scholarly journals Subwavelength Direct Laser Nanopatterning Via Microparticle Arrays for Functionalizing Metallic Surfaces

2019 ◽  
Vol 7 (1) ◽  
Author(s):  
Jean-Michel Romano ◽  
Rajib Ahmed ◽  
Antonio Garcia-Giron ◽  
Pavel Penchev ◽  
Haider Butt ◽  
...  
Keyword(s):  
Focal Length ◽  
Near Field ◽  
Cost Effective ◽  
Spot Size ◽  
Metallic Surface ◽  
Metallic Surfaces ◽  
Large Area ◽  
Transitional State ◽  
Direct Laser ◽  
Surface Patterns

Functionalized metallic nanofeatures can be selectively fabricated via ultrashort laser processing; however, the cost-effective large-area texturing, intrinsically constrained by the diffraction limit of light, remains a challenging issue. A high-intensity near-field phenomenon that takes place when irradiating microsized spheres, referred to as photonic nanojet (PN), was investigated in the transitional state between geometrical optics and dipole regime to fabricate functionalized metallic subwavelength features. Finite element simulations were performed to predict the PN focal length and beam spot size, and nanofeature formation. A systematic approach was employed to functionalize metallic surface by varying the pulse energy, focal offset, and number of pulses to fabricate controlled array of nanoholes and to study the generation of triangular and rhombic laser-induced periodic surface structures (LIPSS). Finally, large-area texturing was investigated to minimize the dry laser cleaning (DLC) effect and improve homogeneity of PN-assisted texturing. Tailored dimensions and densities of achievable surface patterns could provide hexagonal light scattering and selective optical reflectance for a specific light wavelength. Surfaces exhibited controlled wetting properties with either hydrophilicity or hydrophobicity. No correlation was found between wetting and microbacterial colonization properties of textured metallic surfaces after 4 h incubation of Escherichia coli. However, an unexpected bacterial repellency was observed.

scholarly journals Self-Organized Conductive Gratings of Au Nanostripe Dimers Enable Tunable Plasmonic Activity

2020 ◽  
Vol 10 (4) ◽  
pp. 1301
Author(s):  
Maria Caterina Giordano ◽  
Matteo Barelli ◽  
Giuseppe Della Valle ◽  
Francesco Buatier de Mongeot
Keyword(s):  
High Efficiency ◽  
Ion Beam ◽  
Near Field ◽  
Cost Effective ◽  
Localized Surface Plasmon ◽  
Large Area ◽  
Field Amplification ◽  
Self Organized ◽  
Broadband Spectrum ◽  
Out Of Plane

Plasmonic metasurfaces based on quasi-one-dimensional (1D) nanostripe arrays are homogeneously prepared over large-area substrates (cm2), exploiting a novel self-organized nanofabrication method. Glass templates are nanopatterned by ion beam-induced anisotropic nanoscale wrinkling, enabling the maskless confinement of quasi-1D arrays of out-of-plane tilted gold nanostripes, behaving as transparent wire-grid polarizer nanoelectrodes. These templates enable the dichroic excitation of localized surface plasmon resonances, easily tunable over a broadband spectrum from the visible to the near- and mid-infrared, by tailoring the nanostripes’ shape and/or changing the illumination conditions. The controlled self-organized method allows the engineering of the nanoantennas’ morphology in the form of Au-SiO2-Au nanostripe dimers, which show hybridized plasmonic resonances with enhanced tunability. Under this condition, superior near-field amplification is achievable for the excitation of the hybridized magnetic dipole mode, as pointed out by numerical simulations. The high efficiency of these plasmonic nanoantennas, combined with the controlled tuning of the resonant response, opens a variety of applications for these cost-effective templates, ranging from biosensing and optical spectroscopies to high-resolution molecular imaging and nonlinear optics.

scholarly journals Development of a Monitoring Strategy for Laser-Textured Metallic Surfaces Using a Diffractive Approach

Materials ◽  
2019 ◽  
Vol 13 (1) ◽  
pp. 53
Author(s):  
Sascha Teutoburg-Weiss ◽  
Bogdan Voisiat ◽  
Marcos Soldera ◽  
Andrés Fabián Lasagni
Keyword(s):  
Current Status ◽  
Textured Surfaces ◽  
Metallic Surfaces ◽  
Optical Images ◽  
Single Scale ◽  
Direct Laser ◽  
Indirect Evaluation ◽  
Optical Configuration ◽  
Surface Patterns ◽  
Direct Laser Interference Patterning

