexAQS-GoMACCS 2006), the optical, chemical and microphysical properties of atmospheric aerosols were measured on multiple mobile platforms and at ground based stations. In situ measurements of the aerosol light extinction coefficient (σep) were performed by two multi-wavelength cavity ring-down (CRD) instruments, one located on board the NOAA R/V Ronald H. Brown (RHB) and the other located at the University of Houston, Moody Tower (UHMT). An AERONET sunphotometer was also located at the UHMT to measure the columnar aerosol optical depth (AOD). The σep data were used to extract the extinction Ångström exponent (åep), a measure of the wavelength dependence of σep. There was general agreement between the åep (and to a lesser degree σep measurements by the two spatially separated CRD instruments during multi-day periods, suggesting a regional scale consistency of the sampled aerosols. Two spectral models are applied to the σep and AOD data to extract the fine mode fraction of extinction (η) and the fine mode effective radius (Reff f). These two parameters are robust measures of the fine mode contribution to total extinction and the fine mode size distribution respectively. The results of the analysis are compared to Reff f values extracted using AERONET V2 retrievals and calculated from in situ particle size measurements on the RHB and at UHMT. During a time period when fine mode aerosols dominated the extinction over a large area extending from Houston/Galveston Bay and out into the Gulf of Mexico, the various methods for obtaining Reff f agree qualitatively (showing the same temporal trend) and quantitatively (pooled standard deviation=28 nm).

scholarly journals Bias in CMIP6 models as compared to observed regional dimming and brightening

2020 ◽  
Vol 20 (24) ◽  
pp. 16023-16040
Author(s):  
Kine Onsum Moseid ◽  
Michael Schulz ◽  
Trude Storelvmo ◽  
Ingeborg Rian Julsrud ◽  
Dirk Olivié ◽  
...  
Keyword(s):  
Sulfur Dioxide ◽  
Surface Energy ◽  
Coupled Model ◽  
Shortwave Radiation ◽  
Anthropogenic Aerosol ◽  
Surface Energy Fluxes ◽  
Aerosol Emission ◽  
Wrong Reason ◽  
The Right ◽  
Aerosol Emissions

Abstract. Anthropogenic aerosol emissions have increased considerably over the last century, but climate effects and quantification of the emissions are highly uncertain as one goes back in time. This uncertainty is partly due to a lack of observations in the pre-satellite era, making the observations we do have before 1990 additionally valuable. Aerosols suspended in the atmosphere scatter and absorb incoming solar radiation and thereby alter the Earth's surface energy balance. Previous studies show that Earth system models (ESMs) do not adequately represent surface energy fluxes over the historical era. We investigated global and regional aerosol effects over the time period 1961–2014 by looking at surface downwelling shortwave radiation (SDSR). We used observations from ground stations as well as multiple experiments from eight ESMs participating in the Coupled Model Intercomparison Project Version 6 (CMIP6). Our results show that this subset of models reproduces the observed transient SDSR well in Europe but poorly in China. We suggest that this may be attributed to missing emissions of sulfur dioxide in China, sulfur dioxide being a precursor to sulfate, which is a highly reflective aerosol and responsible for more reflective clouds. The emissions of sulfur dioxide used in the models do not show a temporal pattern that could explain observed SDSR evolution over China. The results from various aerosol emission perturbation experiments from DAMIP, RFMIP and AerChemMIP show that only simulations containing anthropogenic aerosol emissions show dimming, even if the dimming is underestimated. Simulated clear-sky and all-sky SDSR do not differ greatly, suggesting that cloud cover changes are not a dominant cause of the biased SDSR evolution in the simulations. Therefore we suggest that the discrepancy between modeled and observed SDSR evolution is partly caused by erroneous aerosol and aerosol precursor emission inventories. This is an important finding as it may help interpret whether ESMs reproduce the historical climate evolution for the right or wrong reason.

scholarly journals Primary anthropogenic aerosol emission trends for China, 1990–2005

2011 ◽  
Vol 11 (3) ◽  
pp. 931-954 ◽  
Author(s):  
Y. Lei ◽  
Q. Zhang ◽  
K. B. He ◽  
D. G. Streets
Keyword(s):  
Emission Factors ◽  
Cement Industry ◽  
Anthropogenic Aerosol ◽  
Residential Sector ◽  
Aerosol Emission ◽  
Metallic Mineral ◽  
Aerosol Emissions ◽  
Industry Sectors ◽  
Mineral Product ◽  
Activity Information

