scholarly journals Unravelling strong electronic interlayer and intralayer correlations in a transition metal dichalcogenide

2021 ◽  
Vol 12 (1) ◽  
Author(s):  
T. J. Whitcher ◽  
Angga Dito Fauzi ◽  
D. Caozheng ◽  
X. Chi ◽  
A. Syahroni ◽  
...  
Keyword(s):  
Transition Metal ◽  
Near Infrared ◽  
Theoretical Calculations ◽  
High Energy ◽  
Low Energy ◽  
Great Effort ◽  
Energy Bands ◽  
Electronic Correlations ◽  
X Ray ◽  
Wide Range

AbstractElectronic correlations play important roles in driving exotic phenomena in condensed matter physics. They determine low-energy properties through high-energy bands well-beyond optics. Great effort has been made to understand low-energy excitations such as low-energy excitons in transition metal dichalcogenides (TMDCs), however their high-energy bands and interlayer correlation remain mysteries. Herewith, by measuring temperature- and polarization-dependent complex dielectric and loss functions of bulk molybdenum disulphide from near-infrared to soft X-ray, supported with theoretical calculations, we discover unconventional soft X-ray correlated-plasmons with low-loss, and electronic transitions that reduce dimensionality and increase correlations, accompanied with significantly modified low-energy excitons. At room temperature, interlayer electronic correlations, together with the intralayer correlations in the c-axis, are surprisingly strong, yielding a three-dimensional-like system. Upon cooling, wide-range spectral-weight transfer occurs across a few tens of eV and in-plane p–d hybridizations become enhanced, revealing strong Coulomb correlations and electronic anisotropy, yielding a two-dimensional-like system. Our result shows the importance of strong electronic, interlayer and intralayer correlations in determining electronic structure and opens up applications of utilizing TMDCs on plasmonic nanolithrography.

scholarly journals Multi-waveband detection of quasi-periodic pulsations in a stellar flare on EK Draconis observed by XMM-Newton

2019 ◽  
Vol 629 ◽  
pp. A147 ◽  
Author(s):  
A.-M. Broomhall ◽  
A. E. L. Thomas ◽  
C. E. Pugh ◽  
J. P. Pye ◽  
S. R. Rosen
Keyword(s):  
Energy Band ◽  
Cross Correlation ◽  
Power Spectra ◽  
High Energy ◽  
Low Energy ◽  
The Sun ◽  
Energy Bands ◽  
X Ray ◽  
High Energy Band ◽  
The Cross

Context. Quasi-periodic pulsations (QPPs) are time variations in the energy emission during a flare that are observed on both the Sun and other stars and thus have the potential to link the physics of solar and stellar flares. Aims. We characterise the QPPs detected in an X-ray flare on the solar analogue, EK Draconis, which was observed by XMM-Newton. Methods. We used wavelet and autocorrelation techniques to identify the QPPs in a detrended version of the flare. We also fitted a model to the flare based on an exponential decay combined with a decaying sinusoid. The flare is examined in multiple energy bands. Results. A statistically significant QPP is observed in the X-ray energy band of 0.2–12.0 keV with a periodicity of 76 ± 2 min. When this energy band is split, a statistically significant QPP is observed in the low-energy band (0.2–1.0 keV) with a periodicity of 73 ± 2 min and in the high-energy band (1.0–12.0 keV) with a periodicity of 82 ± 2 min. When fitting a model to the time series the phases of the signals are also found to be significantly different in the two energy bands (with a difference of 1.8 ± 0.2 rad) and the high-energy band is found to lead the low-energy band. Furthermore, the first peak in the cross-correlation between the detrended residuals of the low- and high-energy bands is offset from zero by more than 3σ (4.1 ± 1.3 min). Both energy bands produce statistically significant regions in the wavelet spectrum, whose periods are consistent with those listed above. However, the peaks are broad in both the wavelet and global power spectra, with the wavelet showing evidence for a drift in period with time, and the difference in period obtained is not significant. The offset in the first peak in the cross-correlation of the detrended residuals of two non-congruent energy bands (0.5−1.0 keV and 4.5−12.0 keV) is found to be even larger (10 ± 2 min). However, the signal-to-noise in the higher of these two energy-bands, covering the range 4.5−12.0 keV, is low. Conclusions. The presence of QPPs similar to those observed on the Sun, and other stars, suggests that the physics of flares on this young solar analogue is similar to the physics of solar flares. It is possible that the differences in the QPPs detected in the two energy bands are seen because each band observes a different plasma structure. However, the phase difference, which differs more significantly between the two energy bands than the period, could also be explained in terms of the Neupert effect. This suggests that QPPs are caused by the modulation of the propagation speeds of charged particles.