The current status of research around the world concurs on the powerful influence of micro- and nano-textured surfaces in terms of surface functionalization. In order to characterize the manufactured topographical morphology with regard to the surface quality or homogeneity, major efforts are still required. In this work, an optical approach for the indirect evaluation of the quality and morphology of surface structures manufactured with Direct Laser Interference Patterning (DLIP) is presented. For testing the designed optical configuration, line-like surface patterns are fabricated at a 1064 nm wavelength on stainless steel with a repetitive distance of 4.9 µm, utilizing a two-beam DLIP configuration. Depending on the pulse to pulse overlap and hatch distance, different single and complex pattern geometries are produced, presenting non-homogenous and homogenous surface patterns. The developed optical system permitted the successfully classification of different pattern geometries, in particular, those showing single-scale morphology (high homogeneity). Additionally, the fabricated structures were measured using confocal microscopy method, and the obtained topographies were correlated with the recorded optical images.

scholarly journals Tailoring optical complex fields with nano-metallic surfaces

Nanophotonics ◽  
2015 ◽  
Vol 4 (1) ◽  
pp. 2-25 ◽  
Author(s):  
Guanghao Rui ◽  
Qiwen Zhan
Keyword(s):  
Near Field ◽  
Photonic Devices ◽  
Metallic Surface ◽  
Strong Interactions ◽  
Metallic Surfaces ◽  
Optical Fields ◽  
Recent Developments ◽  
Quantum Optical ◽  
Light Beams ◽  
Made In

AbstractRecently there is an increasing interest in complex optical fields with spatially inhomogeneous state of polarizations and optical singularities. Novel effects and phenomena have been predicted and observed for light beams with these unconventional states. Nanostructured metallic thin film offers unique opportunities to generate, manipulate and detect these novel fields. Strong interactions between nano-metallic surfaces and complex optical fields enable the development of highly compact and versatile functional devices and systems. In this review, we first briefly summarize the recent developments in complex optical fields. Various nano-metallic surface designs that can produce and manipulate complex optical fields with tailored characteristics in the optical far field will be presented. Nano-metallic surfaces are also proven to be very effective for receiving and detection of complex optical fields in the near field. Advances made in this nascent field may enable the design of novel photonic devices and systems for a variety of applications such as quantum optical information processing and integrated photonic circuits.

scholarly journals On the Interplay of DLIP and LIPSS Upon Ultra-Short Laser Pulse Irradiation

Materials ◽  
2019 ◽  
Vol 12 (7) ◽  
pp. 1018 ◽  
Author(s):  
Sabri Alamri ◽  
Fotis Fraggelakis ◽  
Tim Kunze ◽  
Benjamin Krupop ◽  
Girolamo Mincuzzi ◽  
...  
Keyword(s):  
Stainless Steel ◽  
Surface Morphology ◽  
Spot Size ◽  
Surface Structures ◽  
Laser Source ◽  
Periodic Patterns ◽  
Simultaneous Generation ◽  
Periodic Surface ◽  
Direct Laser ◽  
Surface Patterns

Controlling laser induced surface morphology is essential for developing specialized functional surfaces. This work presents novel, multi-scale periodic patterns with two-dimensional symmetry generated on stainless steel, polyimide and sapphire. The microstructures were realized by combining Direct Laser Interference Patterning with the generation of Laser Induced Periodic Surface Structures in a one-step process. An industrial, fiber femtosecond laser source emitting at 1030 nm with a pulse duration of 500 fs was utilized for the experiments. In the case of stainless steel, it was possible to create line-like or pillar-like surface patterns by rotating the polarization orientation with respect to the interference pattern. In the case of polyimide and sapphire, the absorption of the laser radiation was promoted by a multiphoton mechanism. In polyimide, grooves and pillars of several microns in depth were produced over an area much larger than the spot size. Finally, for sapphire, the simultaneous generation of interference-like pattern and laser induced periodic surface structures was realized. The results reported here provide valuable data on the feasibility to combine two state-of-the-art techniques with an industrial apparatus, to control the induced surface morphology.

