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Molecules ◽  
2022 ◽  
Vol 27 (2) ◽  
pp. 338
Author(s):  
Shigeyuki Kawai ◽  
Wataru Hashimoto

4-Deoxy-l-erythro-5-hexoseulose uronate (DEH), DEH reductase, and alginate lyase have key roles in the metabolism of alginate, a promising carbon source in brown macroalgae for biorefinery. In contrast to the widely reviewed alginate lyase, DEH and DEH reductase have not been previously reviewed. Here, we summarize the current understanding of DEH and DEH reductase, with emphasis on (i) the non-enzymatic and enzymatic formation and structure of DEH and its reactivity to specific amino groups, (ii) the molecular identification, classification, function, and structure, as well as the structural determinants for coenzyme specificity of DEH reductase, and (iii) the significance of DEH for biorefinery. Improved understanding of this and related fields should lead to the practical utilization of alginate for biorefinery.


2021 ◽  
Author(s):  
Rosaria Ciriminna ◽  
Cristina Scolaro ◽  
Antonino Scurria ◽  
Silvia Sfameni ◽  
Gabriella Di Carlo ◽  
...  

The outcomes of adhesion and ecotoxicity tests carried out on metal specimens faithfully representing the surface of real ships, including the primer and tie coat layers typically applied on ship hull prior to deposition of the antifouling paint, show the practical applicability of "AquaSun" antifouling sol-gel coatings. Newly developed AquaSun coatings share superhydrophicity (contact angle >115) and exceptionally high scratch resistance (ASTM 5B). Coupled to the ecofriendly antifouling mechanism based on continuous H2O2 formation upon exposure to solar light and foul release due to low surface energy, these results open the route to the practical utilization of these novel marine coatings.


2021 ◽  
Author(s):  
Antonino Scurria ◽  
Silvia Sfameni ◽  
Gabriella Di Carlo ◽  
Mario Pagliaro ◽  
Anna Maria Visco ◽  
...  

The outcomes of adhesion and ecotoxicity tests carried out on metal specimens faithfully representing the surface of real ships, including the primer and tie coat layers typically applied on ship hull prior to deposition of the antifouling paint, show the practical applicability of "AquaSun" antifouling sol-gel coatings. Newly developed AquaSun coatings share superhydrophicity (contact angle >115) and exceptionally high scratch resistance (ASTM 5B). Coupled to the ecofriendly antifouling mechanism based on continuous H2O2 formation upon exposure to solar light and foul release due to low surface energy, these results open the route to the practical utilization of these novel marine coatings.


Author(s):  
Wasif Yasin ◽  
Muhammad Tayyab ◽  
Muhammad Hanif

It is essential to monitor the mean of a process regarding quality characteristics for the ongoing production. For enhancement of mean monitoring power of the exponentially weighted moving average (EWMA) chart, a new median quartile double ranked set sampling (MQDRSS) based EWMA control chart is proposed and named as EWMA-MQDRSS chart. In order to study the performance of the developed EWMA-MQDRSS chart, performance measures; average run length, and the standard deviation of run length are used. The shift detection ability of the proposed chart has been compared with counterparts, under the simple random sampling and ranking based sampling techniques. The extensive simulation-based results indicate that the EWMA-MQDRSS chart performs better to trace all kinds of shifts than the existing charts. An illustrative application concerning monitoring the diameter of the piston ring of a machine is also provided to demonstrate the practical utilization of the suggested chart.


Catalysts ◽  
2021 ◽  
Vol 11 (12) ◽  
pp. 1534
Author(s):  
Maali-Amel Mersel ◽  
Lajos Fodor ◽  
Péter Pekker ◽  
Miklós Jakab ◽  
Éva Makó ◽  
...  

Photocatalytic H2 production utilizing H2S, an industrial side-product, is regarded as an environmentally friendly process to produce clean energy through direct solar energy conversion. For this purpose, sulfide-based materials, such as photocatalysts, have been widely used due to their good solar response and high photocatalytic activity. In this work, a ZnS–CdS composite was studied, and special attention was dedicated to the influence of the preparation parameters on its H2 production activity. The ZnS–CdS composite, with an enhanced photoactivity for H2 production, was synthesized both from ammine complexes and, in a conventional way, directly from acetates at various pH values. Deviating from the traditional method, the photoactivity of ZnS–CdS prepared from ammine complexes was not affected by the pH. Besides, the hydrothermal treatment and the ammonia content strongly influenced the rate of H2 production in this system. DRS, TEM, SEM, XRD, and quantum yield measurements prove the dependence of the photoactivity of these catalysts on the structural and morphological properties determined by the preparation conditions. The promising photocatalytic efficiency achieved with the application of these ZnS–CdS catalysts, prepared without any metal deposition, encourages further investigations to enhance the rate of hydrogen generation by optimization of the reaction conditions for practical utilization.


2021 ◽  
Vol 2143 (1) ◽  
pp. 012025
Author(s):  
Yu Song ◽  
Jingui Lu

Abstract The application of related tech represented by machine vision in mechanical design has gradually deepened, which has greatly ameliorated the automation of mechanical design. Based on this, this paper first analyses the principle and important composition of machine vision tech, then studies the utilization value of machine vision tech in mechanical design, and finally analyses the typical practical utilization of machine vision tech in workpiece detection, workpiece measurement and high-precision measurement in mechanical design.