scholarly journals MetroMMC: Electron-Capture Spectrometry with Cryogenic Calorimeters for Science and Technology

2019 ◽  
Vol 199 (1-2) ◽  
pp. 441-450 ◽  
Author(s):  
P. C.-O. Ranitzsch ◽  
D. Arnold ◽  
J. Beyer ◽  
L. Bockhorn ◽  
J. J. Bonaparte ◽  
...  
Keyword(s):  
Electron Capture ◽  
Science And Technology ◽  
High Energy ◽  
Low Energy ◽  
Energy Threshold ◽  
High Energy Resolution ◽  
Wide Energy Range ◽  
Good Resolution ◽  
X Ray ◽  
Wide Range

AbstractAccurate decay data of radionuclides are necessary for many fields of science and technology, ranging from medicine and particle physics to metrology. However, data that are in use today are mostly based on measurements or theoretical calculation methods that are rather old. Recent measurements with cryogenic detectors and other methods show significant discrepancies to both older experimental data and theory in some cases. Moreover, the old results often suffer from large or underestimated uncertainties. This is in particular the case for electron-capture (EC) decays, where only a few selected radionuclides have ever been measured. To systematically address these shortcomings, the European metrology project MetroMMC aims at investigating six radionuclides decaying by EC. The nuclides are chosen to cover a wide range of atomic numbers Z, which results in a wide range of decay energies and includes different decay modes, such as pure EC or EC accompanied by $$\gamma $$γ- and/or $$\beta ^{+}$$β+-transitions. These will be measured using metallic magnetic calorimeters (MMCs), cryogenic energy-dispersive detectors with high-energy resolution, low-energy threshold and high, adjustable stopping power that are well suited for measurements of the total decay energy and X-ray spectrometry. Within the MetroMMC project, these detectors are used to obtain X-ray emission intensities of external sources as well as fractional EC probabilities of sources embedded in a $$4\pi $$4π absorber. Experimentally determined nuclear and atomic data will be compared to state-of-the-art theoretical calculations which will be further developed within the project. This contribution introduces the MetroMMC project and in particular its experimental approach. The challenges in EC spectrometry are to adapt the detectors and the source preparation to the different decay channels and the wide energy range involved, while keeping the good resolution and especially the low-energy threshold to measure the EC from outer shells.

scholarly journals Low-Energy Electron Damage to Condensed-Phase DNA and Its Constituents

2021 ◽  
Vol 22 (15) ◽  
pp. 7879
Author(s):  
Yingxia Gao ◽  
Yi Zheng ◽  
Léon Sanche
Keyword(s):  
Condensed Phase ◽  
Genetic Material ◽  
High Energy ◽  
Dna Lesions ◽  
Low Energy ◽  
Experimental Investigations ◽  
Experimental Conditions ◽  
Strand Breaks ◽  
Sequence Of Events ◽  
Wide Range

