anthropogenic pollutant
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2022 ◽  
Author(s):  
Haoyu Jiang ◽  
Yingyao He ◽  
Yiqun Wang ◽  
Sheng Li ◽  
Bin Jiang ◽  
...  

Abstract. The presence of organic sulfur compounds (OSs) at the water surface, acting as organic surfactants, may influence the air-water interaction and contribute to new particle formation in the atmosphere. However, the impact of ubiquitous anthropogenic pollutant emissions, such as SO2 and polycyclic aromatic hydrocarbons (PAHs) on the formation of OSs at the air-water interface still remains unknown. Here, we observe large amounts of OSs formation in presence of SO2, upon irradiation of aqueous solutions containing typical PAHs such as pyrene (PYR), fluoranthene (FLA), and phenanthrene (PHE), as well as dimethylsulfoxide (DMSO). We observe rapid formation of several gaseous OSs from light-induced heterogeneous reactions of SO2 with either DMSO or a mixture of PAHs/DMSO, and some of these OSs (e.g. methanesulfonic acid) are well established secondary organic aerosol (SOA) precursors. A myriad of OSs and unsaturated compounds are produced and detected in the aqueous phase. The tentative reaction pathways are supported by theoretical calculations of the reaction Gibbs energies. Our findings provide new insights into potential sources and formation pathways of OSs occurring at the water (sea, lake, river) surface, that should be considered in future model studies to better represent the air-water interaction and SOA formation processes.


2021 ◽  
Vol 288 (1952) ◽  
pp. 20210454
Author(s):  
Jules Schligler ◽  
Daphne Cortese ◽  
Ricardo Beldade ◽  
Stephen E. Swearer ◽  
Suzanne C. Mills

Artificial light at night (ALAN) is an increasing anthropogenic pollutant, closely associated with human population density, and now well recognized in both terrestrial and aquatic environments. However, we have a relatively poor understanding of the effects of ALAN in the marine realm. Here, we carried out a field experiment in the coral reef lagoon of Moorea, French Polynesia, to investigate the effects of long-term exposure (18–23 months) to chronic light pollution at night on the survival and growth of wild juvenile orange-fin anemonefish, Amphiprion chrysopterus . Long-term exposure to environmentally relevant underwater illuminance (mean: 4.3 lux), reduced survival (mean: 36%) and growth (mean: 44%) of juvenile anemonefish compared to that of juveniles exposed to natural moonlight underwater (mean: 0.03 lux). Our study carried out in an ecologically realistic situation in which the direct effects of artificial lighting on juvenile anemonefish are combined with the indirect consequences of artificial lighting on other species, such as their competitors, predators, and prey, revealed the negative impacts of ALAN on life-history traits. Not only are there immediate impacts of ALAN on mortality, but the decreased growth of surviving individuals may also have considerable fitness consequences later in life. Future studies examining the mechanisms behind these findings are vital to understand how organisms can cope and survive in nature under this globally increasing pollutant.


2021 ◽  
Vol 20 (1) ◽  
Author(s):  
Patrick D. M. C. Katoto ◽  
Amanda S. Brand ◽  
Buket Bakan ◽  
Paul Musa Obadia ◽  
Carsi Kuhangana ◽  
...  

Abstract Background Air pollution is one of the world’s leading mortality risk factors contributing to seven million deaths annually. COVID-19 pandemic has claimed about one million deaths in less than a year. However, it is unclear whether exposure to acute and chronic air pollution influences the COVID-19 epidemiologic curve. Methods We searched for relevant studies listed in six electronic databases between December 2019 and September 2020. We applied no language or publication status limits. Studies presented as original articles, studies that assessed risk, incidence, prevalence, or lethality of COVID-19 in relation with exposure to either short-term or long-term exposure to ambient air pollution were included. All patients regardless of age, sex and location diagnosed as having COVID-19 of any severity were taken into consideration. We synthesised results using harvest plots based on effect direction. Results Included studies were cross-sectional (n = 10), retrospective cohorts (n = 9), ecological (n = 6 of which two were time-series) and hypothesis (n = 1). Of these studies, 52 and 48% assessed the effect of short-term and long-term pollutant exposure, respectively and one evaluated both. Pollutants mostly studied were PM2.5 (64%), NO2 (50%), PM10 (43%) and O3 (29%) for acute effects and PM2.5 (85%), NO2 (39%) and O3 (23%) then PM10 (15%) for chronic effects. Most assessed COVID-19 outcomes were incidence and mortality rate. Acutely, pollutants independently associated with COVID-19 incidence and mortality were first PM2.5 then PM10, NO2 and O3 (only for incident cases). Chronically, similar relationships were found for PM2.5 and NO2. High overall risk of bias judgments (86 and 39% in short-term and long-term exposure studies, respectively) was predominantly due to a failure to adjust aggregated data for important confounders, and to a lesser extent because of a lack of comparative analysis. Conclusion The body of evidence indicates that both acute and chronic exposure to air pollution can affect COVID-19 epidemiology. The evidence is unclear for acute exposure due to a higher level of bias in existing studies as compared to moderate evidence with chronic exposure. Public health interventions that help minimize anthropogenic pollutant source and socio-economic injustice/disparities may reduce the planetary threat posed by both COVID-19 and air pollution pandemics.


