On shock-induced light-fluid-layer evolution

Shock-induced light-fluid-layer evolution is firstly investigated experimentally and theoretically. Specifically, three quasi-one-dimensional helium gas layers with different layer thicknesses are generated to study the wave patterns and interface motions. Six quasi-two-dimensional helium gas layers with diverse layer thicknesses and amplitude combinations are created to explore the Richtmyer–Meshkov instability of a light-fluid layer. Due to the multiple reflected shocks reverberating inside a light-fluid layer, the speeds of the two interfaces gradually converge, and the layer thickness saturates eventually. A general one-dimensional theory is adopted to describe the two interfaces’ motions and the layer thickness variations. It is found that, for the first interface, the end time of its phase reversal determines the influence of the reflected shocks on it. However, the reverberated shocks indeed lead to the second interface being more unstable. When the two interfaces are initially in phase, and the initial fluid layer is very thin, the two interfaces’ spike heads collide and stabilise the two interfaces. Linear and nonlinear models are successfully adopted by considering the interface-coupling effect and the reverberated shocks to predict the two interfaces’ perturbation growths in all regimes. The interfacial instability of a light-fluid layer is quantitatively compared with that of a heavy-fluid layer. It is concluded that the kind of waves reverberating inside a fluid layer significantly affects the fluid-layer evolution.

A Molecular Dynamics Simulation Study: The Inkjet Printing of Graphene Inks on Polyimide Substrates

Inkjet printing-based 2D materials for flexible electronics have aroused much interest due to their highly low-cost customization and manufacturing resolution. However, there is a lack of investigation and essential understanding of the surface adhesion affected by the printing parameters at the atomic scale. Herein, we conducted a systematic molecular dynamics simulation investigating the inkjet printing of graphitic inks on polyimide substrates under various conditions. Simulations under different temperatures, inkjet velocities, and mechanical loadings such as pressure and deformation are performed. The results show that the best adhesion is achieved in the plasma-modified polyimide/graphene-oxide (mPI/GO) interfacial system (the interaction energy (Ein) between mPI and GO is ca. 1.2 times than with graphene). The adhesion strength decreases with increasing temperature, and higher inkjet velocities lead to both larger impact force as well as interfacial fluctuation, while the latter may result in greater interfacial instability. When loaded with pressure, the adhesion strength reaches a threshold without further improvement as continuing compacting of polymer slabs can hardly be achieved. The detachment of the interfaces was also explored and mPI/GO shows better resistance against delamination. Hopefully, our simulation study paves the way for future inkjet printing-based manufacturing of graphene-based flexible electronics.

Instability of a liquid sheet with viscosity contrast in inertial microfluidics

Flows at moderate Reynolds numbers in inertial microfluidics enable high throughput and inertial focusing of particles and cells with relevance in biomedical applications. In the present work, we consider a viscosity-stratified three-layer flow in the inertial regime. We investigate the interfacial instability of a liquid sheet surrounded by a density-matched but more viscous fluid in a channel flow. We use linear stability analysis based on the Orr–Sommerfeld equation and direct numerical simulations with the lattice Boltzmann method (LBM) to perform an extensive parameter study. Our aim is to contribute to a controlled droplet production in inertial microfluidics. In the first part, on the linear stability analysis we show that the growth rate of the fastest growing mode $$\xi ^{*}$$ ξ ∗ increases with the Reynolds number $$\text {Re}$$ Re and that its wavelength $$\lambda ^{*}$$ λ ∗ is always smaller than the channel width w for sufficiently small interfacial tension $$\Gamma $$ Γ . For thin sheets we find the scaling relation $$\xi ^{*} \propto mt^{2.5}_{s}$$ ξ ∗ ∝ m t s 2.5 , where m is viscosity ratio and $$t_{s}$$ t s the sheet thickness. In contrast, for thicker sheets $$\xi ^{*}$$ ξ ∗ decreases with increasing $$t_s$$ t s or m due to the nearby channel walls. Examining the eigenvalue spectra, we identify Yih modes at the interface. In the second part on the LBM simulations, the thin liquid sheet develops two distinct dynamic states: waves traveling along the interface and breakup into droplets with bullet shape. For smaller flow rates and larger sheet thicknesses, we also observe ligament formation and the sheet eventually evolves irregularly. Our work gives some indication how droplet formation can be controlled with a suitable parameter set $$\{\lambda ,t_{s},m,\Gamma ,\text {Re}\}$$ { λ , t s , m , Γ , Re } . Graphical Abstract