The complex physical and chemical reactions between the large number of low-energy (0–30 eV) electrons (LEEs) released by high energy radiation interacting with genetic material can lead to the formation of various DNA lesions such as crosslinks, single strand breaks, base modifications, and cleavage, as well as double strand breaks and other cluster damages. When crosslinks and cluster damages cannot be repaired by the cell, they can cause genetic loss of information, mutations, apoptosis, and promote genomic instability. Through the efforts of many research groups in the past two decades, the study of the interaction between LEEs and DNA under different experimental conditions has unveiled some of the main mechanisms responsible for these damages. In the present review, we focus on experimental investigations in the condensed phase that range from fundamental DNA constituents to oligonucleotides, synthetic duplex DNA, and bacterial (i.e., plasmid) DNA. These targets were irradiated either with LEEs from a monoenergetic-electron or photoelectron source, as sub-monolayer, monolayer, or multilayer films and within clusters or water solutions. Each type of experiment is briefly described, and the observed DNA damages are reported, along with the proposed mechanisms. Defining the role of LEEs within the sequence of events leading to radiobiological lesions contributes to our understanding of the action of radiation on living organisms, over a wide range of initial radiation energies. Applications of the interaction of LEEs with DNA to radiotherapy are briefly summarized.

scholarly journals Combination of Dual-Energy X-ray Transmission and Variable Gas-Ejection for the In-Line Automatic Sorting of Many Types of Scrap in One Measurement

2021 ◽  
Vol 11 (10) ◽  
pp. 4349
Author(s):  
Tianzhong Xiong ◽  
Wenhua Ye ◽  
Xiang Xu
Keyword(s):  
High Efficiency ◽  
Nearest Neighbor ◽  
High Energy ◽  
Dual Energy ◽  
Center Of Gravity ◽  
Low Energy ◽  
Identification Accuracy ◽  
Flow Process ◽  
X Ray ◽  
Automatic Sorting

As an important part of pretreatment before recycling, sorting has a great impact on the quality, efficiency, cost and difficulty of recycling. In this paper, dual-energy X-ray transmission (DE-XRT) combined with variable gas-ejection is used to improve the quality and efficiency of in-line automatic sorting of waste non-ferrous metals. A method was proposed to judge the sorting ability, identify the types, and calculate the mass and center-of-gravity coordinates according to the shading of low-energy, the line scan direction coordinate and transparency natural logarithm ratio of low energy to high energy (R_value). The material identification was satisfied by the nearest neighbor algorithm of effective points in the material range to the R_value calibration surface. The flow-process of identification was also presented. Based on the thickness of the calibration surface, the material mass and center-of-gravity coordinates were calculated. The feasibility of controlling material falling points by variable gas-ejection was analyzed. The experimental verification of self-made materials showed that identification accuracy by count basis was 85%, mass and center-of-gravity coordinates calculation errors were both below 5%. The method proposed features high accuracy, high efficiency, and low operation cost and is of great application value even to other solid waste sorting, such as plastics, glass and ceramics.

A multi-length-scale USAXS/SAXS facility: 10–50 keV small-angle X-ray scattering instrument

2013 ◽  
Vol 46 (5) ◽  
pp. 1508-1512 ◽  
Author(s):  
Byron Freelon ◽  
Kamlesh Suthar ◽  
Jan Ilavsky
Keyword(s):  
Small Angle ◽  
Soft Matter ◽  
High Energy ◽  
X Rays ◽  
X Ray ◽  
X Ray Scattering ◽  
Wide Range ◽  
And Performance ◽  
New Facility ◽  
Ray Scattering

Coupling small-angle X-ray scattering (SAXS) and ultra-small-angle X-ray scattering (USAXS) provides a powerful system of techniques for determining the structural organization of nanostructured materials that exhibit a wide range of characteristic length scales. A new facility that combines high-energy (HE) SAXS and USAXS has been developed at the Advanced Photon Source (APS). The application of X-rays across a range of energies, from 10 to 50 keV, offers opportunities to probe structural behavior at the nano- and microscale. An X-ray setup that can characterize both soft matter or hard matter and high-Zsamples in the solid or solution forms is described. Recent upgrades to the Sector 15ID beamline allow an extension of the X-ray energy range and improved beam intensity. The function and performance of the dedicated USAXS/HE-SAXS ChemMatCARS-APS facility is described.

