Heat Transfer in Encased Graphene

Author(s):  
Zhen Chen ◽  
Wanyoung Jang ◽  
Wenzhong Bao ◽  
Chun Ning Lau ◽  
Chris Dames

Experimentally understanding the heat transfer in graphene (sheets of graphite a few atoms thick) is important for fundamental physics as well as device applications. In particular, measurements of the heat flow through graphene encased by oxide layers are essential for future graphene-based nanoelectronics, interconnects, and thermal management structures. Here we use a “heat spreader method” to study the heat dissipation performance of encased graphene. Measurements show enhanced heat spreading by a graphene layer as compared to control samples without graphene. At room temperature, the in-plane thermal conductivity of encased graphene sheets of thickness 2 nm and 5 nm is measured to be ∼150 W/m-K, more than one order of magnitude smaller than a published report for a freely-suspended graphene sheet [A. A. Balandin et al., Nano Lett. 8, 902], as well as bulk graphite. We also used a differential 3ω method to measure the thermal contact resistance between graphene and SiO2, finding a value around 10−8 m2-K/W at room temperature. Possible reasons for the unexpectedly low thermal conductivity are also discussed.

Author(s):  
Odne S. Burheim ◽  
Jon G. Pharoah ◽  
Hannah Lampert ◽  
Preben J. S. Vie ◽  
Signe Kjelstrup

We report the through-plane thermal conductivities of the several widely used carbon porous transport layers (PTLs) and their thermal contact resistance to an aluminum polarization plate. We report these values both for wet and dry samples and at different compaction pressures. We show that depending on the type of PTL and the existence of residual water, the thermal conductivity of the materials varies from 0.15 W K−1 m−1 to 1.6 W K−1 m−1, one order of magnitude. This behavior is the same for the contact resistance varying from 0.8 m2 K W−1 to 11×10−4 m2 K W−1. For dry PTLs, the thermal conductivity decreases with increasing polytetrafluorethylene (PTFE) content and increases with residual water. These effects are explained by the behavior of air, water, and PTFE in between the PTL fibers. It is also found that Toray papers of differing thickness exhibit different thermal conductivities.


2021 ◽  
Vol 12 (1) ◽  
Author(s):  
Shoufeng Lan ◽  
Xiaoze Liu ◽  
Siqi Wang ◽  
Hanyu Zhu ◽  
Yawen Liu ◽  
...  

AbstractThe interplay between chirality and magnetism generates a distinct physical process, the magneto-chiral effect, which enables one to develop functionalities that cannot be achieved solely by any of the two. Such a process is universal with the breaking of parity-inversion and time-reversal symmetry simultaneously. However, the magneto-chiral effect observed so far is weak when the matter responds to photons, electrons, or phonons. Here we report the first observation of strong magneto-chiral response to excitons in a twisted bilayer tungsten disulfide with the amplitude of excitonic magneto-chiral (ExMCh) anisotropy reaches a value of ~4%. We further found the ExMCh anisotropy features with a spectral splitting of ~7 nm, precisely the full-width at half maximum of the excitonic chirality spectrum. Without an externally applied strong magnetic field, the observed ExMCh effect with a spontaneous magnetic moment from the ferromagnetic substrate of thulium iron garnet at room temperature is favorable for device applications. The unique ExMCh processes provide a new pathway to actively control magneto-chiral applications in photochemical reactions, asymmetric synthesis, and drug delivery.


Author(s):  
G P Voller ◽  
M Tirovic ◽  
R Morris ◽  
P Gibbens

The aim of this investigation was to study automotive disc brake cooling characteristics experimentally using a specially developed spin rig and numerically using finite element (FE) and computational fluid dynamics (CFD) methods. All three modes of heat transfer (conduction, convection and radiation) have been analysed along with the design features of the brake assembly and their interfaces. The spin rig proved to be very valuable equipment; experiments enabled the determination of the thermal contact resistance between the disc and wheel carrier. The analyses demonstrated the sensitivity of this mode of heat transfer to clamping pressure. For convective cooling, heat transfer coefficients were measured and very similar results were obtained from spin rig experiments and CFD analyses. The nature of radiative heat dissipation implies substantial e ects at high temperatures. The results indicate substantial change of emissivity throughout the brake application. The influence of brake cooling parameters on the disc temperature has been investigated by FE modelling of a long drag brake application. The thermal power dissipated during the drag brake application has been analysed to reveal the contribution of each mode of heat transfer.