2021 ◽  
Vol 9 ◽  
Author(s):  
Yun Liang ◽  
Anika Lehmann ◽  
Gaowen Yang ◽  
Eva F. Leifheit ◽  
Matthias C. Rillig

Microplastic as an anthropogenic pollutant accumulates in terrestrial ecosystems over time, threatening soil quality and health, for example by decreasing aggregate stability. Organic matter addition is an efficient approach to promote aggregate stability, yet little is known about whether microplastic can reduce the beneficial effect of organic matter on aggregate stability. We investigated the impacts of microplastic fibers in the presence or absence of different organic materials by carrying out a soil incubation experiment. This experiment was set up as a fully factorial design containing all combinations of microplastic fibers (no microplastic fiber addition, two different types of polyester fibers, and polyacrylic) and organic matter (no organic matter addition, Medicago lupulina leaves, Plantago lanceolata leaves, wheat straw, and hemp stems). We evaluated the percentage of water-stable aggregates (WSA) and activities of four soil enzymes (β-glucosidase, β-D-celluliosidase, N-acetyl-b-glucosaminidase, phosphatase). Organic matter addition increased WSA and enzyme activities, as expected. In particular, Plantago or wheat straw addition increased WSA and enzyme activities by 224.77 or 281.65% and 298.51 or 55.45%, respectively. Microplastic fibers had no effect on WSA and enzyme activities in the soil without organic matter addition, but decreased WSA and enzyme activities by 26.20 or 37.57% and 23.85 or 26.11%, respectively, in the presence of Plantago or wheat straw. Our study shows that the effects of microplastic fibers on soil aggregation and enzyme activities are organic matter dependent. A possible reason is that Plantago and wheat straw addition stimulated soil aggregation to a greater degree, resulting in more newly formed aggregates containing microplastic, the incorporated microplastic fibers led to less stable aggregates, and decrease in enzyme activities This highlights an important aspect of the context dependency of microplastic effects in soil and on soil health. Our results also suggest risks for soil stability associated with organic matter additions, such as is common in agroecosystems, when microplastics are present.


2021 ◽  
Author(s):  
Henk Eskes ◽  
Pieternel Levelt ◽  
Deborah Stein ◽  
Isabelle DeSmedt ◽  
Ilse Aben ◽  
...  

<p>The lockdown measures taken to combat the COVID-19 virus implemented in a majority of countries worldwide have had a dramatic impact on the anthropogenic pollutant emissions, related to a drastic reduction of road and air traffic, as well as part of the industrial activities. In our contribution we investigate the presence of COVID-19-related imprints in air quality as observed from space, focussing on worldwide industrial/highly populated regions where strong lockdown measures have been taken (e.g., China, Europe, US). This is done by exploiting the observations of the TROPOMI instrument onboard the Copernicus Sentinel-5P platform, for a number of trace gases which are indicators of anthropogenic activity. We make use of the TROPOMI operational product portfolio, which includes tropospheric NO2, CO, SO2, and HCHO. These operational data products are complemented by other scientific products such as the BIRA-IASB glyoxal (CHOCHO) retrievals and a new SO2 retrieval algorithm called COBRA. The reductions in NO2 observed by TROPOMI have been documented already in the recent literature for several regions and countries worldwide. In our contribution we focus on the combined observations of multiple trace gases, which provides not only information about how much primary (NOx) emissions decreased, but also gives region-to-region insights and constraints on the overall changes in atmospheric composition as a result of these lockdowns.</p>


2021 ◽  
Author(s):  
Collin J. Weber ◽  
Simone Lechthaler ◽  
Georg Stauch ◽  
Christian Opp