Single Crystal Wurtzitic Aluminum Nitride Growth on Silicon Using Supersonic Gas Jets

1995 ◽  
Vol 395 ◽  
Author(s):  
S. A. Ustin ◽  
L. Lauhon ◽  
K. A. Brown ◽  
D. Q. Hu ◽  
W. Ho
Keyword(s):  
Aluminum Nitride ◽  
Growth Rates ◽  
High Energy ◽  
X Ray Diffraction ◽  
Rutherford Back Scattering ◽  
X Ray ◽  
Supersonic Molecular Beam ◽  
Supersonic Beams ◽  
Wide Range

ABSTRACTHighly oriented aluminum nitride (0001) films have been grown on Si(001) and Si (111) substrates at temperatures between 550° C and 775° C with dual supersonic molecular beam sources. Triethylaluminum (TEA;[(C2H5)3Al]) and ammonia (NH3) were used as precursors. Hydrogen, helium, and nitrogen were used as seeding gases for the precursors, providing a wide range of possible kinetic energies for the supersonic beams due to the disparate masses of the seed gases. Growth rates of AIN were found to depend strongly on the substrate orientation and the kinetic energy of the incident precursor; a significant increase in growth rate is seen when seeding in hydrogen or helium as opposed to nitrogen. Growth rates were 2–3 times greater on Si(001) than on Si(111). Structural characterization of the films was done by reflection high energy electron diffraction (RHEED) and x-ray diffraction (XRD). X-ray rocking curve (XRC) full-width half-maxima (FWHM) were seen as small as 2.5°. Rutherford back scattering (RBS) was used to determine the thickness of the films and their chemical composition. Films were shown to be nitrogen rich, deviating from perfect stoichiometry by 10%–20%. Surface analysis was performed by Auger electron spectroscopy (AES).

scholarly journals Broadband study of blazar 1ES 1959+650 during flaring state in 2016

2018 ◽  
Vol 611 ◽  
pp. A44 ◽  
Author(s):  
S. R. Patel ◽  
A. Shukla ◽  
V. R. Chitnis ◽  
D. Dorner ◽  
K. Mannheim ◽  
...  
Keyword(s):  
High Energy ◽  
Spectral Energy ◽  
Quiescent State ◽  
Energy Bands ◽  
Energy Distributions ◽  
X Ray ◽  
Broadband Emission ◽  
June July ◽  
Power Law Index ◽  
Observation Period

Aims. The nearby TeV blazar 1ES 1959+650 (z = 0.047) was reported to be in flaring state during June–July 2016 by Fermi-LAT, FACT, MAGIC and VERITAS collaborations. We studied the spectral energy distributions (SEDs) in different states of the flare during MJD 57530–57589 using simultaneous multiwaveband data with the aim of understanding the possible broadband emission scenario during the flare. Methods. The UV-optical and X-ray data from UVOT and XRT respectively on board Swift and high energy γ-ray data from Fermi-LAT were used to generate multiwaveband lightcurves as well as to obtain high flux states and quiescent state SEDs. The correlation and lag between different energy bands was quantified using discrete correlation function. The synchrotron self-Compton (SSC) model was used to reproduce the observed SEDs during flaring and quiescent states of the source. Results. A good correlation is seen between X-ray and high energy γ-ray fluxes. The spectral hardening with increase in the flux is seen in X-ray band. The power law index vs. flux plot in γ-ray band indicates the different emission regions for 0.1–3 GeV and 3–300 GeV energy photons. Two zone SSC model satisfactorily fits the observed broadband SEDs. The inner zone is mainly responsible for producing synchrotron peak and high energy γ-ray part of the SED in all states. The second zone is mainly required to produce less variable optical-UV and low energy γ-ray emission. Conclusions. Conventional single zone SSC model does not satisfactorily explain broadband emission during observation period considered. There is an indication of two emission zones in the jet which are responsible for producing broadband emission from optical to high energy γ-rays.

scholarly journals Alternatives to the Existence of Large Cooling Flows

1990 ◽  
Vol 115 ◽  
pp. 232-239
Author(s):  
Wallace Tucker
Keyword(s):  
Surface Brightness ◽  
Large Scale ◽  
Theoretical Calculations ◽  
Central Peak ◽  
High Energy ◽  
Cooling Time ◽  
Radiative Cooling ◽  
Massive Black Hole ◽  
X Ray ◽  
Cooling Flows