Author(s):  
Linghong Xu ◽  
Zhihao Yu ◽  
Junrong Zheng

Abstract Lithium metal is a promising anode utilized in cutting-edge high-energy batteries owing to the low density, low electrochemical potential, and super high theoretical capacity. Unfortunately, continuous uncontrollable lithium dendrite growth and ‘dead’ lithium result in capacity decay, low coulombic efficiency, and short circuit, severely hindering the practical utilization of lithium anode. Herein, we propose a three-dimensional porous lithiophilic current collector for lithium storage. The conductive 3D structure constructed by carbon fiber (CF) can well accommodate the deposited lithium, eliminating volume change between the lithium depositing/stripping process. Moreover, the polydopamine (PDA) coating on the CF surface possesses a large number of polar groups, which can homogenize Li+ ions distribution and apply as the sites for lithium deposition, decreasing nucleation overpotential. As a result, under the 1 mA cm−2 current density, the PDA coated CF (PDA@CF) electrode exhibits high CE (∼98%) for 1000 cycles. Galvanostatic measurements demonstrate that the Li anode using PDA@CF achieves 1000 h cycling life under 1 mA cm−2 with a low overpotential (<15 mV). The LiFePO4 full cell shows enhanced rate performance and stable long-term cycling.


Catalysts ◽  
2021 ◽  
Vol 11 (11) ◽  
pp. 1285
Author(s):  
Ewelina Ksepko ◽  
Rafal Lysowski

This paper contains the results of research on a promising combustion technology known as chemical looping combustion (CLC) and chemical looping with oxygen uncoupling (CLOU). The remarkable advantages of CLC are, among others, that concentrated CO2 stream can be obtained after water condensation without any energy penalty for its separation or significant decrease of NOx emissions. The objective of this work was to prepare a novel bi-metallic Fe–Mn supported on ZrO2 oxygen carriers. Performance of these carriers for the CLOU and CLC process with nitrogen/air and hard coal/air was evaluated. One-cycle CLC tests were conducted with supported Fe–Mn oxygen carriers in thermogravimetric analyzer utilizing hard coal as a fuel. The effects of the oxygen carrier chemical composition and process temperature on the reaction rates were determined. Our study proved that for CLOU, properties formation of bixbyite and spinel forms are responsible. Among iron ferrites, we concluded that iron-rich compounds such as Fe2MnO4 over FeMn2O4 spinel type oxides are more effective for CLOU applications.


Polymers ◽  
2021 ◽  
Vol 13 (20) ◽  
pp. 3458
Author(s):  
Sofia El-Ghazali ◽  
Hisatoshi Kobayashi ◽  
Muzamil Khatri ◽  
Duy-Nam Phan ◽  
Zeeshan Khatri ◽  
...  

Electrospun biobased polymeric nanofiber blends are widely used as biomaterials for different applications, such as tissue engineering and cell adhesion; however, their surface wettability and handling require further improvements for their practical utilization in the assistance of surgical operations. Therefore, Polyglycolic acid (PGA) and collagen-based nanofibers with three different ratios (40:60, 50:50 and 60:40) were prepared using the electrospinning method, and their surface wettability was improved using ozonation and plasma (nitrogen) treatment. The effect on the wettability and the morphology of pristine and blended PGA and collagen nanofibers was assessed using the WCA test and SEM, respectively. It was observed that PGA/collagen with the ratio 60:40 was the optimal blend, which resulted in nanofibers with easy handling and bead-free morphology that could maintain their structural integrity even after the surface treatments, imparting hydrophilicity on the surface, which can be advantageous for cell adhesion applications. Additionally, a cage-type collector was used during the electrospinning process to provide better handling properties to (PGA/collagen 60:40) blend. The resultant nanofiber mat was then incorporated with activated poly (α,β-malic acid) to improve its surface hydrophilicity. The chemical composition of PGA/collagen 60:40 was assessed using FTIR spectroscopy, supported by Raman spectroscopy.


2021 ◽  
Vol 12 (1) ◽  
Author(s):  
Byung Joon Moon ◽  
Sang Jin Kim ◽  
Aram Lee ◽  
Yelin Oh ◽  
Seoung-Ki Lee ◽  
...  

AbstractPhotophysical and photochemical properties of graphene quantum dots (GQDs) strongly depend on their morphological and chemical features. However, systematic and uniform manipulation of the chemical structures of GQDs remains challenging due to the difficulty in simultaneous control of competitive reactions, i.e., growth and doping, and the complicated post-purification processes. Here, we report an efficient and scalable production of chemically tailored N-doped GQDs (NGs) with high uniformity and crystallinity via a simple one-step solvent catalytic reaction for the thermolytic self-assembly of molecular precursors. We find that the graphitization of N-containing precursors during the formation of NGs can be modulated by intermolecular interaction with solvent molecules, the mechanism of wh ich is evidenced by theoretical calculations and various spectroscopic analyses. Given with the excellent visible-light photoresponse and photocatalytic activity of NGs, it is expected that the proposed approach will promote the practical utilization of GQDs for various applications in the near future.


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