Abstract. An inventory of anthropogenic primary aerosol emissions in China was developed for 1990–2005 using a technology-based approach. Taking into account changes in the technology penetration within industry sectors and improvements in emission controls driven by stricter emission standards, a dynamic methodology was derived and implemented to estimate inter-annual emission factors. Emission factors of PM2.5 decreased by 7%–69% from 1990 to 2005 in different industry sectors of China, and emission factors of TSP decreased by 18%–80% as well, with the measures of controlling PM emissions implemented. As a result, emissions of PM2.5 and TSP in 2005 were 11.0 Tg and 29.7 Tg, respectively, less than what they would have been without the adoption of these measures. Emissions of PM2.5, PM10 and TSP presented similar trends: they increased in the first six years of 1990s and decreased until 2000, then increased again in the following years. Emissions of TSP peaked (35.5 Tg) in 1996, while the peak of PM10 (18.8 Tg) and PM2.5 (12.7 Tg) emissions occurred in 2005. Although various emission trends were identified across sectors, the cement industry and biofuel combustion in the residential sector were consistently the largest sources of PM2.5 emissions, accounting for 53%–62% of emissions over the study period. The non-metallic mineral product industry, including the cement, lime and brick industries, accounted for 54%–63% of national TSP emissions. There were no significant trends of BC and OC emissions until 2000, but the increase after 2000 brought the peaks of BC (1.51 Tg) and OC (3.19 Tg) emissions in 2005. Although significant improvements in the estimation of primary aerosols are presented here, there still exist large uncertainties. More accurate and detailed activity information and emission factors based on local tests are essential to further improve emission estimates, this especially being so for the brick and coke industries, as well as for coal-burning stoves and biofuel usage in the residential sector.

Resisting Openness

2020 ◽  
pp. 51-90
Author(s):  
Christian Freudlsperger
Keyword(s):  
Trade Liberalization ◽  
Historical Development ◽  
State Governments ◽  
Best Value ◽  
Short Period ◽  
The Us ◽  
Canadian Provinces ◽  
Run Up ◽  
Municipal Level ◽  
The Eu

The third chapter of Trade Policy in Multilevel Government introduces the field of procurement as a hard case of trade liberalization. Contracting in line with the principle of ‘best value for money’ curtails public actors’ ability to rely on procurement as a directed means of redistribution. Nevertheless, this principle has served as the rallying cry of an international regime of procurement liberalization that has gradually evolved since the 1970s and whose historical development is described here. In a second step, the chapter elaborates on the patterns of openness and resistance to procurement liberalization among the three multilevel polities chosen for analysis. Over the entire period of observation, the US states’ openness has been comparatively low. Intermittently, their resistance had decreased in the run-up to the 1994 GPA. In recent years, however, the number of states willing to be bound by international procurement disciplines plummeted to virtually zero. As for the Canadian provinces and territories, the picture shifted in recent years. Especially in the negotiations on CETA, they permitted the EU wholesale access to their procurement markets. Within a short period, the Canadian provinces’ position on international procurement liberalization thus witnessed a veritable sea change. Finally, in the EU case, openness on part of member state governments has consistently proved highest among the three cases. Already within the scope of the 1979 GATT Code, all EC members’ central procurement was covered, albeit modestly. In the 1994 GPA and its 2012 revision, the EU covered its procurement on the national, regional, and municipal level.

scholarly journals Emission of fine particles (PM2.5) from residential biomass combustion in Croatia and how to reduce it

2020 ◽  
Vol 7 (2) ◽  
pp. 84-94
Author(s):  
Mirela Poljanac
Keyword(s):  
Air Quality ◽  
Human Health ◽  
Urban Areas ◽  
Fine Particles ◽  
Biomass Combustion ◽  
Rural And Urban Areas ◽  
Wood Burning ◽  
Rural And Urban ◽  
The Impact ◽  
Pm2.5 Emissions

Wood burning in residential appliances is very represented in the Republic of Croatia. It is a main or an additional form of heating for many households in rural and urban areas and is therefore an important source of air pollution. The choice of energy and the combustion appliance used in home have a significant impact on PM2.5 emissions. The paper informs the reader about PM2.5 emissions, their main sources and impacts on human health, environment, climate, air quality, and the reason why PM2.5 emissions from residential wood burning are harmful. Paper also gives an overview of spatial PM2.5 emission distribution in Croatia, their five air quality zones and four agglomerations. The paper analyses the sources and their contribution to PM2.5 emissions with the relevance of PM2.5 emissions from residential plants, the use of fuels in residential plants and their contribution to PM2.5 emissions and PM2.5 emissions by fuel combustion technologies in residential sector. Appropriate strategies, policies, and actions to reduce the impact of residential biomass (wood) burning on the environment, air quality and human health are considered.

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