Science ◽  
2020 ◽  
Vol 367 (6475) ◽  
pp. 309-312 ◽  
Author(s):  
Yo Machida ◽  
Nayuta Matsumoto ◽  
Takayuki Isono ◽  
Kamran Behnia

Allotropes of carbon, such as diamond and graphene, are among the best conductors of heat. We monitored the evolution of thermal conductivity in thin graphite as a function of temperature and thickness and found an intimate link between high conductivity, thickness, and phonon hydrodynamics. The room-temperature in-plane thermal conductivity of 8.5-micrometer-thick graphite was 4300 watts per meter-kelvin—a value well above that for diamond and slightly larger than in isotopically purified graphene. Warming enhances thermal diffusivity across a wide temperature range, supporting partially hydrodynamic phonon flow. The enhancement of thermal conductivity that we observed with decreasing thickness points to a correlation between the out-of-plane momentum of phonons and the fraction of momentum-relaxing collisions. We argue that this is due to the extreme phonon dispersion anisotropy in graphite.


2020 ◽  
Vol 11 (1) ◽  
Author(s):  
Ji Qi ◽  
Baojuan Dong ◽  
Zhe Zhang ◽  
Zhao Zhang ◽  
Yanna Chen ◽  
...  

Abstract A solid with larger sound speeds usually exhibits higher lattice thermal conductivity. Here, we report an exception that CuP2 has a quite large mean sound speed of 4155 m s−1, comparable to GaAs, but single crystals show very low lattice thermal conductivity of about 4 W m−1 K−1 at room temperature, one order of magnitude smaller than GaAs. To understand such a puzzling thermal transport behavior, we have thoroughly investigated the atomic structures and lattice dynamics by combining neutron scattering techniques with first-principles simulations. This compound crystallizes in a layered structure where Cu atoms forming dimers are sandwiched in between P atomic networks. In this work, we reveal that Cu atomic dimers vibrate as a rattling mode with frequency around 11 meV, which is manifested to be remarkably anharmonic and strongly scatters acoustic phonons to achieve the low lattice thermal conductivity.


2013 ◽  
Vol 135 (9) ◽  
Author(s):  
Jiajun Xu ◽  
Bao Yang ◽  
Boualem Hammouda

In this work, thermophysical properties, microstructure, and pool boiling characteristics of water-in-polyalphaolefin (PAO) nanoemulsion fluids have been measured in the water concentration range of 0–10.3 vol. %, in order to gain basic data for nanoemulsion boiling. Water-in-PAO nanoemulsion fluids are formed via self-assembly with surfactant: sodium sullfosuccinate (AOT). Thermal conductivity of these fluids is found to increase monotonically with water concentration, as expected from the Maxwell equation. Unlike thermal conductivity, their dynamic viscosity first increases with water concentration, reaches a maximum at 5.3 vol. %, and then decreases. The observed maximum viscosity could be attributed to the attractive forces among water droplets. The microstructures of the water-in-PAO nanoemulsion fluids are measured via the small-angle neutron scattering (SANS) technique, which shows a transition from sphere to elongated cylinder when the water concentration increases above 5.3 vol. %. The pool boiling heat transfer of these water-in-PAO nanoemulsion fluids is measured on a horizontal Pt wire at room temperature (25 °C, subcooled condition). One interesting phenomenon observed is that the pool boiling follows two different curves randomly when the water concentration is in the range of 5.3 vol. % to 7.8 vol. %.