scholarly journals Stimulated compton scattering of surface plasma wave excited over metallic surface by a laser

2015 ◽  
Vol 33 (4) ◽  
pp. 641-646 ◽  
Author(s):  
Deepika Goel ◽  
Prashant Chauhan ◽  
Anshu Varshney ◽  
D.B. Singh ◽  
Vivek Sajal
Keyword(s):  
Compton Scattering ◽  
Plasma Wave ◽  
Spot Size ◽  
Metallic Surface ◽  
Fermi Velocity ◽  
Surface Plasma ◽  
Incident Laser ◽  
Free Electron Density ◽  
Direct Laser ◽  
Electrostatic Plasma Wave

AbstractA high-frequency surface plasma wave (SPW) excited over metallic surface irradiated by a laser beam, can undergo stimulated Compton scattering if phase velocity of daughter plasma wave is equal to the Fermi velocity for metal. The pump SPW${\rm (}{{\rm \omega} _0},{\vec k_{0{\rm z}}})$parametrically excites a quasi-electrostatic plasma wave${\rm (\omega}, {\vec k_{\rm z}})$and a backscattered sideband SPW${\rm (}{{\rm \omega} _1},{\vec k_{1{\rm z}}})$at resonance ω0= ω − ω1and${\vec k_{0{\rm z}}} = {\vec k_{\rm z}} - {\vec k_{1{\rm z}}}$. The growth rate of Compton process increases with the frequency of incident laser and turns out to be 5.425 × 1010rad/s at laser frequency ω0= 0.7595 × 1015rad/s for incident laser amplitudeA0L= 11 × 1011V/m, laser spot size b = 1.38 × 10−5m, and free electron density of metaln0= 5.85 × 1028/m3. The excitation of highly damped quasi-electrostatic plasma wave in this parametric process provide a better nonlinear option for surface heating as compared with direct laser heating. The process can also be used for diagnostics purposes.

scholarly journals High-Resolution Measurement of Molecular Internal Polarization Structure by Photoinduced Force Microscopy

2021 ◽  
Vol 11 (15) ◽  
pp. 6937
Author(s):  
Hidemasa Yamane ◽  
Nobuhiko Yokoshi ◽  
Hajime Ishihara
Keyword(s):  
High Resolution ◽  
Single Molecule ◽  
Near Field ◽  
Critical Role ◽  
Single Molecules ◽  
Atomic Scale ◽  
Metallic Surface ◽  
Metallic Surfaces ◽  
Force Microscopy

Near-field interactions between metallic surfaces and single molecules play an essential role in the application of metamaterials. To reveal the near-field around a photo-irradiated single molecule on the metallic surface, high-resolution photo-assisted scanning microscopy is required. In this study, we theoretically propose photoinduced force microscopy (PiFM) measurements of single molecules at the atomic resolution. For experimental demonstration, we performed a numerical calculation of PiFM images of various transition states, including optical forbidden transitions, and interpreted them in terms of the interaction between the molecular internal polarization structures and localized plasmon. We also clarified the critical role of atomic-scale structures on the tip surface for high-resolution PiFM measurements.

A High Resolution Scanning Microscope

1968 ◽  
Vol 26 ◽  
pp. 356-357
Author(s):  
A. V. Crewe ◽  
J. Wall ◽  
L. M. Welter
Keyword(s):  
High Resolution ◽  
Field Emission ◽  
Spherical Aberration ◽  
Focal Length ◽  
Spot Size ◽  
Emission Source ◽  
Field Of View ◽  
Scanning Microscope ◽  
Magnetic Lens ◽  
High Quality

A scanning microscope using a field emission source has been described elsewhere. This microscope has now been improved by replacing the single magnetic lens with a high quality lens of the type described by Ruska. This lens has a focal length of 1 mm and a spherical aberration coefficient of 0.5 mm. The final spot size, and therefore the microscope resolution, is limited by the aberration of this lens to about 6 Å.The lens has been constructed very carefully, maintaining a tolerance of + 1 μ on all critical surfaces. The gun is prealigned on the lens to form a compact unit. The only mechanical adjustments are those which control the specimen and the tip positions. The microscope can be used in two modes. With the lens off and the gun focused on the specimen, the resolution is 250 Å over an undistorted field of view of 2 mm. With the lens on,the resolution is 20 Å or better over a field of view of 40 microns. The magnification can be accurately varied by attenuating the raster current.