AbstractArguments against the existence of large scale cooling flows in clusters of galaxies are presented. The evidence for cooling flows is all circumstantial, consisting of observations of cool gas or hot gas with a radiative cooling time less than the Hubble time, or a central peak in the x-ray surface brightness profile. There is no evidence for large quantities (several tens to several hundreds of solar masses per year) of matter actually flowing anywhere. On the contrary, several lines of evidence — stellar dynamics, observations of the amount of star formation, x-ray surface brightness observations, theoretical calculations of the growth of thermal instabilities, the amount of cold gas — suggest that cooling flows, if they exist, must be suppressed by one to two orders of magnitude from the values implied by simple estimates based on the radiative cooling time of the x-ray emitting gas. Two heat sources which might accomplish this — thermal conduction and relativistic particles, are considered and an alternative to the standard model for cooling flows is presented: an accretion flow with feedback wherein the accretion of gas into a massive black hole in the central galaxy generates high energy particles that heat the gas and act to limit the accretion.

scholarly journals Long-term multiwavelength view of the blazar 1ES 1218+304

2019 ◽  
Vol 489 (4) ◽  
pp. 5076-5086 ◽  
Author(s):  
K K Singh ◽  
B Bisschoff ◽  
B van Soelen ◽  
A Tolamatti ◽  
J P Marais ◽  
...  
Keyword(s):  
High Energy ◽  
Host Galaxy ◽  
Energy Bands ◽  
X Ray ◽  
Very High Energy ◽  
Γ Ray ◽  
Activity State ◽  
Low Activity ◽  
Very High

ABSTRACT In this work, we present a multiwavelength study of the blazar 1ES 1218+304 using near simultaneous observations over 10 yr during the period 2008 September 1 to 2018 August 31 (MJD 54710–58361). We have analysed data from Swift-UVOT, Swift-XRT, and Fermi-LAT to study the long term behaviour of 1ES 1218+304 in different energy bands over the last decade. We have also used the archival data from OVRO, MAXI, and Swift-BAT available during the above period. The near simultaneous data on 1ES 1218+304 suggest that the long term multiwavelength emission from the source is steady and does not show any significant change in the source activity. The optical/UV fluxes are found to be dominated by the host galaxy emission and can be modelled using the pegase code. However, the time averaged X-ray and γ-ray emissions from the source are reproduced using a single zone leptonic model with log-parabolic distribution for the radiating particles. The intrinsic very high energy γ-ray emission during a low activity state of the source is broadly consistent with the predictions of the leptonic model for blazars. We have investigated the physical properties of the jet and the mass of the supermassive black hole at the centre of the host galaxy using long term X-ray observations from the Swift-XRT which is in agreement with the value derived using blackbody approximation of the host galaxy. We also discuss the extreme nature of the source on the basis of X-ray and γ-ray observations.

Epitaxial growth of BaO and SrO with new crystal structures using mass-separated low-energy O+ beams

1993 ◽  
Vol 8 (2) ◽  
pp. 321-323 ◽  
Author(s):  
Ryusuke Kita ◽  
Takashi Hase ◽  
Hiromi Takahashi ◽  
Kenichi Kawaguchi ◽  
Tadataka Morishita
Keyword(s):  
Lattice Constant ◽  
High Energy ◽  
Low Energy ◽  
Diffraction Reflection ◽  
High Energy Electron ◽  
Bulk Crystals ◽  
X Ray Diffraction ◽  
X Ray ◽  
Transmission Electron ◽  
Cubic Structure

The growth of BaO and SrO on SrTiO3(100) substrates using mass-separated low-energy (50 eV) O+ beams has been studied using x-ray diffraction, reflection high-energy electron diffraction, and high-resolution transmission electron microscopy. It was found that the BaO and SrO films have been epitaxially grown with new structures different from those of corresponding bulk crystals: The BaO films have a cubic structure with a lattice constant of 4.0 Å, and the SrO films have a tetragonal structure with a lattice constant of a = 3.7 Å parallel to the substrate and with c = 4.0 Å normal to the substrate.

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