Author(s):  
Brian K. Ryglowski ◽  
Randall D. Pollak ◽  
Young W. Kwon

Heat dissipation is a major challenge for many technologies. Possible solutions include thermal energy transfer via coolant fluid to a phase change material (PCM), with higher thermal conductivity a design goal. In recent years, heat transfer nanofluids (fluids with suspended nanoparticles) have received attention based on their potential for improving thermal conductivity. Carbon nanotubes (CNTs) are an attractive additive due to their enhanced thermal conductivity and ability to remain suspended over long times. However, characterizing their potential is difficult due to the many design variables and the need for repeated thermal conductivity tests for comparison. Since thermal conductivity enhancement is dependent on a dispersed nanotube network, the electrical conductivity of CNTs can be exploited to monitor the stability of such nanofluids, as such testing is quick and simple. The aim of this research was to evaluate electrical conductivity testing as a means to monitor stability of CNT-enhanced distilled water as a PCM, with varying CNT size, type, and concentration; and various other processing variables. The prepared nanofluids were tested after repeated phase change cycles. Results indicate that electrical conductivity testing is a practical means of monitoring the nanofluid stability, and CNT-based nanofluids show both promise and limitations as a PCM.


Author(s):  
C. Y. Shen ◽  
M. Yang ◽  
L. Li ◽  
Y. W. Zhang

The heat dissipation of current busbur in power plant is one of the important issues in power transmission, usually through the cylinder slotted to strengthen heat dissipation. Natural convection in a cylinder with an internal slotted annulus is the computational model abstracted from it. Natural convection in a cylinder with an concentric slotted annulus is concerned. Attention is focused on the effects of different slotted sizes on natural convection. Numerical results showed that, the equivalent thermal conductivity increases with the increase of Rayleigh number. At high Ra, the system heat transfer exhibit rich nonlinear characteristics. When the slotted direction or the slotted degree changed, it would have an important impact on the flow and heat transfer in the system, and also influence the related nonlinear characteristics.


1997 ◽  
Vol 43 (144) ◽  
pp. 339-351 ◽  
Author(s):  
Richard E. Brandt ◽  
Stephen G. Warren

AbstractTo study near-surface heat flow on the Antarctíc ice sheet, snow temperatures were measured at South Pole Station to a depth of 3 m at 15 min intervals during most of 1992. Solar heating and water-vapor transport were negligible during the 6 month Winter, as was inter-grain net thermal radiation, leaving conduction as the dominant heat-transport mechanism. The rate of temperature change at depth over 15 min intervals was smaller than that at the surface, by one order of magnitude at 20 cm depth and two orders of magnitude at 1 m depth. A finite-difference model, with conduction as the only heat-transfer mechanism and measured temperatures as the upper and lower boundary conditions, was applied to foursets of three thermistors each. The thermal conductivity was estimated as that which minimized the difference between modeled and measured 15 min changes in temperatures at the center thermistor. The thermal conductivity obtained at shallow depths (above 40 cm) was lower than that given by existing parameterizations based on density, probably because the snow grains were freshly deposited, cold and poorly bonded. A model using only vertical conduction explains on average 87% ofthe observed 15 min temperature changes at less than 60 cm depth and 92% below 60 cm. The difference between modeled andmeasured temperature changes decreased with depth. The discrepancies between model and observation correlated more strongly with the air-snow temperature difference than with the product of that difference with the square of the wind speed,suggesting that the residual errors are due more to non-vertical conduction and to sub-grid-scale variabilis of the conductivity than to windpumping. The residual heating rate not explained by the model of vertical conduction exceeds 0.2 W m−3only in the top 60 cm of the near-surface snow.


2016 ◽  
Vol 7 ◽  
pp. 2037-2044 ◽  
Author(s):  
Aparna Zagabathuni ◽  
Sudipto Ghosh ◽  
Shyamal Kumar Pabi

A suspension of particles below 100 nm in size, usually termed as nanofluid, often shows a notable enhancement in thermal conductivity, when measured by the transient hot-wire method. In contrast, when the conductivity of the same nanofluid is measured by the laser flash method, the enhancement reported is about one order of magnitude lower. This difference has been quantitatively resolved for the first time on the basis of the collision-mediated heat transfer model for nanofluids proposed earlier by our research group. Based on the continuum simulation coupled with stochastic analysis, the present theoretical prediction agrees well with the experimental observations from different measuring methods reported in the literature, and fully accounts for the different results from the two measuring methods mentioned above. This analysis also gives an indication that the nanofluids are unlikely to be effective for heat transfer in microchannels.


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