Spot size and effective focal length measurements for a fast axial flow CO2 laser

1997 ◽  
Author(s):  
Robert J. Steele ◽  
Phillip W. Fuerschbach ◽  
Danny O. MacCallum
Keyword(s):  
Co2 Laser ◽  
Focal Length ◽  
Axial Flow ◽  
Spot Size ◽  
Effective Focal Length ◽  
Length Measurements

scholarly journals Strong texture tuning along different crystalline directions in glass-supported CeO2 thin films by ultrasonic spray pyrolysis

2021 ◽  
Vol 11 (1) ◽  
Author(s):  
Inti Zumeta-Dubé ◽  
José Manuel García Rangel ◽  
Jorge Roque ◽  
Issis Claudette Romero-Ibarra ◽  
Mario Fidel García Sánchez
Keyword(s):  
Thin Films ◽  
Spray Pyrolysis ◽  
Spray Pyrolysis Technique ◽  
Morphological Characteristics ◽  
Ultrasonic Spray Pyrolysis ◽  
Cost Effective ◽  
Growth Direction ◽  
Large Area ◽  
Smart Windows ◽  
Ultrasonic Spray

AbstractThe strong facet-dependent performance of glass-supported CeO2 thin films in different applications (catalysis, smart windows, etc.) has been the target of diverse fundamental and technological approaches. However, the design of accurate, cost-effective and scalable methods with the potential for large-area coverage that produce highly textured glass-supported CeO2 thin films remains a technological challenge. In the present work, it is demonstrated that under proper tuning conditions, the ultrasonic spray pyrolysis technique enables one to obtain glass-supported polycrystalline CeO2 films with noticeable texture along both the (100) and (111) directions, as well as with randomly oriented crystallites (no texture). The influence of flow rates, solution molarity, and substrate temperature on the texture and morphological characteristics, as well as optical absorption and Raman response of the deposited films, is evaluated. The obtained results are discussed on the basis of the combined dependence of the CeO2-exposed surfaces on the thermodynamic stability of the corresponding facets and the reaction kinetics, which modulate the crystallite growth direction.

scholarly journals All-Organic, Low Voltage, Transparent and Compliant Organic Field-Effect Transistor Fabricated by Means of Large-Area, Cost-Effective Techniques

2020 ◽  
Vol 10 (19) ◽  
pp. 6656
Author(s):  
Stefano Lai ◽  
Giulia Casula ◽  
Pier Carlo Ricci ◽  
Piero Cosseddu ◽  
Annalisa Bonfiglio
Keyword(s):  
Field Effect ◽  
Low Voltage ◽  
Field Effect Transistors ◽  
High Mobility ◽  
Chemical Vapor ◽  
Cost Effective ◽  
Large Area ◽  
Parylene C ◽  
Biomedical Sensing ◽  
Novel Applications

The development of electronic devices with enhanced properties of transparency and conformability is of high interest for the development of novel applications in the field of bioelectronics and biomedical sensing. Here, a fabrication process for all organic Organic Field-Effect Transistors (OFETs) by means of large-area, cost-effective techniques such as inkjet printing and chemical vapor deposition is reported. The fabricated device can operate at low voltages (as high as 4 V) with ideal electronic characteristics, including low threshold voltage, relatively high mobility and low subthreshold voltages. The employment of organic materials such as Parylene C, PEDOT:PSS and 6,13-Bis(triisopropylsilylethynyl)pentacene (TIPS pentacene) helps to obtain highly transparent transistors, with a relative transmittance exceeding 80%. Interestingly enough, the proposed process can be reliably employed for OFET fabrication over different kind of substrates, ranging from transparent, flexible but relatively thick polyethylene terephthalate (PET) substrates to transparent, 700-nm-thick, compliant Parylene C films. OFETs fabricated on such sub-micrometrical substrates maintain their functionality after being transferred onto complex surfaces, such as human skin and wearable items. To this aim, the electrical and electromechanical stability of proposed devices will be discussed.

Sign in / Sign up

Export Citation Format

Share Document