<p>After approximately two decades of plastic research in freshwater environments, plastics and especially microplastics (d < 5 mm) have entered the scientific consciousness as an anthropogenic pollutant. Even if this pollutant shows certain comparability with heavy metal pollution in soils and sediments, it should be seen as a purely anthropogenic material without geochemical or natural background loads, which leads to the assumption that it might also be a potential marker of the Anthropocene. Regarding the global plastic cycle within the environment, rivers act as main transport paths from land-to-sea. As rivers are embedded into landscapes, accumulation of plastics within riverine (e.g. sediment temporary sink) and accompanied terrestrial environments (e.g., floodplain storage for deposited plastics) has been proven in initial studies.</p><p>In contrast to other natural or anthropogenic pollutants, the approximate time since plastics and microplastic can be introduced into the environment starts in the 1950's with increasing global plastic production and consumption. A steady increase of possible plastic loads with the rising plastic production, probably decreasing with beginning environmental responsibility (approx. 2010 or beyond) leads to the fact, that plastic contents mainly occur in sediments and soils over a period of the last 70 years. This circumstance in connection with the general known sink function of soils and sediments, especially floodplains, nutrients as well as pollutants, allows the consideration of plastic deposits for dating purposes. As different dating methods reach their limits regarding comparatively young sediments, the connection between plastic deposition depth and temporal entry provides a basis for dating recent sediment layers. Possible detailed age differentiations in dependence on the identification of polymer types and additives, particle surface appearance (e.g., fresh/weathered) or spectroscopic criteria (e.g., surface weathering determination) are thinkable.</p><p>The opinion presented here, aims to address this new opportunity on the basis of own research findings within floodplains as well as other studies and highlights two main requirements: The first requirement for a sufficient dating implementation of plastic particles is the particle size: Detection and application for dating purposes is relatively easy to apply for macro- and mesoplastic particles (˃5 mm), due to size and less mobility in soils or sediments (e.g., plastic films embedded in sediment structure). In contrast for particles in the microplastic size class (˂ 5mm down to 1 µm) we recommend only the consideration of coarse microplastics (˃ 2mm) as smaller particles could easily shift in soils and sediments (e.g., bioturbation, preferential flow).  Additionally, the selection of a suitable sampling site as a second requirement depends on the appropriate localization within the floodplain area and surface morphology, sampling depth, flood history and anthropogenic influences.</p><p>Apart from the numerous potential environmental risks of plastics, their purely anthropogenic production and their respectively features, can turn them into a useful dating tool in river and floodplain sediments and thus enabling, besides the detection alone, a further application. This approach could also be transferred to marine or lacustrine sediments in future.</p>


2021 ◽  
Vol 21 (4) ◽  
pp. 2959-2980
Author(s):  
Yao Wang ◽  
Yue Zhao ◽  
Yuchen Wang ◽  
Jian-Zhen Yu ◽  
Jingyuan Shao ◽  
...  

Abstract. Organosulfates (OSs) are ubiquitous in the atmosphere and serve as important tracers for secondary organic aerosols (SOAs). Despite intense research over the years, the abundance, origin, and formation mechanisms of OSs in ambient aerosols, particularly in regions with severe anthropogenic pollution, are still not well understood. In this study, we collected filter samples of ambient fine particulate matter (PM2.5) over four seasons in both 2015–2016 and 2018–2019 at an urban site in Shanghai, China, and comprehensively characterized the OS species in these PM2.5 samples using an ultra-performance liquid chromatography quadrupole time-of-flight mass spectrometer equipped with an electrospray ionization (ESI) source (UPLC-ESI-QToFMS). Overall, we find that while the concentration of organic aerosols (OAs) decreased by 29 % in 2018–2019 compared to that in 2015–2016, mainly as a result of the reduction of anthropogenic pollutant emissions in eastern China, the annually averaged concentrations of 35 quantified OSs were similar in both years (65.5 ± 77.5 ng m−3, 0.57 % ± 0.56 % of OA in 2015–2016 vs. 59.4 ± 79.7 ng m−3, 0.66 % ± 0.56 % of OA in 2018–2019), suggesting an increased contribution of SOAs to OAs in 2018–2019 compared to 2015–2016. Isoprene- and monoterpene-derived OSs were the two most abundant OS families, on average, accounting for 36.3 % and 31.0 % of the quantified OS concentrations, respectively, during both sampling years, suggesting an important contribution of biogenic emissions to the production of OSs and SOAs in Shanghai. The abundance of biogenic OSs, particularly those arising from isoprene, exhibited strong seasonality (peaked in summer) but no significant interannual variability. In contrast, the quantified anthropogenic OSs had little seasonal variability and declined in 2018–2019 compared with those in 2015–2016. The C2 and C3 OS species that have both biogenic and anthropogenic origins contributed, on average, 19.0 % of the quantified OSs, with C2H3O6S−, C3H5O5S−, and C3H5O6S− being the most abundant species, together accounting for 76 % of the C2 and C3 OS concentrations in 2015–2016 and 2018–2019. 2-Methyltetrol sulfate (2-MTS, C5H11O7S−) and monoterpene-derived C10H16NO7S− were the most abundant OSs and nitrooxy OSs in summer, on average, contributing 31 % and 5 % of the quantified OSs, respectively, during the summertime of the sampling years. The substantially larger concentration ratio of 2-MTS to 2-methylglyceric acid sulfate (2-MAS, C4H7O7S−) in summer (6.8–7.8) compared to the other seasons (0.31–0.78) implies that low-NOx oxidation pathways played a dominant role in isoprene-derived SOA formation in summer, while high-NOx reaction pathways were more important in other seasons. We further find that the production of OSs was largely controlled by the level of Ox (Ox= O3+ NO2), namely the photochemistry of OS precursors, particularly in summer, though sulfate concentration, aerosol acidity, and aerosol liquid water content (ALWC) that could affect the heterogeneous chemistry of reactive intermediates leading to OS formation also played a role. Our study provides valuable insights into the characteristics and mechanisms of OS formation in a typical Chinese megacity and implies that the mitigation of Ox pollution can effectively reduce the production of OSs and SOAs in eastern China.