Effect of Periodic Oscillation on the Interfacial Instability of Two Superposed Fluid Layers in a Fully Saturated Porous Media

We investigate the effect of horizontal periodic oscillation on the interfacial instability of two immiscible and viscous fluids of different densities in a fully saturated porous media. A linear stability analysis of the viscous and time-dependent basic flow leads to a periodic oscillator describing the evolution of the interfacial perturbation amplitude. The horizontal oscillation leads to the occurrence of two types of instability, the Kelvin–Helmholtz’s instability and the parametric resonance. These instabilities appear at the frontier between water and petroleum and have a practical interest in oil reservoir engineering. The results show that, an increase of the oscillation frequency destabilizes the Kelvin–Helmholtz instability and displaces the parametric instability regions toward the short wavelength perturbation. Also, we examine mainly how the other physical parameters of the system affect the instabilities for various permeability and porosity values of the porous medium as well as for relative heights of the two fluid layers.

An Idealized 3D Model of Interfacial Instability of Aeolian Bedform

An idealized morphodynamic model is constructed for formation of the aeolian sand ripples from small bottom perturbations of a two-dimensional sand bed. The main goal of the analysis is to evaluate the influence of the gravity flow (including “impact-induced gravity flow” in the reptation flux and “topography-induced gravity flow” in the creep flux) on the formation of the aeolian sand ripples and to clarify the relative contribution of various factors to the bed instability. A 3D linear stability analysis reveals that gravity flow appreciably affects the dynamics behaviors of aeolian sand ripples, which decreases the growth rate of sand ripples, tends to stabilize the sand bed, and leads to longer wavelength. We found that the competition between the destabilizing effect of reptation flow and the stabilizing effects of gravity flow leads to pattern selection. The along-crest diffusion of topography driven by impact and gravity is beneficial to the transverse stability of sand ripples, producing sand ripples with straighter and more continuous crests. For moderate values of D, the most unstable mode has zero value of the transverse wavenumber (ky = 0), thus corresponding to aeolian ripples with crests perpendicular to the wind. Moreover, when the impact angle is 9–16°, it has little effect on the characteristics of sand ripples for the initial stage of ripple development. For every increase of the impact angle by 1°, the initial wavelength only increases by about 1.5%. In conclusion, the influence of the gravity flow on the dynamics of sand ripples formation stage cannot be neglected.

Surface enrichment and diffusion enabling gradient-doping and coating of Ni-rich cathode toward Li-ion batteries

Critical barriers to layered Ni-rich cathode commercialisation include their rapid capacity fading and thermal runaway from crystal disintegration and their interfacial instability. Structure combines surface modification is the ultimate choice to overcome these. Here, a synchronous gradient Al-doped and LiAlO2-coated LiNi0.9Co0.1O2 cathode is designed and prepared by using an oxalate-assisted deposition and subsequent thermally driven diffusion method. Theoretical calculations, in situ X-ray diffraction results and finite-element simulation verify that Al3+ moves to the tetrahedral interstices prior to Ni2+ that eliminates the Li/Ni disorder and internal structure stress. The Li+-conductive LiAlO2 skin prevents electrolyte penetration of the boundaries and reduces side reactions. These help the Ni-rich cathode maintain a 97.4% cycle performance after 100 cycles, and a rapid charging ability of 127.7 mAh g−1 at 20 C. A 3.5-Ah pouch cell with the cathode and graphite anode showed more than a 500-long cycle life with only a 5.6% capacity loss.

Interfacial instability of ferrofluid flow under the influence of a vacuum magnetic field

This study is to numerically test the interfacial instability of ferrofluid flow under the presence of a vacuum magnetic field. The ferrofluid parabolized stability equations (PSEs) are derived from the ferrofluid stability equations and the Rosensweig equations, and the characteristic values of the ferrofluid PSEs are given to describe the ellipticity of ferrofluid flow. Three numerical models representing specific cases considering with/without a vacuum magnetic field or viscosity are created to mathematically examine the interfacial instability by the computation of characteristic values. Numerical investigation shows strong dependence of the basic characteristic of ferrofluid Rayleigh-Taylor instability (RTI) on viscosity of ferrofluid and independence of the vacuum magnetic field. For the shock wave striking helium bubble, the magnetic field is not able to trigger the symmetry breaking of bubble but change the speed of the bubble movement. In the process of droplet formation from a submerged orifice, the collision between the droplet and the liquid surface causes symmetry breaking. Both the viscosity and the magnetic field exacerbate symmetry breaking. The computational results agree with the published experimental results.