2021 ◽  
Vol 9 ◽  
Author(s):  
Krystie A. Miner ◽  
Mar Huertas ◽  
Andrea S. Aspbury ◽  
Caitlin R. Gabor

Human population growth and its associated effects on the environment contribute to the rapid decrease of biodiversity worldwide. Artificial light at night (ALAN) is an anthropogenic pollutant that is increasing with the spread of urbanization and may contribute to biodiversity declines. ALAN alters the migration patterns of birds, communication in frogs, and impacts reproduction, behavior, and physiology of multiple other taxa. However, most of the studies on ALAN are based on terrestrial systems, and overall, the effects of ALAN on freshwater organisms are poorly understood. We investigated how ALAN affects the physiology, behavior, and reproduction of a widespread, tolerant species of freshwater fish. Gambusia affinis are small livebearing fish often found in urban streams. We exposed groups of female G. affinis to either a natural light cycle or a constant 24-h light cycle (ALAN) in the laboratory for 60 days. In another experiment, we exposed female G. affinis to the same treatments in outdoor mesocosms for 32 days. We found that exposure to ALAN lowered glucose levels in the brain and decreased swimming activity, but had no effect on cortisol release rates, reproduction, survival, or growth. This research is strengthened by measuring multiple metrics in response to ALAN and by incorporating both a field and laboratory component which confirm similar results. These results suggest that this tolerant species of fish may behaviorally adjust to ALAN rather than modulate their endocrine stress response.


Water ◽  
2020 ◽  
Vol 12 (9) ◽  
pp. 2560
Author(s):  
Pauline Macharia ◽  
Norbert Kreuzinger ◽  
Nzula Kitaka

This work explores the application of the Water-Energy Nexus concept for water supply in the African context, where its operationalization is quite limited compared to developed regions. Furthermore, water supply and demand drivers and their influence on energy use are examined. This study found that there is limited literature available on the operationalization of the concept, and energy use is not considered a key performance indicator by water regulators and utilities. Regionally, most of the studies were carried out in the northern and southern Africa, where energy demand for water supply through desalination is high. An analysis of water supply and demand drivers show diminishing quantities of available freshwater, and increased anthropogenic pollutant loads in some areas are projected. Consequently, utilities will likely consider alternative energy-intensive water supply options. Increased population growth with the highest global urban growth rate is projected, with about 60% of the total population in Africa as urban dwellers by 2050. This implies huge growth in water demand that calls for investment in technology, infrastructure, and improved understanding of energy use and optimization, as the largest controllable input within utilities boundaries. However, it requires a data-driven understanding of the operational drivers for water supply and incorporation of energy assessment metrics to inform water-energy policies and to exploit the nexus opportunities.


Life ◽  
2020 ◽  
Vol 10 (6) ◽  
pp. 86
Author(s):  
Carla Ferreira ◽  
Catarina Almeida ◽  
Sandra Tenreiro ◽  
Alexandre Quintas

Parkinson’s Disease (PD) is currently the most rapid growing neurodegenerative disease and over the past generation, its global burden has more than doubled. The onset of PD can arise due to environmental, sporadic or genetic factors. Nevertheless, most PD cases have an unknown etiology. Chemicals, such as the anthropogenic pollutant 1-methyl-4-phenyl-1,2,3,6-tetrahydropyridine (MPTP) and amphetamine-type stimulants, have been associated with the onset of PD. Conversely, cannabinoids have been associated with the treatment of the symptoms’. PD and medical cannabis is currently under the spotlight, and research to find its benefits on PD is on-going worldwide. However, the described clinical applications and safety of pharmacotherapy with cannabis products are yet to be fully supported by scientific evidence. Furthermore, the novel psychoactive substances are currently a popular alternative to classical drugs of abuse, representing an unknown health hazard for young adults who may develop PD later in their lifetime. This review addresses the neurotoxic and neuroprotective impact of illicit substance consumption in PD, presenting clinical evidence and molecular and cellular mechanisms of this association. This research area is utterly important for contemporary society since illicit drugs’ legalization is under discussion which may have consequences both for the onset of PD and for the treatment of its symptoms.


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